Studying the relevance of mechanical process to the geochemical evolution in bentonite buffer of repositories for high-level radioactive waste

IF 1.5 3区 化学 Q3 CHEMISTRY, ANALYTICAL
Xiaoyuan Cao, Liange Zheng, Litang Hu
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引用次数: 0

Abstract

In deep geological repositories for high-level radioactive waste, the bentonite buffer undergoes thermal, hydrological, mechanical, and chemical (THMC) processes. This study aims to clarify the significance of the mechanical process in the THC evolution of bentonite by comparing a THC model with a coupled THMC model for a generic repository. The comparison shows that the impact of the mechanical process on hydrological and geochemical changes is significant during the early unsaturated stage but diminishes in the later stages once the bentonite is fully saturated. This suggests that considering mechanical processes may not be essential for long-term radionuclide migration models.

Abstract Image

高放废物处置库膨润土缓冲层力学过程与地球化学演化的相关性研究
在高放射性废物的深层地质储存库中,膨润土缓冲液经历了热、水文、机械和化学(THMC)过程。本研究旨在通过对一般储存库的THC模型与耦合THMC模型进行比较,阐明膨润土THC演化过程中力学过程的意义。对比结果表明,膨润土在非饱和初期,力学过程对水文和地球化学变化的影响显著,而在膨润土完全饱和的后期,力学过程对水文和地球化学变化的影响减弱。这表明,考虑机械过程可能不是长期放射性核素迁移模型所必需的。
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来源期刊
CiteScore
2.80
自引率
18.80%
发文量
504
审稿时长
2.2 months
期刊介绍: An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.
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