Peiyu Luo , Xin Zhang , Yihe Yue , Zhuohang Wang , Changsong Shi , Zhiyang Lyu
{"title":"Directional freeze-casting of aerogels: Structure, properties, and applications","authors":"Peiyu Luo , Xin Zhang , Yihe Yue , Zhuohang Wang , Changsong Shi , Zhiyang Lyu","doi":"10.1016/j.mser.2025.101173","DOIUrl":"10.1016/j.mser.2025.101173","url":null,"abstract":"<div><div>Aerogels are a class of lightweight, porous materials with high porosity and large specific surface area, making them promising candidates for applications in thermal insulation, energy storage, environmental remediation, catalysis, and biomedical engineering. However, conventional aerogels exhibit isotropic pore structure, limited mechanical robustness, and poor control over multiscale structures, which constrain their broader development and applications. Directional freeze-casting (DFC) has emerged as an efficient strategy to address these challenges by regulating ice crystal growth to form directionally aligned micro/nanostructures. When applied to aerogel fabrication, this technique can impart anisotropic features and significantly enhance overall performance. This review systematically summarizes recent advances in the fabrication of aerogels using various DFC approaches, including unidirectional, bidirectional, radial, and physical field-assisted techniques. It further highlights how these approaches enable precise structural control, performance enhancement, and functional optimization across diverse material platforms, including carbon-, ceramic-, polymer-, MXene-, and metal-based aerogels. Finally, current challenges and future research directions are discussed, providing new insights for the continued development of uniquely structured and high-performance aerogels.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"168 ","pages":"Article 101173"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145836427","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Mohammad Reza Gholizadeh , Hossein Roghani-Mamaqani , Vahid Haddadi-Asl
{"title":"Sustainable polymers: Recycling and reprocessing mechanisms using reversible and dynamic covalent bonds","authors":"Mohammad Reza Gholizadeh , Hossein Roghani-Mamaqani , Vahid Haddadi-Asl","doi":"10.1016/j.mser.2025.101174","DOIUrl":"10.1016/j.mser.2025.101174","url":null,"abstract":"<div><div>One of the most critical challenges facing human societies is environmental pollution resulting from the excessive use of polymeric materials and the adherence of their consumption patterns to the linear economy model. To address these challenges, sustainable polymers have garnered significant attention because they can be recycled, composted, or biodegraded at the end of their life cycle, while also demonstrating reduced environmental impact throughout their lifespan. Self-immolative polymers, degradable polymers, and reprocessable polymers are different types of sustainable polymers that have emerged as particularly promising candidates owing to the presence of reversible and dynamic bonds in their structures. Accordingly, this review begins by exploring polymer recycling methods and then discusses sustainable polymers, with a particular focus on the incorporation of reversible and dynamic chemistry into these materials. Reversible covalent bonds are broken and formed by induction of different stimuli or different states of one stimulus. Dynamic chemistry provides powerful molecular tools for designing constitutionally dynamic materials capable of self-healing, adaptation, reprocessing, and recycling. Dynamic covalent bonds (DCBs) are divided into five groups (pH-, redox-, photo-, thermal-, and mechano-responsive linkages) based on their responsiveness to external stimuli and are discussed in detail. Additionally, this review highlights emerging technologies, such as light-based 3D printing, printable vitrimers, and sustainable foams, rubbers, and adhesives, that incorporate reversible or dynamic covalent chemistries into integrated systems, opening new avenues across diverse scientific fields. Finally, the review addresses current challenges and future opportunities, emphasizing the transformative potential of reversible or dynamic covalent polymers in advancing a more sustainable polymer industry.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"168 ","pages":"Article 101174"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145836421","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yifei Pei , Jiaming Zhang , Mengya Guo , Jianhui Zhao , Liyu Wang , Jisiqi Chen , Xiaobing Yan
{"title":"Low-dimensional optoelectronic memristors: From quantum confinement to neuromorphic vision","authors":"Yifei Pei , Jiaming Zhang , Mengya Guo , Jianhui Zhao , Liyu Wang , Jisiqi Chen , Xiaobing Yan","doi":"10.1016/j.mser.2025.101115","DOIUrl":"10.1016/j.mser.2025.101115","url":null,"abstract":"<div><div>The von Neumann architecture's inherent separation of memory and computation has become a critical bottleneck in the era of big data, driving the search for integrated computing-memory solutions. Memristors, with their intrinsic ability to unify storage and processing, have emerged as a transformative platform. The exceptional physical properties of low-dimensional materials have played a critical role in this progress, enabling unprecedented device miniaturization, increased storage density, and tunable optoelectronic functionality through their outstanding electronic, optical, and quantum characteristics. This review explores the pivotal role of low-dimensional materials in revolutionizing optoelectronic memristors, focusing on their quantum confinement effects, tunable optoelectronic properties, and neuromorphic applications. We systematically analyze how 0D quantum dots enable light-modulated conductive pathways through precise carrier trapping, 1D nanowires leverage anisotropic charge transport for ultrafast photoresponse, and 2D materials facilitate heterostructure engineering to enhance switching stability. We then deeply analyze the transformative impact of optoelectronic memristors based on low-dimensional materials in neuromorphic computing, particularly their remarkable advantages in simulating complex synaptic dynamics and developing low-energy artificial vision systems. Finally, we specifically outline future research directions, focusing on overcoming bottlenecks in the precise synthesis and scalable fabrication of low-dimensional materials, and leveraging their exceptional optoelectronic properties and tunable quantum characteristics to emulate more intricate synaptic dynamics, thereby bridging the gap between electronic and biological systems. These efforts aim to amplify the role of optoelectronic memristors in future neuromorphic computing and highly integrated chip applications.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"167 ","pages":"Article 101115"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145026848","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Navakoteswara Rao Vempuluru , Yeongjun Yoon , Jyoti Prakash Das , Vijayakumar Elumalai , Anandhan Ayyappan Saj , Hanna Lee , Tae Kyu Kim , Kyeounghak Kim , Arunprasath Sathyaseelan , Perumalsamy Muthukumar , Sang-Jae Kim
{"title":"Nanocluster catalyst driving ampere-level current density in direct seawater electrolysis quantum leap towards sustainable energy","authors":"Navakoteswara Rao Vempuluru , Yeongjun Yoon , Jyoti Prakash Das , Vijayakumar Elumalai , Anandhan Ayyappan Saj , Hanna Lee , Tae Kyu Kim , Kyeounghak Kim , Arunprasath Sathyaseelan , Perumalsamy Muthukumar , Sang-Jae Kim","doi":"10.1016/j.mser.2025.101092","DOIUrl":"10.1016/j.mser.2025.101092","url":null,"abstract":"<div><div>Direct seawater electrolysis offers a promising route for sustainable hydrogen production, but challenges such as chloride corrosion, high overpotentials, and catalyst instability hinder its scalability. Here, we present a surface-engineered Cu-Ni bimetallic nanocluster catalyst anchored on Ti₃C₂Tₓ MXene via a facile polyvinylpyrrolidone (PVP)-assisted synthesis method. This pioneering design leverages the terminal functional groups (Tx = F, OH, O) of MXene to enhance metal-substrate interactions, optimize intermediate adsorption, and minimize the chloride ions adsorption, enabling efficient and durable seawater splitting. The catalyst achieves ultralow overpotentials of 29 mV (HER) and 250 mV (OER) in ultrapure water, and 49 mV (HER) and 290 mV (OER) in natural seawater at 10 mA cm⁻², closely compute with precious metal-based systems. Remarkably, it delivers a significant current density of 1.5 A cm⁻² at 2.4 V (60 °C) in an anion-exchange membrane (AEM) electrolyzer, demonstrating its potential for industrial-scale hydrogen production. The engineered surface resists chloride-induced corrosion and maintains stability for > 100 h at 100 mA cm⁻² and 70 h at 1000 mA cm⁻² in alkaline seawater. Combined experimental and density functional theory (DFT) analyses reveal the synergistic effects of Cu-Ni nanoclusters and Ti₃C₂Tₓ, elucidating the mechanisms behind enhanced reaction kinetics and durability by In-situ Raman and anticorrosion insights. The scalable, low-cost synthesis method, coupled with seamless integration into photovoltaic-electrolysis systems, achieves a remarkable rate of 1.42 mL/min of H<sub>2</sub> production. This work provides a transformative pathway for sustainable hydrogen production from seawater, addressing global energy and environmental challenges while advancing the fundamental understanding of electrocatalysis.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"167 ","pages":"Article 101092"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144926040","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yuanxi Chang , Yan Jia , Yansong Pan , Jin Wang , Hongrui Yang , Mei Zu , Haifeng Cheng
{"title":"Enhancing water retention in hydrogels under extreme conditions: Strategies, applications and challenges","authors":"Yuanxi Chang , Yan Jia , Yansong Pan , Jin Wang , Hongrui Yang , Mei Zu , Haifeng Cheng","doi":"10.1016/j.mser.2025.101098","DOIUrl":"10.1016/j.mser.2025.101098","url":null,"abstract":"<div><div>Hydrogels have garnered significant research interest for their versatile applications in biomedical, electronic, and agricultural fields—attributes intrinsically linked to their high-water-content matrices. However, hydrogel functionality frequently deteriorates under environmental conditions due to dehydration/freezing-induced structural damage, resulting in performance degradation. To address this challenge, various strategies have been developed to enhance the water retention of hydrogels, employing diverse mechanisms and targeting a range of applications. In this review, strategies for improving the water retention of hydrogels and their corresponding cutting-edge applications have been systematically described. Firstly, the states and importance of water in hydrogels are articulated. Subsequently, five core strategies are categorized and mechanistically analyzed across multi-scale: encapsulation, solvent optimization, ionic incorporation, structural design, and combination approaches. Then, the applications and developments of hydrogels are highlighted and mainly categorized into three promising candidates, including biomedical (tissue engineering, dressing, biosensing), electronic (electrolyte, sensor, wearable device), and agricultural (water retainer of soil, nutrient release, vertical farming) fields. Finally, current challenges and future research directions for hydrogels are critically assessed, emphasizing the need for comprehensive solutions and strategic advancements to unlock their full potential in diverse applications.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"167 ","pages":"Article 101098"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144932592","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Jinwei Chen , Fanbo Meng , Zhenzhong Yang , Yuxuan Liu , Renzong Hu , Min Zhu
{"title":"Insights into the fundamental interactions within Li-ion battery electrolyte components and the solvation structure-property relationships","authors":"Jinwei Chen , Fanbo Meng , Zhenzhong Yang , Yuxuan Liu , Renzong Hu , Min Zhu","doi":"10.1016/j.mser.2025.101134","DOIUrl":"10.1016/j.mser.2025.101134","url":null,"abstract":"<div><div>As an efficient approach, electrolyte optimization has been extensively studied and leads to significant improvements in battery performance. Compared with the specific formulations, the interactions between electrolyte components and the resulting solvation structures have attracted widespread attention. This is because they provide deep insights into the solvation structure-property relationships of electrolytes. Faced with rapid progress in understanding the various interactions within electrolyte in recent years, it is crucial to promptly summarize these advances in detail and establish a theoretical framework. Such a framework will aid in comprehending the essence behind the performance enhancement of numerous existing formulations and guiding future electrolyte design. In this review, we begin by summarizing the processes related to ion transport and interfacial chemistry in electrolytes, along with their relationship to electrolyte solvation structures. Building on this foundation, detailed analysis is provided on how the various interactions within the electrolyte influence the solvation structure and consequently impact the above two key functions. Furthermore, some conflicting aspects and feasible strategies in interaction regulation are discussed. With a comprehensive and deep understanding of the fundamental interactions and solvation structure-property relationships, bottom-up electrolyte design can be achieved, improving the efficiency and precision of electrolyte development.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"167 ","pages":"Article 101134"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145332892","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Feixiang Huang , Binhong Liu , Yujun Guo , Zixu Yang , Siming Li , Zhe Chen , Shaoxing Qu
{"title":"Photodegradable hydrogels: Connecting network evolution and material properties by a photo-chemo-mechanical coupling model","authors":"Feixiang Huang , Binhong Liu , Yujun Guo , Zixu Yang , Siming Li , Zhe Chen , Shaoxing Qu","doi":"10.1016/j.mser.2025.101116","DOIUrl":"10.1016/j.mser.2025.101116","url":null,"abstract":"<div><div>Degradable hydrogels possess excellent biocompatibility, controllable mechanical properties, and mass transfer capabilities, making them widely applicable in wound dressings, drug delivery, and tissue engineering. By incorporating photo-responsive components into the polymer network, degradable hydrogels can respond to precisely controlled light fields. However, mechanical modeling works on photodegradable hydrogels remain relatively limited. A finite deformation theory coupling photochemical principles is needed to comprehensively describe the mechanical behavior of photodegradable hydrogels. In this study, we developed a photo-chemo-mechanical coupling constitutive model of photodegradable hydrogels within the framework of continuum mechanics. The model involves the photochemical kinetics of the photo-induced degradation process and depicts the evolution of networks in the degradation process using sub-networks, providing a microscopic image more consistent with the degradation mechanism. The model characterizes the changes in mechanical properties and swelling deformation after photodegradation, and corresponding experimental validations are conducted. Building upon this theoretical model, specific recipe compositions and degradation conditions are systematically discussed, and the parameter-property relationships are bridged. This constitutive model reveals the photodegradation mechanism of the hydrogel network at the microscopic level and can predict mechanical behavior at the macroscopic level, guiding the synthesis and application of photodegradable hydrogels.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"167 ","pages":"Article 101116"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145060041","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Jingbo Fan , Yuanyuan Tian , Zhi Kai Ng , Hancen Zhang , Yaqi Zhu , Mao See Wu , Kun Zhou
{"title":"Magnetic-assisted 3D printed bioinspired scaffold for high-performance EMI shielding with low reflection, high mechanical robustness, and excellent thermal conductivity","authors":"Jingbo Fan , Yuanyuan Tian , Zhi Kai Ng , Hancen Zhang , Yaqi Zhu , Mao See Wu , Kun Zhou","doi":"10.1016/j.mser.2025.101132","DOIUrl":"10.1016/j.mser.2025.101132","url":null,"abstract":"<div><div>The rapid advancement of fifth-generation (5 G) technologies has spurred an urgent demand for advanced electromagnetic interference (EMI) shielding materials that combine high shielding effectiveness, low reflection, high mechanical robustness, and excellent thermal conductivity. However, achieving all these properties in a single material remains highly challenging, as the excessive functional fillers required to enhance EMI shielding and thermal conductivity often compromise mechanical integrity. Inspired by the comb-like microstructure of butterfly wing scales, renowned for their vivid structural coloration, excellent thermal conductivity, and mechanical properties, we designed and fabricated a gradient multilayered composite scaffold featuring oriented graphite microplatelets and a gradually varying content of nanoscale zero-valent iron across layers, using the developed magnetic-assisted multi-material 3D printing system. The resulting scaffold demonstrates exceptional EMI shielding performance with a high shielding effectiveness of 65 dB and a low reflectance of 0.26, outperforming many conventional materials in mitigating secondary electromagnetic pollution. Importantly, in addition to excellent thermal conductivity, the scaffold also exhibits outstanding mechanical robustness with a compressive strength of 98.1 MPa and a toughness of 587.4 J/m<sup>3</sup>, outperforming many reported EMI shielding materials. This 3D printed bioinspired scaffold successfully addresses the longstanding trade-off between functional performance and mechanical integrity, offering a novel strategy for developing high-performance EMI shielding materials with great application value in 5 G base station modules, data center servers, and aerospace electronics.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"168 ","pages":"Article 101132"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145475287","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Siyan Pan , Erming Su , Yuxi Wang , Zhenyu Wang , Herbert E. Huppert , Zhong Lin Wang , Leo N.Y. Cao
{"title":"Sustainable soil decontamination via triboelectric-electrokinetic heavy metal removal","authors":"Siyan Pan , Erming Su , Yuxi Wang , Zhenyu Wang , Herbert E. Huppert , Zhong Lin Wang , Leo N.Y. Cao","doi":"10.1016/j.mser.2025.101139","DOIUrl":"10.1016/j.mser.2025.101139","url":null,"abstract":"<div><div>Soil heavy metal pollution poses severe threats to ecosystems and human health. Existing remediation methods suffer from high energy costs and secondary pollution. Here, we developed a wind-driven soft-contact triboelectric nanogenerator (SC-TENG) with a ternary electrode structure to power electrokinetic remediation, achieving efficient energy harvesting from natural wind. The SC-TENG converted 65 µA AC into 10 mA pulsed DC via an energy management circuit, increasing the electric field strength. Within seven days, the system achieved 10.45 % Pb²⁺ and 27.05 % Cd²⁺ removal efficiencies. Remediated soil exhibited 100 % pea seed germination and 42.1 % faster seedling growth compared to untreated soil. This work pioneers self-powered electrokinetic remediation using pulsed DC fields generated entirely from wind energy, offering a sustainable and scalable solution for soil decontamination.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"168 ","pages":"Article 101139"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145475288","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Wonryeol Yang , Wantae Park , Youjin Reo , Soohwan Yoo , Sungjae Cho , Hyesun Kim , Sunmin Ryu , Yong-Young Noh
{"title":"Additive-free thermally evaporated tin halide perovskite transistors","authors":"Wonryeol Yang , Wantae Park , Youjin Reo , Soohwan Yoo , Sungjae Cho , Hyesun Kim , Sunmin Ryu , Yong-Young Noh","doi":"10.1016/j.mser.2025.101141","DOIUrl":"10.1016/j.mser.2025.101141","url":null,"abstract":"<div><div>Tin halide perovskites have emerged as promising p-type semiconductors owing to their low effective mass and high defect tolerance. While early development of perovskite thin-film transistors (TFTs) was achieved by solution processing, their reliance on solvents and poor compatibility with high-resolution patterning hindered large-scale integration. By contrast, thermal evaporation offers a solvent-free approach with precise control over the thickness and composition, making it well-suited for scalable and industry-relevant fabrication. Herein, we report the development of additive-free, thermally evaporated FASnI<sub>3</sub> TFTs and systematically investigate how the deposition method and precursor stoichiometry affect the crystallization behavior and device characteristics. Co-deposition enabled complete precursor conversion and (n00, n = 1,2,3)-oriented crystallization, achieving high mobility of ∼14 cm<sup>2</sup> V<sup>−1</sup> s<sup>−1</sup>, while sequential deposition leads to residual SnI<sub>2</sub>, (111)-oriented crystallization, and relatively low mobility of ∼2 cm<sup>2</sup> V<sup>−1</sup> s<sup>−1</sup>. Notably, these thermally evaporated films enable reliable switching behavior without requiring hole suppressors, owing to the intrinsic control over the carrier concentration. These findings underscore the importance of optimizing the deposition strategy and precursor stoichiometry to achieve high-performance tin halide perovskite TFTs and facilitate their integration into large-area electronic systems.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"168 ","pages":"Article 101141"},"PeriodicalIF":31.6,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145475289","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}