Nano Letters最新文献_第4页

Gas-Pressure-DrivenPhase Engineering of PdZn OrderedIntermetallics for Enhanced Oxygen Reduction Electrocatalysis 强化氧还原电催化的PdZn有序金属间化合物气压驱动相工程

IF 10.8 1区材料科学

Nano Letters Pub Date : 2026-10-15 DOI: 10.1021/acs.nanolett.6c03757

Jiabing Yan,Pei Zhang,Xing Hu,Yibo Liu,Hao Han,Ruifan Li,Yanan Feng,Shan Zhu,Kezhu Jiang,Shijian Zheng

{"title":"Gas-Pressure-Driven\u0000Phase Engineering of PdZn Ordered\u0000Intermetallics for Enhanced Oxygen Reduction Electrocatalysis","authors":"Jiabing Yan,Pei Zhang,Xing Hu,Yibo Liu,Hao Han,Ruifan Li,Yanan Feng,Shan Zhu,Kezhu Jiang,Shijian Zheng","doi":"10.1021/acs.nanolett.6c03757","DOIUrl":"https://doi.org/10.1021/acs.nanolett.6c03757","url":null,"abstract":"Abstract Precise phase engineering at the atomic scale is central to advanced catalyst design, yet controlling high-temperature phase transitions remains challenging because of large kinetic barriers. Here, we report a gas-pressure-induced strategy that establishes gas pressure as an independent dimension for nanoscale phase engineering. Mechanistic studies reveal that modulating the gas-phase diffusion coefficient via the gas pressure can control the structural evolution of crystal phases. As a demonstration of this methodology, an optimal pressure effectively overcomes high-temperature constraints and retards the escape of volatile species, enabling the precise construction of phase-pure ordered PdZn intermetallics. This strategy extends to ternary PdZnCu ordered alloys, inducing significant compressive strain while preserving the long-range ordered lattice. The resulting catalyst delivers a high oxygen reduction mass activity of 1.09 A mgPd–1 and long-term durability over 30 000 cycles. This gas-pressure-induced approach circumvents conventional thermodynamic and kinetic constraints, providing a pathway for the design of advanced intermetallic catalysts.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"16 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2026-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149210029","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Molten-Perfusion-FluorinationStrategy To Enable GraphiteLayer Confined Pyrochlore-Phase Iron Hydroxy Fluoride as SustainableConversion-Type Cathode 熔融-灌注-氟化策略使石墨层限烧氯相羟基氟化铁成为可持续转换型阴极

IF 10.8 1区材料科学

Nano Letters Pub Date : 2026-10-15 DOI: 10.1021/acs.nanolett.6c03365

Runyuan Cao,Chuanzhong Lai,Ju Huang,Meng Lei,Keyi Chen,Chilin Li

{"title":"Molten-Perfusion-Fluorination\u0000Strategy To Enable Graphite\u0000Layer Confined Pyrochlore-Phase Iron Hydroxy Fluoride as Sustainable\u0000Conversion-Type Cathode","authors":"Runyuan Cao,Chuanzhong Lai,Ju Huang,Meng Lei,Keyi Chen,Chilin Li","doi":"10.1021/acs.nanolett.6c03365","DOIUrl":"https://doi.org/10.1021/acs.nanolett.6c03365","url":null,"abstract":"Abstract Multielectron-conversion type and economically friendly iron fluorides are labeled as potential cathode candidates over single electron-redox intercalation oxides for Li-driven batteries. Herein, we propose a molten-perfusion-fluorination strategy to introduce pyrochlore-phase iron hydroxy fluoride into nature graphite layers. The macroscopic coralloid-like morphology, sandwich-packing with Fe–C chemical bonds, and 3D open framework endow FeF3 with abundant (surface/bulk) reactive sites and self-adaption ability against consecutive conversion reactions. The microscopic hydroxy anion replacement against F– framework also reduces the Fe–F coordination strength while partially substituting “tough” LiF by “soft” LiOH in discharge products. Consequently, the optimized cathode delivers a good cycling performance (255 mAh g–1 after 150 cycles) at 100 mA g–1 and outstanding capacity retention from 200 to 1000 mA g–1 (with reversible capacity of 327 mAh g–1). Such structural design method also reveals new perspectives for the expansion and exfoliation of graphite and its confinement effect and hybridization with electrode active species.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"4 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2026-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149210022","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

A Thermoelectric Hydrogel-Based Insole with Self-DecoupledTemperature and Pressure Sensing for Diabetic Plantar Monitoring 用于糖尿病足底监测的自解耦温度和压力传感热电水凝胶鞋垫

IF 10.8 1区材料科学

Nano Letters Pub Date : 2026-10-15 DOI: 10.1021/acs.nanolett.6c03487

Yu Niu,Chunjing Wang,Saeed Ahmed Khan,Xinru Yang,Ning Li,Hao Chen,Yanrong Li,Dapeng Yang,Xiaojing Cui,Zhou Li,Hulin Zhang

{"title":"A Thermoelectric Hydrogel-Based Insole with Self-Decoupled\u0000Temperature and Pressure Sensing for Diabetic Plantar Monitoring","authors":"Yu Niu,Chunjing Wang,Saeed Ahmed Khan,Xinru Yang,Ning Li,Hao Chen,Yanrong Li,Dapeng Yang,Xiaojing Cui,Zhou Li,Hulin Zhang","doi":"10.1021/acs.nanolett.6c03487","DOIUrl":"https://doi.org/10.1021/acs.nanolett.6c03487","url":null,"abstract":"Abstract Plantar temperature and pressure reflect the plantar health status of diabetic patients and serve as critical indicators for evaluating disease progression. However, existing plantar monitoring devices are still limited by single-modal signal acquisition, bulky device configurations, and a strong reliance on external power supplies. Herein, we report a thermogalvanic hydrogel-based smart insole integrating self-powered sensing units for self-decoupled plantar monitoring. The insole integrates 16 self-decoupled thermogalvanic hydrogel sensing units, which convert plantar temperature difference and pressure stimuli into decouplable electrical signals via the thermogalvanic effect and the active iontronic piezoresistive effect, respectively. The incorporation of the backend acquisition circuit into the smart monitoring insole enables remote plantar temperature-difference and pressure mapping. Cloud-based machine learning further empowers the insole to assess plantar status in diabetic patients and distinguish disease-associated gait patterns. This work provides a versatile strategy for developing multimodal intelligent wearable platforms for personalized foot health monitoring and disease management.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"4 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2026-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149210026","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Lipoprotein-DrivenRemodeling of Interfacial ChargeGoverns Protein-Mediated Implant Integration 脂蛋白驱动的界面电荷重塑控制蛋白质介导的植入物整合

IF 10.8 1区材料科学

Nano Letters Pub Date : 2026-10-15 DOI: 10.1021/acs.nanolett.6c03394

Chengyue Ou,Fanyu Zhang,Junjia Wang,Muhesen Yashengjiang,Qunli Liu,Jiaqiang Zhang,Yian Shen,Tianman Wang,Wenjie Gan,Caiqun Zhang,Yangqi He,Yufeng Zhang

{"title":"Lipoprotein-Driven\u0000Remodeling of Interfacial Charge\u0000Governs Protein-Mediated Implant Integration","authors":"Chengyue Ou,Fanyu Zhang,Junjia Wang,Muhesen Yashengjiang,Qunli Liu,Jiaqiang Zhang,Yian Shen,Tianman Wang,Wenjie Gan,Caiqun Zhang,Yangqi He,Yufeng Zhang","doi":"10.1021/acs.nanolett.6c03394","DOIUrl":"https://doi.org/10.1021/acs.nanolett.6c03394","url":null,"abstract":"Abstract Hyperlipidemia compromises implant integration, but the molecular mechanisms linking dyslipidemic environments to the biomaterial performance remain largely unknown. Here, we identify interfacial charge remodeling as a key regulator of the protein-mediated cell adhesion. Fibronectin (FN) is shown to govern endothelial attachment under hyperlipidemic conditions through charge-dependent interactions with the material surfaces. Molecular dynamics simulations reveal that the local charge distribution governs FN adsorption and conformational stability, while total internal reflection fluorescence (TIRF) single-molecule tracking demonstrates that charged adhesion domains regulate FN residence and adhesion stability in lipoprotein-rich environments. Deletion of negatively charged residues stabilizes FN–surface interactions, attenuates lipid-dependent disruption of adhesion signaling, and enhances endothelial responses. Similar charge-dependent behavior is observed on poly(lactic acid) (PLA), extending this interfacial charge remodeling from inorganic to organic biomaterials. These findings establish interfacial charge as a molecular determinant of implant integration under hyperlipidemic conditions and provide a general strategy for designing metabolism-responsive biomaterials.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"292 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2026-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149210027","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Probing Inner-TipAccess-Resistance Modulation byssDNA in a Nanopipette Using a Single-Molecule Nanomanipulation System 利用单分子纳米操作系统探测纳米吸管中yssdna的内针尖接入电阻调制

IF 10.8 1区材料科学

Nano Letters Pub Date : 2026-10-15 DOI: 10.1021/acs.nanolett.6c03709

Wenhao Ma,Yongjia Wang,Shaoxi Fang,Shixuan He,Yajie Yin,Bohua Yin,Rong Tian,Ting Weng,Wanyi Xie,Changjun Hou,Danquan Huo,Deqiang Wang

{"title":"Probing Inner-Tip\u0000Access-Resistance Modulation by\u0000ssDNA in a Nanopipette Using a Single-Molecule Nanomanipulation System","authors":"Wenhao Ma,Yongjia Wang,Shaoxi Fang,Shixuan He,Yajie Yin,Bohua Yin,Rong Tian,Ting Weng,Wanyi Xie,Changjun Hou,Danquan Huo,Deqiang Wang","doi":"10.1021/acs.nanolett.6c03709","DOIUrl":"https://doi.org/10.1021/acs.nanolett.6c03709","url":null,"abstract":"Abstract The transport of flexible polyelectrolytes through nanoscale confinements is fundamental to polymer physics and biophysics, yet direct observation remains challenging. Using a nanopipette-based single-molecule nanomanipulation platform, we controllably translocate long single-stranded DNA (ssDNA) through a solid-state nanopore, enabling real-time tracking of chain dynamics with nanoscale precision. We discover that ssDNA generates a characteristic progressive current decrease with terminal oscillations─absent for rigid double-stranded DNA. Evidence indicates this signal arises from inner-tip access-resistance modulation by the ssDNA coil, with a linear relationship between current blockade and relative escape displacement. Systematic variation of voltage and nanopore geometry reveals electric-field-driven stretching of the ssDNA coil and extended interaction with the inner tip region. This provides a framework for interpreting flexible polyelectrolyte transport under nanoconfinement, with implications for polymer physics, nuclear pore transport, and intrinsically disordered proteins.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"11 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2026-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149210025","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Dimensionality-Driven Charge Stabilization of Group-IVColor Centers in Diamond Ultrathin Films 金刚石超薄膜中群- iv色中心的维数驱动电荷稳定

IF 10.8 1区材料科学

Nano Letters Pub Date : 2026-10-15 DOI: 10.1021/acs.nanolett.6c03449

Jijun Huang,Bing Huang,Song Li

{"title":"Dimensionality-Driven Charge Stabilization of Group-IV\u0000Color Centers in Diamond Ultrathin Films","authors":"Jijun Huang,Bing Huang,Song Li","doi":"10.1021/acs.nanolett.6c03449","DOIUrl":"https://doi.org/10.1021/acs.nanolett.6c03449","url":null,"abstract":"Abstract Neutral group-IV vacancy (XV, X = Si, Ge, Sn, and Pb) centers in diamond are promising solid-state spin-photon interfaces owing to favorable spin coherence and inversion-symmetry-protected optical transitions. However, stabilizing their neutral charge state typically requires stringent Fermi-level engineering in high-purity boron-doped diamond, which poses significant materials-growth challenges. Here, dimensional confinement in diamane offers an alternative for charge-state stabilization without intentional doping. Our results show that diamane thickness and surface chemical termination cooperatively tune the electronic structures of XV centers, while their neutral-state thermodynamic stability is enhanced. The zero-field splitting and spin–orbit coupling of XV centers could be tuned while largely preserving their optical transition energies. We find hydrogenated diamane offers the best balance between charge-state stability and magneto-optical performance. More broadly, our findings establish dimensional confinement as a general strategy for engineering the charge, optical, and spin properties of solid-state quantum defects.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"188 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2026-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149210024","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Adaptive andMulticolored Electrochromic Smart Windowwith Transparent–Opaque Switchable Radiative Cooling 自适应和多色电致变色智能窗口与透明-不透明的可切换辐射冷却

IF 10.8 1区材料科学

Nano Letters Pub Date : 2026-10-15 DOI: 10.1021/acs.nanolett.6c03931

Jingjing Mao,Shenghao Jin,Ning Wang,Tao Xie,Run Hu,Lin Zhang,Boxiang Wang

{"title":"Adaptive and\u0000Multicolored Electrochromic Smart Window\u0000with Transparent–Opaque Switchable Radiative Cooling","authors":"Jingjing Mao,Shenghao Jin,Ning Wang,Tao Xie,Run Hu,Lin Zhang,Boxiang Wang","doi":"10.1021/acs.nanolett.6c03931","DOIUrl":"https://doi.org/10.1021/acs.nanolett.6c03931","url":null,"abstract":"Abstract Transparent radiative-cooling windows can reduce cooling demand while preserving daylighting, yet high solar transmission becomes undesirable under strong solar irradiation. Although existing electrochromic windows can regulate solar transmittance, simultaneously achieving strong solar rejection, radiative heat dissipation, and wide-gamut coloration remains challenging. Here, we develop dynamic colorful radiative cooling windows by integrating planar coupled nanocavities with reversible silver electrodeposition. Electrochemically controlled Ag deposition/stripping reconfigures Fabry–Pérot resonances, enabling reversible switching between colored transparent and highly reflective colored opaque states while retaining high mid-infrared emissivity. The devices can achieve &gt;40% modulation in average visible transmittance and cover 99.5% of the sRGB color gamut. Under outdoor conditions, they exhibit temperature drops of ∼7.0 °C compared to conventional glass and ∼8.7 °C relative to commercial electrochromic glass. This work provides a versatile platform for dynamic optical regulation with diverse requirements, paving the way for next-generation multifunctional smart windows, building envelopes, and smart photonic devices.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"80 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2026-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149210028","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Band Degeneracyand Liquid-like Dynamics in IntercalatedLa2O2Te/BiAgSeO Thermoelectrics 插层la2o2te /BiAgSeO热电器件的能带简并及类液体动力学

IF 10.8 1区材料科学

Nano Letters Pub Date : 2026-10-15 DOI: 10.1021/acs.nanolett.6c04158

Yufei Meng,Pengfei Zhang,Shulin Bai,Da Wan,Zhanpeng Xu,Hao Sun,Amondulloi Burhonzoda,Shuwei Tang,Shizhi Dong

{"title":"Band Degeneracy\u0000and Liquid-like Dynamics in Intercalated\u0000La2O2Te/BiAgSeO Thermoelectrics","authors":"Yufei Meng,Pengfei Zhang,Shulin Bai,Da Wan,Zhanpeng Xu,Hao Sun,Amondulloi Burhonzoda,Shuwei Tang,Shizhi Dong","doi":"10.1021/acs.nanolett.6c04158","DOIUrl":"https://doi.org/10.1021/acs.nanolett.6c04158","url":null,"abstract":"Abstract Interlayer modulation of layered oxychalcogenide superlattices provides a strategy to decouple electron–phonon transport for high-performance thermoelectric (TE) materials. Herein, an intercalated oxychalcogenide superlattice (La4Bi2Ag2Se2Te2O6) is theoretically designed by inserting a La2O2Te slab into the BiAgSeO framework to synergistically optimize carrier and phonon transport behaviors and systematically uncover an unprecedented synergy of orbital-driven valence band degeneracy and Ag+ liquid-like ionic dynamics. The La4Bi2Ag2Se2Te2O6 superlattice exhibits a highly anisotropic lattice architecture characterized by strong intralayer covalent bonding and weak interlayer interactions, which simultaneously preserves structural stability and promotes pronounced lattice anharmonicity. Meanwhile, stereochemically active Bi 6s2 lone-pair electrons, four-phonon scattering, and phonon–diffuson conversion drastically suppress the lattice thermal conductivity. This work establishes a dual-regulation intercalation paradigm combining band convergence and liquid-cation dynamics, offering a universal route for designing high-efficiency layered TE materials.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"37 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2026-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149210021","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Scalable, Simple, and Versatile Encapsulation of 2D Materials and Devices 二维材料和器件的可扩展，简单和通用封装

IF 9.1 1区材料科学

Nano Letters Pub Date : 2026-10-14 Epub Date: 2026-10-03 DOI: 10.1021/acs.nanolett.6c03297

Gabriel Natale, Uma Chirkova, Flávio Henriques Feres, Ran Jing, Michael Geiwitz, Wenyao Liu, Emma Low, Josh Leeman, Kyung-Mo Kim, Leslie M. Schoop, Mohamed Shehabeldin, Qiong Ma, Michael A. Susner, Pijush Bhattacharya, Genda Gu, Katherine Lee, James Hone, Mengkun Liu, Kenneth S. Burch

{"title":"Scalable, Simple, and Versatile Encapsulation of 2D Materials and Devices","authors":"Gabriel Natale, Uma Chirkova, Flávio Henriques Feres, Ran Jing, Michael Geiwitz, Wenyao Liu, Emma Low, Josh Leeman, Kyung-Mo Kim, Leslie M. Schoop, Mohamed Shehabeldin, Qiong Ma, Michael A. Susner, Pijush Bhattacharya, Genda Gu, Katherine Lee, James Hone, Mengkun Liu, Kenneth S. Burch","doi":"10.1021/acs.nanolett.6c03297","DOIUrl":"10.1021/acs.nanolett.6c03297","url":null,"abstract":"Air-sensitive 2D materials present fundamental challengesfor deviceintegration. Encapsulation is required to preserve intrinsic properties,yet conventional strategies require complicated fabrication workflowsand fail with thicker flakes. We demonstrate that electron-beam (e-beam)evaporated aluminum oxide (AlOx) servesas an effective encapsulation layer and sacrificial fabrication mask,protecting sensitive flakes from air, photoresists, and chemicals.Unlike transfer-based approaches, this scalable technique requiresno stacking and enables contacts without postencapsulation etchingor harsh chemistry. Using rare-earth tritellurides (RTe3, R = La, Er), semimetallic WTe2, and superconductingFeTexSe1–x, we show that AlOx suppressesoxidation and preserves optical and electronic properties. We establishsubstrate-dependent optimization of encapsulation across a range offlake thicknesses, demonstrate that ultrathin AlOx preserves WTe2’s plasmonic response, andenhances superconducting performance in FeTexSe1–x devices when employedas a mask. Thus, we overcome the longstanding trade-off between encapsulationand straightforward device fabrication in fragile quantum materials.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"26 40","pages":"13904–13912"},"PeriodicalIF":9.1,"publicationDate":"2026-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149088199","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Disordered Near-Field Metasurfaces for On-Chip Wavelength Demultiplexing 片上波长解复用的无序近场元表面

IF 9.1 1区材料科学

Nano Letters Pub Date : 2026-10-14 Epub Date: 2026-10-02 DOI: 10.1021/acs.nanolett.6c03564

L. Schmid, J. Schwab, F. Kadriu, R. Horvat, C. Li, S. A. Maier, H. Giessen, H. Ren, M. Hentschel

{"title":"Disordered Near-Field Metasurfaces for On-Chip Wavelength Demultiplexing","authors":"L. Schmid, J. Schwab, F. Kadriu, R. Horvat, C. Li, S. A. Maier, H. Giessen, H. Ren, M. Hentschel","doi":"10.1021/acs.nanolett.6c03564","DOIUrl":"10.1021/acs.nanolett.6c03564","url":null,"abstract":"Plasmonic and dielectric building blocks shape the flowof lightat boundaries and interfaces. While metasurfaces that consist of plasmonicor dielectric nanophotonic elements have established a framework forshaping the far field, control over near fields remains largely unexplored.Here, we introduce disordered metasurfaces for near-field light shaping.Near-field distributions are created by engineering the interferenceof surface plasmons launched from scatterers on metallic surfaces.We demonstrate near-field metasurfaces to direct, focus, and demultiplexlight. These structures use a strip-off process, resulting in ultrasmoothmetallic surfaces suitable for efficient surface plasmon propagation.An optical imaging setup enables retrieval of the local near-fieldby mapping it into the far-field. Our concept can be generalized toarbitrary near-field distributions, permitting nanoscale routing andsorting of light based on polarization and orbital angular momentum,as well as coupling schemes to emitters and nanoscale systems in ultracompactintegrated photonic receivers and demultiplexers.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"26 40","pages":"13955–13961"},"PeriodicalIF":9.1,"publicationDate":"2026-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149088203","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0