Current Opinion in Electrochemistry最新文献_第2页

Recent advances in graphene-based electrochemical biosensors for major non-communicable diseases 用于重大非传染性疾病的石墨烯电化学生物传感器的最新进展

IF 6.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-25 DOI: 10.1016/j.coelec.2025.101737

Tathagata Bhattacharjya , Martin–Alex Nalepa , Ivan Dědek , Petr Jakubec , David Panáček , Michal Otyepka

{"title":"Recent advances in graphene-based electrochemical biosensors for major non-communicable diseases","authors":"Tathagata Bhattacharjya , Martin–Alex Nalepa , Ivan Dědek , Petr Jakubec , David Panáček , Michal Otyepka","doi":"10.1016/j.coelec.2025.101737","DOIUrl":"10.1016/j.coelec.2025.101737","url":null,"abstract":"<div><div>Non-communicable diseases, including cancer, cardiovascular diseases, diabetes, and neurological disorders, represent a growing global health challenge, driving an urgent need for rapid, sensitive, and affordable diagnostic technologies. Graphene-based materials, with their exceptional physicochemical properties, offer transformative potential for the development of next-generation electrochemical biosensors. This review highlights recent advancements in the use of graphene derivatives (such as reduced graphene oxide, graphene quantum dots, laser-induced graphene, and covalently functionalized graphene) for the electrochemical detection of key biomarkers associated with major non-communicable diseases. We critically analyze strategies for enhancing biosensor performance, discuss innovations in biomarker recognition and real-sample validation, and underscore emerging trends toward wearable, minimally invasive platforms. Particular emphasis is placed on the challenges of selectivity, stability, and clinical translation, as well as on the need for reproducible material synthesis and device standardization. By bridging material science with biomedical applications, graphene-based biosensors are poised to enable earlier diagnosis, continuous monitoring, and improved management of non-communicable diseases, ultimately contributing to the advancement of global healthcare.</div></div>","PeriodicalId":11028,"journal":{"name":"Current Opinion in Electrochemistry","volume":"53 ","pages":"Article 101737"},"PeriodicalIF":6.9,"publicationDate":"2025-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144829523","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Impedimetric aptasensors: Emerging tools for sensitive detection in health, food, and environmental monitoring 阻抗感应传感器：用于健康、食品和环境监测中敏感检测的新兴工具

IF 6.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-25 DOI: 10.1016/j.coelec.2025.101736

Arzum Erdem, Huseyin Senturk, Cengiz Altınsoy

{"title":"Impedimetric aptasensors: Emerging tools for sensitive detection in health, food, and environmental monitoring","authors":"Arzum Erdem, Huseyin Senturk, Cengiz Altınsoy","doi":"10.1016/j.coelec.2025.101736","DOIUrl":"10.1016/j.coelec.2025.101736","url":null,"abstract":"<div><div>Electrochemical impedance spectroscopy (EIS)-based aptasensors combine the high selectivity of aptamers as biorecognition elements with the label-free, sensitive, and noninvasive measurement capabilities of EIS. Owing to these features, they have recently attracted considerable attention, offering a wide range of applications from the early diagnosis of numerous biomarkers in the field of healthcare to food safety and environmental analysis. In this review, the fundamental principles of impedimetric aptasensors are discussed, and studies published over the last two years in the fields of health, food, and environment are comprehensively examined. In this context, recent original research on the development of aptasensors for the detection of various analytes including cancer biomarkers, viral and bacterial pathogens, mycotoxins, antibiotic residues, hormones, and heavy metals has been analyzed in detail. Moreover, recent findings supporting the applicability of these aptasensors in complex biological (e.g. serum, plasma, saliva, urine), food (e.g. milk, fruit juice, cereal products), and environmental (e.g. wastewater, river water) sample matrices have been summarized. Additionally, key application-oriented challenges such as optimization of surface chemistry for aptamer immobilization, minimization of matrix effects, sensor surface stability, repeatability/reproducibility, multiplex detection, and integration into portable platforms have been thoroughly discussed. Furthermore, innovative solutions that could facilitate the transition of this technology into clinical and field applications, as well as future perspectives regarding commercialization, have been presented. In this regard, it is emphasized that impedimetric aptasensors possess strong potential not only at the laboratory scale but also as powerful tools for real-world diagnostic and monitoring applications.</div></div>","PeriodicalId":11028,"journal":{"name":"Current Opinion in Electrochemistry","volume":"53 ","pages":"Article 101736"},"PeriodicalIF":6.9,"publicationDate":"2025-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144863194","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Next-generation plasma-sprayed electrodes for water electrolysis and beyond: Recent advances and future directions 用于水电解及其他领域的下一代等离子喷涂电极：最新进展和未来方向

IF 6.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-22 DOI: 10.1016/j.coelec.2025.101732

Glen McClea , Laura Titheridge , Steven Matthews , Aaron T. Marshall

{"title":"Next-generation plasma-sprayed electrodes for water electrolysis and beyond: Recent advances and future directions","authors":"Glen McClea , Laura Titheridge , Steven Matthews , Aaron T. Marshall","doi":"10.1016/j.coelec.2025.101732","DOIUrl":"10.1016/j.coelec.2025.101732","url":null,"abstract":"<div><div>Conventional industrial alkaline water electrolysis electrodes made using plasma spray deposition are unable to produce and sustain the demanding performance requirements needed to achieve economic targets. State-of-the-art lab-scale alkaline electrolysis configurations can achieve these higher performances; however, given their complex electrode architecture and production methods, often suffer from practical limitations regarding scale-up. Proven and trusted by industry, plasma spraying offers a pragmatic and cost-effective method for fabricating these next-generation electrodes at scale. This review explores the most recent advances in plasma-sprayed electrode development, covering its use to form both the active catalyst layer and the porous transport layer. We also highlight how these findings can be transferred to benefit the development of other industrial process electrodes. This review aims to provide pathways for future research, showing how novel lab-scale electrodes can be replicated at scale, with the latest in plasma-spray technology.</div></div>","PeriodicalId":11028,"journal":{"name":"Current Opinion in Electrochemistry","volume":"53 ","pages":"Article 101732"},"PeriodicalIF":6.9,"publicationDate":"2025-07-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144828230","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Organic and molecular electrochemistry: Tools, interfaces and interdisciplinary frontiers 有机和分子电化学：工具、界面和跨学科前沿

IF 6.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-22 DOI: 10.1016/j.coelec.2025.101735

Serena Arnaboldi, Sara Grecchi

引用次数: 0

Reactor designs for pH-swing electrochemical CO2 capture ph -摆动电化学CO2捕获反应器设计

IF 6.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-19 DOI: 10.1016/j.coelec.2025.101731

Yuesheng Zhang, Haoxiang Bai, Yuhang Wang

引用次数: 0

Shaping the next-generation of fused deposition modeling three-dimensional-printing-based electrochemical (bio)sensing: Drawing a realistic horizon 塑造下一代熔融沉积建模三维打印电化学（生物）传感：绘制现实的地平线

IF 6.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-15 DOI: 10.1016/j.coelec.2025.101730

Miriam Chávez , Fabiana Arduini , Alberto Escarpa

引用次数: 0

Local pH engineering to impact electrocatalysis 局部pH工程影响电催化

IF 6.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-09 DOI: 10.1016/j.coelec.2025.101728

Maxime Decker , Quentin Lenne , Jalal Ghilane , Carlos M. Sánchez-Sánchez

引用次数: 0

Magnetic support-driven electrochemical affinity biosensing: Advancing sensitive, rapid, and simplified determination of clinically relevant analytes 磁支持驱动的电化学亲和生物传感：推进敏感，快速和简化的测定临床相关分析物

IF 7.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-08 DOI: 10.1016/j.coelec.2025.101729

Susana Campuzano , Maria Gamella , José M. Pingarrón

{"title":"Magnetic support-driven electrochemical affinity biosensing: Advancing sensitive, rapid, and simplified determination of clinically relevant analytes","authors":"Susana Campuzano , Maria Gamella , José M. Pingarrón","doi":"10.1016/j.coelec.2025.101729","DOIUrl":"10.1016/j.coelec.2025.101729","url":null,"abstract":"<div><div>The demand to determine analytes at increasingly lower concentrations in complex samples, while minimizing sample size, treatment and test duration, has driven innovation in electrochemical biotechnologies. Inspired by the principle that affinity reactions gain in efficiency and speed when the biosensing surface seeks the analyte, bioelectrochemical technologies leverage their unique strengths along with those provided by magnetic carriers to improve affinity testing, pushing the boundaries of accuracy and efficiency.</div><div>This minireview focuses primarily on magnetic beads, motors, and gold-coated magnetic nanoparticles dispersible electrodes, considering the remarkable improvements they provide in electrochemical affinity biotechnologies. A timely, comparative, and critical analysis of the opportunities offered by these three magnetic supports in electrochemical affinity biodetection is carried out by highlighting and discussing some of the most innovative research. This minireview also dares to forecast the future potential of these technologies for advancing modern analytical capabilities and accelerating their integration into next-generation point-of-care devices.</div></div>","PeriodicalId":11028,"journal":{"name":"Current Opinion in Electrochemistry","volume":"53 ","pages":"Article 101729"},"PeriodicalIF":7.9,"publicationDate":"2025-07-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144711096","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Progress and pitfalls in measuring the double-layer capacitance of platinum electrodes 铂电极双层电容测量的进展与缺陷

IF 7.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-05 DOI: 10.1016/j.coelec.2025.101727

Nicci L. Fröhlich, Marc T.M. Koper

{"title":"Progress and pitfalls in measuring the double-layer capacitance of platinum electrodes","authors":"Nicci L. Fröhlich, Marc T.M. Koper","doi":"10.1016/j.coelec.2025.101727","DOIUrl":"10.1016/j.coelec.2025.101727","url":null,"abstract":"<div><div>Despite extensive research, the double-layer structure at Pt/aqueous electrolyte interfaces (quantified by the double-layer capacitance, <em>C</em><sub>dl</sub>) remains incompletely understood as even for the model Pt(111)/HClO<sub>4</sub> interface, anomalous <em>C</em><sub>dl</sub> trends have been reported. These trends were previously ascribed to differences in measurement techniques (<em>i.e.</em> dc methods such as cyclic voltammetry versus ac methods such as electrochemical impedance spectroscopy [EIS]). However, by repeating these measurements using EIS, we clarify that these anomalous <em>C</em><sub>dl</sub> trends are not measurement artefacts but instead reflect intrinsic properties of the Pt(111)/HClO<sub>4</sub> interface, necessitating continued investigation. We further highlight the complexity introduced by electrosorbed H<sub>ads</sub> and/or OH<sub>ads</sub> species resulting from catalytic H<sub>2</sub>O dissociation, which contribute an adsorption (pseudo)capacitance, <em>C</em><sub>ads</sub>. This complicates the deconvolution of <em>C</em><sub>dl</sub> from total capacitance, a challenge further exacerbated by structure-dependent adsorption between different Pt facets. Our goal is to clarify how these factors affect capacitance interpretation at Pt/aqueous electrolyte interfaces, particularly highlighting the progress and challenges in accurately extracting <em>C</em><sub>dl</sub> values from prior studies.</div></div>","PeriodicalId":11028,"journal":{"name":"Current Opinion in Electrochemistry","volume":"53 ","pages":"Article 101727"},"PeriodicalIF":7.9,"publicationDate":"2025-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144687538","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Time: The potentially powerful, often-overlooked variable in electrochemical sensing of per- and polyfluoroalkyl substances 时间：全氟烷基和多氟烷基物质电化学传感中潜在的强大的、经常被忽视的变量

IF 6.9 2区化学

Current Opinion in Electrochemistry Pub Date : 2025-07-02 DOI: 10.1016/j.coelec.2025.101726

Samantha C. Cullom , Jeffrey E. Dick

{"title":"Time: The potentially powerful, often-overlooked variable in electrochemical sensing of per- and polyfluoroalkyl substances","authors":"Samantha C. Cullom , Jeffrey E. Dick","doi":"10.1016/j.coelec.2025.101726","DOIUrl":"10.1016/j.coelec.2025.101726","url":null,"abstract":"<div><div>Modern electrochemistry places a heavy emphasis on the importance of thermodynamic measurements for environmental sensing. While most electrochemical sensors require some type of binding mechanism, analytes do not bind to sensors instantaneously; the binding process takes time, suggesting that we must examine reaction kinetics as well. With emerging environmental pollutants of concern, such as per- and polyfluoroalkyl substances (PFAS), electrochemists must consider the kinetic relationship between the electrochemical sensor and the analyte. Various types of environmental electrochemical sensors, such as enzymes, antibodies, aptamers, and molecularly imprinted polymers (MIPs), exist. Each type of sensor can be used in the environment, but MIPs have recently demonstrated strong potential to qualitatively and quantitatively detect and identify PFAS species at the earliest onset of environmental contamination. Additionally, the mathematical and experimental approaches to MIP binding have room to expand beyond the thermodynamic isotherm models and into a time-dependent kinetic model.</div></div>","PeriodicalId":11028,"journal":{"name":"Current Opinion in Electrochemistry","volume":"53 ","pages":"Article 101726"},"PeriodicalIF":6.9,"publicationDate":"2025-07-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144780048","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0