Journal of Photochemistry and Photobiology A-chemistry最新文献_第3页

Dy3+/Cr4+ doped CaLuGaO4 phosphors emitting white and broad NIR light Dy3+/Cr4+掺杂的CaLuGaO4荧光粉发出白光和宽近红外光

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-11 DOI: 10.1016/j.jphotochem.2025.116494

Wenfeng Yuan, Xianke Sun, Meng Wu

{"title":"Dy3+/Cr4+ doped CaLuGaO4 phosphors emitting white and broad NIR light","authors":"Wenfeng Yuan, Xianke Sun, Meng Wu","doi":"10.1016/j.jphotochem.2025.116494","DOIUrl":"10.1016/j.jphotochem.2025.116494","url":null,"abstract":"<div><div>A phosphor that emits both white light and broad near-infrared (NIR) light is of significant interest across various fields, as it enables both visual inspection and NIR spectroscopic detection. In this study, we designed Dy<sup>3+</sup>/Cr<sup>4+</sup> codoped CaLuGaO<sub>4</sub> phosphors that emit both white light and broad NIR light ranging from 1100 nm to 1700 nm when excited at 450 nm. The white light is produced by the <sup>4</sup>F<sub>9/2</sub> → <sup>6</sup>H<sub>15/2</sub>, <sup>6</sup>H<sub>13/2</sub>, <sup>6</sup>H<sub>11/2</sub> transitions of Dy<sup>3+</sup>. The broad NIR light arises from the <sup>3</sup>T<sub>2</sub> to <sup>3</sup>A<sub>2</sub> transition of Cr<sup>4+</sup>. Additionally, energy transfer from Dy<sup>3+</sup> to Cr<sup>4+</sup> occurs in the Dy<sup>3+</sup>/Cr<sup>4+</sup> codoped CaLuGaO<sub>4</sub> phosphors, allowing for tunable ratios of white light to NIR light by varying the concentrations of Dy<sup>3+</sup> and Cr<sup>4+</sup>. A phosphor-converted light-emitting-diode was constructed by encapsulating the synthesized phosphors around a commercial blue LED chip, demonstrating potential applications in lighting sources and non-destructive spectral analysis.</div></div>","PeriodicalId":16782,"journal":{"name":"Journal of Photochemistry and Photobiology A-chemistry","volume":"468 ","pages":"Article 116494"},"PeriodicalIF":4.1,"publicationDate":"2025-05-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143935762","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Preparation of flower globule Pd@Bi2WO6 catalyst and its photocatalytic performance in imines synthesis reaction 花球Pd@Bi2WO6催化剂的制备及其在亚胺合成反应中的光催化性能

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-11 DOI: 10.1016/j.jphotochem.2025.116493

Xiaojie Zhao, Xiujuan Yu, Yejun Feng, Luwei Wang, Manjia Yang, Xinyuan Zhao

{"title":"Preparation of flower globule Pd@Bi2WO6 catalyst and its photocatalytic performance in imines synthesis reaction","authors":"Xiaojie Zhao, Xiujuan Yu, Yejun Feng, Luwei Wang, Manjia Yang, Xinyuan Zhao","doi":"10.1016/j.jphotochem.2025.116493","DOIUrl":"10.1016/j.jphotochem.2025.116493","url":null,"abstract":"<div><div>The Bi<sub>2</sub>WO<sub>6</sub> (BWO) catalyst and <em>x</em>-Pd@Bi<sub>2</sub>WO<sub>6</sub> (<em>x</em>-Pd@BWO) catalysts with varying loading ratios were synthesized using the hydrothermal method and NaBH<sub>4</sub> reduction method. The BWO catalyst exhibits a unique flower-like globule composed of interlaced nanosheets, demonstrating excellent photocatalytic properties. The incorporation of palladium nanoparticles (Pd NPs) further enhances its light absorption capability and promotes efficient separation and migration of photogenerated charge carriers. Experimental results show that 3 wt% Pd@BWO achieves a high conversion rate of 86.2 % for the catalytic synthesis of imine under visible light irradiation, along with excellent stability and recyclability under experimental conditions. A variety of characterization techniques were employed to systematically analyze the crystal structure, morphology, optical properties, charge separation efficiency, and specific surface area of the catalyst. Combined with the results of capturing experiments, density functional theory (DFT) calculations were performed to elucidate the band structure, density of states, electronic density difference, and adsorption energies, providing deep theoretical insights into the photocatalytic performance of <em>x</em>-Pd@BWO. Based on these findings, the plausible reaction mechanism for the photocatalytic generation of imines was further proposed. This work provides useful reference for the preparation of high-performance BWO based photocatalysts.</div></div>","PeriodicalId":16782,"journal":{"name":"Journal of Photochemistry and Photobiology A-chemistry","volume":"468 ","pages":"Article 116493"},"PeriodicalIF":4.1,"publicationDate":"2025-05-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143947283","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

1,8-Naphthalimide-based hybrid inorganic–organic materials for visualization of latent fingerprints: Intracellular Cu2+ detection and anti-counterfeiting ink 1,8-萘酰亚胺基无机-有机杂化材料用于潜在指纹的可视化：细胞内Cu2+检测和防伪油墨

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-11 DOI: 10.1016/j.jphotochem.2025.116495

Vishakha Thakur , Sanjeev Kumar , Mandeep Kaur , Ananay Sharma , Sheikh Showkat Ahmad , Satwinderjeet Kaur , Prabhpreet Singh

{"title":"1,8-Naphthalimide-based hybrid inorganic–organic materials for visualization of latent fingerprints: Intracellular Cu2+ detection and anti-counterfeiting ink","authors":"Vishakha Thakur , Sanjeev Kumar , Mandeep Kaur , Ananay Sharma , Sheikh Showkat Ahmad , Satwinderjeet Kaur , Prabhpreet Singh","doi":"10.1016/j.jphotochem.2025.116495","DOIUrl":"10.1016/j.jphotochem.2025.116495","url":null,"abstract":"<div><div>The ethylene glycol appended 4,5-disubstituted-1,8-naphthalimide (<strong>NBG</strong>) is reported for the detection of the Cu<sup>2+</sup> ions in aqueous medium, live cells and for the imaging of latent fingerprints (LFPs). The NBG showed a decrease in the fluorescence and absorbance intensities at 382 and 446 nm, respectively upon addition of Cu<sup>2+</sup> ions in 20 % HEPES buffer–CH<sub>3</sub>CN medium or CH<sub>3</sub>CN with limit of detection as low as 90 nM (in CH<sub>3</sub>CN). The solution of NBG in ethanol and ethanol–glycerol (7:3, v/v) has been explored as the security ink to write full page text, drawings and chemical structures with ease. The NBG was non-covalently adsorbed on silica nanoparticles (NBG@SiO<sub>2</sub>) and Montmorillonite clay (NBG@MM) to make hybrid inorganic–organic materials for the imaging of latent fingerprints on 13–16 different surfaces up to levels 1–3. The NBG@SiO<sub>2</sub> and NBG@MM fluorescent powders showed sebaceous content enhanced visualization of LFPs on different surfaces and can be used for the analysis, differentiation of different subjects. The physically stressed LFPs have been successfully developed using NBG@ SiO<sub>2</sub> and NBG@MM fluorescent powders with excellent contrast.</div></div>","PeriodicalId":16782,"journal":{"name":"Journal of Photochemistry and Photobiology A-chemistry","volume":"468 ","pages":"Article 116495"},"PeriodicalIF":4.1,"publicationDate":"2025-05-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144068998","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Tailoring CdTe colloidal quantum dots growth kinetics with Ag and In dopants for dazzling white-light emission 银和铟掺杂的CdTe胶体量子点生长动力学研究

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-10 DOI: 10.1016/j.jphotochem.2025.116492

Vijayaraj Venkatachalam , Sasikala Ganapathy , Ilaiyaraja Perumal , Priyadarshini N , Santhosh Jeferson Joseph Stanley , Davis Jacob Inbaraj

{"title":"Tailoring CdTe colloidal quantum dots growth kinetics with Ag and In dopants for dazzling white-light emission","authors":"Vijayaraj Venkatachalam , Sasikala Ganapathy , Ilaiyaraja Perumal , Priyadarshini N , Santhosh Jeferson Joseph Stanley , Davis Jacob Inbaraj","doi":"10.1016/j.jphotochem.2025.116492","DOIUrl":"10.1016/j.jphotochem.2025.116492","url":null,"abstract":"<div><div>CdTe quantum dots (QDs) were synthesized using an aqueous colloidal method with 3-mercaptopropionic acid (3-MPA) serving as the capping agent. Silver (Ag<sup>+</sup>) doping accelerates crystal growth and causes a red shift in CdTe QDs, while indium (In<sup>3+</sup>) doping leads to a slight blue shift due to controlled growth from free chloride ions in InCl<sub>3</sub> precursor, in conjunction with the 3-mercaptopropionic acid (3-MPA) capping agent. As the reflux time increases, particle size grows accordingly, leading to a progressive narrowing of the bandgap: from 2.67 to 2.15 eV for CdTe, 2.7 to 2.19 eV for In-doped CdTe (In:CdTe), and 2.37 to 1.74 eV for Ag-doped CdTe (Ag:CdTe). In<sup>3+</sup> doping in CdTe QDs introduce a shallow level, while Ag<sup>+</sup> doping creates both shallow and deep levels below the conduction band. Emission tuning from deep green to deep red was achieved, effectively addressing the “green gap.” The absorption spectra revealed s- and p-state saturation in CdTe and In:CdTe QDs, whereas Ag:CdTe QDs exhibited additional d-state filling. Both dopants enhanced the optical quality and photoluminescence. A white-light nanocomposite was developed using a blue-emitting organic fluorophore, green-emitting In:CdTe (1 %), and red-emitting Ag:CdTe (5 %) QDs. Optimized mixing produced white light with CIE coordinates (0.33, 0.34), a correlated color temperature (CCT) of 5181 K, and a color rendering index (CRI) of 87 demonstrating strong potential for future white LED and display applications.</div></div>","PeriodicalId":16782,"journal":{"name":"Journal of Photochemistry and Photobiology A-chemistry","volume":"468 ","pages":"Article 116492"},"PeriodicalIF":4.1,"publicationDate":"2025-05-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144068999","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Time-dependent DFT-based study of bacteriochlorophyll a optical properties within the B800 part of LH2 Rhodoblastus acidophilus light-harvesting complex LH2嗜酸Rhodoblastus acidophilus光收集复合物B800部分细菌叶绿素a光学特性的时变dft研究

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-09 DOI: 10.1016/j.jphotochem.2025.116489

E.A. Kovaleva , L.V. Begunovich , M.M. Korshunov

引用次数: 0

Construction of Z-scheme BiVO4/CNTs/Cu2O ternary heterojunction with enhanced photocatalytic activity for round-the-clock antibacterial application

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-08 DOI: 10.1016/j.jphotochem.2025.116474

Rongqing Wang , Jiajia Wu , Jiaqi Wan , Peng Wang , Dun Zhang

引用次数: 0

Efficient photocatalytic removal of drugs in aqueous dispersions by using different TiO2 based semiconductors under UV and simulated solar light irradiation 不同TiO2基半导体在紫外光和模拟太阳光照下的高效光催化脱除水中药物

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-07 DOI: 10.1016/j.jphotochem.2025.116465

Vittorio Loddo, Muhammad Umair, Tayyaba Kanwal, Leonardo Palmisano, Marianna Bellardita

{"title":"Efficient photocatalytic removal of drugs in aqueous dispersions by using different TiO2 based semiconductors under UV and simulated solar light irradiation","authors":"Vittorio Loddo, Muhammad Umair, Tayyaba Kanwal, Leonardo Palmisano, Marianna Bellardita","doi":"10.1016/j.jphotochem.2025.116465","DOIUrl":"10.1016/j.jphotochem.2025.116465","url":null,"abstract":"<div><div>Antibiotics are an important class of environmental pollutants. Due to their widespread use, low metabolism by organisms and persistence in the aquatic environment, they pose a serious risk to human health and environmental quality. The effective removal of pharmaceuticals and their metabolites from aqueous wastewater represents an audacious challenge for the scientific community. Heterogeneous photocatalysis has been applied as an effective technology for the removal of organic pollutants because it can induce their complete mineralization into CO<sub>2</sub>, H<sub>2</sub>O and inorganic species when heteroatoms are present in the degraded molecules without giving rise to the so-called secondary pollution. This study is addressed to enhance the efficiency of differently modified commercial and home-prepared TiO<sub>2</sub> based photocatalysts (heterojunctions with Cu<sub>2</sub>O and WO<sub>3</sub>, and samples doped with N were also prepared) towards some representative drugs (tetracycline, oxytetracycline and lincomycin). N-doped TiO<sub>2</sub> revealed high photocatalytic activity under both UV and simulated solar light irradiation, allowing not only the drugs removal but also a higher mineralization degree. O<sub>2</sub><sup>•−</sup> radicals was found to be the main active species in the drugs degradation. Mechanistic investigations revealed a first order kinetics.</div></div>","PeriodicalId":16782,"journal":{"name":"Journal of Photochemistry and Photobiology A-chemistry","volume":"468 ","pages":"Article 116465"},"PeriodicalIF":4.1,"publicationDate":"2025-05-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143935763","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Photodegradation of polystyrene microplastics exposed to natural sunlight 聚苯乙烯微塑料暴露在自然阳光下的光降解

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-06 DOI: 10.1016/j.jphotochem.2025.116462

Zeynep Kilinc , Gamze Yesilay , Demet Cetin , Zekiye Suludere , Suad Rashdan , Layla Hazeem , Mohamed Bououdina , George Z. Kyzas

{"title":"Photodegradation of polystyrene microplastics exposed to natural sunlight","authors":"Zeynep Kilinc , Gamze Yesilay , Demet Cetin , Zekiye Suludere , Suad Rashdan , Layla Hazeem , Mohamed Bououdina , George Z. Kyzas","doi":"10.1016/j.jphotochem.2025.116462","DOIUrl":"10.1016/j.jphotochem.2025.116462","url":null,"abstract":"<div><div>In the present study, we investigated the photodegradation of polystyrene microplastics (PS-MPs) exposed to natural sunlight over an extended period. Changes in particle size, surface charge, morphology, and chemical structure of PS-MPs were evaluated using Dynamic Light Scattering (DLS), Zeta potential measurements, Scanning Electron Microscopy (SEM), and Raman spectroscopy. Our findings revealed that exposure to natural sunlight significantly accelerates MP degradation process, resulting in pronounced fragmentation and chemical alterations compared to samples kept in dark conditions. While degradation occurs in the dark, light enhances the process. Therefore, researchers conducting studies on the toxicity of MP should include photodegradation parameter in the environmental impact assessment of MPs. Our findings highlight the importance of photodegradation in understanding the environmental fate and impact of PS-MPs. Further research can focus on the ecological implications of these chemical changes and the interactions of degraded particles with marine biota.</div></div>","PeriodicalId":16782,"journal":{"name":"Journal of Photochemistry and Photobiology A-chemistry","volume":"468 ","pages":"Article 116462"},"PeriodicalIF":4.1,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143924848","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Three fluorescent probes based on the D-π-A configuration to detect changes in endoplasmic reticulum polarity 基于D-π-A结构的三种荧光探针检测内质网极性的变化

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-05 DOI: 10.1016/j.jphotochem.2025.116480

Jie Wang , Sichen Zhang , Jiale Li , Aobo Sun , Aixiang Ding , Lei Hu , Chunfei Wang , Hui Wang

{"title":"Three fluorescent probes based on the D-π-A configuration to detect changes in endoplasmic reticulum polarity","authors":"Jie Wang , Sichen Zhang , Jiale Li , Aobo Sun , Aixiang Ding , Lei Hu , Chunfei Wang , Hui Wang","doi":"10.1016/j.jphotochem.2025.116480","DOIUrl":"10.1016/j.jphotochem.2025.116480","url":null,"abstract":"<div><div>Abnormal fluctuations in the polarity of the endoplasmic reticulum (ER), a critical intracellular organelle, have been closely associated with the onset and progression of various diseases. Consequently, monitoring ER polarity fluctuations is of significant practical importance for the diagnosis and treatment of these conditions. In this study, we designed and synthesized three ER-targeted polarity fluorescent probes, <strong>TCF1-TCF3</strong>  <strong>TCF3</strong> <!-->achieved high-quality imaging even at a low concentration of 0.5 μM. These properties enable <strong>TCF3</strong> to effectively monitor ER polarity changes induced by a variety of conditions such as DTT, tunicamycin, etc., highlighting its potential as a valuable tool for studying ER-related cellular processes.</div></div>","PeriodicalId":16782,"journal":{"name":"Journal of Photochemistry and Photobiology A-chemistry","volume":"468 ","pages":"Article 116480"},"PeriodicalIF":4.1,"publicationDate":"2025-05-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143913170","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Novel antifouling and photocatalytic immobilized iron-doped cerium oxide@halloysite nanotubes decorated polyethersulfone membranes 新型防污光催化固定化铁掺杂铈oxide@halloysite纳米管修饰聚醚砜膜

IF 4.1 3区化学

Journal of Photochemistry and Photobiology A-chemistry Pub Date : 2025-05-05 DOI: 10.1016/j.jphotochem.2025.116478

Kgolofelo I. Malatjie , Richard M. Moutloali , Ajay K. Mishra , Shivani B. Mishra , Edward N. Nxumalo

{"title":"Novel antifouling and photocatalytic immobilized iron-doped cerium oxide@halloysite nanotubes decorated polyethersulfone membranes","authors":"Kgolofelo I. Malatjie , Richard M. Moutloali , Ajay K. Mishra , Shivani B. Mishra , Edward N. Nxumalo","doi":"10.1016/j.jphotochem.2025.116478","DOIUrl":"10.1016/j.jphotochem.2025.116478","url":null,"abstract":"<div><div>Novel polyethersulfone (PES) ultrafiltration (UF) membranes were prepared by incorporating different contents of iron-doped cerium oxide-halloysite nanotubes (FC@NHT) nanocomposites onto the PES membranes. The properties of the prepared nanocomposite membranes were investigated using Attenuated Total Reflectance-Fourier Transform Infrared spectroscopy (ATR-FTIR), X-ray diffraction (XRD), thermo-gravimetric analyzer (TGA) and scanning electron microscope (SEM). The results showed that iron dopped cerium oxide (FC) was indeed successfully loaded on the surface of halloysite nanotubes (HNTs). SEM characterization of FC@HNT/PES membranes showed an increase in pore sizes and microvoids which resulted in an increase in both hydrophilicity and flux due to the impact of FC@HNT. Pure water flux of 2% FC@HNT/PES (M4) was increased from 55.9 L.m<sup>−2</sup>.h<sup>−1</sup> (0% FC@HNT/PES) to 320.4 L.m<sup>−2</sup>.h<sup>−1</sup>. The membranes also showed high antifouling properties towards humic acid (HA). This was attributed to the membranes becoming more hydrophilic upon modification. Subsequently, this reduced membrane-foulant hydrophobic interactions and made it difficult for hydrophobic contaminants to be attached onto the membranes surface. Photocatalytic ability of the modified membranes was tested against imidacloprid (IMD) insecticides. The membrane (M4) showed high photocatalytic activity of about 79% in 120 mins and 85.7% in 180 mins. The immobilization of FC onto the surface of the HNTs was for the homogenous dispersion of the nanoparticles and to mitigate the issue of agglomeration. Other remarkable functionalities are also provided by this integration. The membrane’s ability to function as system for water filtration and for the degradation of imidacloprid pesticide with high antifouling propensity is by far its most intriguing aspect of this work.</div></div>","PeriodicalId":16782,"journal":{"name":"Journal of Photochemistry and Photobiology A-chemistry","volume":"468 ","pages":"Article 116478"},"PeriodicalIF":4.1,"publicationDate":"2025-05-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144083882","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0