{"title":"金刚石中时间分辨荧光探测的耗散自旋动力学离轴磁传感。","authors":"Baiqiang Zhu,Fei Liu,Jia-Xin Peng,Zhifei Yu,Jianpei Geng,Keye Zhang,Bing Chen","doi":"10.1021/acs.nanolett.5c03898","DOIUrl":null,"url":null,"abstract":"Magnetic field sensing with a nitrogen-vacancy (NV) center in diamond typically relies on coherent spin manipulation, which is susceptible to spin dephasing noise. Here, we demonstrate an alternative protocol that exploits dissipative spin dynamics, probed through time-resolved fluorescence, to extract off-axis magnetic field information without relying on spin coherence. The approach operates under continuous optical excitation and leverages spin-dependent transition channels to encode both the strength and orientation of the magnetic field into the fluorescence dynamics. Numerical simulations incorporating Gaussian magnetic noise confirm that the protocol remains robust against spin dephasing, maintaining a stable estimation performance even under short coherence times. We further develop a general parameter estimation framework based on photoluminescence trajectories, enabling off-axis field reconstruction from experimental measurements. The method is experimentally validated and may be adapted to other fluorescence-based spin defect platforms including silicon carbide and hexagonal boron nitride.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"24 1","pages":""},"PeriodicalIF":9.1000,"publicationDate":"2025-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Off-Axis Magnetic Sensing via Dissipative Spin Dynamics Probed by Time-Resolved Fluorescence in Diamond.\",\"authors\":\"Baiqiang Zhu,Fei Liu,Jia-Xin Peng,Zhifei Yu,Jianpei Geng,Keye Zhang,Bing Chen\",\"doi\":\"10.1021/acs.nanolett.5c03898\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Magnetic field sensing with a nitrogen-vacancy (NV) center in diamond typically relies on coherent spin manipulation, which is susceptible to spin dephasing noise. Here, we demonstrate an alternative protocol that exploits dissipative spin dynamics, probed through time-resolved fluorescence, to extract off-axis magnetic field information without relying on spin coherence. The approach operates under continuous optical excitation and leverages spin-dependent transition channels to encode both the strength and orientation of the magnetic field into the fluorescence dynamics. Numerical simulations incorporating Gaussian magnetic noise confirm that the protocol remains robust against spin dephasing, maintaining a stable estimation performance even under short coherence times. We further develop a general parameter estimation framework based on photoluminescence trajectories, enabling off-axis field reconstruction from experimental measurements. The method is experimentally validated and may be adapted to other fluorescence-based spin defect platforms including silicon carbide and hexagonal boron nitride.\",\"PeriodicalId\":53,\"journal\":{\"name\":\"Nano Letters\",\"volume\":\"24 1\",\"pages\":\"\"},\"PeriodicalIF\":9.1000,\"publicationDate\":\"2025-09-30\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.nanolett.5c03898\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.5c03898","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Off-Axis Magnetic Sensing via Dissipative Spin Dynamics Probed by Time-Resolved Fluorescence in Diamond.
Magnetic field sensing with a nitrogen-vacancy (NV) center in diamond typically relies on coherent spin manipulation, which is susceptible to spin dephasing noise. Here, we demonstrate an alternative protocol that exploits dissipative spin dynamics, probed through time-resolved fluorescence, to extract off-axis magnetic field information without relying on spin coherence. The approach operates under continuous optical excitation and leverages spin-dependent transition channels to encode both the strength and orientation of the magnetic field into the fluorescence dynamics. Numerical simulations incorporating Gaussian magnetic noise confirm that the protocol remains robust against spin dephasing, maintaining a stable estimation performance even under short coherence times. We further develop a general parameter estimation framework based on photoluminescence trajectories, enabling off-axis field reconstruction from experimental measurements. The method is experimentally validated and may be adapted to other fluorescence-based spin defect platforms including silicon carbide and hexagonal boron nitride.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.