Nature Reviews Materials最新文献_第6页

Topological fibres expand the horizons of fibre materials 拓扑纤维拓展了纤维材料的视野

IF 79.8 1区材料科学

Nature Reviews Materials Pub Date : 2025-03-17 DOI: 10.1038/s41578-025-00791-5

Hanwei Wang, Cheng Zeng, Qingfeng Sun, Huiqiao Li

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2D non-layered crystals with high hole mobility enter the scene 具有高空穴迁移率的二维非分层晶体进入场景

IF 79.8 1区材料科学

Nature Reviews Materials Pub Date : 2025-03-13 DOI: 10.1038/s41578-025-00794-2

Giulia Pacchioni

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Context dependence in assembly code for supramolecular peptide materials and systems 超分子肽材料和系统汇编代码中的上下文依赖性

IF 86.2 1区材料科学

Nature Reviews Materials Pub Date : 2025-03-13 DOI: 10.1038/s41578-025-00782-6

Kübra Kaygisiz, Deborah Sementa, Vignesh Athiyarath, Xi Chen, Rein V. Ulijn

{"title":"Context dependence in assembly code for supramolecular peptide materials and systems","authors":"Kübra Kaygisiz, Deborah Sementa, Vignesh Athiyarath, Xi Chen, Rein V. Ulijn","doi":"10.1038/s41578-025-00782-6","DOIUrl":"10.1038/s41578-025-00782-6","url":null,"abstract":"Living systems provide the most sophisticated materials known. These materials are created from a few dozen building blocks that are driven to self-organize by covalent and non-covalent interactions. Biology’s building blocks can be repurposed for the design of synthetic materials that life has not explored. In this Review, we examine the bottom-up design, discovery and evolution of self-assembling peptides by considering the entire supramolecular interaction space available to their constituent amino acids. Our approach focuses on sequence context, or how peptide sequence and environmental conditions collectively influence peptide self-assembly outcomes. We discuss examples of peptides that assemble through multimodal backbone, side chain and water interactions. We conclude that a more systematic (comparing sequences side-by-side), integrated (pairing computation and experiment) and holistic (considering peptide, solvent and environment) approach is required to better understand and fully exploit amino acids as a universal assembly code. This goal is particularly timely, because laboratory automation and artificial intelligence now have the potential to accelerate discoveries in these highly modular and complex materials, beyond the limited sequence space that biology uses. Living systems create exceptional materials from simple amino acid building blocks. This Review explores how a systems-based approach — considering peptide, solvent and environment, and integrating computation and experimentation — can unlock peptide sequence space as a universal materials assembly code, enabling designs beyond biology’s natural scope.","PeriodicalId":19081,"journal":{"name":"Nature Reviews Materials","volume":"10 6","pages":"449-472"},"PeriodicalIF":86.2,"publicationDate":"2025-03-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143618892","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Palestinian and German researchers meet to strengthen scientific ties 巴勒斯坦和德国科学家会面加强科学联系

IF 79.8 1区材料科学

Nature Reviews Materials Pub Date : 2025-03-06 DOI: 10.1038/s41578-025-00790-6

Giulia Pacchioni

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Biodegradable origami soft robot 可生物降解的折纸软机器人

IF 79.8 1区材料科学

Nature Reviews Materials Pub Date : 2025-02-27 DOI: 10.1038/s41578-025-00786-2

Charlotte Allard

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Bridging theory and experiment in defect-tolerant semiconductors for photovoltaics 光电容错半导体的桥接理论与实验

IF 79.8 1区材料科学

Nature Reviews Materials Pub Date : 2025-02-27 DOI: 10.1038/s41578-024-00769-9

Maria S. Hammer, Hannah Schlott, Larry Lüer, Christoph J. Brabec, Mykhailo Sytnyk, Johannes Will, Bernd Meyer, Wolfgang Heiss

{"title":"Bridging theory and experiment in defect-tolerant semiconductors for photovoltaics","authors":"Maria S. Hammer, Hannah Schlott, Larry Lüer, Christoph J. Brabec, Mykhailo Sytnyk, Johannes Will, Bernd Meyer, Wolfgang Heiss","doi":"10.1038/s41578-024-00769-9","DOIUrl":"10.1038/s41578-024-00769-9","url":null,"abstract":"Defect tolerance is a concept applied in photovoltaics to explain semiconductors such as lead-halide perovskites that excel without relying on single-crystalline growth. It differentiates from the mere absence of defects, emphasizing on minimizing the influence of defects on minority carrier lifetimes. Whether defect tolerance is the only reason for the superiority of lead-halide-perovskite-based solution-processed solar cells is still controversial. However, the defect tolerance of various semiconductor structures and materials has been experimentally suggested and, in some cases, proven. In this Perspective, we explore defect tolerance across material science, defect characterization and computational modelling. With a primary focus on electrically or optically active defects, we systematically compare computational and experimental results from the literature. We aim to address the complexity arising from diverse theoretical approaches that have yielded partially contradictory results. Additionally, experimental findings have been subject to varied interpretations, ranging from defect signals to ion migration. We endeavour to chart a course through this intricacy and seek to establish a rigorous framework for the identification and quantitative assessment of defect tolerance. Semiconductors that are insensitive to defects hold considerable promise for advancing photovoltaics. This Perspective highlights the importance of combining theoretical predictions with experimental validation to identify viable non-toxic, earth-abundant and cost-effective alternatives to existing materials.","PeriodicalId":19081,"journal":{"name":"Nature Reviews Materials","volume":"10 4","pages":"311-325"},"PeriodicalIF":79.8,"publicationDate":"2025-02-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143506947","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

A kosmotropic solution to cathode manufacturing 阴极制造的全向性解决方案

IF 79.8 1区材料科学

Nature Reviews Materials Pub Date : 2025-02-27 DOI: 10.1038/s41578-025-00788-0

Ariane Vartanian

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Low-cost recycling of perovskite photovoltaics 钙钛矿光伏电池的低成本回收

IF 79.8 1区材料科学

Nature Reviews Materials Pub Date : 2025-02-26 DOI: 10.1038/s41578-025-00787-1

Giulia Pacchioni

引用次数: 0

Publisher Correction: Materials for high-temperature digital electronics 出版者更正：材料高温数码电子

IF 79.8 1区材料科学

Nature Reviews Materials Pub Date : 2025-02-24 DOI: 10.1038/s41578-025-00789-z

Dhiren K. Pradhan, David C. Moore, A. Matt Francis, Jacob Kupernik, W. Joshua Kennedy, Nicholas R. Glavin, Roy H. Olsson III, Deep Jariwala

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Resilience pathways for halide perovskite photovoltaics under temperature cycling 温度循环下卤化物钙钛矿光伏电池的回弹途径

IF 86.2 1区材料科学

Nature Reviews Materials Pub Date : 2025-02-19 DOI: 10.1038/s41578-025-00781-7

Luyan Wu , Shuaifeng Hu , Feng Yang , Guixiang Li , Junke Wang , Weiwei Zuo , José J. Jerónimo-Rendon, Silver-Hamill Turren-Cruz, Michele Saba, Michael Saliba, Mohammad Khaja Nazeeruddin, Jorge Pascual, Meng Li , Antonio Abate

{"title":"Resilience pathways for halide perovskite photovoltaics under temperature cycling","authors":"Luyan Wu \u0000 , Shuaifeng Hu \u0000 , Feng Yang \u0000 , Guixiang Li \u0000 , Junke Wang \u0000 , Weiwei Zuo \u0000 , José J. Jerónimo-Rendon, Silver-Hamill Turren-Cruz, Michele Saba, Michael Saliba, Mohammad Khaja Nazeeruddin, Jorge Pascual, Meng Li \u0000 , Antonio Abate","doi":"10.1038/s41578-025-00781-7","DOIUrl":"10.1038/s41578-025-00781-7","url":null,"abstract":"Metal-halide perovskite solar cells have achieved power conversion efficiencies comparable to those of silicon photovoltaic (PV) devices, approaching 27% for single-junction devices. The durability of the devices, however, lags far behind their performance. Their practical implementation implies the subjection of the material and devices to temperature cycles of varying intensity, driven by diurnal cycles or geographical characteristics. Thus, it is vital to develop devices that are resilient to temperature cycling. This Perspective analyses the behaviour of perovskite devices under temperature cycling. We discuss the crystallographic structural evolution of the perovskite layer, reactions and/or interactions among stacked layers, PV properties and photocatalysed thermal reactions. We highlight effective strategies for improving stability under temperature cycling, such as enhancing material crystallinity or relieving interlayer thermal stress using buffer layers. Additionally, we outline existing standards and protocols for temperature cycling testing and we propose a unified approach that could facilitate valuable cross-study comparisons among scientific and industrial research laboratories. Finally, we share our outlook on strategies to develop perovskite PV devices with exceptional real-world operating stability. Device resilience under temperature cycling is critical for the practical implementation of perovskite photovoltaics. This Perspective highlights how stability evolves with thermal cycling, emphasizing the need for adequate protocols and a deeper understanding of the material and interface changes.","PeriodicalId":19081,"journal":{"name":"Nature Reviews Materials","volume":"10 7","pages":"536-549"},"PeriodicalIF":86.2,"publicationDate":"2025-02-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143443723","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0