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Phosphorus-32 labelled irradiated bovine hydroxyapatite for radiosynovectomy
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-16 DOI: 10.1007/s10967-024-09917-5
Asep Rizaludin, Isa Mahendra, Muhamad Basit Febrian, Ahmad Kurniawan, Basril Abbas, Yessy Warastuti, Army Adi Sutanningsih, Wira Y. Rahman, Fajar Lukitowati, Arie Hardian
{"title":"Phosphorus-32 labelled irradiated bovine hydroxyapatite for radiosynovectomy","authors":"Asep Rizaludin,&nbsp;Isa Mahendra,&nbsp;Muhamad Basit Febrian,&nbsp;Ahmad Kurniawan,&nbsp;Basril Abbas,&nbsp;Yessy Warastuti,&nbsp;Army Adi Sutanningsih,&nbsp;Wira Y. Rahman,&nbsp;Fajar Lukitowati,&nbsp;Arie Hardian","doi":"10.1007/s10967-024-09917-5","DOIUrl":"10.1007/s10967-024-09917-5","url":null,"abstract":"<div><p>Radiosynovectomy is a treatment for patients with rheumatoid arthritis (RA) that affects joints by injecting beta-emitting radiopharmaceuticals into the synovial membrane of inflamed joints. In this study, we established <sup>32</sup>Phosphorus labelled hydroxyapatite (<sup>32</sup>P-HAp) using gamma-irradiated hydroxyapatite material from bovine. Our results showed that gamma-irradiation of bovine HAp tends to agglomerate the particle and form a micro-sized HAp. In addition, irradiated HAp exhibited Ca/P ratio higher than non-irradiated HAp. The ex-vivo biodistribution studies exhibited a high accumulation of irradiated <sup>32</sup>P-HAp in the inflamed joints, resulting in good therapeutic effectiveness. Our study demonstrated the potential of <sup>32</sup>P-HAp from irradiated bovine hydroxyapatite for radiosynovectomy therapy.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1195 - 1204"},"PeriodicalIF":1.5,"publicationDate":"2024-12-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481173","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Distribution characteristics and health risk assessments in different surface and profile soils near a uranium mine tailings pond of Southeast China
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-12 DOI: 10.1007/s10967-024-09903-x
Yanhe Guan, Zhongkui Zhou, Yadan Guo, Binyu Lu, Renyu Zeng, Jingying Chen, Zhanxue Sun
{"title":"Distribution characteristics and health risk assessments in different surface and profile soils near a uranium mine tailings pond of Southeast China","authors":"Yanhe Guan,&nbsp;Zhongkui Zhou,&nbsp;Yadan Guo,&nbsp;Binyu Lu,&nbsp;Renyu Zeng,&nbsp;Jingying Chen,&nbsp;Zhanxue Sun","doi":"10.1007/s10967-024-09903-x","DOIUrl":"10.1007/s10967-024-09903-x","url":null,"abstract":"<div><p>The study investigates the radioactive nuclides <sup>238</sup>U, <sup>226</sup>Ra, <sup>232</sup>Th, and <sup>40</sup>K in surface and profile soils near the Lefu uranium mine tailings pond in southern China. It is found that concentrations of <sup>238</sup>U, <sup>226</sup>Ra, and <sup>232</sup>Th are significantly elevated (4.10, 13.57, 2.83, and 1.90 times the global average, respectively), and they decrease with soil depth, while <sup>40</sup>K remains stable in both surface and profile. Health risk assessments reveal that all soils in the bordering area and surface soils in nearby areas of the tailings pond poses higher risks, although overall risk levels are low. Correlation analysis indicates a strong positive correlation among <sup>238</sup>U, <sup>226</sup>Ra and <sup>232</sup>Th, suggesting a potential common source for them. These findings enhance understanding of contamination in uranium mining areas and inform remediation strategies.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 3","pages":"2001 - 2011"},"PeriodicalIF":1.5,"publicationDate":"2024-12-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707122","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Calculation of space radiation risks for astronauts and high-level natural radiation exposure area residents: two different exposure categories
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-12 DOI: 10.1007/s10967-024-09904-w
Akbar Abbasi, Nouf Almousa, Hesham M.H. Zakaly, Fatemeh Mirekhtiary
{"title":"Calculation of space radiation risks for astronauts and high-level natural radiation exposure area residents: two different exposure categories","authors":"Akbar Abbasi,&nbsp;Nouf Almousa,&nbsp;Hesham M.H. Zakaly,&nbsp;Fatemeh Mirekhtiary","doi":"10.1007/s10967-024-09904-w","DOIUrl":"10.1007/s10967-024-09904-w","url":null,"abstract":"<div><p>In the present paper, the health risks to astronauts due to space radiation exposure and the excess cancer risk (ECR) caused by high-level natural radiation exposure area residents were estimated manes on the National Aeronautics and Space Administration (NASA) Space Cancer Risk (NSCR)-2012 model and RESRAD code, respectively. The total risk of exposure-induced cancer (REIC) and total risk of exposure-induced death (REID) were calculated for different ages and genders. In contrast, the mortality and morbidity due to High Natural Background Radiation Exposure areas (HNBRAs) were simulated for different genders and ages. The results showed that the morbidity of the HNBRAs area for males and females was less than the REIC value of the 6-month mission at the International Space Station (ISS). Also, the results indicated that the mortality of the HNBRAs area was equal to the REIC 6-month mission for males. The mortality rate in the HNBRA area was higher than the average rate for females in the REIC 6-month mission.</p><h3>Graphical abstract</h3><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1445 - 1454"},"PeriodicalIF":1.5,"publicationDate":"2024-12-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143480991","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Research on the mechanism of uranium pollution caused by SUP gene transformation of Deinococcus Radiodurans
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-10 DOI: 10.1007/s10967-024-09905-9
Luomn Li, Fan Jiang, Lianyun Wang, Yuping Deng, Yuchun Hu, Fangzhu Xiao
{"title":"Research on the mechanism of uranium pollution caused by SUP gene transformation of Deinococcus Radiodurans","authors":"Luomn Li,&nbsp;Fan Jiang,&nbsp;Lianyun Wang,&nbsp;Yuping Deng,&nbsp;Yuchun Hu,&nbsp;Fangzhu Xiao","doi":"10.1007/s10967-024-09905-9","DOIUrl":"10.1007/s10967-024-09905-9","url":null,"abstract":"<div><p>This study reveals the transformation of the Super Uranyl-binding Protein (SUP) gene with high uranium selectivity and binding affinity into Deinococcus Radiodurans, a genetically modified bacterium with high uranium adsorption capacity and resistance to radiation. The optimal adsorption conditions and mechanism of <i>Deino-SUP</i> for uranium under different environmental conditions were investigated. The results demonstrated the successful construction of <i>Deino-SUP</i>, a recombinant strain with excellent uranium adsorption capacity and radiation resistance. The adsorption of uranium by <i>Deino-SUP</i> is mainly controlled by chemisorption, and the adsorption rate of uranium by <i>Deino-SUP</i> is better than that by <i>Deino-wt</i>.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1595 - 1611"},"PeriodicalIF":1.5,"publicationDate":"2024-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481011","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Development of the equilibrium adsorption layer model for describing the dynamic adsorption of radioactive gases
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-10 DOI: 10.1007/s10967-024-09826-7
Eldar P. Magomedbekov, Aleksei O. Merkushkin, Alexander V. Obruchikov, Veronika S. Pokalchuk, Elena A. Vanina
{"title":"Development of the equilibrium adsorption layer model for describing the dynamic adsorption of radioactive gases","authors":"Eldar P. Magomedbekov,&nbsp;Aleksei O. Merkushkin,&nbsp;Alexander V. Obruchikov,&nbsp;Veronika S. Pokalchuk,&nbsp;Elena A. Vanina","doi":"10.1007/s10967-024-09826-7","DOIUrl":"10.1007/s10967-024-09826-7","url":null,"abstract":"<div><p>The technique of adsorption is commonly employed to capture volatile radionuclides, finding extensive use in various fields, including gas treatment in nuclear power plants, protection of personnel, and capture systems for medical radioactive isotopes. An adequate mathematical description is essential for the design, calculation, and prediction of the output concentration and distribution of radionuclides in the sorbent bed over time. The theory of chromatography for non-radioactive adsorptives can now be considered detailed. However, its applications for radioactive gases are not as numerous and are generally limited to the simplest cases (stationary adsorption mode, linear isotherm). The present investigation improves upon the current model of the equilibrium adsorption layer by incorporating the radioactive decay of the adsorptive. At any given time, the complete description of the radionuclide distribution in the mobile and solid phase can be obtained through the resulting equation system, regardless of the type of adsorption isotherm. Simple analytical solutions were also obtained for the most practical case of linear adsorption isotherm. The frontal adsorption of the short-lived isotope <sup>220</sup>Rn on activated AG-3 at 30 °C was studied in the air flow rate from 1 to 8 l/min (superficial linear air velocity from 50 to 430 cm/min). The experimental results were fully corresponded to the theoretical representations described in the paper.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1375 - 1389"},"PeriodicalIF":1.5,"publicationDate":"2024-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481010","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
111In-hydroxyapatite nanoparticles: sorption studies
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-06 DOI: 10.1007/s10967-024-09913-9
Oľga Rosskopfová, Martina Bugriová, Eva Viglašová, Marek Hupian, Michal Galamboš
{"title":"111In-hydroxyapatite nanoparticles: sorption studies","authors":"Oľga Rosskopfová,&nbsp;Martina Bugriová,&nbsp;Eva Viglašová,&nbsp;Marek Hupian,&nbsp;Michal Galamboš","doi":"10.1007/s10967-024-09913-9","DOIUrl":"10.1007/s10967-024-09913-9","url":null,"abstract":"<div><p>This research examines the ability of hydroxyapatite to adsorb and desorb <sup>111</sup>In under various conditions. High crystallinity hydroxyapatite showed rapid <sup>111</sup>In sorption within just 3 min, with consistent pH levels. Adsorption remained stable over a broad pH range, and the results were well-fitted by Langmuir and Freundlich isotherms, with maximum capacities of 0.437 and 0.605 mmol g<sup>−1</sup>. Organic ligands maintained high sorption while competitive ions like Fe<sup>3+</sup> and Al<sup>3+</sup> reduced <sup>111</sup>In sorption efficiency significantly. Oxalic acid and carbonate ions proved most effective for desorption of <sup>111</sup>In, highlighting hydroxyapatite´s potential as a sorbent for this radioisotope.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1631 - 1641"},"PeriodicalIF":1.5,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10967-024-09913-9.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481159","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Projections of future ambient dose rates in a mountainous area in the Fukushima evacuation zone, Japan
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-06 DOI: 10.1007/s10967-024-09908-6
Katsumi Shozugawa, Mayumi Hori, Thomas E. Johnson, Yo Ishigaki, Yoshinori Matsumoto
{"title":"Projections of future ambient dose rates in a mountainous area in the Fukushima evacuation zone, Japan","authors":"Katsumi Shozugawa,&nbsp;Mayumi Hori,&nbsp;Thomas E. Johnson,&nbsp;Yo Ishigaki,&nbsp;Yoshinori Matsumoto","doi":"10.1007/s10967-024-09908-6","DOIUrl":"10.1007/s10967-024-09908-6","url":null,"abstract":"<div><p>We measured ambient dose rates in a mountainous area in the evacuation zone (Namie town, Fukushima prefecture, Japan) to predict ambient dose rates several decades ahead based on collected data. The survey was conducted on a ridge in a mountainous area that had not been previously decontaminated. Future ambient dose rate projections based on observed dose rates suggest a faster dose rate decline than those based on the physical decay of radiocesium. Specifically, the projections based on observed data indicate that the Japanese decontamination threshold in the area would be reached 15 years earlier than predicted based on physical decay.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1643 - 1648"},"PeriodicalIF":1.5,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10967-024-09908-6.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481160","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Investigation into the chemical mechanism of praseodymium extraction for rare earth elements through high-temperature electrochemical extraction
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-04 DOI: 10.1007/s10967-024-09865-0
Qi Zeng, Daqing Huang, Yuanping Jiang, Yuhui Liu, Yubo Shen, Zhimin Dong, Xiaohong Cao, Jun Gao, Zhibin Zhang, Yingcai Wang, Yunhai Liu
{"title":"Investigation into the chemical mechanism of praseodymium extraction for rare earth elements through high-temperature electrochemical extraction","authors":"Qi Zeng,&nbsp;Daqing Huang,&nbsp;Yuanping Jiang,&nbsp;Yuhui Liu,&nbsp;Yubo Shen,&nbsp;Zhimin Dong,&nbsp;Xiaohong Cao,&nbsp;Jun Gao,&nbsp;Zhibin Zhang,&nbsp;Yingcai Wang,&nbsp;Yunhai Liu","doi":"10.1007/s10967-024-09865-0","DOIUrl":"10.1007/s10967-024-09865-0","url":null,"abstract":"<div><p>The experiment is based on the dry post-treatment of spent fuel, employing high-temperature electrolysis to eliminate rare earth elements from spent fuel. Electrochemical methods such ascyclic voltammetry, square-wave voltammetry and open-circuit chronopotentiometry, were employed to examine the electrochemical properties of target nuclide at an inert tungsten electrode in the LiCl–KCl molten salt system. The results demonstrate that Pr(III) ions undergo a three-electron exchange process under diffusion control, leading to the reduction of Pr(III) ions to Pr(0). Additionally, it is observed that the redox reaction of Pr(III) ions is reversible and governed by diffusion control. The determination of the electron transfer number for Pr(III) yielded a value of 3 through the utilization of square-wave voltammetry. The diffusion coefficients of Pr(III) ions and the thermodynamics of various Pr-Bi intermetallic compounds were computed. Based on its exhibited characteristics, this electrochemical method provides suitable conditions for preparing rare earth alloys through constant potential electrolysis, and the average extraction rate of Pr was validated as 92.90%.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1541 - 1552"},"PeriodicalIF":1.5,"publicationDate":"2024-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481039","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Yttrium-90 recovery from carbonate media with binary extractants based on hydroxyaromatic compounds and methyltrioctylammonium carbonate
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-12-03 DOI: 10.1007/s10967-024-09910-y
Ahmed H. A. Harb, Igor V. Balantsev, Maria D. Karavan, Igor V. Smirnov
{"title":"Yttrium-90 recovery from carbonate media with binary extractants based on hydroxyaromatic compounds and methyltrioctylammonium carbonate","authors":"Ahmed H. A. Harb,&nbsp;Igor V. Balantsev,&nbsp;Maria D. Karavan,&nbsp;Igor V. Smirnov","doi":"10.1007/s10967-024-09910-y","DOIUrl":"10.1007/s10967-024-09910-y","url":null,"abstract":"<div><p>A new method of yttrium recovery with a mixture of hydroxyaromatic compound (8-hydroxyquinoline, 2,3-dihydroxynaphthalene) and methyltrioctylammonium carbonate separation from strontium in carbonate media has been proposed. Yttrium extraction from carbonate media has been studied. The structures of yttrium solvates with ligands formed during extraction have been proposed. The suggested method for yttrium recovery from soil by sample calcination followed by carbonate leaching and extraction with the specified mixture allows the efficient separation of yttrium-strontium pair and yttrium recovery.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 3","pages":"2131 - 2138"},"PeriodicalIF":1.5,"publicationDate":"2024-12-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143706883","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Optimum storage temperature of a reusable radiochromic gel dosimeter composed of PVA, iodine, and silicananoparticles (PAISiN)
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-11-30 DOI: 10.1007/s10967-024-09900-0
Sophia E. Welti, Hirokazu Miyoshi, Hiroshi Yasuda
{"title":"Optimum storage temperature of a reusable radiochromic gel dosimeter composed of PVA, iodine, and silica\u0000nanoparticles (PAISiN)","authors":"Sophia E. Welti,&nbsp;Hirokazu Miyoshi,&nbsp;Hiroshi Yasuda","doi":"10.1007/s10967-024-09900-0","DOIUrl":"10.1007/s10967-024-09900-0","url":null,"abstract":"<div><p>A recently introduced radiochromic complex composed of polyvinyl alcohol, iodide, and silica nanoparticles named “PAISiN” has potential as an extremity dosimeter because of its easily recognizable color change and reusability. In this study, the influence of temperature on the decolorization process of PAISiN after X-ray irradiation was investigated at four different temperatures. The results indicated that the optimal storage temperature for maintaining the post-irradiation coloration status of PAISiN was judged to be 10–11 °C.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1589 - 1594"},"PeriodicalIF":1.5,"publicationDate":"2024-11-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10967-024-09900-0.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481150","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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