Frontiers of Optoelectronics最新文献

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Achievable information rate optimization in C-band optical fiber communication system. c波段光纤通信系统可实现的信息速率优化。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-06-29 DOI: 10.1007/s12200-023-00072-5
Zheng Liu, Tianhua Xu, Ji Qi, Joshua Uduagbomen, Jian Zhao, Tiegen Liu
{"title":"Achievable information rate optimization in C-band optical fiber communication system.","authors":"Zheng Liu,&nbsp;Tianhua Xu,&nbsp;Ji Qi,&nbsp;Joshua Uduagbomen,&nbsp;Jian Zhao,&nbsp;Tiegen Liu","doi":"10.1007/s12200-023-00072-5","DOIUrl":"https://doi.org/10.1007/s12200-023-00072-5","url":null,"abstract":"<p><p>Optical fiber communication networks play an important role in the global telecommunication network. However, nonlinear effects in the optical fiber and transceiver noise greatly limit the performance of fiber communication systems. In this paper, the product of mutual information (MI) and communication bandwidth is used as the metric of the achievable information rate (AIR). The MI loss caused by the transceiver is also considered in this work, and the bit-wise MI, generalized mutual information (GMI), is used to calculate the AIR. This loss is more significant in the use of higher-order modulation formats. The AIR analysis is carried out in the QPSK, 16QAM, 64QAM and 256QAM modulation formats for the communication systems with different communication bandwidths and transmission distances based on the enhanced Gaussian noise (EGN) model. The paper provides suggestions for the selection of the optimal modulation format in different transmission scenarios.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"17"},"PeriodicalIF":5.4,"publicationDate":"2023-06-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10307731/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"10105186","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Impact of film thickness in laser-induced periodic structures on amorphous Si films. 激光诱导周期结构中薄膜厚度对非晶硅薄膜的影响。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-06-20 DOI: 10.1007/s12200-023-00071-6
Liye Xu, Jiao Geng, Liping Shi, Weicheng Cui, Min Qiu
{"title":"Impact of film thickness in laser-induced periodic structures on amorphous Si films.","authors":"Liye Xu,&nbsp;Jiao Geng,&nbsp;Liping Shi,&nbsp;Weicheng Cui,&nbsp;Min Qiu","doi":"10.1007/s12200-023-00071-6","DOIUrl":"https://doi.org/10.1007/s12200-023-00071-6","url":null,"abstract":"<p><p>We report self-organized periodic nanostructures on amorphous silicon thin films by femtosecond laser-induced oxidation. The dependence of structural periodicity on the thickness of silicon films and the substrate materials is investigated. The results reveal that when silicon film is 200 nm, the period of self-organized nanostructures is close to the laser wavelength and is insensitive to the substrates. In contrast, when the silicon film is 50 nm, the period of nanostructures is much shorter than the laser wavelength, and is dependent on the substrates. Furthermore, we demonstrate that, for the thick silicon films, quasi-cylindrical waves dominate the formation of periodic nanostructures, while for the thin silicon films, the formation originates from slab waveguide modes. Finite-difference time-domain method-based numerical simulations support the experimental discoveries.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"16"},"PeriodicalIF":5.4,"publicationDate":"2023-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10281936/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"10066284","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Optical engineering of infrared PbS CQD photovoltaic cells for wireless optical power transfer systems. 无线光功率传输系统红外PbS CQD光伏电池的光学工程。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-06-15 DOI: 10.1007/s12200-023-00069-0
Mengqiong Zhu, Yuanbo Zhang, Shuaicheng Lu, Zijun Wang, Junbing Zhou, Wenkai Ma, Ruinan Zhu, Guanyuan Chen, Jianbing Zhang, Liang Gao, Jiancan Yu, Pingqi Gao, Jiang Tang
{"title":"Optical engineering of infrared PbS CQD photovoltaic cells for wireless optical power transfer systems.","authors":"Mengqiong Zhu,&nbsp;Yuanbo Zhang,&nbsp;Shuaicheng Lu,&nbsp;Zijun Wang,&nbsp;Junbing Zhou,&nbsp;Wenkai Ma,&nbsp;Ruinan Zhu,&nbsp;Guanyuan Chen,&nbsp;Jianbing Zhang,&nbsp;Liang Gao,&nbsp;Jiancan Yu,&nbsp;Pingqi Gao,&nbsp;Jiang Tang","doi":"10.1007/s12200-023-00069-0","DOIUrl":"https://doi.org/10.1007/s12200-023-00069-0","url":null,"abstract":"<p><p>Infrared photovoltaic cells (IRPCs) have attracted considerable attention for potential applications in wireless optical power transfer (WOPT) systems. As an efficient fiber-integrated WOPT system typically uses a 1550 nm laser beam, it is essential to tune the peak conversion efficiency of IRPCs to this wavelength. However, IRPCs based on lead sulfide (PbS) colloidal quantum dots (CQDs) with an excitonic peak of 1550 nm exhibit low short circuit current (J<sub>sc</sub>) due to insufficient absorption under monochromatic light illumination. Here, we propose comprehensive optical engineering to optimize the device structure of IRPCs based on PbS CQDs, for 1550 nm WOPT systems. The absorption by the device is enhanced by improving the transmittance of tin-doped indium oxide (ITO) in the infrared region and by utilizing the optical resonance effect in the device. Therefore, the optimized device exhibited a high short circuit current density of 37.65 mA/cm<sup>2</sup> under 1 sun (AM 1.5G) solar illumination and 11.91 mA/cm<sup>2</sup> under 1550 nm illumination 17.3 mW/cm<sup>2</sup>. Furthermore, the champion device achieved a record high power conversion efficiency (PCE) of 7.17% under 1 sun illumination and 10.29% under 1550 nm illumination. The PbS CQDs IRPCs under 1550 nm illumination can even light up a liquid crystal display (LCD), demonstrating application prospects in the future.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"15"},"PeriodicalIF":5.4,"publicationDate":"2023-06-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10271996/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"9654629","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Revealing the interaction mechanism of pulsed laser processing with the application of acoustic emission. 揭示了脉冲激光加工与声发射应用的相互作用机理。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-06-14 DOI: 10.1007/s12200-023-00070-7
Weinan Liu, Youmin Rong, Ranwu Yang, Congyi Wu, Guojun Zhang, Yu Huang
{"title":"Revealing the interaction mechanism of pulsed laser processing with the application of acoustic emission.","authors":"Weinan Liu,&nbsp;Youmin Rong,&nbsp;Ranwu Yang,&nbsp;Congyi Wu,&nbsp;Guojun Zhang,&nbsp;Yu Huang","doi":"10.1007/s12200-023-00070-7","DOIUrl":"https://doi.org/10.1007/s12200-023-00070-7","url":null,"abstract":"<p><p>The mechanisms of interaction between pulsed laser and materials are complex and indistinct, severely influencing the stability and quality of laser processing. This paper proposes an intelligent method based on the acoustic emission (AE) technique to monitor laser processing and explore the interaction mechanisms. The validation experiment is designed to perform nanosecond laser dotting on float glass. Processing parameters are set differently to generate various outcomes: ablated pits and irregular-shaped cracks. In the signal processing stage, we divide the AE signals into two bands, main and tail bands, according to the laser processing duration, to study the laser ablation and crack behavior, respectively. Characteristic parameters extracted by a method that combines framework and frame energy calculation of AE signals can effectively reveal the mechanisms of pulsed laser processing. The main band features evaluate the degree of laser ablation from the time and intensity scales, and the tail band characteristics demonstrate that the cracks occur after laser dotting. In addition, from the analysis of the parameters of the tail band very large cracks can be efficiently distinguished. The intelligent AE monitoring method was successfully applied in exploring the interaction mechanism of nanosecond laser dotting float glass and can be used in other pulsed laser processing fields.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"14"},"PeriodicalIF":5.4,"publicationDate":"2023-06-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10267076/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"9642400","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Two types of ultrafast mode-locking operations from an Er-doped fiber laser based on germanene nanosheets. 锗烯纳米片掺铒光纤激光器的两种超快锁模操作。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-06-07 DOI: 10.1007/s12200-023-00068-1
Baohao Xu, Zhiyuan Jin, Lie Shi, Huanian Zhang, Qi Liu, Peng Qin, Kai Jiang, Jing Wang, Wenjing Tang, Wei Xia
{"title":"Two types of ultrafast mode-locking operations from an Er-doped fiber laser based on germanene nanosheets.","authors":"Baohao Xu,&nbsp;Zhiyuan Jin,&nbsp;Lie Shi,&nbsp;Huanian Zhang,&nbsp;Qi Liu,&nbsp;Peng Qin,&nbsp;Kai Jiang,&nbsp;Jing Wang,&nbsp;Wenjing Tang,&nbsp;Wei Xia","doi":"10.1007/s12200-023-00068-1","DOIUrl":"https://doi.org/10.1007/s12200-023-00068-1","url":null,"abstract":"<p><p>As a member of Xenes family, germanene has excellent nonlinear saturable absorption characteristics. In this work, we prepared germanene nanosheets by liquid phase exfoliation and measured their saturation intensity as 0.6 GW/cm<sup>2</sup> with a modulation depth of 8%. Then, conventional solitons with a pulse width of 946 fs and high-energy noise-like pulses with a pulse width of 784 fs were obtained by using germanene nanosheet as a saturable absorber for a mode-locked Erbium-doped fiber laser. The characteristics of the two types of pulses were investigated experimentally. The results reveal that germanene has great potential for modulation devices in ultrafast lasers and can be used as a material for creation of excellent nonlinear optical devices to explore richer applications in ultrafast photonics.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"13"},"PeriodicalIF":5.4,"publicationDate":"2023-06-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10247613/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"9598243","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Generation of mode-locked states of conventional solitons and bright-dark solitons in graphene mode-locked fiber laser. 在石墨烯锁模光纤激光器中产生传统孤子和明暗孤子的锁模态。
IF 4.1 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-06-02 DOI: 10.1007/s12200-023-00067-2
Zixiong Li, Mingyu Li, Xinyi Hou, Lei Du, Lin Xiao, Tianshu Wang, Wanzhuo Ma
{"title":"Generation of mode-locked states of conventional solitons and bright-dark solitons in graphene mode-locked fiber laser.","authors":"Zixiong Li, Mingyu Li, Xinyi Hou, Lei Du, Lin Xiao, Tianshu Wang, Wanzhuo Ma","doi":"10.1007/s12200-023-00067-2","DOIUrl":"10.1007/s12200-023-00067-2","url":null,"abstract":"<p><p>This paper proposes a mode-locked fiber laser based on graphene-coated microfiber. The total length of the fiber laser resonant cavity is 31.34 m. Under the condition of stable output of bright-dark soliton pairs from the fiber laser, dual-wavelength tuning is realized by adjusting the polarization controller (PC), and the wavelength tuning range is 11 nm. Furthermore, the effects of polarization states on bright-dark solitons are studied. It is demonstrated that the mode-locking state can be switched between conventional solitons and bright-dark solitons in the graphene mode-locked fiber laser. Bright-dark soliton pairs with different shapes and nanosecond pulse width can be obtained by adjusting the PC and pump power.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"12"},"PeriodicalIF":4.1,"publicationDate":"2023-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10238347/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"9928995","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A broadband integrated microwave photonic mixer based on balanced photodetection. 一种基于平衡光探测的宽带集成微波光子混频器。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-05-26 DOI: 10.1007/s12200-023-00064-5
Zhenzhu Xu, Li Mei, Yuhua Chong, Xudong Gao, Shoubao Han, Chengkun Yang, Lin Li
{"title":"A broadband integrated microwave photonic mixer based on balanced photodetection.","authors":"Zhenzhu Xu,&nbsp;Li Mei,&nbsp;Yuhua Chong,&nbsp;Xudong Gao,&nbsp;Shoubao Han,&nbsp;Chengkun Yang,&nbsp;Lin Li","doi":"10.1007/s12200-023-00064-5","DOIUrl":"https://doi.org/10.1007/s12200-023-00064-5","url":null,"abstract":"<p><p>An integrated microwave photonic mixer based on silicon photonic platforms is proposed, which consist of a dual-drive Mach-Zehnder modulator and a balanced photodetector. The modulated optical signals from microwave photonic links can be directly demodulated and down-converted to intermediate frequency (IF) signals by the photonic mixer. The converted signal is obtained by conducting off-chip subtraction of the outputs from the balanced photodetector, and subsequent filtering of the high frequency items by an electrical low-pass filter. Benefiting from balanced detection, the conversion gain of the IF signal is improved by 6 dB, and radio frequency leakage and common-mode noise are suppressed significantly. System-level simulations show that the frequency mixing system has a spurious-free dynamic range of 89 dB·Hz<sup>2/3</sup>, even with deteriorated linearity caused by the two cascaded modulators. The spur suppression ratio of the photonic mixer remains higher than 40 dB when the IF varies from 0.5 to 4 GHz. The electrical-electrical 3 dB bandwidth of frequency conversion is 11 GHz. The integrated frequency mixing approach is quite simple, requiring no extra optical filters or electrical 90° hybrid coupler, which makes the system more stable and with broader bandwidth so that it can meet the potential demand in practical applications.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"11"},"PeriodicalIF":5.4,"publicationDate":"2023-05-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10219908/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"9536352","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Recent progress of in-fiber WGM microsphere resonator. 光纤内WGM微球谐振器研究进展。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-05-25 DOI: 10.1007/s12200-023-00066-3
Yong Yang, Zijie Wang, Xiaobei Zhang, Qi Zhang, Tingyun Wang
{"title":"Recent progress of in-fiber WGM microsphere resonator.","authors":"Yong Yang,&nbsp;Zijie Wang,&nbsp;Xiaobei Zhang,&nbsp;Qi Zhang,&nbsp;Tingyun Wang","doi":"10.1007/s12200-023-00066-3","DOIUrl":"https://doi.org/10.1007/s12200-023-00066-3","url":null,"abstract":"<p><p>In-fiber whispering gallery mode (WGM) microsphere resonators have received remarkable attention due to the superiorities of compact structure, high stability and self-alignment. As an in-fiber structure, WGM microsphere resonators have been demonstrated in various applications, such as sensors, filters and lasers, which have significant impacts on modern optics. Herein, we review recent progress of in-fiber WGM microsphere resonators, which involve fibers of diverse structures and microspheres of different materials. First, a brief introduction is given to in-fiber WGM microsphere resonators, from structures to applications. Then, we focus on recent progresses in this field, including in-fiber couplers based on conventional fibers, capillaries and micro-structure hollow fibers, and passive/active microspheres. Finally, future developments of the in-fiber WGM microsphere resonators are envisioned.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"10"},"PeriodicalIF":5.4,"publicationDate":"2023-05-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10209386/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"9895373","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Light response and adsorption interaction of black phosphorus quantum dots and single-layer graphene phototransistor. 黑磷量子点与单层石墨烯光电晶体管的光响应及吸附相互作用。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-05-24 DOI: 10.1007/s12200-023-00065-4
Qi Han, Yadong Jiang, Xianchao Liu, Chaoyi Zhang, Jun Wang
{"title":"Light response and adsorption interaction of black phosphorus quantum dots and single-layer graphene phototransistor.","authors":"Qi Han,&nbsp;Yadong Jiang,&nbsp;Xianchao Liu,&nbsp;Chaoyi Zhang,&nbsp;Jun Wang","doi":"10.1007/s12200-023-00065-4","DOIUrl":"https://doi.org/10.1007/s12200-023-00065-4","url":null,"abstract":"<p><p>Black phosphorus quantum dots (BPQDs) are synthesized and combined with graphene sheet. The fabricated BPQDs/graphene devices are capable of detecting visible and near infrared radiation. The adsorption effect of BPQDs in graphene is clarified by the relationship of the photocurrent and the shift of the Dirac point with different substrate. The Dirac point moves toward a neutral point under illumination with both SiO<sub>2</sub>/Si and Si<sub>3</sub>N<sub>4</sub>/Si substrates, indicating an anti-doped feature of photo-excitation. To our knowledge, this provides the first observation of photoresist induced photocurrent in such systems. Without the influence of the photoresist the device can respond to infrared light up to 980 nm wavelength in vacuum in a cryostat, in which the photocurrent is positive and photoconduction effect is believed to dominate the photocurrent. Finally, the adsorption effect is modeled using a first-principle method to give a picture of charge transfer and orbital contribution in the interaction of phosphorus atoms and single-layer graphene.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"9"},"PeriodicalIF":5.4,"publicationDate":"2023-05-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10209371/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"9526233","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Efficient soluble PTCBI-type non-fullerene acceptor materials for organic solar cells. 有机太阳能电池用高效可溶性ptcbi型非富勒烯受体材料。
IF 5.4 3区 工程技术
Frontiers of Optoelectronics Pub Date : 2023-04-23 DOI: 10.1007/s12200-023-00063-6
Xiang Gao, Fengbo Sun, Xinzhu Tong, Xufan Zheng, Yinuo Wang, Cong Xiao, Pengcheng Li, Renqiang Yang, Xunchang Wang, Zhitian Liu
{"title":"Efficient soluble PTCBI-type non-fullerene acceptor materials for organic solar cells.","authors":"Xiang Gao,&nbsp;Fengbo Sun,&nbsp;Xinzhu Tong,&nbsp;Xufan Zheng,&nbsp;Yinuo Wang,&nbsp;Cong Xiao,&nbsp;Pengcheng Li,&nbsp;Renqiang Yang,&nbsp;Xunchang Wang,&nbsp;Zhitian Liu","doi":"10.1007/s12200-023-00063-6","DOIUrl":"https://doi.org/10.1007/s12200-023-00063-6","url":null,"abstract":"<p><p>Single perylene diimide (PDI) used as a non-fullerene acceptor (NFA) in organic solar cells (OSCs) is enticing because of its low cost and excellent stability. To improve the photovoltaic performance, it is vital to narrow the bandgap and regulate the stacking behavior. To address this challenge, we synthesize soluble perylenetetracarboxylic bisbenzimidazole (PTCBI) molecules with a bulky side chain at the bay region, by replacing the widely used \"swallow tail\" type alkyl chains at the imide position of PDI molecules with a planar benzimidazole structure. Compared with PDI molecules, PTCBI molecules exhibit red-shifted UV-vis absorption spectra with larger extinction coefficient, and one magnitude higher electron mobility. Finally, OSCs based on one soluble PTCBI-type NFA, namely MAS-7, exhibit a champion power conversion efficiency (PCE) of 4.34%, which is significantly higher than that of the corresponding PDI-based OSCs and is the highest PCE of PTCBI-based OSCs reported. These results highlight the potential of soluble PTCBI derivatives as NFAs in OSCs.</p>","PeriodicalId":12685,"journal":{"name":"Frontiers of Optoelectronics","volume":"16 1","pages":"8"},"PeriodicalIF":5.4,"publicationDate":"2023-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10122612/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"9423006","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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