Nano Letters最新文献_第2页

A Novel Approach to Harnessing Acoustic A-Lines to Detect Circulating Tumor Cells in Flowing Blood. 利用声 A 线检测流动血液中循环肿瘤细胞的新方法。

IF 9.6 1区材料科学

Nano Letters Pub Date : 2024-11-18 DOI: 10.1021/acs.nanolett.4c03982

Shu Kang, Stephen Skapek, Sunil Krishnan, Sanjiv S Gambhir, Yushun Zeng, Qifa Zhou, Raiyan Zaman

引用次数: 0

Engineering Two-Dimensional Magnetic Heterostructures: A Theoretical Perspective. 二维磁性异质结构工程：理论视角。

IF 9.6 1区材料科学

Nano Letters Pub Date : 2024-11-18 DOI: 10.1021/acs.nanolett.4c04251

Jinbo Pan, Yan-Fang Zhang, Yu-Yang Zhang, Shixuan Du

{"title":"Engineering Two-Dimensional Magnetic Heterostructures: A Theoretical Perspective.","authors":"Jinbo Pan, Yan-Fang Zhang, Yu-Yang Zhang, Shixuan Du","doi":"10.1021/acs.nanolett.4c04251","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c04251","url":null,"abstract":"Two-dimensional (2D) magnetic materials have attracted great attention due to their promise for applications in future high-speed, low-energy quantum computing and memory devices. By integrating 2D magnetic materials with other magnetic or nonmagnetic materials to form heterostructures, the synergistic effects of interlayer orbital hybridization, spin-orbit coupling, and symmetry breaking can surpass the performance of single-layer materials and lead to novel physical phenomena. This review provides a comprehensive theoretical analysis of engineering 2D magnetic heterostructures, emphasizing the fundamental physics of interlayer interactions and the resulting enhancements and novel properties. It reviews the mechanisms and progress in tuning the magnetic ordering, enhancing the Curie temperature (Tc) and modulating properties such as topological magnetic structures, spin polarization, electronic band topology, valley polarization, and magnetoelectric coupling through the construction of 2D magnetic heterostructures. Additionally, this review discusses the current challenges faced by 2D magnetic heterostructures, aiming to guide the future design of higher-performance magnetic heterostructures.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":" ","pages":""},"PeriodicalIF":9.6,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142646503","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Regulating Li2S Deposition and Accelerating Conversion Kinetics through Intracavity ZnS toward Low-Temperature Lithium–Sulfur Batteries 通过腔内 ZnS 调节 Li2S 沉积并加速转换动力学，实现低温锂硫电池的目标

IF 10.8 1区材料科学

Nano Letters Pub Date : 2024-11-15 DOI: 10.1021/acs.nanolett.4c04427

Hao Ding, Zhonghui Chen, Huiyu Li, Huadong Suo, Chaozhong Liu, Huanan Yu, Jingkun Yuan, Zixu Sun, Yanyan Zhu, Bo Song

{"title":"Regulating Li2S Deposition and Accelerating Conversion Kinetics through Intracavity ZnS toward Low-Temperature Lithium–Sulfur Batteries","authors":"Hao Ding, Zhonghui Chen, Huiyu Li, Huadong Suo, Chaozhong Liu, Huanan Yu, Jingkun Yuan, Zixu Sun, Yanyan Zhu, Bo Song","doi":"10.1021/acs.nanolett.4c04427","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c04427","url":null,"abstract":"The uncontrolled deposition behavior and sluggish conversion kinetics of the discharging product (solid Li2S) severely deteriorate the electrochemical performance of lithium–sulfur (Li–S) batteries, especially under high S loading and low-temperature conditions. Herein, a multifunctional S cathode host consisting of ZnS nanoparticles (NPs) confined in hollow porous carbon spheres (ZnS@HPCS) is synthesized via a unique capillary force-driven melting-diffusion strategy. The porous carbon shell of ZnS@HPCS provides a space-confined reservoir for soluble polysulfides and solid Li2S, while the intracavity ZnS NPs trap polysulfides, induce Li2S inside deposition, and accelerate conversion kinetics. Thus, Li–S batteries with ZnS@HPCS-S cathodes exhibit excellent electrochemical performance at both room and low temperatures (−40 °C) and high reversible capacities under high S loading (5.2 mg cm–2). Furthermore, Li2S nucleation/deposition, in situ Raman, and theoretical analyses reveal the underlying mechanism. This work offers fundamental insights into regulating Li2S deposition and designing S hosts for high-performance Li–S batteries.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"128 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2024-11-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142637848","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Nanoscale Mapping of Carrier Distribution Regulated by Polarization in 2D FeFETs. 二维铁氧体场效应晶体管中受极化调控的载流子分布的纳米级绘图。

IF 9.6 1区材料科学

Nano Letters Pub Date : 2024-11-15 DOI: 10.1021/acs.nanolett.4c03962

Shengyao Su, Yingli Zhang, Fengyuan Zhang, Chuanlai Ren, Longji Lyu, Mengkang Xu, Changjian Li, Boyuan Huang

引用次数: 0

Time-Domain-Filtered Terahertz Nanoscopy of Intrinsic Light–Matter Interactions 时域滤波太赫兹纳米镜观察光与物质的内在相互作用

IF 10.8 1区材料科学

Nano Letters Pub Date : 2024-11-15 DOI: 10.1021/acs.nanolett.4c03715

Xiaoqiuyan Zhang, Xin Zhang, Zhuocheng Zhang, Tianyu Zhang, Xingxing Xu, Fu Tang, Jing Yang, Jiakun Wang, Hui Jiang, Zhaoyun Duan, Yanyu Wei, Yubin Gong, Hui Zhang, Peining Li, Min Hu

{"title":"Time-Domain-Filtered Terahertz Nanoscopy of Intrinsic Light–Matter Interactions","authors":"Xiaoqiuyan Zhang, Xin Zhang, Zhuocheng Zhang, Tianyu Zhang, Xingxing Xu, Fu Tang, Jing Yang, Jiakun Wang, Hui Jiang, Zhaoyun Duan, Yanyu Wei, Yubin Gong, Hui Zhang, Peining Li, Min Hu","doi":"10.1021/acs.nanolett.4c03715","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03715","url":null,"abstract":"Terahertz (THz) technology holds great potential across diverse applications, including biosensing and information communications, but conventional far-field techniques are limited by diffraction. Near-field optical microscopy overcomes this barrier through a sharp tip that concentrates incident THz waves into nanometric volumes, detecting scattered near-field to reveal nanoscale optical properties. However, owing to the large THz wavelengths, resonant surface waves arising on the tip and cantilever obscure the intrinsic response. Here we combine near-field microscopy with THz time-domain spectroscopy and implement time-domain filtering with an elongated cantilever to eliminate this artifact, achieving intrinsic nanospectroscopy and nanoimaging. By applying this technique, we distinguish and characterize historical pigments of an ancient sculpture, such as vermilion and red lead, on the nanoscale. We also unravel deep-subwavelength localized resonance modes in THz optical antennas, demonstrating capabilities for THz nanophotonics. Our work advances THz nanoimaging and nanospectroscopy techniques to probe intrinsic nanoscale THz light-matter interactions.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"62 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2024-11-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142637659","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Self-Rectifying Memristor-Based Reservoir Computing for Real-Time Intrusion Detection in Cybersecurity. 基于自整流 Memristor 的水库计算用于网络安全中的实时入侵检测。

IF 9.6 1区材料科学

Nano Letters Pub Date : 2024-11-15 DOI: 10.1021/acs.nanolett.4c04385

Guobin Zhang, Zijian Wang, Xuemeng Fan, Pengtao Li, Dawei Gao, Zhenyong Zhang, Qing Wan, Yishu Zhang

引用次数: 0

Water-Vapor-Triggered Dual-Mode Optical Responses in Rare-Earth-Doped Hollow Nanospheres. 稀土掺杂空心纳米球中的水蒸气触发双模光学响应

IF 9.6 1区材料科学

Nano Letters Pub Date : 2024-11-15 DOI: 10.1021/acs.nanolett.4c03714

Hongji Huang, Zixian Chen, Hanqi Zheng, Yingyi Ou, Jianing Zhang, Kang Xiao, Jinqing Huang, Zhao-Qing Liu, Yibo Chen

{"title":"Water-Vapor-Triggered Dual-Mode Optical Responses in Rare-Earth-Doped Hollow Nanospheres.","authors":"Hongji Huang, Zixian Chen, Hanqi Zheng, Yingyi Ou, Jianing Zhang, Kang Xiao, Jinqing Huang, Zhao-Qing Liu, Yibo Chen","doi":"10.1021/acs.nanolett.4c03714","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c03714","url":null,"abstract":"Multimode responsive optical materials are garnering ever-increasing attention due to their diverse applications. This work showcases a film assembled with rare-earth-doped CaF2 hollow nanospheres that exhibit water-vapor-triggered dual-mode optical responses. Upon exposure to flowing water vapor, the film rapidly (less than 1.5 s for a 7.7 μm thickness) transitions to a transparent state and simultaneously undergoes a sharp decrease in the photoluminescence intensity. Both of these changes fully reverse upon water evaporation, demonstrating an impressive reversibility over at least 200 cycles. The water-vapor-induced dual-mode responses are attributed to the altered incident light propagation path stemming from the similar refractive indices between CaF2 and water, coupled with the water-induced energy loss of the rare-earth ions. The fabrication of encryption patterns displaying separate signals in multiple channels, as well as the demonstration of noncontact sensing for water vapor distribution, underscore the promising application potential of this dual-mode responsive system.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":" ","pages":""},"PeriodicalIF":9.6,"publicationDate":"2024-11-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142638129","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Highly Monodisperse Stable Gold Nanorod Powder for Optical Sensor 用于光学传感器的高单分散稳定金纳米棒粉末

IF 10.8 1区材料科学

Nano Letters Pub Date : 2024-11-15 DOI: 10.1021/acs.nanolett.4c04640

Zhiyang Zhang, Yanzhou Wu, Xin Cao, Junpeng Gao, Shuoyang Yan, Shuang Su, Yixuan Wu, Na Zhou, Xiaoyan Wang, Lingxin Chen

{"title":"Highly Monodisperse Stable Gold Nanorod Powder for Optical Sensor","authors":"Zhiyang Zhang, Yanzhou Wu, Xin Cao, Junpeng Gao, Shuoyang Yan, Shuang Su, Yixuan Wu, Na Zhou, Xiaoyan Wang, Lingxin Chen","doi":"10.1021/acs.nanolett.4c04640","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c04640","url":null,"abstract":"Gold nanorods (GNRs) as plasmonic metal nanoparticles are valuable for optical applications due to their tunable plasmonic properties. However, conventional colloidal GNRs face significant optical instability during storage, which limits their practical use. In this work, we developed a highly dispersible GNR powder using an octadecyl trimethylammonium bromide (C18TAB)-assisted freeze-drying method, preserving the optical and chemical sensing properties of GNRs for over 4 months. Compared with C16TAB, C18TAB significantly enhances the GNRs dispersibility even at lower concentrations. Our study demonstrates that C18TAB forms a sponge-like crystal structure that prevents aggregation during the freeze-drying process. The resulting GNR powder retains its plasmonic features and water dispersibility, achieving near-identical optical properties to those of fresh GNR solutions. This stability enabled creation of a liquid-free colorimetric test kit with a long shelf life. This work marks a significant step forward in the use of GNRs as standard analytical reagents, opening new avenues for real-world applications.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"21 1","pages":""},"PeriodicalIF":10.8,"publicationDate":"2024-11-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142637657","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Identifying the Role of Interfacial Long-Range Order in Regulating the Solid Electrolyte Interphase in Lithium Metal Batteries. 确定界面长程有序性在调节锂金属电池固态电解质相间中的作用。

IF 9.6 1区材料科学

Nano Letters Pub Date : 2024-11-15 DOI: 10.1021/acs.nanolett.4c04018

Xiaohan Cai, Hao Xu, Cong Ma, Jiale Zheng, Ke Yue, Juxin Yue, Yao Wang, Jianwei Nai, Jianmin Luo, Huadong Yuan, Shihui Zou, Xinyong Tao, Yujing Liu

{"title":"Identifying the Role of Interfacial Long-Range Order in Regulating the Solid Electrolyte Interphase in Lithium Metal Batteries.","authors":"Xiaohan Cai, Hao Xu, Cong Ma, Jiale Zheng, Ke Yue, Juxin Yue, Yao Wang, Jianwei Nai, Jianmin Luo, Huadong Yuan, Shihui Zou, Xinyong Tao, Yujing Liu","doi":"10.1021/acs.nanolett.4c04018","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c04018","url":null,"abstract":"The self-assembled monolayer (SAM) technique, known for its customizable molecular segments and active end groups, is widely recognized as a powerful tool for regulating the interfacial properties of high-energy-density lithium metal batteries. However, it remains unclear how the degree of long-range order in SAMs affects the solid electrolyte interphase (SEI). In this study, we precisely controlled the hydrolysis of silanes to construct monolayers with varying degrees of long-range order and investigated their effects on the SEI nanostructure and lithium anode performance. The results indicate that the degree of long-range order in SAMs significantly influences the decomposition kinetics of the carbon-fluorine bond in lithium bis(trifluoromethanesulfonyl)imide (LiTFSI), promoting the formation of a LiF-rich SEI and profoundly affecting the long-term stability of the highly sensitive anode during electrochemical processes. These findings provide new insights and directions for the molecular design of SAMs tailored for long-lasting lithium metal interfaces.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":" ","pages":""},"PeriodicalIF":9.6,"publicationDate":"2024-11-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142638122","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

High-Performance Radiative Cooling Sunscreen 高性能辐射冷却防晒霜

IF 10.8 1区材料科学

Nano Letters Pub Date : 2024-11-15 DOI: 10.1021/acs.nanolett.4c04969

Jiaqi Xu, Xueke Wu, Yunrui Li, Siming Zhao, Fan Lan, Aike Xi, Ya Huang, Yilin Ding, Rufan Zhang

引用次数: 0