Progress in Materials Science最新文献_第9页

Advanced strategies to boost sustainable high-rate Ni-rich cathodes toward durable LIBs 先进的策略，促进可持续的高速率富镍阴极到耐用的锂离子电池

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-09-08 DOI: 10.1016/j.pmatsci.2025.101574

Parnaz Asghari , Farshad Boorboor Ajdari , Fereshteh Abbasi , Sasan Rostami , Ali Asghar Sadeghi Ghazvini , Ali Molaei Aghdam

{"title":"Advanced strategies to boost sustainable high-rate Ni-rich cathodes toward durable LIBs","authors":"Parnaz Asghari , Farshad Boorboor Ajdari , Fereshteh Abbasi , Sasan Rostami , Ali Asghar Sadeghi Ghazvini , Ali Molaei Aghdam","doi":"10.1016/j.pmatsci.2025.101574","DOIUrl":"10.1016/j.pmatsci.2025.101574","url":null,"abstract":"<div><div>The rapid rise in demand for high-performance lithium-ion batteries (LIBs) highlights the importance of high-rate nickel-rich cathode materials as a key step toward next-generation LIBs, offering high discharge capacity, increased energy density, stable operating voltage, and cost-effectiveness. However, issues such as cation mixing, side reactions, microcrack formation, and thermal instability limit their rate capability and long-term durability. This review provides a detailed assessment of these challenges. It outlines strategies to overcome them, including surface coating, doping, core–shell structures, full-concentration gradients, and particle or additive engineering. Surface coatings improve surface stability and ion transport, while doping methods, including pillar and gradient doping, reduce cation mixing and strengthen structural stability. Core–shell and full-concentration gradients designs relieve mechanical stress and suppress phase transitions, and advanced particle engineering reduces microcrack formation. Computational tools such as density functional theory and machine learning, together with <em>in-situ</em> characterization, provide valuable insights into degradation mechanisms, enabling more precise material optimization. Importantly, combined and modified approaches that integrate multiple strategies show the greatest potential to address these challenges while maintaining sustainability and scalability. This work clarifies operational mechanisms, aiding researchers in developing advanced high-rate Ni-rich cathode LIBs for future energy storage.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"156 ","pages":"Article 101574"},"PeriodicalIF":40.0,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145017730","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Elaborately designed intelligent responsive sensing materials for development of flexible gas sensors 为开发柔性气体传感器精心设计了智能响应传感材料

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-09-04 DOI: 10.1016/j.pmatsci.2025.101565

Yonghui Deng , Luyang Liu , Yidan Chen , Yu Deng , Jichun Li , Xiaoqing Liu , Yidong Zou , Limin Wu , Wenhe Xie

{"title":"Elaborately designed intelligent responsive sensing materials for development of flexible gas sensors","authors":"Yonghui Deng , Luyang Liu , Yidan Chen , Yu Deng , Jichun Li , Xiaoqing Liu , Yidong Zou , Limin Wu , Wenhe Xie","doi":"10.1016/j.pmatsci.2025.101565","DOIUrl":"10.1016/j.pmatsci.2025.101565","url":null,"abstract":"<div><div>With the development of artificial intelligence and Internet of Things, flexible gas sensors have emerged as vital functional devices by integrating with smart wearable electronics, which exhibit irreplaceable advantages in medical diagnosis, aerospace, environmental remediation, robotics, and electronic skin. The elaborately designed sensing materials are critical to developing high-performance gas sensors in terms of sensitivity, selectivity, stability, and response/recovery dynamics. In addition, to achieve the reliable and consistent operation of the flexible sensing devices, it is essential to ensure an effective and stable integration between sensing materials and device substrates. Consequently, it is distinctly meaningful to comprehensively summarize the design principles and surface properties of gas-sensitive materials in flexible gas sensors. This review originates from the precise synthesis, regulation and structure optimization of sensing materials for flexible gas sensors, and the new concept of “chemical microenvironment” is proposed to elucidate the sensing mechanism from molecular-atomic level. Specifically, various carrier migration models (e.g., electron, proton, ion) and surface/interfacial interaction are highlighted. Finally, the emerging opportunities and challenges in flexible gas sensors are proposed and predicted, aiming to provide insight about the development of flexible gas sensors into the next-generation sensing applications and further satisfy the growing requirements of smart sensors for long-life, biocompatibility, and real-time communication capabilities.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"156 ","pages":"Article 101565"},"PeriodicalIF":40.0,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144995178","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Recent advances and remaining challenges of solid-state electrolytes for lithium batteries 锂电池固态电解质的最新进展与挑战

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-08-30 DOI: 10.1016/j.pmatsci.2025.101559

Qing Qiao , Yingxue Li , Chang Song , Mariyam Niyaz , Yang Zhang , Songqiang Zhu , Tengfei Zhang , Weiming Teng , Hongge Pan , Xuebin Yu

{"title":"Recent advances and remaining challenges of solid-state electrolytes for lithium batteries","authors":"Qing Qiao , Yingxue Li , Chang Song , Mariyam Niyaz , Yang Zhang , Songqiang Zhu , Tengfei Zhang , Weiming Teng , Hongge Pan , Xuebin Yu","doi":"10.1016/j.pmatsci.2025.101559","DOIUrl":"10.1016/j.pmatsci.2025.101559","url":null,"abstract":"<div><div>All-solid-state lithium batteries (ASSLBs) have garnered significant attention as a next-generation energy storage technology, providing superior safety, enhanced stability, and high energy density. However, current research predominantly remains confined to laboratory-scale demonstrations, with limited translation into scalable technological solutions. Addressing this academia-industry disconnect is critical to unlocking the commercial viability of ASSLBs. This review focuses on bridging this gap by systematically analyzing advancements in solid-state electrolytes (SSEs)—the cornerstone of ASSLB technology. We delve into the structural characteristics, ion transport mechanisms, and performance metrics of various SSEs, alongside a comprehensive summary of modification strategies. Beyond theoretical advancements, we emphasize the practical implications of these strategies in addressing energy density limitations, interfacial instability, and safety concerns. A distinctive feature of this review lies in its multidimensional analysis of early-stage ASSLB industrialization hurdles, integrating perspectives from materials synthesis scalability, electrode processing innovations, device-level performance validation, advanced characterization methodologies, and application-specific requirements. This work not only maps current research frontiers but also establishes actionable guidelines for academia–industry collaboration, offering scientists a roadmap for targeted innovation and equipping enterprises with evidence-based insights to streamline technology development and commercialization strategies.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"156 ","pages":"Article 101559"},"PeriodicalIF":40.0,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144920904","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Corrigendum to “Progress in recent sustainable materials for greenhouse gas (NOx and SOx) emission mitigation”. [Prog. Mater. Sci. 132 (2023) 101033] “减少温室气体（氮氧化物和硫氧化物）排放的近期可持续材料的进展”的勘误。[掠夺。板牙。科学通报，132 (2023)101033]

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-09-21 DOI: 10.1016/j.pmatsci.2025.101566

Aminul Islam , Siow Hwa Teo , Chi Huey Ng , Yun Hin Taufiq-Yap , Shean Yaw Thomas Choong , Md. Rabiul Awual

引用次数: 0

Towards preferential lithium recovery from spent lithium-ion batteries: phase transition mechanisms, technical innovation and future perspectives 从废锂离子电池中优先回收锂：相变机制、技术创新和未来展望

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-08-22 DOI: 10.1016/j.pmatsci.2025.101557

Mengyu Lin , Yongqiang Chen , Chengyan Wang , Shengming Xu , Jialiang Zhang

{"title":"Towards preferential lithium recovery from spent lithium-ion batteries: phase transition mechanisms, technical innovation and future perspectives","authors":"Mengyu Lin , Yongqiang Chen , Chengyan Wang , Shengming Xu , Jialiang Zhang","doi":"10.1016/j.pmatsci.2025.101557","DOIUrl":"10.1016/j.pmatsci.2025.101557","url":null,"abstract":"<div><div>Lithium is an indispensable element for the sustainable development of the new energy industry. However, the strong market demand for LIBs has led to a shortage of lithium resources. Recycling lithium from spent LIBs is an effective approach to alleviate the lithium shortage. However, LIBs are all artificially synthesized complex materials, and phase transition is an indispensable pathway to extract lithium selectively and efficiently. The phase transition methods can be divided into two types: lithium selective leaching in the liquid phase and lithium preferential extraction in the solid phase. This review systematically summarizes the available methods for selective lithium recovery and analyzes the phase transition mechanism from a thermodynamic perspective. The environmental impact and economic benefits analysis were presented for selective lithium extraction methods in liquid phase systems. Innovatively, the “reactivity-selectivity principle” was first employed to evaluate the main solid phase transition methods, indicating the importance of phase transition control for higher lithium recovery efficiency and selectivity. Finally, the prospects of lithium recycling development were outlined from four dimensions of technological innovation, entire-process optimization, economical efficiency and environmental friendliness. This review aims to provide references and enlightenment for the efficient recycling of spent LIBs from the perspective of phase transition and assist in the healthy and long-term development of new energy industry.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"156 ","pages":"Article 101557"},"PeriodicalIF":40.0,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144916650","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Advanced fast-charging anode designs for sodium-ion batteries 用于钠离子电池的先进快速充电阳极设计

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-08-29 DOI: 10.1016/j.pmatsci.2025.101564

Jiaxin Wang , Yanling Yang , Jingeng Chen , Xiao-Lei Shi , Yu Sun , Xuefeng Tian , Hao Che , Yuefeng Chen , Zhi-Gang Chen

{"title":"Advanced fast-charging anode designs for sodium-ion batteries","authors":"Jiaxin Wang , Yanling Yang , Jingeng Chen , Xiao-Lei Shi , Yu Sun , Xuefeng Tian , Hao Che , Yuefeng Chen , Zhi-Gang Chen","doi":"10.1016/j.pmatsci.2025.101564","DOIUrl":"10.1016/j.pmatsci.2025.101564","url":null,"abstract":"<div><div>Sodium-ion batteries (SIBs) are emerging as a promising next-generation fast-charging technology due to their abundant raw resources, low cost, and low desolvation energy advantages that are especially beneficial under low-temperature conditions. However, achieving ultra-fast charging (i.e., charging times under 15 min) remains challenging. The kinetics of Na<sup>+</sup> ions are primarily hindered by Na<sup>+</sup> desolvation sluggish, restricted ion transport within the solid electrolyte interphase (SEI), and slow solid-state diffusion in the anode. Moreover, several fundamental challenges, such as significant volume changes during sodiation/desodiation and interfacial chemistry-induced side reactions, are further exacerbated. This review provides a comprehensive analysis of the key factors limiting the fast-charging capability of SIB anodes and outlines targeted optimization strategies, including bulk structure engineering, synergistic electrolyte design, and the controlled formation of favorable SEI layers. Representative case studies are presented to illustrate both the challenges and recent advances. Finally, this review presents future perspectives and potential pathways to guide the rational design of advanced fast-charging anode materials for SIBs.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"156 ","pages":"Article 101564"},"PeriodicalIF":40.0,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144919105","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Regenerated cellulose fibres and their composites: From fundamental properties to advanced applications 再生纤维素纤维及其复合材料：从基本特性到高级应用

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-08-07 DOI: 10.1016/j.pmatsci.2025.101547

Tim Huber , Nina Graupner , Jörg Müssig

{"title":"Regenerated cellulose fibres and their composites: From fundamental properties to advanced applications","authors":"Tim Huber , Nina Graupner , Jörg Müssig","doi":"10.1016/j.pmatsci.2025.101547","DOIUrl":"10.1016/j.pmatsci.2025.101547","url":null,"abstract":"<div><div>Despite their good mechanical properties, especially their toughness, there are hardly any industrial applications for regenerated cellulose fibre-reinforced composites (RCFCs) apart from the classic elastomer applications in the automotive sector (tyres and hoses). The present review demonstrates that although there is some research work dealing with RCFCs, the amount of data is considered to be rather low compared to, e.g., natural fibre-reinforced composites. This review paper provides an overview of different regenerated cellulose fibres (RCFs) and their areas of application, as well as the processing of RCFs into RCFCs. It shows a comprehensive comparison of the mechanical properties of different fibre types and semi-finished products in various polymer matrices, an assessment of biodegradation and durability, and an overview of applications. RCFCs demonstrate significant potential for lightweight construction of composite materials, particularly in applications involving surface loads under bending and high toughness, due to their low density and environmental benefits compared to, e.g., glass fibres. However, further optimisation of stiffness and tensile strength is required to enhance their competitiveness for highly stressed composite materials, while increased attention to material perception is essential for successful product development and market adoption. Further research should be focused on standardising processing methods and achievable properties to transfer the technology to advanced industrial applications.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"156 ","pages":"Article 101547"},"PeriodicalIF":40.0,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144797513","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Corrigendum to “Roadmap for integrating deep eutectic solvents into adsorption processes: A critical review & design blueprint” [Progress Mater. Sci. 154 (2025) 101501] “将深共晶溶剂整合到吸附过程的路线图：一个关键的审查和设计蓝图”的勘误表[进展材料]。科学通报。154 (2025)101501]

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-10-29 DOI: 10.1016/j.pmatsci.2025.101598

Ghaiath Almustafa , Rawan Abu Alwan , Ho Kyong Shon , Jorge Rodriguez , Inas AlNashef

引用次数: 0

Advancing ionic thermoelectric materials for heat recovery 热回收离子热电材料的研究进展

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-09-06 DOI: 10.1016/j.pmatsci.2025.101575

Yifan Wang , Ibrahim Mwamburi Mwakitawa , Hao Yang , Mingyu Song , Qian Huang , Xinzhe Li , Pengchi Zhang , Wei Fang , Lijun Hu , Yongli Zhou , Chen Li , Jianyong Ouyang , Kuan Sun

{"title":"Advancing ionic thermoelectric materials for heat recovery","authors":"Yifan Wang , Ibrahim Mwamburi Mwakitawa , Hao Yang , Mingyu Song , Qian Huang , Xinzhe Li , Pengchi Zhang , Wei Fang , Lijun Hu , Yongli Zhou , Chen Li , Jianyong Ouyang , Kuan Sun","doi":"10.1016/j.pmatsci.2025.101575","DOIUrl":"10.1016/j.pmatsci.2025.101575","url":null,"abstract":"<div><div>Ionic thermoelectrics (i-TEs) are emerging as a promising, sustainable technology for low-grade heat recovery, notable for their absence of moving mechanical parts. In recent years, significant advancements in i-TE materials and devices have been propelled by their advantages in thermal power generation, compatibility with room-temperature operation, and potential for integration into flexible, wearable devices. However, challenges remain to be addressed for practical future applications, primarily due to insufficient evaluations of innovative operational modes and materials. This review aims to bridge this gap by summarizing key existing theories and providing an in-depth analysis of ion migration mechanisms within i-TE capacitors. We also highlight significant contributions from leading studies, focusing on material selection, operational modes, performance characteristics, and pivotal discoveries. Ultimately, this review seeks to identify transformative approaches in i-TEs to foster innovative designs for practical applications.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"156 ","pages":"Article 101575"},"PeriodicalIF":40.0,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145007200","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Progress in cathode materials for rechargeable Zinc-Ion batteries: from inorganic and organic systems to hybrid frameworks and biomass-derived innovations 可充电锌离子电池正极材料的进展：从无机和有机系统到混合框架和生物质衍生的创新

IF 4 1区材料科学

Progress in Materials Science Pub Date : 2026-02-01 Epub Date: 2025-07-31 DOI: 10.1016/j.pmatsci.2025.101543

Amjad Ali , Jamile Mohammadi Moradian , Ahmad Naveed , Shu Zhang , Mudassir Hussain Tahir , Khurram Shehzad , Mika Sillanpää

{"title":"Progress in cathode materials for rechargeable Zinc-Ion batteries: from inorganic and organic systems to hybrid frameworks and biomass-derived innovations","authors":"Amjad Ali , Jamile Mohammadi Moradian , Ahmad Naveed , Shu Zhang , Mudassir Hussain Tahir , Khurram Shehzad , Mika Sillanpää","doi":"10.1016/j.pmatsci.2025.101543","DOIUrl":"10.1016/j.pmatsci.2025.101543","url":null,"abstract":"<div><div>Zinc-ion batteries (ZIBs) have gained significant attention as promising candidates for large-scale energy storage systems owing to their low cost, environmental friendliness, and inherent safety, and have become a key focus of both academic research and industrial development strategies. However, significant challenges must be resolved, such as suboptimal charge kinetics, inadequate electrode structural stability, and complicated and costly manufacturing methods, prior to achieving meaningful advancements. Building on this foundation, this review offers a comprehensive overview of electrode materials, beginning with the fundamental factors that influence their electrochemical performance, such as electronic conductivity, ion diffusion pathways, structural stability, redox activity, and surface/interface characteristics. A clear understanding of these parameters is essential for guiding the rational design and optimization of high-performance electrodes for ZIBs. Secondly, we critically assess the current progress, identify persistent limitations, and explore potential strategies to overcome the challenges in achieving long-term cycling stability and fast reaction kinetics. Detailed analyses of structural engineering approaches, electrochemical behavior, and zinc-ion storage mechanisms across diverse material systems are presented to provide deep insights into the design principles driving next-generation AZB development. Finally, we also included a comprehensive outlook on the future development of ZIBs by identifying critical challenges and promising opportunities to drive their rapid progress and extensive practical deployment in the field.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"156 ","pages":"Article 101543"},"PeriodicalIF":40.0,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144756495","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0