Nature reviews. Chemistry最新文献_第9页

Author Correction: Chemistry advances driving industrial carbon capture technologies 作者更正：化学进步推动工业碳捕获技术。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-26 DOI: 10.1038/s41570-026-00811-0

Jeannie Z. Y. Tan, Joao M. Uratani, Steve Griffiths, John M. Andresen, M. Mercedes Maroto-Valer

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Understanding the degradation complexity of ultrahigh-energy lithium metal batteries 了解超高能量锂金属电池的降解复杂性。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-20 DOI: 10.1038/s41570-026-00801-2

Wei Deng (, ), Bao Qiu (, ), Jiahang Chen, Zhen Li, Yongbing Tang (, ), Zhaoping Liu (, ), Ying Shirley Meng

{"title":"Understanding the degradation complexity of ultrahigh-energy lithium metal batteries","authors":"Wei Deng \u0000 (, ), Bao Qiu \u0000 (, ), Jiahang Chen, Zhen Li, Yongbing Tang \u0000 (, ), Zhaoping Liu \u0000 (, ), Ying Shirley Meng","doi":"10.1038/s41570-026-00801-2","DOIUrl":"10.1038/s41570-026-00801-2","url":null,"abstract":"The combination of Li-rich layered oxide cathodes and lithium metal anodes enables lithium metal batteries (LMBs) to achieve specific energies exceeding 600 Wh kg−1, which is a crucial threshold requiring the activation of anionic oxygen-redox of cathode. The specific energy is attained owing to oxygen-redox reactions at the cathode and reversible Li plating–stripping at the anode, but these processes also induce distinct failure mechanisms. Structural destabilization at the cathode and anodic dendrite growth cause cell-level failures that impact the lifespan of LMBs more profoundly than material degradation alone. Moreover, the presence of lithium metal anodes obscures the detection of active Li loss, often leading to misinterpretations related to capacity fading and cycle life. This Review examines the progress in realizing 600 Wh kg−1 LMBs and understanding their lifespan failure mechanisms. We discuss the challenges in accurately assessing the lifespan and Li loss pathways of LMBs, and we elucidate the fundamental chemistry mechanisms driving both material-level and cell-level failures. In particular, the electrochemical implications of cell parameters, cell assembly and operating conditions on the lifespan are highlighted. We also outline the gaps in knowledge and advanced techniques required to decipher detailed failure modes for LMBs with oxygen-redox reactions and Li plating–stripping. This Review discusses the lifespan failure chemistry of lithium metal batteries beyond 600 Wh kg−1, highlighting the challenges in assessing active Li loss. We correlate material degradation, cell parameters, cell assembly and operating conditions to the overall performance and failure of a lithium metal battery.","PeriodicalId":18849,"journal":{"name":"Nature reviews. Chemistry","volume":"10 5","pages":"315-331"},"PeriodicalIF":51.7,"publicationDate":"2026-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146258695","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Empowering the next generation of scientists 赋予下一代科学家力量

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-18 DOI: 10.1038/s41570-026-00806-x

Arismel Tena Meza, Caitlyn Fick, Erin M. Bucci, Jordan A. M. Gonzalez, Katherine McCarthy, Katherine Snell, Luca McDermott, Madeline E. Ruos

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Carbon capture with COFs COFs的碳捕获。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-13 DOI: 10.1038/s41570-026-00802-1

Liang Zhang (, ), Jun Jiang (, )

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Foundation models for atomistic simulation of chemistry and materials 化学和材料原子模拟的基础模型。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-11 DOI: 10.1038/s41570-025-00793-5

Eric C.-Y. Yuan, Yunsheng Liu, Junmin Chen, Peichen Zhong, Sanjeev Raja, Tobias Kreiman, Santiago Vargas, Wenbin Xu, Martin Head-Gordon, Chao Yang, Samuel M. Blau, Bingqing Cheng, Aditi Krishnapriyan, Teresa Head-Gordon

{"title":"Foundation models for atomistic simulation of chemistry and materials","authors":"Eric C.-Y. Yuan, Yunsheng Liu, Junmin Chen, Peichen Zhong, Sanjeev Raja, Tobias Kreiman, Santiago Vargas, Wenbin Xu, Martin Head-Gordon, Chao Yang, Samuel M. Blau, Bingqing Cheng, Aditi Krishnapriyan, Teresa Head-Gordon","doi":"10.1038/s41570-025-00793-5","DOIUrl":"10.1038/s41570-025-00793-5","url":null,"abstract":"Conventional computational methods for modeling chemical and materials systems are limited by system size and timescale, forcing a trade-off between quantum-mechanical accuracy and the sampling needed for realistic observables. Large language and vision foundation models — pre-trained on massive datasets using transformer architectures — have revolutionized many fields. It is thus interesting to ask whether a foundation model — subject to suitable data, parameter scaling and training — could enable learned simulations of chemistry and materials. Here, we review the field of machine-learned interatomic potentials (MLIPs) and posit that scaling up large and diverse chemical and materials datasets and highly expressive architectures using advanced training strategies should result in models that are: more efficient, transferable, robust to out-of-distribution scenarios, and easier to fine-tune to a variety of downstream physical observables than models trained from scratch on small datasets corresponding to specific, targeted atomistic simulation tasks. We provide specific criteria for creating such large-scale MLIP foundation models, coordinated strategies for their development, evaluation and deployment, and highlight potential emergent capabilities that could transform predictive simulations in chemistry and materials science and accelerate discovery across multiple technological domains. We examine the historical development and underlying principles of foundation models realized in language and vision, and propose how physics-infused machine learning interaction potentials could dramatically transform at scale to create transformative foundation models for chemistry and materials science.","PeriodicalId":18849,"journal":{"name":"Nature reviews. Chemistry","volume":"10 3","pages":"212-230"},"PeriodicalIF":51.7,"publicationDate":"2026-02-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146165993","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Author Correction: Substitution and electrochemistry in layered oxide cathode materials for sodium-ion batteries 作者更正：钠离子电池层状氧化物正极材料的替代和电化学。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-06 DOI: 10.1038/s41570-026-00804-z

Liangtao Yang, Xingxing Yin, Jun Wang, Yanan Sun, Yongchun Li, Zhenggang Zhang, Zhongqing Liu, Si-Min Huang, Philipp Adelhelm, Dong Zhou

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A conversation with a chemical biology pioneer 与化学生物学先驱的对话。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-06 DOI: 10.1038/s41570-026-00803-0

Stuart Schreiber, Stephanie Greed

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Towards effective and ethical GenAI in chemistry education 在化学教育中实现有效、道德的基因教育。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-06 DOI: 10.1038/s41570-026-00799-7

Kirsty Tinto, Lorraine Gibson van Mil, Fraser J. Scott

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A call for chemical safety and sustainability 呼吁化学品安全和可持续性。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-02-06 DOI: 10.1038/s41570-026-00798-8

Oskar Karlsson, Berit Olofsson, Aji P. Mathew

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Substitution and electrochemistry in layered oxide cathode materials for sodium-ion batteries 钠离子电池层状氧化物正极材料的替代与电化学。

IF 51.7 1区化学

Nature reviews. Chemistry Pub Date : 2026-01-29 DOI: 10.1038/s41570-025-00795-3

Liangtao Yang, Xingxing Yin, Jun Wang, Yanan Sun, Yongchun Li, Zhenggang Zhang, Zhongqing Liu, Si-Min Huang, Philipp Adelhelm, Dong Zhou

{"title":"Substitution and electrochemistry in layered oxide cathode materials for sodium-ion batteries","authors":"Liangtao Yang, Xingxing Yin, Jun Wang, Yanan Sun, Yongchun Li, Zhenggang Zhang, Zhongqing Liu, Si-Min Huang, Philipp Adelhelm, Dong Zhou","doi":"10.1038/s41570-025-00795-3","DOIUrl":"10.1038/s41570-025-00795-3","url":null,"abstract":"Substitution is a vital strategy for developing high-performance sodium layered oxides (SLOs), which demonstrates great potential for making sodium-ion batteries a viable alternative to lithium-ion batteries. Numerous studies have been conducted on substituted SLOs; however, each substitute exhibits varied effects on the structure and electrochemical performance of the SLOs, and no clear design principles have been established. Clarifying the relationship among substitution, structure and performance is therefore important to enable a rational design strategy for high-performance SLOs. In this Review, the up-to-date substitution guidelines and the current understanding of how substitution affects the structure and electrochemistry in SLOs are discussed, and the site preference and characteristic redox features of different types of substitutes are outlined. The inherent challenges and opportunities for the innovation of better-performing SLOs are summarized, paving the way for accelerating the commercialization of SLO-based sodium-ion batteries and the realization of their applications ranging from electric vehicles to grid energy storage systems. The impact of atomic substitution in sodium-layered oxides and how substitutions affect the properties and performances of battery materials are discussed, with the aim of improving sodium-layered oxides and accelerating the commercialization of sodium-ion batteries.","PeriodicalId":18849,"journal":{"name":"Nature reviews. Chemistry","volume":"10 3","pages":"196-211"},"PeriodicalIF":51.7,"publicationDate":"2026-01-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146073354","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0