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TexSe1–x Shortwave Infrared Photodiode Arrays with Monolithic Integration 单片集成的 TexSe1-x 短波红外线光电二极管阵列
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-26 DOI: 10.1021/acs.nanolett.4c03728
Meng Peng, Yuming He, Yuxuan Hu, Zunyu Liu, Xinyi Chen, Zhiqiang Liu, Junrui Yang, Maohua Chen, Weijie Liu, Feng Wu, Luying Li, Jiangnan Dai, Changqing Chen, Jungang He, Long Hu, Chao Chen, Jiang Tang
{"title":"TexSe1–x Shortwave Infrared Photodiode Arrays with Monolithic Integration","authors":"Meng Peng, Yuming He, Yuxuan Hu, Zunyu Liu, Xinyi Chen, Zhiqiang Liu, Junrui Yang, Maohua Chen, Weijie Liu, Feng Wu, Luying Li, Jiangnan Dai, Changqing Chen, Jungang He, Long Hu, Chao Chen, Jiang Tang","doi":"10.1021/acs.nanolett.4c03728","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03728","url":null,"abstract":"Te<sub><i>x</i></sub>Se<sub>1–<i>x</i></sub> shortwave infrared (SWIR) photodetectors show promise for monolithic integration with readout integrated circuits (ROIC), making it a potential alternative to conventional expensive SWIR photodetectors. However, challenges such as a high dark current density and insufficient detection performance hinder their application in large-scale monolithic integration. Herein, we develop a ZnO/Te<sub><i>x</i></sub>Se<sub>1–<i>x</i></sub> heterojunction photodiode and synergistically address the interfacial elemental diffusion and dangling bonds via inserting a well-selected 0.3 nm amorphous TeO<sub>2</sub> interfacial layer. The optimized device achieves a reduced dark current density of −3.5 × 10<sup>–5</sup> A cm<sup>–2</sup> at −10 mV, a broad response from 300 to 1700 nm, a room-temperature detectivity exceeding 2.03 × 10<sup>11</sup> Jones, and a 3 dB bandwidth of 173 kHz. Furthermore, for the first time, we monolithically integrate the Te<sub><i>x</i></sub>Se<sub>1–<i>x</i></sub> photodiodes on ROIC (64 × 64 pixels) with the largest-scale array among all Te<sub><i>x</i></sub>Se<sub>1–<i>x</i></sub>-based detectors. Finally, we demonstrate its applications in transmission imaging and substance identification.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142321208","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Acoustic Modulation of Individual Nanowire Quantum Dots Integrated into a Hybrid Thin-Film Lithium Niobate Photonic Platform 集成到混合薄膜铌酸锂光子平台中的单个纳米线量子点的声学调制
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-26 DOI: 10.1021/acs.nanolett.4c03402
Thomas Descamps, Tanguy Schetelat, Jun Gao, Philip J. Poole, Dan Dalacu, Ali W. Elshaari, Val Zwiller
{"title":"Acoustic Modulation of Individual Nanowire Quantum Dots Integrated into a Hybrid Thin-Film Lithium Niobate Photonic Platform","authors":"Thomas Descamps, Tanguy Schetelat, Jun Gao, Philip J. Poole, Dan Dalacu, Ali W. Elshaari, Val Zwiller","doi":"10.1021/acs.nanolett.4c03402","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03402","url":null,"abstract":"Surface acoustic waves are a powerful tool for controlling quantum systems, including quantum dots (QDs), where the oscillating strain field can modulate the emission wavelengths. We integrate InAsP/InP nanowire QDs onto a thin-film lithium niobate platform and embed them within Si<sub>3</sub>N<sub>4</sub>-loaded waveguides. We achieve a 0.70 nm peak-to-peak wavelength modulation at 13 dBm using a single focused interdigital transducer (FIDT) operating at 400 MHz, and we double this amplitude to 1.4 nm by using two FIDTs as an acoustic cavity. Additionally, we independently modulate two QDs with an initial wavelength difference of 0.5 nm, both integrated on the same chip. We show that their modulated emissions overlap, demonstrating the potential to bring them to a common emission wavelength after spectral filtering. This local strain-tuning represents a significant step toward generating indistinguishable single photons from remote emitters heterogeneously integrated on a single chip, advancing on-chip quantum information processing with multiple QDs.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142321206","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Achieving a Noise Limit with a Few-layer WSe2 Avalanche Photodetector at Room Temperature 在室温条件下实现几层 WSe2 雪崩光电探测器的噪声极限
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-25 DOI: 10.1021/acs.nanolett.4c03450
Xin Li, Jin Chen, Feilong Yu, Xiaoshuang Chen, Wei Lu, Guanhai Li
{"title":"Achieving a Noise Limit with a Few-layer WSe2 Avalanche Photodetector at Room Temperature","authors":"Xin Li, Jin Chen, Feilong Yu, Xiaoshuang Chen, Wei Lu, Guanhai Li","doi":"10.1021/acs.nanolett.4c03450","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03450","url":null,"abstract":"We engineered a two-dimensional Pt/WSe<sub>2</sub>/Ni avalanche photodetector (APD) optimized for ultraweak signal detection at room temperature. By fine-tuning the work functions, we achieved an ultralow dark current of 10<sup>–14</sup> A under small bias, with a noise equivalent power (NEP) of 8.09 fW/Hz<sup>1/2</sup>. This performance is driven by effective dark barrier blocking and a record-long electron mean free path (123 nm) in intrinsic WSe<sub>2</sub>, minimizing dark carrier replenishment and suppressing noise under an ultralow electric field. Our APD exhibits a high gain of 5 × 10<sup>5</sup> at a modulation frequency of 20 kHz, effectively balancing gain and bandwidth, a common challenge in traditional photovoltaic-based APDs. By addressing the typical challenges of high noise and low gain and minimizing dependence on high electric fields, this work highlights the potential of 2D materials in developing efficient, low-power, and ultrasensitive photodetections.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317176","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Simultaneously Enhancing Brightness and Purity of WSe2 Single Photon Emitter Using High-Aspect-Ratio Nanopillar Array on Metal 在金属上使用高宽比纳米柱阵列同时提高 WSe2 单光子发射器的亮度和纯度
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-25 DOI: 10.1021/acs.nanolett.4c03168
Mayank Chhaperwal, Himanshu Madhukar Tongale, Patrick Hays, Kenji Watanabe, Takashi Taniguchi, Seth Ariel Tongay, Kausik Majumdar
{"title":"Simultaneously Enhancing Brightness and Purity of WSe2 Single Photon Emitter Using High-Aspect-Ratio Nanopillar Array on Metal","authors":"Mayank Chhaperwal, Himanshu Madhukar Tongale, Patrick Hays, Kenji Watanabe, Takashi Taniguchi, Seth Ariel Tongay, Kausik Majumdar","doi":"10.1021/acs.nanolett.4c03168","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03168","url":null,"abstract":"A monolayer semiconductor transferred on nanopillar arrays provides site-controlled, on-chip single photon emission, which is a scalable light source platform for quantum technologies. However, the brightness of these emitters reported to date often falls short of the perceived requirement for such applications. Also, the single photon purity usually degrades as the brightness increases. Hence, there is a need for a design methodology to achieve an enhanced emission rate while maintaining high single photon purity. By using WSe<sub>2</sub> on high-aspect-ratio (∼3, at least 2-fold higher than previous reports) nanopillar arrays, here we demonstrate &gt;10 MHz single photon emission rate in the 770–800 nm band that is compatible with quantum memory and repeater networks (Rb-87-D1/D2 lines) and satellite quantum communication. The emitters exhibit excellent purity (even at high emission rates) and improved out-coupling due to the use of a gold back reflector that quenches the emission away from the nanopillar.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317183","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Magnetic Detection of Neural Activity by Nanocoil Transducers 利用纳米线圈传感器对神经活动进行磁探测
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-25 DOI: 10.1021/acs.nanolett.4c02784
Ilhan Bok, Jack Phillips, Tianxiang Zhu, Jennifer Lu, Elizabeth Detienne, Eduardo Andrade Lima, Benjamin P. Weiss, Alan Jasanoff, Aviad Hai
{"title":"Magnetic Detection of Neural Activity by Nanocoil Transducers","authors":"Ilhan Bok, Jack Phillips, Tianxiang Zhu, Jennifer Lu, Elizabeth Detienne, Eduardo Andrade Lima, Benjamin P. Weiss, Alan Jasanoff, Aviad Hai","doi":"10.1021/acs.nanolett.4c02784","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c02784","url":null,"abstract":"Electrophysiological recordings from brain cells are performed routinely using implanted electrodes, but they traditionally require a wired connection to the outside of the brain. A completely passive, wireless device that does not require on-board power for active transmission but that still facilitates remote detection could open the door for mass-scale direct recording of action potentials and transform the way we acquire brain signals. We present a nanofabricated coil that forms a neuroelectromagnetic junction, yielding a highly enhanced magnetic field transduction of electrophysiology. We show that this micrometer-scale device enables remote magnetic detection of neuronal fields from the center of the coil using room temperature superconducting quantum interference device (SQUID) microscopy. Further, time-locked stimulation in conjunction with magnetometry demonstrates thresholding behavior that affirms the viability of the technology for detection with no requirement for wires or on-board power. This strategy may permit unprecedented detection of electrophysiology using magnetoencephalography and magnetic resonance imaging.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317180","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Large-Area Perovskite Nanocrystal Metasurfaces for Direction-Tunable Lasing 用于定向可调激光的大面积 Perovskite 纳米晶体金属表面
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-25 DOI: 10.1021/acs.nanolett.4c03921
Nanli Mou, Bing Tang, Bowen Han, Jingyue Yu, Delin Zhang, Zichun Bai, Mou Zhong, Biye Xie, Zhaoyu Zhang, Shikai Deng, Andrey L. Rogach, Jingtian Hu, Jun Guan
{"title":"Large-Area Perovskite Nanocrystal Metasurfaces for Direction-Tunable Lasing","authors":"Nanli Mou, Bing Tang, Bowen Han, Jingyue Yu, Delin Zhang, Zichun Bai, Mou Zhong, Biye Xie, Zhaoyu Zhang, Shikai Deng, Andrey L. Rogach, Jingtian Hu, Jun Guan","doi":"10.1021/acs.nanolett.4c03921","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03921","url":null,"abstract":"Perovskite nanocrystals (PNCs) are attractive emissive materials for developing compact lasers. However, manipulation of PNC laser directionality has been difficult, which limits their usage in photonic devices that require on-demand tunability. Here we demonstrate PNC metasurface lasers with engineered emission angles. We fabricated millimeter-scale CsPbBr<sub>3</sub> PNC metasurfaces using an all-solution-processing technique based on soft nanoimprinting lithography. By designing band-edge photonic modes at the high-symmetry X point of the reciprocal lattice, we achieved four linearly polarized lasing beams along a polar angle of ∼30° under optical pumping. The device architecture further allows tuning of the lasing emission angles to 0° and ∼50°, respectively, by adjusting the PNC thickness to shift other high-symmetry points (Γ and M) to the PNC emission wavelength range. Our laser design strategies offer prospects for applications in directional optical antennas and detectors, 3D laser projection displays, and multichannel visible light communication.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317178","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Light-Armed Nitric Oxide-Releasing Micromotor In Vivo 体内光臂一氧化氮释放微马达
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-25 DOI: 10.1021/acs.nanolett.4c03120
Tiange Zhang, Haojiang Ren, Haifeng Qin, Xiaoshuai Liu, Baojun Li, Xianchuang Zheng
{"title":"Light-Armed Nitric Oxide-Releasing Micromotor In Vivo","authors":"Tiange Zhang, Haojiang Ren, Haifeng Qin, Xiaoshuai Liu, Baojun Li, Xianchuang Zheng","doi":"10.1021/acs.nanolett.4c03120","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03120","url":null,"abstract":"The delivery of NO at a high spatiotemporal precision is important but still challenging for existing NO-releasing platforms due to the lack of precise motion control and limited biomedical functions. In this work, we propose an alternative strategy for developing the light-armed nitric oxide-releasing micromotor (LaNorM), in which a main light beam was employed to navigate the microparticle and stimulate NO release and an auxiliary light beam was used to cooperate with the released NO to act as a remotely controlled scalpel for cell separation. Benefiting from the advantages of fully controlled locomotion, photostimulated NO release, and microsurgery ability at the single-cell level, the proposed LaNorM could enable a series of biomedical applications <i>in vivo</i>, including the separation of flowing emboli, selective removal of a specific thrombus, and inhibition of thrombus growth, which may provide new insight into the precise delivery of NO and the treatment of cardiovascular diseases.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317187","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High-Active Surface of Centimeter-Scale β-In2S3 for Attomolar-Level Hg2+ Sensing 用于阿托摩尔级 Hg2+ 传感的厘米级 β-In2S3 高活性表面
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-25 DOI: 10.1021/acs.nanolett.4c04047
Weixuan Zhang, Xuanlin Pan, Junxin Yan, Lixuan Liu, Anmin Nie, Yingchun Cheng, Fusheng Wen, Congpu Mu, Kun Zhai, Jianyong Xiang, Bochong Wang, Tianyu Xue, Zhongyuan Liu
{"title":"High-Active Surface of Centimeter-Scale β-In2S3 for Attomolar-Level Hg2+ Sensing","authors":"Weixuan Zhang, Xuanlin Pan, Junxin Yan, Lixuan Liu, Anmin Nie, Yingchun Cheng, Fusheng Wen, Congpu Mu, Kun Zhai, Jianyong Xiang, Bochong Wang, Tianyu Xue, Zhongyuan Liu","doi":"10.1021/acs.nanolett.4c04047","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c04047","url":null,"abstract":"Recognition layer materials play a crucial role in the functionality of chemical sensors. Although advancements in two-dimensional (2D) materials have promoted sensor development, the controlled fabrication of large-scale recognition layers with highly active sites remains crucial for enhancing sensor sensitivity, especially for trace detection applications. Herein, we propose a strategy for the controlled preparation of centimeter-scale non-layered ultrathin β-In<sub>2</sub>S<sub>3</sub> materials with tailored high-active sites to design ultrasensitive Hg<sup>2+</sup> sensors. Our results reveal that the highly active sites of non-layered β-In<sub>2</sub>S<sub>3</sub> materials are pivotal for achieving superior sensing performance. Selective detection of Hg<sup>2+</sup> at the 1 aM level is achieved via selective Hg–S bonding. Additionally, we evaluate that this sensor exhibits excellent performance in detecting Hg<sup>2+</sup> in the tap water matrix. This work provides a proof-of-concept for utilizing non-layered 2D films in high-performance sensors and highlights their potential for diverse analyte sensing applications.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317179","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Direct Detection of the Magnetic Force and Field Coupling of Electronic Spins Using Photoinduced Magnetic Force Microscopy 利用光诱导磁力显微镜直接检测电子自旋的磁力和磁场耦合
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-25 DOI: 10.1021/acs.nanolett.4c03437
Zhenrong Zhang, Qiang Zhu, Liangjie Li, Huan Fei Wen, Hao Guo, Zongmin Ma, Ye Tian, Yasuhiro Sugawara, Yan Jun Li, Jun Tang, Jun Liu
{"title":"Direct Detection of the Magnetic Force and Field Coupling of Electronic Spins Using Photoinduced Magnetic Force Microscopy","authors":"Zhenrong Zhang, Qiang Zhu, Liangjie Li, Huan Fei Wen, Hao Guo, Zongmin Ma, Ye Tian, Yasuhiro Sugawara, Yan Jun Li, Jun Tang, Jun Liu","doi":"10.1021/acs.nanolett.4c03437","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03437","url":null,"abstract":"The intrinsic spin of the electron and its associated magnetic moment can provide insights into spintronics. However, the interaction is extremely weak, as is the case with the coupling between an electron’s spin and a magnetic field, and it poses significant experimental challenges. Here we demonstrate the direct measurement of polarized single NV<sup>–</sup> centers and their spin–spin coupling behaviors in diamond. By using photoinduced magnetic force microscopy, we obtain the extremely weak magnetic force coupling originating from the electron spin. The polarized spin state of NV<sup>–</sup> centers, transitioning from |0⟩ to |±1⟩, and their corresponding Zeeman effect can be characterized through their interaction with a magnetic tip. The result presents an advancement in achieving electron spin measurements by magnetic force, avoiding the need for manufacturing conductive substrates. This facilitates a better understanding and control of electron spin to novel electronic states for future quantum technologies.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317184","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Significant Power Consumption Reduction and Speed Boosting in Phase Change Memory with Nanocurrent Channels 利用纳米电流通道大幅降低相变存储器功耗并提高速度
IF 10.8 1区 材料科学
Nano Letters Pub Date : 2024-09-24 DOI: 10.1021/acs.nanolett.4c03900
Yuntao Zeng, Ge Ma, Han Li, Xiaomin Cheng, Xiangshui Miao
{"title":"Significant Power Consumption Reduction and Speed Boosting in Phase Change Memory with Nanocurrent Channels","authors":"Yuntao Zeng, Ge Ma, Han Li, Xiaomin Cheng, Xiangshui Miao","doi":"10.1021/acs.nanolett.4c03900","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03900","url":null,"abstract":"The excessive power consumption is challenging for phase change memory (PCM) on its way to becoming universal memory in complex hierarchies of memory systems. Here, from the perspective of device structure, by adding a nanocurrent-channel (NCC) layer between the electrode layer and phase change layer, a RESET power consumption reduction by more than 95% and 10 times faster SET speed were realized simultaneously. Through the first principle calculations, Au and SiO<sub>2</sub> were screened as the metal and insulating matrix material of NCC layer, respectively. Our PCM device with a Au-SiO<sub>2</sub> NCC layer shows an ultralow RESET power consumption, down to 381 fJ, and an ultrafast SET speed (8 ns). Much higher current density near NCC in the phase change layer and thermal barrier effect of insulating matrix material were confirmed by finite element analysis (FEA), and the role of Au nanochannels was revealed by transmission electron microscopy (TEM). Our NCC layer structure provides a simple and practicable method to significantly decrease PCM power consumption.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":10.8,"publicationDate":"2024-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142313539","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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