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Stabilizing Layered Cathodes by High-Entropy Doping. 通过高熵掺杂稳定层状阴极。
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-23 eCollection Date: 2024-01-01 DOI: 10.34133/research.0503
Yuan Ma, Zihao Zhou, Torsten Brezesinski, Yanjiao Ma, Yuping Wu
{"title":"Stabilizing Layered Cathodes by High-Entropy Doping.","authors":"Yuan Ma, Zihao Zhou, Torsten Brezesinski, Yanjiao Ma, Yuping Wu","doi":"10.34133/research.0503","DOIUrl":"https://doi.org/10.34133/research.0503","url":null,"abstract":"<p><p>Layered Ni-rich oxide cathodes in lithium-ion batteries (LIBs) often struggle with poor thermal safety and capacity fade. Xin and colleagues' studies in <i>Nature</i> and <i>Nature Energy</i> demonstrate a novel high-entropy (compositionally complex) doping strategy, introducing \"cocktail effects\" from multiple constituents. This approach substantially improves cycling performance and stability, reduces material cost, and may pave the way toward the development of advanced electrodes for next-generation LIBs.</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0503"},"PeriodicalIF":11.0,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11496606/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142506906","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A Universal Framework for General Prediction of Physicochemical Properties: The Natural Growth Model. 物理化学性质一般预测的通用框架：自然生长模型
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-23 eCollection Date: 2024-01-01 DOI: 10.34133/research.0510
Jinming Fan, Chao Qian, Shaodong Zhou
{"title":"A Universal Framework for General Prediction of Physicochemical Properties: The Natural Growth Model.","authors":"Jinming Fan, Chao Qian, Shaodong Zhou","doi":"10.34133/research.0510","DOIUrl":"https://doi.org/10.34133/research.0510","url":null,"abstract":"<p><p>To precisely and reasonably describe the contribution of interatomic and intermolecular interactions to the physicochemical properties of complex systems, a chemical message passing strategy as driven by graph neural network is proposed. Thus, by distinguishing inherent and environmental features of atoms, as well as proper delivering of these messages upon growth of systems from atoms to bulk level, the evolution of system features affords eventually the target properties like the adsorption wavelength, emission wavelength, solubility, photoluminescence quantum yield, ionization energy, and lipophilicity. Considering that such a model combines chemical principles and natural behavior of atom aggregation crossing multiple scales, most likely, it will be proven to be rational and efficient for more general aims in dealing with complex systems.</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0510"},"PeriodicalIF":11.0,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11496607/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142506904","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A Wearable Integrated Microneedle Electrode Patch for Exercise Management in Diabetes. 用于糖尿病患者运动管理的可穿戴式集成微针电极贴。
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-21 eCollection Date: 2024-01-01 DOI: 10.34133/research.0508
Boyu Zhu, Lihang Zhu, Xinru Li, Ziyi Zhao, Jiayi Cao, Min Qi, Zhigang Gao, Lin Zhou, Bin Su
{"title":"A Wearable Integrated Microneedle Electrode Patch for Exercise Management in Diabetes.","authors":"Boyu Zhu, Lihang Zhu, Xinru Li, Ziyi Zhao, Jiayi Cao, Min Qi, Zhigang Gao, Lin Zhou, Bin Su","doi":"10.34133/research.0508","DOIUrl":"10.34133/research.0508","url":null,"abstract":"<p><p>Exercise is one of the preferred management strategies for diabetic patients, but the exercise mode including type, intensity, and duration time is quite different for each patient because of individual differences. Inadequate exercise has no effect on the blood glucose control, while overexercise may cause serious side effects, such as hypoglycemia and loss of blood glucose control. In this work, we report a closed-loop feedback mode for exercise management in diabetes. A minimally invasive, biocompatible microneedle electrode patch was fabricated and used for continuously monitoring the glucose in the interstitial fluid. Further, in conjunction with using a wireless electrochemical device, the glucose signals can be analyzed to output the potency of exercise and give advice on exercise management. A custom exercise given by this closed-loop feedback mode can reduce the used dose of insulin and avoid side effect during and after exercise. We believe that this work can provide a novel comprehensive guidance for diabetic patients.</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0508"},"PeriodicalIF":11.0,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11491670/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142473586","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Discovery of High-Risk Clinical Factors That Accelerate Brain Aging in Adults: A Population-Based Machine Learning Study. 发现加速成人大脑老化的高危临床因素：基于人群的机器学习研究。
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-21 eCollection Date: 2024-01-01 DOI: 10.34133/research.0500
Jing Sun, Luyao Wang, Yiwen Gao, Ying Hui, Shuohua Chen, Shouling Wu, Zhenchang Wang, Jiehui Jiang, Han Lv
{"title":"Discovery of High-Risk Clinical Factors That Accelerate Brain Aging in Adults: A Population-Based Machine Learning Study.","authors":"Jing Sun, Luyao Wang, Yiwen Gao, Ying Hui, Shuohua Chen, Shouling Wu, Zhenchang Wang, Jiehui Jiang, Han Lv","doi":"10.34133/research.0500","DOIUrl":"10.34133/research.0500","url":null,"abstract":"<p><p><b>Introduction:</b> Brain age prediction using neuroimaging data and machine learning algorithms holds significant promise for gaining insights into the development of neurodegenerative diseases. The estimation of brain age may be influenced not only by the imaging modality but also by multidomain clinical factors. However, the degree to which various clinical factors in individuals are associated with brain structure, as well as the comprehensive relationship between these factors and brain aging, is not yet clear. <b>Methods:</b> In this study, multimodal brain magnetic resonance imaging data and longitudinal clinical information were collected from 964 participants in a population-based cohort with 16 years of follow-up in northern China. We developed a machine learning-based algorithm to predict multimodal brain age and compared the estimated brain age gap (BAG) differences among the 5 groups characterized by varying exposures to these high-risk clinical factors. We then estimated modality-specific brain age in the hypertension group based on hypertension-related regional imaging metrics. <b>Results:</b> The results revealed a significantly larger BAG estimated from multimodal neuroimaging in subjects with 4 or 5 risk factors compared to other groups, suggesting an acceleration of brain aging under cumulative exposure to multiple risk factors. The estimated T1-based BAG exhibited a significantly higher level in the hypertensive subjects compared to the normotensive individuals. <b>Conclusion:</b> Our study provides valuable insights into a range of health factors across lifestyle, metabolism, and social context that are reflective of brain aging and also contributes to the advancement of interventions and public health initiatives targeted at the general population aimed at promoting brain health.</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0500"},"PeriodicalIF":11.0,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11491671/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142473588","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Intelligent Transmissive Microwave Metasurface with Optical Sensing and Transparency. 具有光学传感和透明度的智能透射微波元表面。
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-21 eCollection Date: 2024-01-01 DOI: 10.34133/research.0514
Ya Lun Sun, Xin Ge Zhang, Zhixiang Huang, Han Wei Tian, Tie Jun Cui, Wei Xiang Jiang
{"title":"Intelligent Transmissive Microwave Metasurface with Optical Sensing and Transparency.","authors":"Ya Lun Sun, Xin Ge Zhang, Zhixiang Huang, Han Wei Tian, Tie Jun Cui, Wei Xiang Jiang","doi":"10.34133/research.0514","DOIUrl":"10.34133/research.0514","url":null,"abstract":"<p><p>Transmissive metasurfaces are essentially conducive to stealth, absorbers, and communications. However, most of the current schemes only allow microwave to transmit and generally adopt multilayer structures or thick dielectric substrates to improve the electromagnetic performance, restricting optical transmission and conformal application. In addition, most metasurfaces still require metal wires and external power suppliers for programmability. Here, we propose and design an intelligent transmissive microwave metasurface with optical sensing and transparency, which provides both microwave and optical channels without redundant optical devices and power suppliers, and the 2 transmission channels are associated with each other. The metasurface is realized by validly integrating photosensitive materials into microwave meta-structures. As a demonstration, we fabricate an ultrathin optically transparent transmissive metasurface based on polyethylene terephthalate substrate and photoresistors, whose thickness is only 0.125 mm. We further construct cross-wavelength transmission links based on the metasurface sample and experimentally validate that the microwave transmissions vary with light intensities under full-polarization and large-angle incidences, and this metasurface possesses high optical transparency. The intelligent transmissive microwave metasurface with optical sensing and transparency has potential applications in optical-microwave hybrid transmission devices and stealth technology.</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0514"},"PeriodicalIF":11.0,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11491669/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142473591","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Compartmentalized Biomolecular Condensates via Controlled Nucleation. 通过受控成核实现分区化生物分子凝聚体
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-17 eCollection Date: 2024-01-01 DOI: 10.34133/research.0505
Chong Wang, Linyi Zhang, Luoran Shang
{"title":"Compartmentalized Biomolecular Condensates via Controlled Nucleation.","authors":"Chong Wang, Linyi Zhang, Luoran Shang","doi":"10.34133/research.0505","DOIUrl":"https://doi.org/10.34133/research.0505","url":null,"abstract":"<p><p>This commentary underscores the importance and implications of the study \"Biomolecular condensates with complex architectures via controlled nucleation,\" led by Jan C. M. van Hest and Tuomas P. J. Knowles, published in <i>Nature Chemical Engineering</i>. The research team developed a novel system to investigate the structure of biological condensates using quaternized amylose, carboxymethylated amylose, and single-stranded DNA. They successfully created multiphase droplets with distinct dense phases and demonstrated that droplet architecture can be controlled through temperature and salt concentration adjustments. This study offers valuable insights into the formation and function of membraneless organelles in cells and suggests promising applications for designing biomimetic materials and therapeutic strategies.</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0505"},"PeriodicalIF":11.0,"publicationDate":"2024-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11483777/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142473587","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
One-Dimensional Implantable Sensors for Accurately Monitoring Physiological and Biochemical Signals. 用于准确监测生理和生化信号的一维植入式传感器。
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-16 eCollection Date: 2024-01-01 DOI: 10.34133/research.0507
Qianming Li, Wen Wang, Haotian Yin, Kuangyi Zou, Yiding Jiao, Ye Zhang
{"title":"One-Dimensional Implantable Sensors for Accurately Monitoring Physiological and Biochemical Signals.","authors":"Qianming Li, Wen Wang, Haotian Yin, Kuangyi Zou, Yiding Jiao, Ye Zhang","doi":"10.34133/research.0507","DOIUrl":"https://doi.org/10.34133/research.0507","url":null,"abstract":"<p><p>In recent years, one-dimensional (1D) implantable sensors have received considerable attention and rapid development in the biomedical field due to their unique structural characteristics and high integration capability. These sensors can be implanted into the human body with minimal invasiveness, facilitating real-time and accurate monitoring of various physiological and pathological parameters. This review examines the latest advancements in 1D implantable sensors, focusing on the material design of sensors, device integration, implantation methods, and the construction of the stable sensor-tissue interface. Furthermore, a comprehensive overview is provided regarding the applications and future research directions for 1D implantable sensors with an ultimate aim to promote their utilization in personalized healthcare and precision medicine.</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0507"},"PeriodicalIF":11.0,"publicationDate":"2024-10-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11480832/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142473593","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Glycyrrhizic Acid Hydrogel Microparticles Encapsulated with Mesenchymal Stem Cell Exosomes for Wound Healing. 甘草酸水凝胶微粒包裹间充质干细胞外泌体用于伤口愈合
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-14 eCollection Date: 2024-01-01 DOI: 10.34133/research.0496
Luting Zhang, Zhiqiang Luo, Hanxu Chen, Xiangyi Wu, Yuanjin Zhao
{"title":"Glycyrrhizic Acid Hydrogel Microparticles Encapsulated with Mesenchymal Stem Cell Exosomes for Wound Healing.","authors":"Luting Zhang, Zhiqiang Luo, Hanxu Chen, Xiangyi Wu, Yuanjin Zhao","doi":"10.34133/research.0496","DOIUrl":"https://doi.org/10.34133/research.0496","url":null,"abstract":"<p><p>Hydrogel microparticles have been proved to be curative to diabetic wounds. Current trends focus on the integration of bioactive matrix and their smart stimulus-responsive release to meet the complex demand of regeneration in diabetic wound. In this paper, we present novel stem cell exosome-encapsulated Chinese herb glycyrrhizic acid (GA) hydrogel microparticles for wound healing. The integrated GA endows the hydrogel microparticles with antibacterial properties, while the encapsulated exosomes impart them with pro-angiogenesis ability. In addition, as the black phosphorus is incorporated into these hybrid hydrogel microparticles, the release profile of GA and exosomes could be controllable under near-infrared irradiation due to the excellent photothermal effect of black phosphorus and the reversible phase transformation properties of GA. Based on these features, we have demonstrated that these microparticles can effectively kill bacteria, scavenge free radical, and promote angiogenesis from in vitro experiments. Besides, they could also markedly accelerate the wound healing process by down-regulating inflammation and promoting collagen deposition and angiogenesis in bacteria-infected in vivo diabetic wound. These results indicate that the proposed exosome-integrated GA hydrogel microparticles present great potential for clinical diabetic wound treatment.</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0496"},"PeriodicalIF":11.0,"publicationDate":"2024-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11471873/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142473590","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Noninvasive Novel Transdermal Drug Delivery System for Deep Drug Permeability. 用于深层药物渗透的无创新型透皮给药系统
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-14 eCollection Date: 2024-01-01 DOI: 10.34133/research.0504
Huijie Han, Hélder A Santos
{"title":"Noninvasive Novel Transdermal Drug Delivery System for Deep Drug Permeability.","authors":"Huijie Han, Hélder A Santos","doi":"10.34133/research.0504","DOIUrl":"https://doi.org/10.34133/research.0504","url":null,"abstract":"","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0504"},"PeriodicalIF":11.0,"publicationDate":"2024-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11471872/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142473592","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Erratum to "Enhanced Effects of Intermittent Fasting by Magnetic Fields in Severe Diabetes". 对 "磁场增强间歇性禁食对严重糖尿病患者的影响 "的勘误。
IF 11 1区 综合性期刊
Research Pub Date : 2024-10-11 eCollection Date: 2024-01-01 DOI: 10.34133/research.0501
Ying Wang, Chuanlin Feng, Biao Yu, Junjun Wang, Weili Chen, Chao Song, Xinmiao Ji, Ruowen Guo, Guofeng Cheng, Hanxiao Chen, Xinyu Wang, Lei Zhang, Zhiyuan Li, Jialiang Jiang, Can Xie, Haifeng Du, Xin Zhang
{"title":"Erratum to \"Enhanced Effects of Intermittent Fasting by Magnetic Fields in Severe Diabetes\".","authors":"Ying Wang, Chuanlin Feng, Biao Yu, Junjun Wang, Weili Chen, Chao Song, Xinmiao Ji, Ruowen Guo, Guofeng Cheng, Hanxiao Chen, Xinyu Wang, Lei Zhang, Zhiyuan Li, Jialiang Jiang, Can Xie, Haifeng Du, Xin Zhang","doi":"10.34133/research.0501","DOIUrl":"https://doi.org/10.34133/research.0501","url":null,"abstract":"<p><p>[This corrects the article DOI: 10.34133/2022/9873203.].</p>","PeriodicalId":21120,"journal":{"name":"Research","volume":"7 ","pages":"0501"},"PeriodicalIF":11.0,"publicationDate":"2024-10-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11467416/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142473589","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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