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Advanced electrode materials for microbial extracellular electron transfer 用于微生物细胞外电子传递的先进电极材料
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-02-22 DOI: 10.1016/j.trechm.2024.01.005
Shriya Grover, Lucinda Elizabeth Doyle
{"title":"Advanced electrode materials for microbial extracellular electron transfer","authors":"Shriya Grover, Lucinda Elizabeth Doyle","doi":"10.1016/j.trechm.2024.01.005","DOIUrl":"https://doi.org/10.1016/j.trechm.2024.01.005","url":null,"abstract":"Bioelectrochemical systems using electroactive microorganisms have applications including energy generation, microbial electrosynthesis, electrofermentation, and biosensing. Enhancing extracellular electron transfer (EET) between microorganisms and electrodes in these systems is a rapidly evolving field. This Review presents recent and emerging advances in the development of novel electrode materials, including incorporation of conductive polymers (CPs), common nanomaterials, MXenes, and metal–organic frameworks (MOFs) to increase the conductivity and surface area available for microbial electrochemical reactions. We also discuss electrodes of the future, focusing on computational rational design and approaches that consider the microorganisms’ perspective in the design process. These include patterning to achieve biologically relevant surface architecture and mimicking the extracellular matrix to form artificial biofilms.","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"96 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-02-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139951530","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Semiconductor cooperative photocatalysis with TEMPO 使用 TEMPO 的半导体协同光催化技术
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-02-20 DOI: 10.1016/j.trechm.2024.01.002
Fengwei Huang, Fulin Zhang, Yuexin Wang, Xianjun Lang
{"title":"Semiconductor cooperative photocatalysis with TEMPO","authors":"Fengwei Huang, Fulin Zhang, Yuexin Wang, Xianjun Lang","doi":"10.1016/j.trechm.2024.01.002","DOIUrl":"https://doi.org/10.1016/j.trechm.2024.01.002","url":null,"abstract":"","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"50 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139926224","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Subscription and Copyright Information 订阅和版权信息
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-02-14 DOI: 10.1016/s2589-5974(24)00012-1
{"title":"Subscription and Copyright Information","authors":"","doi":"10.1016/s2589-5974(24)00012-1","DOIUrl":"https://doi.org/10.1016/s2589-5974(24)00012-1","url":null,"abstract":"","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"12 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-02-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139926210","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advisory Board and Contents 咨询委员会和内容
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-02-14 DOI: 10.1016/s2589-5974(24)00009-1
{"title":"Advisory Board and Contents","authors":"","doi":"10.1016/s2589-5974(24)00009-1","DOIUrl":"https://doi.org/10.1016/s2589-5974(24)00009-1","url":null,"abstract":"","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"34 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-02-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139926214","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Emerging green approaches for valorization of plastics with saturated carbon backbones 对具有饱和碳骨架的塑料进行价值评估的新兴绿色方法
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-02-05 DOI: 10.1016/j.trechm.2024.01.001
Bao-Nguyen T. Nguyen, Jason Y.C. Lim
{"title":"Emerging green approaches for valorization of plastics with saturated carbon backbones","authors":"Bao-Nguyen T. Nguyen, Jason Y.C. Lim","doi":"10.1016/j.trechm.2024.01.001","DOIUrl":"https://doi.org/10.1016/j.trechm.2024.01.001","url":null,"abstract":"<p>Plastics possess highly unsustainable linear life cycles that are environmentally damaging. With low recycling rates worldwide, plastics upcycling is emerging as a promising alternative by using these abundant waste products as chemical feedstock for the production of materials and essential chemicals of higher economic value. However, the saturated C–C polymer backbones of polymers constituting ~60% of all plastic waste are unreactive and challenging to upcycle, often necessitating energy-intensive processes. This review examines state-of-the-art sustainable approaches employing the Principles of Green Chemistry to functionalize or cleave these unreactive polymer backbones, including alternative solvents, Earth-abundant metal catalysis, emerging low-energy approaches, and biocatalysis. Such sustainable strategies will enhance the attractiveness and practical feasibility of plastics upcycling to achieve a circular materials economy.</p>","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"38 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139758908","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Asymmetric radical aziridination of alkenes 烯的不对称自由基氮丙啶化反应
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-01-24 DOI: 10.1016/j.trechm.2023.12.003
Wan-Chen Cindy Lee, X. Peter Zhang
{"title":"Asymmetric radical aziridination of alkenes","authors":"Wan-Chen Cindy Lee, X. Peter Zhang","doi":"10.1016/j.trechm.2023.12.003","DOIUrl":"https://doi.org/10.1016/j.trechm.2023.12.003","url":null,"abstract":"Abstract not available","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"19 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139553195","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Tailoring chemistry for inorganic 3D micro-optics 为无机 3D 微型光学量身定制化学材料
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-01-19 DOI: 10.1016/j.trechm.2023.12.005
J.P. Winczewski, J. Arriaga-Dávila, C. Rosero-Arias, A. Susarrey-Arce
{"title":"Tailoring chemistry for inorganic 3D micro-optics","authors":"J.P. Winczewski, J. Arriaga-Dávila, C. Rosero-Arias, A. Susarrey-Arce","doi":"10.1016/j.trechm.2023.12.005","DOIUrl":"https://doi.org/10.1016/j.trechm.2023.12.005","url":null,"abstract":"<p>Additive manufacturing of metal oxides possesses immense potential in micro-optics, enabling intricate glass and ceramic structures at the highest definition. However, a limited range of inorganic–organic monomeric precursors restrains its advancements. New inorganic–organic precursors should be developed to unlock optical functionalities to manipulate light in the third dimension.</p>","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"23 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-01-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139506911","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Harnessing chemical functionality of lignin towards stimuli-responsive materials 利用木质素的化学功能性开发刺激响应材料
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-01-11 DOI: 10.1016/j.trechm.2023.12.001
Yong Zheng, Adrian Moreno, Yiqi Zhang, Mika H. Sipponen, Lin Dai
{"title":"Harnessing chemical functionality of lignin towards stimuli-responsive materials","authors":"Yong Zheng, Adrian Moreno, Yiqi Zhang, Mika H. Sipponen, Lin Dai","doi":"10.1016/j.trechm.2023.12.001","DOIUrl":"https://doi.org/10.1016/j.trechm.2023.12.001","url":null,"abstract":"<p>The mysteries of chemical structures and properties of lignin are gradually being unveiled. In parallel, lignin is gaining ground as a versatile resource for the development of stimuli-responsive materials with environmentally friendly, high-performance, and multifunctional characters. This review focuses on synthesis and mechanisms of lignin-based stimuli-responsive materials, highlighting the chemical structures linked to responses to various different stimuli, such as pH and temperature. We also highlight applications of these materials in drug carriers, bioimaging, shape memory, strain sensors, and substance detection, with the objective to showcase the untapped potential of lignin, challenging the prevailing notion that lignin is merely a by-product of the pulp industry. Finally, we identify challenges and propose future directions for the development of lignin-based stimuli-responsive materials.</p>","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"111 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-01-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139421178","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Converting heterotrophic Saccharomyces cerevisiae to a synthetic methylotroph 将异养型酿酒酵母转化为合成甲基营养体
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-01-10 DOI: 10.1016/j.trechm.2023.12.004
Pan Zhu, Ziqi Zhang, Yufei Li
{"title":"Converting heterotrophic Saccharomyces cerevisiae to a synthetic methylotroph","authors":"Pan Zhu, Ziqi Zhang, Yufei Li","doi":"10.1016/j.trechm.2023.12.004","DOIUrl":"https://doi.org/10.1016/j.trechm.2023.12.004","url":null,"abstract":"<p>It is challenging to convert a non-methylotrophic yeast to a synthetic methylotroph. In a recently described new method, <span>Nielsen, Keasling, Chen, Bai, and coworkers</span><svg aria-label=\"Opens in new window\" focusable=\"false\" height=\"8px\" viewbox=\"0 0 8 8\" width=\"8px\"><path d=\"M1.12949 2.1072V1H7V6.85795H5.89111V2.90281L0.784057 8L0 7.21635L5.11902 2.1072H1.12949Z\"></path></svg> show that <em>Saccharomyces cerevisiae</em> can be engineered to grow solely on methanol, which potentially emerges as a promising platform for one-carbon (C1)-based biomanufacturing.</p>","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"67 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139421403","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advisory Board and Contents 咨询委员会和内容
IF 15.7 2区 化学
Trends in Chemistry Pub Date : 2024-01-10 DOI: 10.1016/s2589-5974(23)00272-1
{"title":"Advisory Board and Contents","authors":"","doi":"10.1016/s2589-5974(23)00272-1","DOIUrl":"https://doi.org/10.1016/s2589-5974(23)00272-1","url":null,"abstract":"Abstract not available","PeriodicalId":48544,"journal":{"name":"Trends in Chemistry","volume":"6 1","pages":""},"PeriodicalIF":15.7,"publicationDate":"2024-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139465060","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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