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Construction of spirotetrahydroquinolines fused with medium-sized rings via TBHP/base-promoted spirocyclization reactions thbhp /碱促进螺旋环化反应合成中型环型螺旋四氢喹啉
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-05 DOI: 10.1039/d5qo00648a
Peng He, Yuanyang Mu, Zongkang Wang, Nana Fei, Chengyu Wang, Yanzhong Li
{"title":"Construction of spirotetrahydroquinolines fused with medium-sized rings via TBHP/base-promoted spirocyclization reactions","authors":"Peng He, Yuanyang Mu, Zongkang Wang, Nana Fei, Chengyu Wang, Yanzhong Li","doi":"10.1039/d5qo00648a","DOIUrl":"https://doi.org/10.1039/d5qo00648a","url":null,"abstract":"An efficient and straightforward methodology for synthesising spirotetrahydroquinolines fused with medium-sized rings (including 7, 8, and 9-membered rings) by TBHP/base-promoted spirocyclization reactions has been developed. The present report provides a transition-metal-free method with a wide range of substitution patterns, functional group compatibility and good diastereoselectivity.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"5 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144219155","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chiral Bifunctional N, N, P-Ligand-Enabled Cooperative Cu Catalysis: One-Pot Two-Step Propargylic Substitution of Propargylic Alcohols 手性双功能N， N， p配体支持的Cu协同催化：丙炔醇的一锅两步丙炔取代
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-05 DOI: 10.1039/d5qo00595g
Ruinan Zhao, Zihao Wang, Ting Fang, Chibin Zhang, Lijun Tang, Cuiju Zhu, Hao Xu
{"title":"Chiral Bifunctional N, N, P-Ligand-Enabled Cooperative Cu Catalysis: One-Pot Two-Step Propargylic Substitution of Propargylic Alcohols","authors":"Ruinan Zhao, Zihao Wang, Ting Fang, Chibin Zhang, Lijun Tang, Cuiju Zhu, Hao Xu","doi":"10.1039/d5qo00595g","DOIUrl":"https://doi.org/10.1039/d5qo00595g","url":null,"abstract":"Propargyl moieties are important structural features that are ubiquitously found in numerous natural products and pharmaceutical molecules. Due to the high reaction barrier, copper-catalyzed enantioselective propargylation with propargylic alcohol has not been reported so far. Herein, we describe the first example of copper catalytic asymmetric propargylic substitution reactions of propargylic alcohols. The N, N, P-ligand functioned as a bifunctional reagent, acting as a base catalyst to promote the esterification of propargylic alcohols and serving as a tridentate ligand to coordinate with copper salts, thereby forming the catalyst that activates propargylic esters. The methodology proceeds under mild reaction conditions and is tolerant of N-, C-, and O-nucleophiles, generating propargylic substitution products in good to excellent yields with high enantioselectivities (up to 95% yield, 97% ee). This methodology might open a new avenue for designing copper-catalyzed propargylic substitution reactions with propargylic alcohols.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"52 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144219153","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ni-catalyzed reductive cross-couplings of diaryl disulfides with aryl bromides for biaryl synthesis through C-S bond cleavage 镍催化二芳基二硫化物与芳基溴的还原交叉偶联，通过C-S键裂解合成联芳基
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-04 DOI: 10.1039/d5qo00546a
Xuan-Qi Zhang, Cai-Yu He, Shuang-Feng Song, Xue-Qiang Chu, Hao Xu, Xiaocong Zhou, Weidong Rao, Zhi-Liang Shen
{"title":"Ni-catalyzed reductive cross-couplings of diaryl disulfides with aryl bromides for biaryl synthesis through C-S bond cleavage","authors":"Xuan-Qi Zhang, Cai-Yu He, Shuang-Feng Song, Xue-Qiang Chu, Hao Xu, Xiaocong Zhou, Weidong Rao, Zhi-Liang Shen","doi":"10.1039/d5qo00546a","DOIUrl":"https://doi.org/10.1039/d5qo00546a","url":null,"abstract":"In previous reports, the cross-couplings of diaryl disulfides with aryl halides in the presence of transition metal catalyst (e.g., Ni, Cu) and metal mediator (e.g., Mg, Zn) usually led to the corresponding aryl sulfides via old S-S bond cleavage and new C-S bond formation. In the present study, we found that the reductive cross-couplings of diaryl disulfides with aryl bromides proceeded via unusual C-S bond cleavage in the presence of nickel catalyst, magnesium, and lithium chloride in THF at room temperature, leading to a variety of biaryls in modest to good yields. In addition, the reaction could be scaled-up with ease. Mechanistic studies showed that the reaction possibly proceeds via the in situ production of arylmagnesium compound as reaction intermediate via LiCl-facilitated Mg insertion into aryl bromide. Most importantly, the combinatory use of Ni(II) catalyst and Mg mediator is the key for the unusual cleavage of the C-S bond in diaryl disulfide to form the corresponding arylnickel(II) species which serves as another important intermediate of the present desulfurated cross-coupling reaction.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"32 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144211687","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The construction of aromatic rings by photocatalytic radical-induced cyclization reactions 光催化自由基诱导环化反应构建芳环
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-04 DOI: 10.1039/d5qo00667h
Xi-Ni Luo, Dong-Qing Yang, Hong-Lin Wu, Jia-Yao Feng, Sheng Du, Yu He, Rongnan Yi, Jun-Qi Zhang, Keqi Tang, Wenting Wei
{"title":"The construction of aromatic rings by photocatalytic radical-induced cyclization reactions","authors":"Xi-Ni Luo, Dong-Qing Yang, Hong-Lin Wu, Jia-Yao Feng, Sheng Du, Yu He, Rongnan Yi, Jun-Qi Zhang, Keqi Tang, Wenting Wei","doi":"10.1039/d5qo00667h","DOIUrl":"https://doi.org/10.1039/d5qo00667h","url":null,"abstract":"Photocatalytic radical-induced cyclization reactions offer an efficient paradigm for constructing aromatic rings due to their unique environmental friendliness, independence from electronic effects, and high functional group tolerance. However, the high reactivity of intermediates in radical reactions, particularly the challenges of controlling it proceeds in an orderly manner according to the expected pathway and the reaction terminates after the ring is formed, which leads to diminished precision in the construction of aromatic rings. Compared to traditional cyclization methods for synthesizing aromatic rings, photocatalysis enables direct cleavage of high-bond-energy chemical bonds under mild conditions, eliminating the need for high temperature, high pressure, or stoichiometric oxidants. Furthermore, photocatalytic systems can serve as a bridge to connect multiple reaction steps, thereby streamlining the process and enhancing efficiency. Recently, significant progress has been made in applying photocatalytic radical-induced cyclization for the construction of aromatic rings. However, to date, there has been no comprehensive summary of this area reported. In this review, we try to provide a comprehensive perspective on the construction of aromatic rings via photocatalytic radical-induced cyclization. The discussion is organized into five sections based on the type of aromatic ring formed: monoheteroatom-doped aromatic rings, diheteroatom-doped aromatic rings, triheteroatom-doped aromatic rings, all-carbon aromatic ring, and non-classical aromatic rings. This review with a particular focus on elucidating reaction mechanisms, the synergistic effect of catalysts and light sources, and the applications of this strategy in pharmaceutical synthesis and materials science.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"17 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144211686","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Facile Synthesis of a Contorted Polycyclic Aromatic Hydrocarbon Derivative 一种扭曲多环芳烃衍生物的简易合成
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-04 DOI: 10.1039/d5qo00604j
Xiaoxia Duan, Kai Lan, Yue Su, Chuyang Cheng
{"title":"Facile Synthesis of a Contorted Polycyclic Aromatic Hydrocarbon Derivative","authors":"Xiaoxia Duan, Kai Lan, Yue Su, Chuyang Cheng","doi":"10.1039/d5qo00604j","DOIUrl":"https://doi.org/10.1039/d5qo00604j","url":null,"abstract":"A facile bottom-up synthesis of a contorted polycyclic aromatic hydrocarbon (PAH) derivative was reported. The structure features three expanded heptagonal rings, constructed by structural extension of a triscycloheptenylene core with integration of three anthraquinone units into the π-conjugated architecture. This strategy enables gram-scale synthesis with decent yield under mild conditions. Single crystal X-ray crystallographic analysis confirmed a saddle-shaped geometry induced by the three heptagons. This work provides a generalizable strategy for designing highly curved PAHs with tunable optoelectronic functionalities.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"11 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144211683","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Oligomeric Monoterpenoid Indole Alkaloids from the Flowers of Gelsemium elegans with Anti-inflammatory and Anti-fibrotic Activities 具有抗炎和抗纤维化活性的葛兰花低聚单萜类吲哚生物碱
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-03 DOI: 10.1039/d5qo00551e
Ji-Hong Gu, Ni-Ping Li, Hao-Ting Lin, Ling-Na Dai, Min-Jing Cheng, Jian Hong, Yi-Yi Li, Jun-Shan Liu, Wen-Cai Ye, Lei Wang
{"title":"Oligomeric Monoterpenoid Indole Alkaloids from the Flowers of Gelsemium elegans with Anti-inflammatory and Anti-fibrotic Activities","authors":"Ji-Hong Gu, Ni-Ping Li, Hao-Ting Lin, Ling-Na Dai, Min-Jing Cheng, Jian Hong, Yi-Yi Li, Jun-Shan Liu, Wen-Cai Ye, Lei Wang","doi":"10.1039/d5qo00551e","DOIUrl":"https://doi.org/10.1039/d5qo00551e","url":null,"abstract":"Gelsepolycines A–F (1–6), six oligomeric monoterpenoid indole alkaloids with new skeletons, together with their biosynthetic precursors (7–8), were isolated from the flowers of Gelsemium elegans. Compounds 1 and 4–6 represented the first examples of trimeric Gelsemium alkaloids that featuring complex sterically compact frameworks with 17-19 chiral centers. Furthermore, these compounds were constructed through unprecedented C14–C19 and C14–N4 linkages. Interestingly, all these oligomeric alkaloids (1–6) could be derived from the same monomer precursor 7 in the proposed biogenetic pathway. The anti-inflammatory and anti-fibrotic activities of these isolates were evaluated, and compound 3 demonstrated potent effects in vitro and in vivo. The biomimetic synthesis of 3 was achieved according to the proposed biogenetic pathway.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"11 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144201545","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dinickel-Catalyzed Regio- and Enantioselective α-Alkylation of Cyclic Ketones with Unactivated Alkyl Halides 镍催化环酮与非活化卤化烷基的区域和对映选择性α-烷基化反应
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-03 DOI: 10.1039/d5qo00448a
Liangwei Zhu, Lin Zhang, Jian Zhang, Peigen Wang, Ruopeng Bai, Zhonglin Tao
{"title":"Dinickel-Catalyzed Regio- and Enantioselective α-Alkylation of Cyclic Ketones with Unactivated Alkyl Halides","authors":"Liangwei Zhu, Lin Zhang, Jian Zhang, Peigen Wang, Ruopeng Bai, Zhonglin Tao","doi":"10.1039/d5qo00448a","DOIUrl":"https://doi.org/10.1039/d5qo00448a","url":null,"abstract":"The asymmetric α-alkylation of simple ketones with unactivated alkyl halides remains a longstanding challenge in organic synthesis. Herein, we report a dinickel-catalyzed asymmetric α-alkylation of cyclic ketones using unactivated alkyl halides as alkylating agents. This methodology accommodates a broad range of substrates, including benzo-fused cyclic ketones, α-aryl and α-alkyl cyclic ketones, and diverse alkyl halides, enabling the construction of chiral ketones with α-quaternary centers in high regio- and enantioselectivity. Mechanistic studies, combining experimental and computational approaches, reveal that this transformation proceeds via a redox-neutral SN2 pathway catalyzed by nickel(I) species intead of commonly seen Ni(II) salt. The unique bimetallic ligand framework plays a dual role: (1) stabilizing adjacent dinickel(I) centers through halogen-bridging interactions, thereby enabling the formation of a highly nucleophilic nickel(I) enolate, and (2) providing a chiral pocket to control the stereochemistry of the reaction.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"169 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144201547","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Remote Activating Strategy Enabled (RASE) π-Bond Migratory Dealkylative C-N coupling Utilising N-Fluorobenzenesulfonimide (NFSI) as A Bifunctional Domino Reagent 利用n -氟苯磺酰亚胺（NFSI）作为双功能多米诺试剂的远程激活策略激活(RASE) π键迁移脱烷基C-N偶联
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-03 DOI: 10.1039/d5qo00480b
Jiahao Gu, Zhenyang Wan, Yuhong Lu, Xiangmin Tian, Ziyue Zeng, Dailin Zhuang, Ziyuan Li
{"title":"Remote Activating Strategy Enabled (RASE) π-Bond Migratory Dealkylative C-N coupling Utilising N-Fluorobenzenesulfonimide (NFSI) as A Bifunctional Domino Reagent","authors":"Jiahao Gu, Zhenyang Wan, Yuhong Lu, Xiangmin Tian, Ziyue Zeng, Dailin Zhuang, Ziyuan Li","doi":"10.1039/d5qo00480b","DOIUrl":"https://doi.org/10.1039/d5qo00480b","url":null,"abstract":"Remote activating strategy enabled (RASE) π-bond migratory dealkylative C(sp3)-N and C(sp2)-N coupling with 2-alkoxylthiazole through C(sp3)-H and C(sp2)-H cleavage, giving N-benzyl or N-phenyl thiazol-2(3H)-one, respectively, are achieved under mild conditions. N-Fluorobenzenesulfonimide (NFSI) serves as a crucial bifunctional domino reagent which not only generates nitrogen-centred radical that initiates N-C or N-N radical relay, offering electrophile coupling partner, but also provides the key carbocation scavenger, N-hydrobenzenesulfonimide (NHSI), triggering π-bond migratory dealkylation of 2-alkoxylthiazole which offers nucleophilic thiazol-2(3H)-one coupling partner. Plausible mechanism has been proposed based on the results of mechanistic studies.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"37 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144201544","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemodivergent Temperature Controlled Switchable Iron Catalysed Annulation of o-vinylaniline with Isatin Derivatives 化学发散温控可切换铁催化邻乙烯苯胺与Isatin衍生物的环化
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-02 DOI: 10.1039/d5qo00626k
Sakshi Singh, Samir Kumar Mondal, Shantanu Pal
{"title":"Chemodivergent Temperature Controlled Switchable Iron Catalysed Annulation of o-vinylaniline with Isatin Derivatives","authors":"Sakshi Singh, Samir Kumar Mondal, Shantanu Pal","doi":"10.1039/d5qo00626k","DOIUrl":"https://doi.org/10.1039/d5qo00626k","url":null,"abstract":"Chemo-divergent approach enables to achieve regioselective and site-divergent transformations of multiple products by changing the parameter from identical, readily accessible starting materials are ideal but challenging due to the complexity of precisely controlling the chemo-diversity. Herein, we reported a novel FeCl₃-catalyzed one-pot strategy enabling the selective synthesis of 5-methyl-7-phenyldibenzo[b,h][1,6] naphthyridin-6(5H)-one or 3-phenyl-1H-indole from o-vinylaniline and N-substituted isatin by switching the temperature. Notably, the reaction exhibits temperature-controlled chemo-divergence, selectively yielding either intramolecular or intermolecular products. This approach demonstrates wide substrate, affording structurally diverse scaffolds under mild conditions. Furthermore, it provides an efficient route for synthesis of symmetrical urea derivatives and offers a potential pathway for the direct synthesis of tryptanthrin and related bioactive molecules.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"98 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144193343","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
NCI-driven regioselectivity and enantioreversal in chiral phosphoric acid-catalyzed arylamine functionalization nci驱动的手性磷酸催化芳胺功能化的区域选择性和对反性
IF 5.4 1区 化学
Organic Chemistry Frontiers Pub Date : 2025-06-02 DOI: 10.1039/d5qo00673b
Zi-Hao Li, Abing Duan, Shu-Yu Zhang
{"title":"NCI-driven regioselectivity and enantioreversal in chiral phosphoric acid-catalyzed arylamine functionalization","authors":"Zi-Hao Li, Abing Duan, Shu-Yu Zhang","doi":"10.1039/d5qo00673b","DOIUrl":"https://doi.org/10.1039/d5qo00673b","url":null,"abstract":"Non-covalent interactions (NCIs) have emerged as pivotal elements in asymmetric catalysis, enabling precise control over reactivity and selectivity in complex transformations. Despite their central role in designing catalytic systems, mechanistic understanding remains limited for reactions where NCIs concurrently govern regio- and enantioselectivity. The inherent complexity of CPA-catalyzed asymmetric reactions, characterized by diverse NCIs—particularly with arylamine substrates bearing multiple NCI-active motifs—presents formidable challenges for theoretical analysis and data-driven mechanistic modeling. This challenge becomes particularly pronounced when examining the enantioreversal phenomenon, where minute NCI perturbations orchestrate divergent catalytic pathways. Crucially, substrate-controlled enantioreversal operating independently of CPA groups modifications remain conspicuously undercharacterized in multi-selective reactions, particularly at the mechanistic level. In this study, we investigate three representative multi-site CPA-catalyzed asymmetric functionalizations of arylamines, utilizing detailed theoretical calculations to explore the influence of steric effects and NCIs, as well as the interplay between regioselectivity and enantioreversal. Our findings clarify the factors governing regioselectivity and enantioreversal, leading to a detailed elucidation of the mechanistic roles of key variables in existing frameworks. This work provides a robust theoretical foundation for optimizing CPA-catalyzed asymmetric reactions involving arylamines, while paving the way for future machine learning-driven advancements in this domain.","PeriodicalId":97,"journal":{"name":"Organic Chemistry Frontiers","volume":"163 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144193316","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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