{"title":"Nanocatalytic NO gas therapy against orthotopic oral squamous cell carcinoma by single iron atomic nanocatalysts","authors":"Yuting Xie, Jiaxin Zuo, Angang Ding, Ping Xiong","doi":"10.1080/14686996.2024.2368452","DOIUrl":"https://doi.org/10.1080/14686996.2024.2368452","url":null,"abstract":"Oral squamous cell carcinoma (OSCC) has been being one of the most malignant carcinomas featuring high metastatic and recurrence rates. The current OSCC treatment modalities in clinics severely det...","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"35 1","pages":""},"PeriodicalIF":5.5,"publicationDate":"2024-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141501618","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Decoding thermal properties in polymer-inorganic heat dissipators: a data-driven approach using pyrolysis mass spectrometry.","authors":"Yusuke Hibi, Yasuhiro Tsuyuki, Satoshi Ishii, Eiichi Ide, Masanobu Naito","doi":"10.1080/14686996.2024.2362125","DOIUrl":"10.1080/14686996.2024.2362125","url":null,"abstract":"<p><p>Polymeric materials can boost their performances by strategically incorporating inorganic substances. Heat dissipators are a representative class of such composite materials, where inorganic fillers and matrix polymers contribute to high thermal conductivity and strong adhesion, respectively, resulting in excellent heat dissipation performance. However, due to the complex interaction between fillers and polymers, even slight differences in structural parameters, e.g. dispersion/aggregation degree of fillers and crosslink density of polymers, may significantly impact material performance, complicating the quality management and guidelines for material developments. Therefore, we introduce pyrolysis mass spectra (MS) as material descriptors. On the basis of these spectra, we construct prediction models using a data-driven approach, specifically focusing on thermal conductivity and adhesion, which are key indicators for heat dissipating performance. Pyrolysis-MS observes thermally decomposable polymers, which occupy only 0.1 volume fraction of the heat dissipators; nevertheless, the physical states of non-decomposable inorganic fillers are implicitly reflected in the pyrolyzed fragment patterns of the matrix polymers. Consequently, pyrolysis-MS provides sufficient information to construct accurate models for predicting heat dissipation performance, simplifying quality management by substituting time-consuming performance evaluations with rapid pyrolysis-MS measurements. Furthermore, we elucidate that higher crosslinking density of the matrix polymers enhances thermal conductivity. This data-driven method promises to streamline the identification of key functional factors in complex composite materials.</p>","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"25 1","pages":"2362125"},"PeriodicalIF":5.5,"publicationDate":"2024-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11177714/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141331690","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Ball-milled MoS<sub>2</sub> with graphene shows enhanced catalytic activity for hydrogen evolution reaction.","authors":"Linghui Li, Satish Laxman Shinde, Takeshi Fujita, Takahiro Kondo","doi":"10.1080/14686996.2024.2359360","DOIUrl":"10.1080/14686996.2024.2359360","url":null,"abstract":"<p><p>The hydrogen evolution reaction (HER) is an important phenomenon in water splitting. Consequently, the development of an active, earth-abundant, and inexpensive HER catalyst is highly desired. MoS<sub>2</sub> has drawn considerable interest as an HER catalyst because it is composed of non-precious metal and exhibits high catalytic activity in the nanosheet form. In this study, size-controlled MoS<sub>2</sub> particles were synthesized by ball milling. The as-prepared samples exhibited significantly enhanced electrochemical and catalytic properties compared to those of pristine bulk MoS<sub>2</sub>. Furthermore, the HER activity improved further upon the introduction of graphene into the as-prepared ball-milled samples. In particular, the MoS<sub>2</sub> sample ball-milled for 12 h mixed with graphene exhibited optimal performance, showing an overpotential (160 mV at 10 mA cm<sup>-2</sup>) that was ~ 335 mV lower than that of pristine bulk MoS<sub>2</sub>. The superior catalytic activity was ascribed to the exposed edge sites, sulfur vacancies, and 1T phase of MoS<sub>2</sub>, as well as the noteworthy fortifying effect of the electronically conductive flexible material, graphene. The results provide a promising strategy for its application as an efficient and stable HER catalyst.</p>","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"25 1","pages":"2359360"},"PeriodicalIF":5.5,"publicationDate":"2024-05-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11177716/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141331660","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Metal–organic framework adhesives with exceptionally high heat resistance","authors":"Izuru Miyazaki, Yumi Masuoka, Akitoshi Suzumura, Shinya Moribe, Hisaaki Takao, Mitsutaro Umehara","doi":"10.1080/14686996.2024.2347193","DOIUrl":"https://doi.org/10.1080/14686996.2024.2347193","url":null,"abstract":"We synthesized high-heat-resistant adhesives based on metal – organic frameworks owing to their high decomposition temperature and the absence of a glass transition. Heat-resistance tests were perf...","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"44 1","pages":""},"PeriodicalIF":5.5,"publicationDate":"2024-04-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140925972","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Alkyl anchor–modified artificial viral capsid budding outside-to-inside and inside-to-outside giant vesicles","authors":"Kazunori Matsuura, Miu Hirahara, Kentarou Sakamoto, Hiroshi Inaba","doi":"10.1080/14686996.2024.2347191","DOIUrl":"https://doi.org/10.1080/14686996.2024.2347191","url":null,"abstract":"The budding of human immunodeficiency virus from an infected host cell is induced by the modification of structural proteins bearing long-chain fatty acids, followed by their anchoring to the cell ...","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"79 1","pages":""},"PeriodicalIF":5.5,"publicationDate":"2024-04-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140811759","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Stefano Felicioni, Alberta Aversa, Erica Librera, Federica Bondioli, Paolo Fino
{"title":"Directed energy deposition of 18NiM300 steel: effect of process and post processing conditions on microstructure and properties.","authors":"Stefano Felicioni, Alberta Aversa, Erica Librera, Federica Bondioli, Paolo Fino","doi":"10.1080/14686996.2024.2346071","DOIUrl":"10.1080/14686996.2024.2346071","url":null,"abstract":"<p><p>This current study investigates the effect of Direct Energy Deposition (DED) process conditions on the properties and microstructure of M300 maraging steel samples. The investigation centers on two key factors: laser power and deposition environment. The microstructure of this tool steel is analyzed by computing the Primary Cellular Arm Spacing. The findings revealed a significant influence of both inert atmosphere and laser power on cooling conditions. These different cooling rates influence the phase content as demonstrated by X-Ray Diffraction and Electron Backscatter Diffraction measurements. It was demonstrated the presence of different content of residual austenite at cell boundaries. These distinct microstructural features caused variations in the hardness values of the printed samples. Furthermore, a direct aging heat treatment was implemented, that was chosen from Differential Scanning Calorimetry measurements results. This heat treatment proves effective in achieving consistent hardness increases and eliminated the differences among samples built in different process conditions. This outcome suggests the possibility of selecting the most economically viable DED parameters for optimal results.</p>","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"25 1","pages":"2346071"},"PeriodicalIF":5.5,"publicationDate":"2024-04-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11107851/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141075027","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Rafael Giorjao, Kaue C. Riffel, Eric Brizes, Katherine Sebeck, Antonio J. Ramirez
{"title":"Heat affected zone liquation cracking evaluation on FeMnAl alloys","authors":"Rafael Giorjao, Kaue C. Riffel, Eric Brizes, Katherine Sebeck, Antonio J. Ramirez","doi":"10.1080/14686996.2024.2342232","DOIUrl":"https://doi.org/10.1080/14686996.2024.2342232","url":null,"abstract":"FeMnAl steels are currently generating a lot of interest with potential applications for structural parts in armored vehicles due to their lower density and outstanding mechanical properties. Despi...","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"121 1","pages":""},"PeriodicalIF":5.5,"publicationDate":"2024-04-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140625462","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Solid polymer electrolyte-based atomic switches: from materials to mechanisms and applications","authors":"Tohru Tsuruoka, Kazuya Terabe","doi":"10.1080/14686996.2024.2342772","DOIUrl":"https://doi.org/10.1080/14686996.2024.2342772","url":null,"abstract":"As miniaturization of semiconductor memory devices is reaching its physical and technological limits, there is a demand for memory technologies that operate on new principles. Atomic switches are n...","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"16 1","pages":""},"PeriodicalIF":5.5,"publicationDate":"2024-04-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140597447","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Han Zhong, Yangying Zhou, Cong Wang, Chunlei Wan, Kunihito Koumoto, Zhiping Wang, Hong Lin
{"title":"A perovskite solar cell-photothermal-thermoelectric tandem system for enhanced solar energy utilization","authors":"Han Zhong, Yangying Zhou, Cong Wang, Chunlei Wan, Kunihito Koumoto, Zhiping Wang, Hong Lin","doi":"10.1080/14686996.2024.2336399","DOIUrl":"https://doi.org/10.1080/14686996.2024.2336399","url":null,"abstract":"Photovoltaic-thermoelectric (PV-TE) tandem system has been considered as an effective way to fully utilize the solar spectrum, and has been demonstrated in a perovskite solar cell (PSC)-thermoelect...","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"4 1","pages":""},"PeriodicalIF":5.5,"publicationDate":"2024-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140597543","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Microstructure and wear behaviour of AlCoCrFeNi-coated SS316L by atmospheric plasma spray process","authors":"Niveditha Noble, Nachimuthu Radhika, Jeyaprakash Natarajan","doi":"10.1080/14686996.2024.2341611","DOIUrl":"https://doi.org/10.1080/14686996.2024.2341611","url":null,"abstract":"The capacity to endure harsh wear in demanding conditions in stainless steel drops under extreme nature and applications. Protecting the surface by providing a coating layer supports the usage in h...","PeriodicalId":21588,"journal":{"name":"Science and Technology of Advanced Materials","volume":"50 1","pages":""},"PeriodicalIF":5.5,"publicationDate":"2024-04-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140563860","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}