Materials Science and Engineering: R: Reports最新文献

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Bifunctional electrocatalysts for Zn–air batteries: A comprehensive review of design optimization and in-situ characterization 锌空气电池双功能电催化剂:设计优化和原位表征的综合综述
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-28 DOI: 10.1016/j.mser.2025.101058
Jagadis Gautam , Roop L. Mahajan , Seul-Yi Lee , Soo-Jin Park
{"title":"Bifunctional electrocatalysts for Zn–air batteries: A comprehensive review of design optimization and in-situ characterization","authors":"Jagadis Gautam ,&nbsp;Roop L. Mahajan ,&nbsp;Seul-Yi Lee ,&nbsp;Soo-Jin Park","doi":"10.1016/j.mser.2025.101058","DOIUrl":"10.1016/j.mser.2025.101058","url":null,"abstract":"<div><div>Rechargeable Zinc-Air Batteries (ZABs) stand out for their superior energy density, safety, cost-effectiveness, and environmental sustainability, making them a promising energy storage solution. Their performance depends on the oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) at the air electrode but is hindered by sluggish kinetics, limited bifunctionality, precious metal dependence, and corrosion. This review explores cutting-edge bifunctional electrocatalysts, focusing on strategies that enhance ORR and OER activity. It critically examines ZAB fundamentals, reaction mechanisms, and innovations in catalyst design—optimizing micro/nano-architectures, electronic structures, binding energies, and surface properties to improve activity, selectivity, and durability. A detailed analysis of electronic, geometric, and synergistic effects at a microscopic scale sheds light on catalytic performance enhancement. <em>In situ</em> characterization techniques are emphasized to unravel electrode-electrolyte interfacial dynamics, surface reconstruction, and mechanistic pathways. Finally, key challenges and future research directions are outlined, driving the next generation of high-performance ZABs.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101058"},"PeriodicalIF":31.6,"publicationDate":"2025-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144502195","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Interfacial and solvent dehydrogenation engineering enables long-life high-voltage lithium-ion batteries 界面和溶剂脱氢工程实现了长寿命高压锂离子电池
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-27 DOI: 10.1016/j.mser.2025.101051
Said Amzil , Yiyao Xiao , Denghui Ma , Jiapei Li , Tonghui Xu , Zhengzheng Ru , Longhao Cao , Ming Yang , Shengyao Luo , Mengqi Wu , Meilan Peng , Yinghui Li , Shuang Tian , Jie Gao , Ying Yu , Peter Müller-Buschbaum , Tao Cai , Fei Zhao , Qian Li , Ya-Jun Cheng , Yonggao Xia
{"title":"Interfacial and solvent dehydrogenation engineering enables long-life high-voltage lithium-ion batteries","authors":"Said Amzil ,&nbsp;Yiyao Xiao ,&nbsp;Denghui Ma ,&nbsp;Jiapei Li ,&nbsp;Tonghui Xu ,&nbsp;Zhengzheng Ru ,&nbsp;Longhao Cao ,&nbsp;Ming Yang ,&nbsp;Shengyao Luo ,&nbsp;Mengqi Wu ,&nbsp;Meilan Peng ,&nbsp;Yinghui Li ,&nbsp;Shuang Tian ,&nbsp;Jie Gao ,&nbsp;Ying Yu ,&nbsp;Peter Müller-Buschbaum ,&nbsp;Tao Cai ,&nbsp;Fei Zhao ,&nbsp;Qian Li ,&nbsp;Ya-Jun Cheng ,&nbsp;Yonggao Xia","doi":"10.1016/j.mser.2025.101051","DOIUrl":"10.1016/j.mser.2025.101051","url":null,"abstract":"<div><div>High-voltage lithium-ion batteries (LIBs) using LiNi<sub>0.8</sub>Mn<sub>0.1</sub>Co<sub>0.1</sub>O<sub>2</sub> (NCM811) cathode materials present a promising avenue for increasing energy density. However, achieving stable operation at elevated voltages is hindered by chemical instability in ethylene carbonate (EC)-based electrolytes, leading to parasitic interfacial reactions. Herein, we introduce 2-hydroxy-5-nitro-3-(trifluoromethyl) pyridine (HNTFP) as a multifunctional electrolyte additive to mitigate EC dehydrogenation and minimize interfacial side reactions. Leveraging the unique functional groups of HNTFP (NO<sub>2</sub>, CF<sub>3</sub>, and C<img>O), we demonstrate the formation of a robust hybrid/inorganic cathode electrolyte interphase (CEI) on high-voltage cathodes and a fluorine-rich solid electrolyte interphase (SEI) on graphite anodes. These interphases enable 4.5 V-charged NCM811||graphite full cells to achieve a capacity retention of 92 % over 500 cycles, while commercial 1 Ah pouch cells retain 89 % over 1000 cycles. This study provides a fresh perspective on electrolyte additive design and underscores the transformative potential of HNTFP in enabling long-life, high-voltage LIBs with superior stability and performance.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101051"},"PeriodicalIF":31.6,"publicationDate":"2025-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144502194","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
3D printing for all-solid-state batteries 全固态电池的3D打印
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-25 DOI: 10.1016/j.mser.2025.101053
Lutong Wang , Chuang Yi , Jixian Luo , Zhiwei Zhang , Hong Li , Liquan Chen , Fan Wu
{"title":"3D printing for all-solid-state batteries","authors":"Lutong Wang ,&nbsp;Chuang Yi ,&nbsp;Jixian Luo ,&nbsp;Zhiwei Zhang ,&nbsp;Hong Li ,&nbsp;Liquan Chen ,&nbsp;Fan Wu","doi":"10.1016/j.mser.2025.101053","DOIUrl":"10.1016/j.mser.2025.101053","url":null,"abstract":"<div><div>3D printing technology has garnered significant attention due to its capability for precise fabrication of complex battery structures, as well as its advantages of low cost and environmental sustainability. By integrating computer-aided design (CAD) with advanced manufacturing processes, 3D printing enables rapid prototyping, accelerated design, testing, and iteration of novel battery structures. Consequently, a growing number of researchers are exploring the use of 3D printing technology for the production of all-solid-state batteries (ASSBs), presenting new possibilities for breakthroughs in future energy storage technologies. In this review, we discuss the differences between traditional battery manufacturing methods and the application of 3D printing techniques for ASSBs fabrication. The working principles, advantages, and limitations of various 3D printing technologies in solid-state battery production are specifically highlighted, along with the challenges that can be addressed by 3D printing. The perspectives on the future development of 3D printing technology in battery manufacturing are proposed.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101053"},"PeriodicalIF":31.6,"publicationDate":"2025-06-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144469801","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bioinspired, piezoelectrically-actuated deployable miniature robots 仿生,压电驱动可展开的微型机器人
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-20 DOI: 10.1016/j.mser.2025.101054
Hongyi Liu , Jinxin Sun , Yanhu Zhang , Yi Zhang , Chen Chen , Penghong Ci , Shuxiang Dong
{"title":"Bioinspired, piezoelectrically-actuated deployable miniature robots","authors":"Hongyi Liu ,&nbsp;Jinxin Sun ,&nbsp;Yanhu Zhang ,&nbsp;Yi Zhang ,&nbsp;Chen Chen ,&nbsp;Penghong Ci ,&nbsp;Shuxiang Dong","doi":"10.1016/j.mser.2025.101054","DOIUrl":"10.1016/j.mser.2025.101054","url":null,"abstract":"<div><div>The continuous breakthroughs in flexible and intelligent materials have paved the way for flexible devices, which further promote the fast development of flexible, intelligent mini robots. This review systematically investigates the progress of the bioinspired, piezoelectrically actuated deployable miniature robots (BPDMRs), including their structures integrated with piezoelectric materials, bionic working mechanisms and multifunctional control method, manufacturing technology, and application scenarios etc., which have become a research hotspot in the area of microscale robotics. The BPDMRs exhibit the features of flexible, intelligent, and deployable structures, including naturally imitated structures, bioinspired functional structures, and origami structures; while their working mechanisms mainly imitate biological behaviors or biologically inspired motion fashions, including their motion control, energy transmission, implementation functions etc. This review also highlights insights and designing strategy of piezo-actuated robots, the advanced manufacturing technology, and future developing direction. Despite facing technological challenges in enhancing energy efficiency, improving adaptability in extreme environments, and multifunctional integrated control systems, BPDMRs offer promising prospects in the future in performing tasks in special environments, including danger industrial reconnaissance, environmental pollution monitoring, earthquake hazard rescue and survey, and other extreme environment investigations, etc.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101054"},"PeriodicalIF":31.6,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144321959","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bi: A rising star for low-temperature fast-charging sodium-ion batteries 毕:低温快充钠离子电池的后起之秀
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-20 DOI: 10.1016/j.mser.2025.101056
Jie Bai, Hui Ping Li, Yu Fei Zheng, Hong Zhang, Chun Cheng Yang, Qing Jiang
{"title":"Bi: A rising star for low-temperature fast-charging sodium-ion batteries","authors":"Jie Bai,&nbsp;Hui Ping Li,&nbsp;Yu Fei Zheng,&nbsp;Hong Zhang,&nbsp;Chun Cheng Yang,&nbsp;Qing Jiang","doi":"10.1016/j.mser.2025.101056","DOIUrl":"10.1016/j.mser.2025.101056","url":null,"abstract":"<div><div>The rising demand for energy storage, such as electric vehicles in extreme conditions, polar and deep-sea exploration, necessitates batteries with exceptional low-temperature performance. Sodium-ion batteries (SIBs) exhibit wide temperature range adaptability and superior rate capability owing to smaller Stokes radius compared with Li<sup>+</sup>. Bi-based materials are characterized by low cost, moderate reaction potential and high volumetric capacity. In addition, the integration with ether-based electrolyte endows the Bi electrode with a continuous three-dimensional (3D) porous nanostructure, rendering it a promising candidate for fast-charging anode. Nevertheless, the low-temperature capabilities are constrained by a multitude of factors, including sluggish solid-state diffusion, diminished ionic conductivity, and slow Na<sup>+</sup> desolvation kinetics. In this review, the challenges of huge volume expansion and opportunities of high diffusion coefficient intermediate phases for Bi-based materials are highlighted. A series of low-temperature high-performance Bi-based materials are also summarized, along with chemical design strategies tailored to enhance their performance. This review culminates in an overview of the prevailing challenges and prospects for the advancement of Bi-based materials as fast-charging anodes in low-temperature environments.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101056"},"PeriodicalIF":31.6,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144331098","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Angular selective optical metasurfaces: Fundamentals, progress and applications 角选择光学超表面:基本原理、进展与应用
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-19 DOI: 10.1016/j.mser.2025.101055
Yile Fan , Hexiang Han , Pan Wang , Mengqi Zhang , Jin Zhang , Chengyu Xiao , Shaowen Chen , Xing Lou , Di Zhang , Han Zhou
{"title":"Angular selective optical metasurfaces: Fundamentals, progress and applications","authors":"Yile Fan ,&nbsp;Hexiang Han ,&nbsp;Pan Wang ,&nbsp;Mengqi Zhang ,&nbsp;Jin Zhang ,&nbsp;Chengyu Xiao ,&nbsp;Shaowen Chen ,&nbsp;Xing Lou ,&nbsp;Di Zhang ,&nbsp;Han Zhou","doi":"10.1016/j.mser.2025.101055","DOIUrl":"10.1016/j.mser.2025.101055","url":null,"abstract":"<div><div>Light manipulation over spatial angular dispersion is a fundamental challenge. The advent of metasurfaces promotes the manipulation of electromagnetic waves in the energy-momentum space. By adjusting the spatial dispersion characteristics, metasurfaces can realize diverse angular selective functionalities, which manifest as unique optical effects customized over particular angular ranges and have garnered increasing interest to address growing application demands. This review introduces state-of-the-art developments of angular selective optical metasurfaces, emphasizing the significant breakthroughs realized until now. We start by introducing fundamental design strategies enabling angular dispersion. Then, the recent progress in angular selective optical metasurfaces, i.e., emission, reflection, transmission, and dynamic directional metasurfaces, are systemically overviewed. Subsequently, their diverse applications such as thermal management, information transfer and encryption, imaging and advanced light detection and ranging systems are addressed. Finally, existing challenges, and potential directions are presented with perspectives in the concluding part, aiming to provide guidance for the future development of advanced angular selective optical metasurfaces.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101055"},"PeriodicalIF":31.6,"publicationDate":"2025-06-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144313155","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Revolutionary NiCo layered double hydroxide electrodes: Advances, challenges, and future prospects for high-performance supercapacitors 革命性的NiCo层状双氢氧化物电极:高性能超级电容器的进展、挑战和未来前景
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-19 DOI: 10.1016/j.mser.2025.101041
Syed Shaheen Shah , Md. Abdul Aziz , Takaya Ogawa , Laiq Zada , Mohsin Ali Marwat , Syed Muhammad Abdullah , Abdul Jabbar Khan , Muhammad Usman , Ibrahim Khan , Zafar Said , Munetaka Oyama
{"title":"Revolutionary NiCo layered double hydroxide electrodes: Advances, challenges, and future prospects for high-performance supercapacitors","authors":"Syed Shaheen Shah ,&nbsp;Md. Abdul Aziz ,&nbsp;Takaya Ogawa ,&nbsp;Laiq Zada ,&nbsp;Mohsin Ali Marwat ,&nbsp;Syed Muhammad Abdullah ,&nbsp;Abdul Jabbar Khan ,&nbsp;Muhammad Usman ,&nbsp;Ibrahim Khan ,&nbsp;Zafar Said ,&nbsp;Munetaka Oyama","doi":"10.1016/j.mser.2025.101041","DOIUrl":"10.1016/j.mser.2025.101041","url":null,"abstract":"<div><div>The increasing global energy demand and transition to renewable sources emphasize the critical need for advanced energy storage technologies. Supercapacitors, with their high power density, rapid charge/discharge rates, and long cycle life, have emerged as a promising solution. Among various electrode materials, NiCo layered double hydroxides (NiCoLDHs) are particularly notable due to their tunable composition, large surface area, high electrical conductivity, multiple redox states, and exceptional redox activity. This review comprehensively explores the structural and electrochemical properties of NiCoLDHs, highlighting recent advancements in their development as revolutionary electrode materials for supercapacitors. Strategies for enhancing capacitance, such as doping with metals/non-metals, hybridization with carbon materials (e.g., graphene, carbon nanotubes, biomass-derived carbon), and integration with metal oxides, sulfides, selenides, MXenes, MOFs, and conducting polymers, are systematically discussed. Additionally, synthetic methodologies and their impact on electrochemical performance are explored. Current challenges, including scalable synthesis, structural stability, and enhanced energy and power densities, are addressed. Insights from computational modeling and density functional theory provide guidance for optimizing performance at commercial scales. This work provides an overview of advances in NiCoLDHs for next-generation, cost-effective, and sustainable energy storage devices.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101041"},"PeriodicalIF":31.6,"publicationDate":"2025-06-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144313154","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High-energy LiFePO4 battery with methodically controlled dry electrode processing 高能LiFePO4电池与有条不紊地控制干电极加工
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-18 DOI: 10.1016/j.mser.2025.101048
Jimin Park , Chaerin Gim , Chihyun Hwang , Jonghyun Park , Yun–Chae Jung , Jang–Yeon Hwang
{"title":"High-energy LiFePO4 battery with methodically controlled dry electrode processing","authors":"Jimin Park ,&nbsp;Chaerin Gim ,&nbsp;Chihyun Hwang ,&nbsp;Jonghyun Park ,&nbsp;Yun–Chae Jung ,&nbsp;Jang–Yeon Hwang","doi":"10.1016/j.mser.2025.101048","DOIUrl":"10.1016/j.mser.2025.101048","url":null,"abstract":"<div><div>Batteries using the LiFePO<sub>4</sub> (LFP) cathode have emerged as the most notable option for electric vehicle applications owing to their low cost and safety relative to other chemistries. However, the fabrication of a high-energy electrode through the conventional wet electrode processing with the LFP nanoparticles faces challenges because the polymer binders heterogeneously agglomerate with the nanoplate LFP cathode throughout the electrode owing to the capillary traction in the solvent drying process. Herein, a high-energy LFP electrode is innovatively fabricated through methodical control of dry electrode processing from the particle to electrode level. The high tap density micron-sized LFP particles coated with a small amount (0.3 wt%) of carbon nanotubes (CNTs) are used as cathode materials (LFP@CNTs). In the dry electrode processing, the continuous fibrillation between LFP@CNTs (99 wt%) and polytetrafluoroethylene (PTFE) binder (1 wt%) enabled by regulating the shear force can produce the robust and elastic network, ensuring high electrode density over 2.4 g cc<sup>−1</sup> of the dry-processed LFP electrode (LFP-DE) without mechanical rupture of LFP@CNTs. The uniform pore distribution and robust electrical pathways in LFP-DE enhances the Li<sup>+</sup> diffusion and electron transport kinetics during the charge<img>discharge processes. Even under a high capacity loading of 5 mAh cm<sup>−2</sup>, the LFP-DE demonstrates a high reversible capacity of 148.4 mAh g<sup>−1</sup>, an excellent capacity retention of 99 % over 100 cycles at 5 mA cm<sup>−2</sup>, and outstanding power capability up to 15 mA cm<sup>−2</sup>. The LFP-DE demonstrates practical applicability with long-term cycling over 700 cycles in a pouch-type full-cell with a graphite anode.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101048"},"PeriodicalIF":31.6,"publicationDate":"2025-06-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144306377","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A general framework to govern machine learning oriented materials data quality 管理面向机器学习的材料数据质量的通用框架
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-18 DOI: 10.1016/j.mser.2025.101050
Yue Liu , Zhengwei Yang , Xinxin Zou , Yuxiao Lin , Shuchang Ma , Wei Zuo , Zheyi Zou , Hong Wang , Maxim Avdeev , Siqi Shi
{"title":"A general framework to govern machine learning oriented materials data quality","authors":"Yue Liu ,&nbsp;Zhengwei Yang ,&nbsp;Xinxin Zou ,&nbsp;Yuxiao Lin ,&nbsp;Shuchang Ma ,&nbsp;Wei Zuo ,&nbsp;Zheyi Zou ,&nbsp;Hong Wang ,&nbsp;Maxim Avdeev ,&nbsp;Siqi Shi","doi":"10.1016/j.mser.2025.101050","DOIUrl":"10.1016/j.mser.2025.101050","url":null,"abstract":"<div><div>Machine learning (ML) is increasingly applied in materials discovery and property prediction, mainly due to its advantage of low-cost and efficient data analysis process. The materials data quality can heavily influence the performance of ML models. However, most current data quality improvement approaches are purely data-driven, neglecting materials domain knowledge and data quality issues latent in the entire process of ML modelling. Here, we address the definition of high-quality data and propose a general framework for ML-oriented MATerials Data Quality Governance incorporating domain knowledge (MAT-DQG), involving nine dimensions defining WHAT materials data quality should be evaluated, lifecycle models guiding WHEN to execute data governance activities in the entire process of ML modelling, and processing models guiding HOW to detect and address issues related to materials data quality. 60 datasets from materials ML studies are assembled to demonstrate potential utility and applications of MAT-DQG, including mining complicated structure-activity relationships in metals, inorganic non-metals, polymers, and composite materials. MAT-DQG identifies and resolves issues in 17 datasets and as a result prediction accuracy improvements of up to 49 % are achieved. Our work lays a foundation for governing ML-oriented materials data and ensuring its reusability and reliability, which advances the frontiers of materials discovery and design.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101050"},"PeriodicalIF":31.6,"publicationDate":"2025-06-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144306378","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Carbon allotropes/fabrics-based triboelectric nanogenerators: Current progress and future perspectives 基于碳同素异形体/织物的摩擦电纳米发电机:目前进展和未来展望
IF 31.6 1区 材料科学
Materials Science and Engineering: R: Reports Pub Date : 2025-06-17 DOI: 10.1016/j.mser.2025.101049
Shan He , Matt Jellicoe , Aniket Chakraborthy , Md. Eshrat E. Alahi , Anindya Nag , Warwick Powell
{"title":"Carbon allotropes/fabrics-based triboelectric nanogenerators: Current progress and future perspectives","authors":"Shan He ,&nbsp;Matt Jellicoe ,&nbsp;Aniket Chakraborthy ,&nbsp;Md. Eshrat E. Alahi ,&nbsp;Anindya Nag ,&nbsp;Warwick Powell","doi":"10.1016/j.mser.2025.101049","DOIUrl":"10.1016/j.mser.2025.101049","url":null,"abstract":"<div><div>The paper presents a substantial review of triboelectric nanogenerators (TENG) development using different carbon allotropes and fabric materials. TENG has been state-of-the-art since the last decade due to its low cost, simple construction, high output and multifunctional applications. Based on their working mechanism, these prototypes have been developed using a wide range of nanomaterials and polymers to induce high open-circuit voltage and short-circuit current. Certain carbon-based nanomaterials, such as carbon nanotubes, graphene and others, have been found to be very effective due to their excellent electrical properties and biocompatibility. These carbon materials have been intertwined and fused with polymers to form effective energy generators and harvesters. Conjugating these carbon materials into certain flexible fabrics, like cotton, silk, polyester and others, has been largely successful. In addition to some of the factors that affect the performance of the nanogenerators, this paper also showcases some of the fabric-based prototypes, the performance of which has been enhanced by adding carbon materials. The market survey and the future perspectives have also been shown.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101049"},"PeriodicalIF":31.6,"publicationDate":"2025-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144297561","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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