Journal of water process engineering最新文献

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Influence of organic matter in wetland substrate on vanadium removal: A batch and column study 湿地基质中有机物对脱钒的影响:间歇式和柱式研究
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106359
A. Hudson , J.G. Murnane , T. O'Dwyer , R. Courtney
{"title":"Influence of organic matter in wetland substrate on vanadium removal: A batch and column study","authors":"A. Hudson ,&nbsp;J.G. Murnane ,&nbsp;T. O'Dwyer ,&nbsp;R. Courtney","doi":"10.1016/j.jwpe.2024.106359","DOIUrl":"10.1016/j.jwpe.2024.106359","url":null,"abstract":"<div><div>Long term Vanadium (V) releases from alkaline wastewaters and associated risks to aquatic environments has highlighted the need to further develop the potential of passive treatment systems, including constructed wetlands (CWs). However, understanding the role and composition of CW substrate, including organic matter content, for V removal is limited.</div><div>This work used batch and column studies to measure V removal and retention by adsorption in mixed compost and soil substrates, at both alkaline and neutral pH's (11 and 6). Batch studies carried out on (i) unamended topsoil, (ii) topsoil with 10 % compost, and (iii) topsoil with 20 % compost, showed that maximum V uptake was highest in the 20 % compost mix (1.47 mg/g) compared to unamended soil (0.76 mg/g) after 24 h contact time.</div><div>A column leaching study using the 20 % compost to topsoil soil mix was batch loaded twice weekly with 50 mL of 100 mg V/ L at pH 6 and pH 11. After 18-weeks, the columns had retained 97 % and 87 % V for the pH 6 and pH 11 solutions respectively. Highest accumulated V was in the top 0–5 cm for the pH 6 (44.8 mg) and top 5-10 cm for pH 11 (56.4 mg) columns, reducing significantly with depth. Soluble V accounted for 46 % of the total in the pH 11 treatment, and 39 % in the pH 6 treatment. Results of this applied study imply a potential means of improving V retention in CW substrate by compost inclusion. Further investigations are needed to assess performance containing multiple trace elements.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106359"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142527054","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhancement of Tunisian groundwater treatment through the simultaneous removal of sulfate, nitrate and nitrogen by-products using a hybrid electrochemical process 利用混合电化学工艺同时去除硫酸盐、硝酸盐和氮副产物,加强突尼斯地下水处理能力
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106374
Maha Ben Arfa , Anis Attour , Alina-Violeta Ursu , Fabrice Audonnet , Hamza Elfil , Christophe Vial
{"title":"Enhancement of Tunisian groundwater treatment through the simultaneous removal of sulfate, nitrate and nitrogen by-products using a hybrid electrochemical process","authors":"Maha Ben Arfa ,&nbsp;Anis Attour ,&nbsp;Alina-Violeta Ursu ,&nbsp;Fabrice Audonnet ,&nbsp;Hamza Elfil ,&nbsp;Christophe Vial","doi":"10.1016/j.jwpe.2024.106374","DOIUrl":"10.1016/j.jwpe.2024.106374","url":null,"abstract":"<div><div>Combined electrocoagulation (<em>EC</em>) and electrooxidation (<em>EO</em>) process was applied to increase Tunisia's drinking water potential from a highly sulfate and nitrate contaminated groundwater. Firstly, batch <em>EC</em> experiments were carried out using Al electrodes under current density (7.2 to 59.5 mA cm<sup>−2</sup>), initial pH (3.0 to 11.0), and temperature (10.0 to 50.0 °C). The results showed that high removal efficiencies, 83.2 % and 82.1 % for sulfate and nitrate, respectively, were achieved at 42.8 mA cm<sup>−2</sup>, initial pH 7.0, and 30.0 °C, while excessive amounts of 0.4 mg NO<sub>2</sub><sup>−</sup>_N L<sup>−1</sup> and 11.6 mg NH<sub>4</sub><sup>+</sup>_N L<sup>−1</sup> were produced. The mechanism study revealed that, at ambient temperature (20–30 °C), sulfate removal by adsorption on Al hydroxides was dependent of generated amount of hydroxide anions resulting from nitrate reduction into nitrogen by-products on the cathode. In second step, <em>EO</em> using a novel electrodes' combination (Ti/RuO<sub>2</sub> anode and Ti cathode), under current density (7.5 to 30.0 mA cm<sup>−2</sup>), initial pH (8.5, 10.0), and initial temperature (10.0 to 50.0 °C), was implemented. The optimized conditions were found at 15.0 mA cm<sup>−2</sup>, initial pH 8.5, and 20.0 °C, leading to complete removal of NO<sub>2</sub><sup>−</sup> and NH<sub>4</sub><sup>+</sup> in the form of N<sub>2</sub> in &lt;20 min.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106374"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142527515","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Conceptual design of an improved ammonia refining process for coal chemical wastewater 煤化工废水改进型氨精制工艺的概念设计
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106371
Jingtao Guo , Chao Pan , Yaping Liu , Xingming Jin , Bingxiao Feng , Hengjun Gai
{"title":"Conceptual design of an improved ammonia refining process for coal chemical wastewater","authors":"Jingtao Guo ,&nbsp;Chao Pan ,&nbsp;Yaping Liu ,&nbsp;Xingming Jin ,&nbsp;Bingxiao Feng ,&nbsp;Hengjun Gai","doi":"10.1016/j.jwpe.2024.106371","DOIUrl":"10.1016/j.jwpe.2024.106371","url":null,"abstract":"<div><div>A large amount of wastewater will be produced in the process of coal chemical production, which has always been one of the most challenging wastewaters to treat. In the actual industry, the phenol ammonia recovery process is mainly used to reduce the content of pollutants in wastewater, and ammonia is recovered as a by-product. Due to the high impurity content in the wastewater, the current process can only produce ammonia with a purity of 98 wt%, which does not meet industrial production requirements. Based on this, a new cascade purification process for by-product ammonia in coal chemical wastewater was proposed and conceptually designed. The results show that 99.8 wt% liquid ammonia can be produced by ammonia washing-ammonia distillation, and 20 wt% ammonia aqueous solution can be produced by ammonia washing-low temperature purification. Both refining methods can reduce inorganics, organics, and oils to &lt;5 mg/L, 35 mg/L, and 10 mg/L, respectively, and the total content of impurities is &lt;50 mg/L, which can produce ammonia products in line with actual industrial production. This work successfully solves the shortcomings of coal chemical wastewater's current ammonia recovery process and has a good application prospect.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106371"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142538388","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhanced tetracycline degradation by manganic iron‑manganese compounds with peroxymonosulfate(PMS): Experimental optimization and environmental fate estimation 过一硫酸锰(PMS)锰铁锰化合物对四环素的强化降解:实验优化和环境归宿评估
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106363
Ruixi Ni, Jiale Tan, Rong Tan, Yineng Lu, Jiangwei Shang, Xiuwen Cheng
{"title":"Enhanced tetracycline degradation by manganic iron‑manganese compounds with peroxymonosulfate(PMS): Experimental optimization and environmental fate estimation","authors":"Ruixi Ni,&nbsp;Jiale Tan,&nbsp;Rong Tan,&nbsp;Yineng Lu,&nbsp;Jiangwei Shang,&nbsp;Xiuwen Cheng","doi":"10.1016/j.jwpe.2024.106363","DOIUrl":"10.1016/j.jwpe.2024.106363","url":null,"abstract":"<div><div>Antibiotics have earned wide attention because of its direct and indirect health and environment risks. As a result, numerous techniques have been explored for deep degradation of antibiotics. Among them, advanced oxidation technologies with Fe-Mn-based catalysts have a great potential on efficient wastewater purification mainly due to low expense, abundant reserves, chemical stabilities and strong oxidation. Herein, we propose a novel wastewater degradation system (Fe<sub>3</sub>O<sub>4</sub>-FeMn<sub>2</sub>O<sub>4</sub>/(peroxymonosulfate)PMS degradation system) as an efficient method for TC decontamination via sulfate radicals based-advanced oxidation processes (SR-AOPs). The results showed that nearly 100 % TC was eliminated in 70 min with the condition of [FM1:3] = 0.50 g/L, [PMS] = 0.25 g/L, pH = 6 and reaction temperature in 25 °C. Based on morphological structure and operating mechanism analysis, the as-prepared Fe<sub>3</sub>O<sub>4</sub>-FeMn<sub>2</sub>O<sub>4</sub> displays obvious porous structures and rich surface functional groups, which positively promotes the oxidative ability of degradation system. Otherwise, dominant active species and possible intermediates are revealed with the results of EPR, HPLC-MS and scavenging experiments, illustrating that nine transformation pathways are ascribed to sulfate radical (SO<sub>4</sub>·<sup>−</sup>) and singlet oxygen (<sup>1</sup>O<sub>2</sub>). This study provides a new method for the development of SR-AOPs towards higher sustainability and more environmental suitability.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106363"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142527055","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Design and optimization of an integrated UF-NF membrane process for treating rare earth refining wastewater 设计和优化处理稀土提炼废水的 UF-NF 一体化膜工艺
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106401
Yiwen Wang , Shuanglin Gui , Qinliang Jiang , Pei Han , Hong Wang , Jianping Deng , Tao Chen , Jianxin Li
{"title":"Design and optimization of an integrated UF-NF membrane process for treating rare earth refining wastewater","authors":"Yiwen Wang ,&nbsp;Shuanglin Gui ,&nbsp;Qinliang Jiang ,&nbsp;Pei Han ,&nbsp;Hong Wang ,&nbsp;Jianping Deng ,&nbsp;Tao Chen ,&nbsp;Jianxin Li","doi":"10.1016/j.jwpe.2024.106401","DOIUrl":"10.1016/j.jwpe.2024.106401","url":null,"abstract":"<div><div>As the rare earth industry develops and energy efficiency improves, high-salinity rare earth smelting wastewater poses a significant environmental concern. This study applied integrated ultrafiltration (UF) - nanofiltration (NF) membrane technology to treat high-salt rare earth smelting wastewater (Ca<sup>2</sup>⁺: 10.75 g/L, COD: 3.5 g/L, turbidity: 1.36 NTU) for salt removal and recovery. The effects of UF pretreatment were explored, and the operating parameters for NF were optimized, with the performance of various commercial NF membranes being evaluated. Membrane fouling conditions were also investigated to determine appropriate cleaning methods. The experimental results demonstrate that the UF-NF integrated process is effective in actual wastewater treatment. The calcium ion content in the permeate was reduced from 10.75 g/L in the feed solution to 0.96 g/L, achieving a removal rate of 91.1 %, which meets reuse water standards. Trace amounts of organic molecules in the water, such as 2-Ethylhexyl phosphonic acid mono-2-ethylhexyl ester (P507), were also effectively removed. The removal rates for COD and TOC were notably high at 97.7 % and 98.3 %, respectively. Acid washing, alkaline washing, and water washing were employed to clean the membranes, all of which achieved flux recovery rates exceeding 95.0 %. In summary, the integrated UF-NF process demonstrated outstanding performance in salt recovery/separation of different valence salts from rare earth smelting wastewater. Its excellent operational stability and high flux recovery rates highlight its strong industrial applicability. The exceptional treatment efficacy it displays provides a feasible technological pathway for resource recovery and water recycling in practical applications.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106401"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142526871","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Molybdenum recovery from acid leaching solution of copper smelting dust using solvent extraction 利用溶剂萃取从铜冶炼粉尘的酸浸出液中回收钼
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106345
Jiawei Wu , Shan Qing , Yina Li , Mingyue Wang
{"title":"Molybdenum recovery from acid leaching solution of copper smelting dust using solvent extraction","authors":"Jiawei Wu ,&nbsp;Shan Qing ,&nbsp;Yina Li ,&nbsp;Mingyue Wang","doi":"10.1016/j.jwpe.2024.106345","DOIUrl":"10.1016/j.jwpe.2024.106345","url":null,"abstract":"<div><div>The massive accumulation of dust produced in the copper smelting process will cause waste of resources and environmental pollution. The selective separation and recovery of valuable metals in copper smelting dust is particularly important. In this study, we proposed a process for extracting molybdenum from acid leaching solution of copper smelting dust with extractant N235. The effects of different process parameters on the extraction and stripping of molybdenum were studied. Under the optimum conditions, the single-stage extraction and stripping efficiency were 94.35 % and 97.77 %, respectively. The extraction efficiency of molybdenum was 99.26 % after three stages of countercurrent extraction. The loaded organic phase was scrubbed with 15 g/L sulfuric acid solution to remove impurities. The stripping efficiency of molybdenum was 99.66 % by three-stage countercurrent stripping with 8 mol/L NH<sub>3</sub>∙H<sub>2</sub>O. Furthermore, the organic phase still maintains a high extraction efficiency after regeneration cycle. Based on the slope method and FT-IR analysis, it is speculated that the extraction complex of molybdenum is [(R<sub>3</sub>NH)<sub>2</sub>·[Mo<sub>2</sub>O<sub>5</sub>(SO<sub>4</sub>)<sub>2</sub>]]. The extraction of molybdenum from acid leaching solution by N235 is an entropy increase and spontaneous endothermic reaction. The recovery of molybdenum from secondary resources reduces the demand for virgin molybdenum ore and improves the efficiency of resource utilization. This study provides an efficient, economical, and environmentally friendly method for industrial recovery of molybdenum.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106345"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142538389","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
UV photoreduction-driven heterogeneous fenton-like process: Long-term reactivation of fenton sludge-derived biochar and enhanced acetaminophen degradation 紫外光还原驱动的异质芬顿类过程:芬顿污泥衍生生物炭的长期再活化和对乙酰氨基酚的强化降解
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106411
Heejin Yang , Sung-Hyo Jung , Jong Ho Lee , In Sun Cho , Seong-Jik Park , Chang-Gu Lee
{"title":"UV photoreduction-driven heterogeneous fenton-like process: Long-term reactivation of fenton sludge-derived biochar and enhanced acetaminophen degradation","authors":"Heejin Yang ,&nbsp;Sung-Hyo Jung ,&nbsp;Jong Ho Lee ,&nbsp;In Sun Cho ,&nbsp;Seong-Jik Park ,&nbsp;Chang-Gu Lee","doi":"10.1016/j.jwpe.2024.106411","DOIUrl":"10.1016/j.jwpe.2024.106411","url":null,"abstract":"<div><div>The Fenton process has been employed in a wide range of applications, including the treatment of wastewater, due to its distinctive characteristics, but disposing of the iron sludge waste that it generates remains a challenge. As a sustainable and effective solution to this problem, the preparation of Fenton sludge (FS) biochar (FSB) and its subsequent use in water treatment has been proposed. In the present study, FSB was employed as a catalyst for the UVC-induced activation of potassium peroxydisulfate (PDS) in the removal of the target contaminant acetaminophen (ACP). The FSB was prepared by pyrolyzing FS (900 °C, 120 min, N<sub>2</sub> atmosphere), and X-ray diffraction analysis confirmed the presence of iron such as zero-valent iron (Fe<sup>0</sup>) and iron carbide (Fe<sub>3</sub>C) on its surface. The FSB/PDS/UVC system achieved an ACP removal efficiency of 100.0 ± 0.0 % in a batch experiment (ACP = 20 mg/L, FSB = 0.2 g/L, PDS = 1 mM, time = 60 min), while the ACP removal rate constant was higher in the FSB/PDS/UVC photo-Fenton-like system (0.309 /min) than in the FSB/PDS Fenton-like system (0.281 /min). The reusability of the FSB in the FSB/PDS/UVC system was tested over 15 cycles and the results showed that, unlike the FSB/PDS system, the catalytic performance of the ACP degradation rate remained consistent (99 %). Overall, UVC irradiation promoted photoreduction, accelerating the in-situ Fe(II)/Fe(III) redox cycle and improving the regeneration of the FSB. This work provides insights into sustainable FS treatment strategies and highlights the potential for the use of FSB in wastewater treatment.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106411"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142526873","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Synergizing photothermal and pyroelectric effects: Coal gangue assisted simultaneous ZnS/CuS for degradation of mineral processing wastewater 光热和热电效应的协同作用:煤矸石辅助 ZnS/CuS 同时降解选矿废水
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106393
Meng Li, Weiji Sun, Wangkai Hui, Lang Liu
{"title":"Synergizing photothermal and pyroelectric effects: Coal gangue assisted simultaneous ZnS/CuS for degradation of mineral processing wastewater","authors":"Meng Li,&nbsp;Weiji Sun,&nbsp;Wangkai Hui,&nbsp;Lang Liu","doi":"10.1016/j.jwpe.2024.106393","DOIUrl":"10.1016/j.jwpe.2024.106393","url":null,"abstract":"<div><div>Photocatalytic oxidation technology is a green and low carbon approach for degradation of mineral processing wastewater, which is extensively applied to ecological environment restoration. In this research, coal gangue-ZnS/CuS pyroelectric/photothermal composite photocatalyst is constructed by high temperature calcination method. The temperature difference between heat converted from light energy absorbed by CuS and the circulating condensate water provides the impelling force for the pyroelectric effect. The porous structure of coal gangue acts as a “heat capacitor”, which furnishes greater temperature fluctuation for pyroelectric effect. Furthermore, the hydroxyl groups on the surface of coal gangue can availably adsorb oxygen and facilely form superoxide radicals with electrons. The degradation efficiency of xanthate is as high as 99.5 % within 50 min. This research has significant implications for designing and developing highly efficient photocatalysts for the degradation of mining wastewater.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106393"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142526872","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of zero-valent iron and magnetite on mitigating sulfate and lincomycin stress in anaerobic digestion: microbial succession and antibiotic resistant genes removal 零价铁和磁铁矿对减轻厌氧消化过程中硫酸盐和林可霉素压力的影响:微生物演替和抗生素耐药基因的去除
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106376
Jing Xie , Jiaxin Zhu , Bolin Min , Rong He , Wenbiao Wang , Li Xie
{"title":"Effect of zero-valent iron and magnetite on mitigating sulfate and lincomycin stress in anaerobic digestion: microbial succession and antibiotic resistant genes removal","authors":"Jing Xie ,&nbsp;Jiaxin Zhu ,&nbsp;Bolin Min ,&nbsp;Rong He ,&nbsp;Wenbiao Wang ,&nbsp;Li Xie","doi":"10.1016/j.jwpe.2024.106376","DOIUrl":"10.1016/j.jwpe.2024.106376","url":null,"abstract":"<div><div>This study investigated the enhancement performance of zero valent iron (ZVI) and Fe<sub>3</sub>O<sub>4</sub> on sulfate, lincomycin and combination stressed anaerobic digestion. The cumulative methane yield were both promoted by ZVI and Fe<sub>3</sub>O<sub>4</sub> under different stressed conditions. ZVI significantly elevated maximum methane production rate to 1.8 ± 0.1 mL/h under sulfate stress, which was 2.25-fold of control group. Fe<sub>3</sub>O<sub>4</sub> revealed its superior performance on lincomycin degradation with a removal efficiency of 56.7 ± 1.3 % under combined stress. Besides, the formation of coenzyme F<sub>420</sub> and hydrogenotrophic methanogenesis were stimulated by ZVI. Regarding microbial community succession, <em>Mesotoga</em> and <em>unclassified_f__Thermotogaceae</em> were enriched by ZVI and Fe<sub>3</sub>O<sub>4</sub>, both of which profited propionate degradation. Iron-based materials similarly enriched hydrogenotrophic methanogens, especially with introduction of Fe<sub>3</sub>O<sub>4</sub>. Insight into metagenomic analysis, genes encoding hydrogenotrophic methanogenesis and direct interspecies electron transfer, such as pliA and chpA, were up-regulated by ZVI and Fe<sub>3</sub>O<sub>4</sub> under different stress conditions. Moreover, Fe<sub>3</sub>O<sub>4</sub> revealed its higher potential to decrease antibiotic resistant genes than ZVI. Overall, this study demonstrated the potential of ZVI and Fe<sub>3</sub>O<sub>4</sub> to enhance anaerobic digestion under high sulfate/lincomycin conditions and provided fundamental basis for further researches.</div></div>","PeriodicalId":17528,"journal":{"name":"Journal of water process engineering","volume":"68 ","pages":"Article 106376"},"PeriodicalIF":6.3,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142527516","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Use of clay honeycomb monoliths for the removal of tetracycline antibiotic from water 利用粘土蜂窝状单体去除水中的四环素抗生素
IF 6.3 2区 工程技术
Journal of water process engineering Pub Date : 2024-10-29 DOI: 10.1016/j.jwpe.2024.106381
Félix Sumariva , F. Javier Moreno-Dorado , Francisco M. Guerra , Daniel Goma , Hilario Vidal , José Manuel Gatica
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