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Sequential electro-coagulation and electro-Fenton processes for the treatment of textile wastewater. 用于处理纺织废水的序贯电凝和电-芬顿工艺。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-09-01 DOI: 10.1002/wer.11118
Palak Agarwal, Vikas K Sangal, Sanjay Mathur
{"title":"Sequential electro-coagulation and electro-Fenton processes for the treatment of textile wastewater.","authors":"Palak Agarwal, Vikas K Sangal, Sanjay Mathur","doi":"10.1002/wer.11118","DOIUrl":"https://doi.org/10.1002/wer.11118","url":null,"abstract":"<p><p>Textile wastewater, laden with persistent dyes and non-biodegradable organics, poses a challenge for treatment in common effluent treatment plants (CETPs) using conventional methods. Pre-treatment of textile effluents is essential to ensure compatibility with CETPs. The present study employed three-dimensional (3D) aluminum and graphite electrodes for a sequential electro-coagulation and electro-Fenton (EC + EF) process. An experimental plan of 25 experiments was constructed using Taguchi method. The combination resulted in high removal efficiencies: 99.91% for color, 93.20% for chemical oxygen demand (COD), and 91.75% for total organic carbon (TOC) for the operating parameters; for EC, current density (J): 20 mA/cm<sup>2</sup>, time (t): 45 min, speed of rotation (N): 55 rpm; and for EF, current density (J): 25 mA/cm<sup>2</sup>, time (t): 50 min, iron concentration: 40 mg/L. Post-treatment, the wastewater exhibited an enhanced biodegradability index of 0.875, rendering it suitable for CETPs. There was an increase of 11% in the total energy consumption when energy spent during rotation and aeration at the time of EC and EF, respectively, were considered. This energy increases the cost and is not accounted for, in previous research. The energy consumption in kWh per g of COD removed at optimum condition for the hybrid treatment was 0.0314, which is lower than the energy consumption by other electrochemical processes employing plate electrodes. This indicates that 3D electrodes are more energy efficient than plate electrodes. PRACTITIONER POINTS: Hybrid electrochemical processes can be used as pre-treatment method for textile effluents. Three-dimensional electrodes improve removal rates with lower energy consumption. Significant color, COD, and TOC abatement were noted post-hybrid treatment of textile wastewater. Biodegradability of the textile effluent improves after the hybrid treatment.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 9","pages":"e11118"},"PeriodicalIF":2.5,"publicationDate":"2024-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142120696","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Identification of carbon fixation microorganisms and pathways in an aquifer contaminated with long-chain petroleum hydrocarbons. 鉴定受长链石油碳氢化合物污染的含水层中的碳固定微生物和途径。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11078
Shuang Gan, Zhuo Ning, Shuaiwei Wang, Weichao Sun, Zhe Xu, He Di, Jinjin Ti, Caijuan Guo, Yahong Zhou, Ze He, Siyu Kong, Min Zhang
{"title":"Identification of carbon fixation microorganisms and pathways in an aquifer contaminated with long-chain petroleum hydrocarbons.","authors":"Shuang Gan, Zhuo Ning, Shuaiwei Wang, Weichao Sun, Zhe Xu, He Di, Jinjin Ti, Caijuan Guo, Yahong Zhou, Ze He, Siyu Kong, Min Zhang","doi":"10.1002/wer.11078","DOIUrl":"https://doi.org/10.1002/wer.11078","url":null,"abstract":"<p><p>Petroleum hydrocarbons (PHCs) can be biodegraded into CO<sub>2</sub>, and PHC-contaminated aquifers are always deemed as carbon sources. Fortunately, some carbon fixation microorganisms have been found in PHC-contaminated sites. However, most of the studies are related to volatile short-chain PHC, and few studies focus on long-chain PHC-contaminated sites. To reveal the carbon fixation microorganisms in these sites, in the study, a long-chain PHC polluted site in North China was selected. Through hydrochemical and metagenomics analysis, the structure and capacity of carbon fixing microorganisms in the site were revealed. Results showed that there were many kinds of carbon fixed microorganisms that were identified such as Flavobacterium, Pseudomonas. HP/4HB, rTCA, and DC/4HB cycles were dominated carbon fixation pathways. The long-chain PHC were weakly correlated with carbon fixation microorganisms, but it may stimulate the growth of some carbon fixation microorganisms, such as microorganisms involved in rTCA cycle. PRACTITIONER POINTS: The microorganisms with carbon fixation gene exist in the aquifer contaminated by long-chain petroleum hydrocarbon. Microorganisms that have the ability to degrade petroleum also have the ability to carbon fixation. Long-chain petroleum hydrocarbon may promote the growth of carbon fixation microorganisms.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11078"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141861076","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hydrogeochemical features, genesis, and quality appraisal of confined groundwater in a typical large sedimentary plain. 典型大型沉积平原封闭地下水的水文地球化学特征、成因和水质评价。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11088
Yuqing Zhang, Yong Xiao, Hongjie Yang, Liwei Wang, Jie Wang, Wenxu Hu, Ning Wang, Zhongyuan Xu, Gongxi Liu, Feiyu Chen, Xu Guo
{"title":"Hydrogeochemical features, genesis, and quality appraisal of confined groundwater in a typical large sedimentary plain.","authors":"Yuqing Zhang, Yong Xiao, Hongjie Yang, Liwei Wang, Jie Wang, Wenxu Hu, Ning Wang, Zhongyuan Xu, Gongxi Liu, Feiyu Chen, Xu Guo","doi":"10.1002/wer.11088","DOIUrl":"https://doi.org/10.1002/wer.11088","url":null,"abstract":"<p><p>The confined groundwater of arid sedimentary plains has been disturbed by long-term anthropogenic extraction, and its hydrochemical quality is required for sustainable development. The present research investigates the hydrochemical characteristics, formation, potential health threats, and quality suitability of the confined groundwater in the central North China Plain. Results show that the confined groundwater has a slightly alkaline nature in the study area, predominantly dominated by fresh-soft Cl-Na and HCO<sub>3</sub>-Na types. Water chemistry is governed by water-rock interactions, including dissolution of evaporites and cation exchange. Approximately 97% of the sampled confined groundwaters exceed the prescribed standard for F<sup>-</sup>. It is mainly due to geological factors such as mineral dissolution, cation exchange, and competitive adsorption of HCO<sub>3</sub> <sup>-</sup> and may also be released from compacted soils because of groundwater extraction. Enriched F<sup>-</sup> in the confined groundwater can pose an intermediate and higher non-carcinogenic risk to more than 90% of the population. It poses the greatest health threat to the population in the north-eastern part of the study area, especially to infants and children. For sustainable development, the long-term use of confined groundwater for irrigation in the area should be avoided, and attention should also be paid to the potential soil salinization and infiltration risks. In the study area, 97% of the confined groundwaters are found to be excellent or good quality for domestic purposes based on Entropy-weighted Water Quality Index. However, the non-carcinogenic health risk caused by high contents of F<sup>-</sup> cannot be ignored. Therefore, it is recommended that differential water supplies should be implemented according to the spatial heterogeneity of confined groundwater quality to ensure the scientific and rational use of groundwater resources. PRACTITIONER POINTS: The hydrochemistry quality of confined groundwater in an arid sedimentary plain disturbed by long-term anthropogenic extraction was investigated. The suitability of confined groundwater for multiple purposes such as irrigation and drinking were evaluated. The hydrochemical characteristics and formation mechanism of confined groundwater under the influence of multiple factors were revealed.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11088"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141876145","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Occurrence of biofilm forming Escherichia coli in drinking water supply system in Kathmandu. 加德满都饮用水供应系统中形成生物膜的大肠埃希氏菌。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11096
Saraswati Gaihre, Kamil Prajapati, Sujata Dhungel, Prabin Dawadi, Dev Raj Joshi, Tista Prasai Joshi
{"title":"Occurrence of biofilm forming Escherichia coli in drinking water supply system in Kathmandu.","authors":"Saraswati Gaihre, Kamil Prajapati, Sujata Dhungel, Prabin Dawadi, Dev Raj Joshi, Tista Prasai Joshi","doi":"10.1002/wer.11096","DOIUrl":"https://doi.org/10.1002/wer.11096","url":null,"abstract":"<p><p>Biofilm development in gram negative bacterial contaminants in water supply systems is linked to persistence as well as antibiotic resistance, which threatens water quality and hence the public health. This study aimed to investigate phenotypic and genetic capacity of biofilm formation by Escherichia coli isolated from supply water with their antibiotic susceptibility pattern. Altogether fifty water samples collected from a city supply water distribution scheme in Kathmandu were analyzed to assess the physicochemical and microbiological quality. Comparing Nepal's national drinking water quality standards 2022, conductivity (4%), turbidity (18%), iron (28%), and residual chlorine (8%) were found exceeding the values above the standards. Among total, 40% of water samples were contaminated with total coliform bacteria. E. coli and Citrobacter species were dominant and isolated from 20 (64.52%) and 11 (35.48%) water samples, respectively. Antibiotic susceptibility testing revealed that E. coli isolates were resistant to ampicillin (20%), nitrofurantoin (10%), and cefotaxime (10%). Citrobacter spp. (54.54%) were found multidrug resistant (MDR) while none of the isolates of E. coli were MDR. Of total, 45% of the isolates developed biofilm while testing with the Microtiter plate method. Biofilm-forming genes bcsA and csgD in E. coli isolates were detected with polymerase chain reaction (PCR) employing specific primers. bcsA and csgD genes were detected in 55% and 45% of the isolates, respectively. This study confirms the occurrences of biofilm forming and antibiotic resistant bacteria like E. coli in the drinking water supply system in Kathmandu alarming its environmental circulation and possible public health threat. Although further study is warranted, this study suggests public health and drinking water treatment interventions to mitigate the biofilm forming antibiotic resistant potential pathogens from supply water in Kathmandu, Nepal. PRACTITIONER POINTS: Forty percent of tested drinking water samples in Kathmandu were contaminated with total coliform bacteria. E. coli and half of Citrobacter spp. isolates were resistant to multiple antibiotics. bcsA and csgD genes were detected in biofilm producing E.coli isolates.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11096"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141971953","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A probabilistic risk assessment of heavy metal in water and sediment: An industrially affected urban river in Bangladesh. 水和沉积物中重金属的概率风险评估:孟加拉国一条受工业影响的城市河流。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11097
Booshra Ahmed, Shamaila Islam, Shamshad Begum Quraishi, Md Nur E Alam, Md Sabbir Ahsan, Alamgir Kabir
{"title":"A probabilistic risk assessment of heavy metal in water and sediment: An industrially affected urban river in Bangladesh.","authors":"Booshra Ahmed, Shamaila Islam, Shamshad Begum Quraishi, Md Nur E Alam, Md Sabbir Ahsan, Alamgir Kabir","doi":"10.1002/wer.11097","DOIUrl":"https://doi.org/10.1002/wer.11097","url":null,"abstract":"<p><p>Human welfare and biodiversity are at risk due to the deterioration of water and sediment quality. Particularly, in last few decades, global water and sediment quality degraded due to the rapid industrialization and urbanization. This study aimed to determine the concentration of nine heavy metals and metalloid (Pb, Cr, Cd, Hg, As, Mn, Ni, Cu, and Zn) and assess the ecological risks using different pollution indices (e.g., heavy metal pollution index [HPI], Nemerow pollution index [NI], geo-accumulation index [Igeo], contamination factor [CF], degree of contamination [CD] and pollution load index [PLI], ecological risk index [ERI]) in water and sediment of the Shitalakshya River, an industrially affected urban river of Bangladesh. For the first time, 20 water and sediment samples were collected across a wider geographical area of the Shitalakshya River during both monsoon and dry seasons and analyzed using the atomic absorption spectrometer. Average concentrations of heavy metals and metalloid in water were within the Bangladesh standard except for Cr (51.69 ppb) and Mn (228.20 ppb) during monsoon season, portraying potential ecological and human health risks. Besides, average concentration of Mn (549.75 and 370.93 ppb), Ni (549.75 and 370.93 ppb), and Cu (45.34 and 36.09 ppb) in sediment during both seasons were above international standard, implying risk to aquatic sediment biota. The average HPI values indicated moderate to high contamination, whereas the NI values implied polluted water in monsoon season with severe pollution in port area of the river. Similarly, Igeo, CF, CD, and PLI elucidated different levels of contamination in the sediment, particularly during dry season. The ERI values also referred moderate ecological risk in the sediment during dry season. Overall, our findings highlight the alarming level of heavy metal pollution in the Shitalakshya River, necessitating immediate action to protect the aquatic environment, sediment biota, and human health. PRACTITIONER POINTS: This study determined the concentration of heavy metals and metalloid in water and sediment of the Shitalakshya River, Bangladesh. The study revealed that the average concentration of Cr and Mn in water exceeded national standard, whereas Mn, Ni, and Cu in sediment exceeded international limit. Potential ecological risk of heavy metals was also assessed using different pollution indices. Calculated pollution indices indicated different degree of pollution, implying critical ecological condition due to heavy metal pollution in aquatic environment and sediment biota.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11097"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142000771","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Radioactive elements in wastewater and potable water: Sources, effects, and methods of analysis and removal. 废水和饮用水中的放射性元素:来源、影响以及分析和清除方法。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11106
Shubham Sharma, Vivek Sharma, Ankit Mittal, Dipak Kumar Das, Sonika Sethi, Suman Yadav, Bhaskar Vallamkonda, Vinod Kumar Vashistha
{"title":"Radioactive elements in wastewater and potable water: Sources, effects, and methods of analysis and removal.","authors":"Shubham Sharma, Vivek Sharma, Ankit Mittal, Dipak Kumar Das, Sonika Sethi, Suman Yadav, Bhaskar Vallamkonda, Vinod Kumar Vashistha","doi":"10.1002/wer.11106","DOIUrl":"https://doi.org/10.1002/wer.11106","url":null,"abstract":"<p><p>Radioactive effluents, originating from nuclear power plants, medical-nuclear applications, and various extraction industries worldwide, present a significant and dangerous contamination challenge. The concentrations of radioactive substances in wastewater, surface water, and potable water vary widely depending on the source and location. For example, cesium-137 levels in wastewater from nuclear facilities can range from 0.1 to 10 Bq/L, while tritium concentrations in surface water near nuclear plants can reach up to 100 Bq/L. Regulatory guidelines, like the maximum contaminant level of 0.185 Bq/L for combined radium-226 and radium-228 in drinking water, are critical for ensuring safety and environmental protection. Specifically, in Fukushima, Japan, cesium-137 levels in surface water range from 0.1 to 10 Bq/L due to the nuclear accident. In contrast, regions with natural uranium deposits, like parts of the United States, have reported radium-226 concentrations in potable water up to 1 Bq/L. These variations highlight the necessity for focused monitoring and evaluation to protect water quality and community health. Among various methods, Gamma spectrometry and inductively coupled plasma mass spectrometry are precise for radionuclide quantification, scintillation detectors, and ion exchange, and adsorption techniques efficiently remove radioactive substances from water. This critical review examines the sources, adverse effects, and analysis and remediation strategies for various radioactive elements in wastewater. By thoroughly evaluating the origins and potential dangers associated with radioactive effluents, this report emphasizes the urgent need for rigorous monitoring and effective treatment practices to maintain the integrity of water resources and ecosystems. PRACTITIONER POINTS: Comprehensive analysis of the radioactive elements frequently found in wastewater and drinking water. Assess the negative effects of radioactive elements in water systems. Examine the treatment methods used to eliminate radioactive pollutants from water sources. Outline effective methods and tactics for addressing and controlling radioactive contamination occurrences. Analyze the latest advancements in technology, regulatory enhancements, and optimal methods to guarantee the safety of drinking water and the sustainable handling of radioactive substances in wastewater.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11106"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142005435","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Examining temporal trends in heavy metal levels to analyze sediment pollution dynamics in the Saida urban watershed (N-W Algeria). 研究重金属含量的时间趋势,分析赛达城市流域(阿尔及利亚西北部)的沉积物污染动态。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11084
Belaid Fatmi, Abdelkrim Hazzab, Asmaa Rahmani, Abdellah Ghenaim
{"title":"Examining temporal trends in heavy metal levels to analyze sediment pollution dynamics in the Saida urban watershed (N-W Algeria).","authors":"Belaid Fatmi, Abdelkrim Hazzab, Asmaa Rahmani, Abdellah Ghenaim","doi":"10.1002/wer.11084","DOIUrl":"https://doi.org/10.1002/wer.11084","url":null,"abstract":"&lt;p&gt;&lt;p&gt;The study focuses on current pollution in the Saïda basin, a semi-arid region in north-western Algeria. By analyzing sediments, the study provides interesting results on urban pollution and its environmental impact. The research consists of two main phases, each addressing different aspects of pollution. In the first phase, different pollution indicators are used to analyze heavy metals and organic pollutants in urban drainage sediments. The results are compared with sediment quality guidelines, regulatory thresholds, and local and international references. Most of the metallic contaminants exceed the toxicity levels established by the continental crust and sediment quality guidelines, suggesting an anthropogenic origin. In addition, contamination indices show significant accumulation. In this context, the results highlight the importance of accumulation and transport processes in urban sediments. Hydrological parameters significantly influence heavy metal distribution mechanisms. Remarkable variations between copper (Cu) and lead (Pb) suggest a combined or singular source during transport. Conversely, chromium (Cr), nickel (Ni), and iron (Fe) are mainly derived from natural lithological sources. Cadmium (Cd) is associated with anthropogenic sources related to the agricultural use of phosphate fertilizers, whereas zinc (Zn) is mainly derived from physical corrosion processes. In the second phase, a combined descriptive and multivariate statistical analysis examines the mobility and distribution of heavy metals and their relationships with organic matter (OM) over time. Pronounced temporal variations in Cd, Zn, and Cu concentrations are attributed to human activities. Strong correlations exist between OM and cobalt (Co), Cu and Pb, confirming the ability of OM to adsorb these metals under specific geochemical conditions associated with waste disposal. Conversely, Zn, Cd, Cr, and Ni show weak or negative correlations with OM, suggesting diverse sources, including potential agricultural, industrial, and natural origins. The dendrogram confirms the existence of previously identified contaminant groups, suggesting common sources and potential co-occurrence patterns. This analysis highlights the role of the drainage network as a physico-chemical reactor in the mobilization of contaminants. It underlines the importance of sediment interactions in urban pollution processes. Finally, recommendations are proposed to ensure effective pollution control and remediation. PRACTITIONER POINTS: Useful information on pollution and its environmental impact is provided by the analysis of sediments in the urban basin of Saida (NW-Algeria). The results of this study indicate high levels of heavy metals in the sediments, in excess of toxicity limits, and evidence of anthropogenic sources. Temporal variations in metal concentrations indicate the influence of human activities. The study has made it possible to identify the sources, to understand the mobility and di","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11084"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141907734","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Organochlorine pesticides (OCPs) and polychlorinated biphenyls (PCBs) distribution, origins, and risk evaluation in the Egyptian Mediterranean coast sediments. 埃及地中海沿岸沉积物中有机氯农药 (OCP) 和多氯联苯 (PCB) 的分布、来源和风险评估。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11093
Mohamed A Hassaan, Safaa Ragab, Marwa R Elkatory, Ahmed El Nemr
{"title":"Organochlorine pesticides (OCPs) and polychlorinated biphenyls (PCBs) distribution, origins, and risk evaluation in the Egyptian Mediterranean coast sediments.","authors":"Mohamed A Hassaan, Safaa Ragab, Marwa R Elkatory, Ahmed El Nemr","doi":"10.1002/wer.11093","DOIUrl":"https://doi.org/10.1002/wer.11093","url":null,"abstract":"<p><p>A study was conducted on 31 surface sediments located in different sectors of the Egyptian Mediterranean coast. The sediments were analyzed for their pollution levels of organochlorine pesticides (OCPs) and polychlorinated biphenyls (PCBs). The sediments were collected from various depths in harbors, coastal lakes, bays, and lagoons, covering the southeastern Mediterranean of the Nile Delta region. The study aimed at determining the distribution, origin, and potential ecological impact of OCP and PCB pollutants. The researchers used the SRM method of GC-MS/MS to measure the concentration of 18 PCBs and 16 OCPs residues. The study found that the total concentration of OCPs in the samples ranged from 3.091 to 20.512 ng/g, with a mean of 8.749 ± 3.677 ng/g. The total concentration of PCB residues ranged from 2.926 to 20.77 ng/g, with a mean of 5.68 ± 3.282 ng/g. The concentration of DDTs exceeded the effect range low (ERL) (1.00) and threshold effect level (TEL) (1.19) in several stations, but it was still below the effect range median (ERM) (7.00) and the probable effect level (PEL) (4.77). This indicates a low ecological risk. The principal component analysis (PCA) was also conducted to determine the sources of all pollutants in the sediment. The PCA showed significant correlations between the concentrations of Gama-HCH and Beta-HCH (0.741), suggesting similar sources. PRACTITIONER POINTS: OCPs and PCBs residues were analyzed in the sediment of the southeastern Mediterranean. The concentration, existence, and causes of OCPs and PCBs were investigated. OCPs and PCBs ecological risk and ecotoxicological calculation were investigated in detail. Cluster analysis, PCA, and correlation coefficient were also investigated.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11093"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141917523","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Temporal and spatial changes in the abundance of antibiotic resistance gene markers in a wastewater treatment plant. 污水处理厂中抗生素耐药性基因标记丰度的时空变化。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11104
Guillaume Cailleau, Thomas Junier, Christophe Paul, Mathilda Fatton, Andrea Corona-Ramirez, Ophelie Gning, Karin Beck, Jacques Vidal, Helmut Bürgmann, Pilar Junier
{"title":"Temporal and spatial changes in the abundance of antibiotic resistance gene markers in a wastewater treatment plant.","authors":"Guillaume Cailleau, Thomas Junier, Christophe Paul, Mathilda Fatton, Andrea Corona-Ramirez, Ophelie Gning, Karin Beck, Jacques Vidal, Helmut Bürgmann, Pilar Junier","doi":"10.1002/wer.11104","DOIUrl":"https://doi.org/10.1002/wer.11104","url":null,"abstract":"<p><p>In this study, we investigated the temporal and spatial quantitative changes in the concentration of antibiotic resistance gene (ARG) markers in a municipal wastewater treatment plant (WWTP). Four ARGs conferring resistance to different classes of antibiotics (ermB, sul1, tet[W], and bla<sub>CTXM</sub>) and a gene used as a proxy for ARG pollution (intl1) were quantified in two separate sampling campaigns covering two and half years of operation of the WWTP. First, a systematic monthly monitoring of multiple points in the inlet and the outlet revealed an absolute decrease in the concentration of all analyzed ARGs. However, the relative abundance of sul1 and intl1 genes relative to the total bacterial load (estimated using the universal marker 16S rDNA) increased in the outlet samples as compared to the inlet. To pinpoint the exact stage of removal and/or enrichment within the WWTP, a second sampling including the stages of the biological treatment was performed bimonthly. This revealed a distinct enrichment of sul1 and intl1 genes during the biological treatment phase. Moreover, the temporal and spatial variations in ARG abundance patterns within the WWTP underscored the complexity of the dynamics associated with the removal of ARGs during wastewater treatment. Understanding these dynamics is pivotal for developing efficient strategies to mitigate the dissemination of ARGs in aquatic environments. PRACTITIONER POINTS: Regular monitoring of ARG markers in WWTPs is essential to assess temporal and spatial changes, aiding in the development of effective mitigation strategies. Understanding the dynamics of ARG abundance during biological treatment is crucial for optimizing processes and minimizing dissemination in aquatic environments. Increased relative abundance of certain ARGs highlights potential enrichment during wastewater treatment, necessitating targeted interventions. Systematic monitoring of multiple points within WWTPs can provide valuable insights into the efficacy of treatment processes in reducing ARG levels over time. The complexity of ARG abundance patterns underscores the need to develop holistic approaches to tackle antibiotic resistance in wastewater systems.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11104"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142009573","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Arsenic-contaminated groundwater of the Western Banat (Pannonian basin): Hydrogeochemical appraisal, pollution source apportionment, and Monte Carlo simulation of source-specific health risks. 西巴纳特(潘诺尼亚盆地)受砷污染的地下水:水文地质化学评估、污染源划分和特定污染源健康风险的蒙特卡罗模拟。
IF 2.5 4区 环境科学与生态学
Water Environment Research Pub Date : 2024-08-01 DOI: 10.1002/wer.11087
Jelena Vesković, Sandra Bulatović, Slavica Ražić, Milica Lučić, Andrijana Miletić, Aleksandra Nastasović, Antonije Onjia
{"title":"Arsenic-contaminated groundwater of the Western Banat (Pannonian basin): Hydrogeochemical appraisal, pollution source apportionment, and Monte Carlo simulation of source-specific health risks.","authors":"Jelena Vesković, Sandra Bulatović, Slavica Ražić, Milica Lučić, Andrijana Miletić, Aleksandra Nastasović, Antonije Onjia","doi":"10.1002/wer.11087","DOIUrl":"https://doi.org/10.1002/wer.11087","url":null,"abstract":"<p><p>Due to rapid urbanization and industrial growth, groundwater globally is continuously deteriorating, posing significant health risks to humans. This study employed a comprehensive methodology to analyze groundwater in the Western Banat Plain (Serbia). Using Piper and Gibbs plots, hydrogeochemistry was assessed, while the entropy-weighted water quality index (EWQI) was used to evaluate groundwater quality. Pollution sources were identified using positive matrix factorization (PMF) accompanied by Pearson correlation and hierarchical cluster analysis, while Monte Carlo simulation assessed health risks associated with groundwater consumption. Results showed that groundwater, mainly Ca-Mg-HCO<sub>3</sub> type, is mostly suitable for drinking. Geogenic pollution, agricultural activities, and sewage were major pollution sources. Consumption of contaminated groundwater poses serious non-carcinogenic and carcinogenic health risks. Additionally, arsenic from geogenic source was found to be the main health risks contributor, considering its worryingly elevated concentration, ranging up to 364 μg/L. These findings will be valuable for decision-makers and researchers in managing groundwater vulnerability. PRACTITIONER POINTS: Groundwater is severely contaminated with As in the northern part of the study area. The predominant hydrochemical type of groundwater in the area is Ca-Mg-HCO<sub>3</sub>. The PMF method apportioned three groundwater pollution sources. Monte Carlo identified rock dissolution as the primary health risk contributor. Health risks and mortality in the study area are positively correlated.</p>","PeriodicalId":23621,"journal":{"name":"Water Environment Research","volume":"96 8","pages":"e11087"},"PeriodicalIF":2.5,"publicationDate":"2024-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141876144","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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