Applied physics reviews最新文献

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Heterogeneous oxide/sulfide materials as superior bifunctional electrocatalysts for carbon-neutral green hydrogen production: A short review 异质氧化物/硫化物材料作为优异的双功能电催化剂用于碳中和绿色制氢:简评
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-24 DOI: 10.1063/5.0221098
Akbar I. Inamdar, Amol S. Salunke, Nabeen K. Shrestha, Hyunsik Im
{"title":"Heterogeneous oxide/sulfide materials as superior bifunctional electrocatalysts for carbon-neutral green hydrogen production: A short review","authors":"Akbar I. Inamdar, Amol S. Salunke, Nabeen K. Shrestha, Hyunsik Im","doi":"10.1063/5.0221098","DOIUrl":"https://doi.org/10.1063/5.0221098","url":null,"abstract":"Maintaining an acceptable quality of life worldwide increasingly depends on the availability of clean and cost-effective energy, with power consumption expected to double by 2050. Therefore, the need for sustainable and affordable green energy has spurred innovative electrocatalysis research with the goal to develop materials and processes that are capable of producing environmentally friendly, carbon-neutral, clean, and green hydrogen fuel as an alternative to fossil fuel. In particular, heterostructured catalysts consisting of transition metal oxides and sulfides have emerged as a capable component of green energy technology. The dual functionality of these catalysts allows for water splitting, while the selectivity of the catalytic materials creates synergetic effects based on their electronic structure, surface composition, and electrochemical surface area. In this review, we examine the latest research and developments, synthesis methods, design strategies, reaction mechanisms, and performance outcomes for oxide/sulfide heterostructures. The review begins by introducing the current demand for hydrogen energy and electrocatalytic water-splitting and then describes the fundamental design principles for oxide/sulfide heterostructures and their hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) performance. A large part of the review is then dedicated to a comprehensive discussion of the various transition metal oxide/sulfide heterostructures designed for the OER, the HER, and two-electrode electrolyzer applications. In addition, the use of in situ and operando techniques, which provide crucial information for the design of effective electrocatalysts, is described. We also discuss the present status of electrocatalysis technology, including the challenges it faces and its future prospects as a means to achieve carbon-neutral hydrogen production. Overall, this review delivers a summary of the latest developments in electrocatalysis based on oxide/sulfide heterostructures for use in green hydrogen production.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142489529","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Self-powered MXene/GaN van der Waals Schottky ultraviolet photodetectors with exceptional responsivity and stability 自供电型 MXene/GaN 范德瓦尔斯肖特基紫外线光电探测器,具有卓越的响应性和稳定性
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-24 DOI: 10.1063/5.0209698
Yu Ding, Xiangming Xu, Zhe Zhuang, Yimeng Sang, Mei Cui, Wenxin Li, Yu Yan, Tao Tao, Weizong Xu, Fangfang Ren, Jiandong Ye, Dunjun Chen, Hai Lu, Rong Zhang, Husam N. Alshareef, Bin Liu
{"title":"Self-powered MXene/GaN van der Waals Schottky ultraviolet photodetectors with exceptional responsivity and stability","authors":"Yu Ding, Xiangming Xu, Zhe Zhuang, Yimeng Sang, Mei Cui, Wenxin Li, Yu Yan, Tao Tao, Weizong Xu, Fangfang Ren, Jiandong Ye, Dunjun Chen, Hai Lu, Rong Zhang, Husam N. Alshareef, Bin Liu","doi":"10.1063/5.0209698","DOIUrl":"https://doi.org/10.1063/5.0209698","url":null,"abstract":"High-responsivity and energy-saving ultraviolet photodetectors become crucial components for modern optoelectronic information sensing and communication systems. This study presents an advanced self-powered MXene/GaN Schottky ultraviolet photodetector that features a high-quality van der Waals interface to enhance photoresponsivity. The photodetector exhibits a high responsivity of 681.6 mA W−1 and a significant detectivity of 7.65 × 1013 Jones at zero bias. In a self-powered mode, the detector can operate robustly even under dim illumination (0.15 μW cm−2) due to the excellent Schottky contact and low amount of defect states at the MXene/GaN interface, which presents a strong intrinsic electric field. The photodetector has a high ultraviolet/visible rejection ratio (R360 nm/R400 nm) of 3.9 × 103 and a signal to noise ratio (SNR) of 2.4 × 105, which enable discrimination against visible light interference in real-world scenarios. We also demonstrated that the photodetectors worked well as ultraviolet signal receivers in an optical information communication system to accurately recognize pulsed signals transmitted from an ultraviolet light-emitting diode. These findings imply the great potential of van der Waals Schottky junctions between 2D MXenes and III-nitrides for high-performance photodetection and sensing in many integrated optoelectronic platforms.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142489528","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Spin-torque nano-oscillators and their applications 自旋扭矩纳米振荡器及其应用
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-23 DOI: 10.1063/5.0221877
Sheng Jiang, Linrong Yao, Shun Wang, Di Wang, Long Liu, Akash Kumar, Ahmad A. Awad, Artem Litvinenko, Martina Ahlberg, Roman Khymyn, Sunjae Chung, Guozhong Xing, Johan Åkerman
{"title":"Spin-torque nano-oscillators and their applications","authors":"Sheng Jiang, Linrong Yao, Shun Wang, Di Wang, Long Liu, Akash Kumar, Ahmad A. Awad, Artem Litvinenko, Martina Ahlberg, Roman Khymyn, Sunjae Chung, Guozhong Xing, Johan Åkerman","doi":"10.1063/5.0221877","DOIUrl":"https://doi.org/10.1063/5.0221877","url":null,"abstract":"Spin-torque nano-oscillators (STNOs) have emerged as an intriguing category of spintronic devices based on spin transfer torque to excite magnetic moment dynamics. The ultra-wide frequency tuning range, nanoscale size, and rich nonlinear dynamics have positioned STNOs at the forefront of advanced technologies, holding substantial promise in wireless communication, and neuromorphic computing. This review surveys recent advances in STNOs, including architectures, experimental methodologies, magnetodynamics, and device properties. Significantly, we focus on the exciting applications of STNOs, in fields ranging from signal processing to energy-efficient computing. Finally, we summarize the recent advancements and prospects for STNOs. This review aims to serve as a valuable resource for readers from diverse backgrounds, offering a concise yet comprehensive introduction to STNOs. It is designed to benefit newcomers seeking an entry point into the field and established members of the STNOs community, providing them with insightful perspectives on future developments.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142488398","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A novel tapered quartz tuning fork-based laser spectroscopy sensing 基于激光光谱传感的新型锥形石英音叉
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-23 DOI: 10.1063/5.0214874
Yufei Ma, Shunda Qiao, Runqiu Wang, Ying He, Chao Fang, Tiantian Liang
{"title":"A novel tapered quartz tuning fork-based laser spectroscopy sensing","authors":"Yufei Ma, Shunda Qiao, Runqiu Wang, Ying He, Chao Fang, Tiantian Liang","doi":"10.1063/5.0214874","DOIUrl":"https://doi.org/10.1063/5.0214874","url":null,"abstract":"A novel tapered quartz tuning fork (QTF) was designed to enhance its stress magnitude and charge distribution in QTF-based laser spectroscopy, which had a low resonant frequency of 7.83 kHz and a wide fork gap for long energy accumulation time and easy optical alignment. Compared to the reported rectangular QTF, this tapered QTF transfers the maximum stress position from the root to the middle to improve its sensing performance. Furthermore, the unique design eliminates the 90° right angles typically found in standard QTFs, which often lead to undesired “webs” and “facets” during the etching process. This design minimizes performance degradation by reducing the presence of residual unexpected materials. QTF-based laser spectroscopy of quartz-enhanced photoacoustic spectroscopy (QEPAS) and light-induced thermoelastic spectroscopy (LITES) were adopted to verify its performance. Compared with the widely used standard QTF, the total surface charge of the tapered QTF was improved 5.08 times and 5.69 times in QEPAS and LITES simulations, respectively. Experiments revealed that this tapered QTF-based QEPAS sensor had a 3.02 times improvement in signal-to-noise-ratio (SNR) compared to the standard QTF-based system. Adding an acoustic micro-resonator to this tapered QTF-based QEPAS sensor improved the signal level by 97.20 times. The minimum detection limit (MDL) for acetylene (C2H2) detection was determined to be 16.45 ppbv. In the LITES technique, compared to the standard QTF, this tapered QTF-based sensor had a 3.60 times improvement in SNR. The MDL for C2H2 detection was determined to be 146.39 ppbv.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142488418","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Time-resolved x-ray imaging of nanoscale spin-wave dynamics at multi-GHz frequencies using low-alpha synchrotron operation 利用低阿尔法同步加速器对多千兆赫频率下的纳米级自旋波动力学进行时间分辨 X 射线成像
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-22 DOI: 10.1063/5.0206576
S. Mayr, J. Förster, S. Finizio, K. Schultheiss, R. A. Gallardo, R. Narkovicz, G. Dieterle, A. Semisalova, J. Bailey, E. Kirk, A. Suszka, J. Lindner, J. Gräfe, J. Raabe, G. Schütz, M. Weigand, H. Stoll, S. Wintz
{"title":"Time-resolved x-ray imaging of nanoscale spin-wave dynamics at multi-GHz frequencies using low-alpha synchrotron operation","authors":"S. Mayr, J. Förster, S. Finizio, K. Schultheiss, R. A. Gallardo, R. Narkovicz, G. Dieterle, A. Semisalova, J. Bailey, E. Kirk, A. Suszka, J. Lindner, J. Gräfe, J. Raabe, G. Schütz, M. Weigand, H. Stoll, S. Wintz","doi":"10.1063/5.0206576","DOIUrl":"https://doi.org/10.1063/5.0206576","url":null,"abstract":"Time-resolved x-ray microscopy is used in a low-alpha synchrotron operation mode to image spin dynamics at an unprecedented combination of temporal and spatial resolution. Thereby, nanoscale spin waves with wavelengths down to 70 nm and frequencies up to 30 GHz are directly observed in ferromagnetic thin film microelements with spin vortex ground states. In an antiparallel ferromagnetic bilayer system, we detect the propagation of both optic and acoustic modes, the latter exhibiting even a strong non-reciprocity. In single-layer systems, quasi-uniform spin waves are observed together with modes of higher order (up to the 4th order), bearing precessional nodes over the thickness of the film. Furthermore, the effects of magnetic material properties, film thickness, and magnetic fields on the spin-wave spectrum are determined experimentally. Our experimental results are consistent with numerical calculations from a micromagnetic theory even on these so-far unexplored time- and length scales.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142487358","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Exploring anti-ferroelectric thin films with high energy storage performance by moderating phase transition 通过缓和相变探索具有高储能性能的反铁电体薄膜
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-22 DOI: 10.1063/5.0226576
Tianfu Zhang, Yangyang Si, Xudong Li, Yijie Li, Tao Wang, Qinghua Zhang, Yunlong Tang, Zuhuang Chen
{"title":"Exploring anti-ferroelectric thin films with high energy storage performance by moderating phase transition","authors":"Tianfu Zhang, Yangyang Si, Xudong Li, Yijie Li, Tao Wang, Qinghua Zhang, Yunlong Tang, Zuhuang Chen","doi":"10.1063/5.0226576","DOIUrl":"https://doi.org/10.1063/5.0226576","url":null,"abstract":"Anti-ferroelectric thin films are renowned for their signature double hysteresis loops and sheds light on the distinguished energy storage capabilities of dielectric capacitors in modern electronic devices. However, anti-ferroelectric capacitors are still facing the dual challenges of low energy density and efficiency to achieve state-of-the-art performance. Their large hysteresis and sharp first-order phase transition usually results in a low energy storage efficiency and easy breakdown, severely obscuring its future application. In this study, we demonstrate that anti-ferroelectric (Pb0.97La0.02)(Zr1−xSnx)O3 epitaxial thin films exhibit enhanced energy storage performance through local structural heterogeneity to moderate the first-order phase transition by calculating the corresponding polarization as a function of switching time for the first time. The films exhibit remarkable enhanced breakdown strength (∼3.47 MV/cm, ∼5 times the value for PbZrO3) and energy storage performance. Our endeavors have culminated in the ingenious formulation of a novel strategy, namely, the postponement of polarization processes, thereby elevating the breakdown strength and total energy storage performance. This landmark achievement has unveiled a fresh vista of investigative opportunities for advancing the energy storage prowess of electric dielectrics.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142487197","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
2D layered halide perovskite for field-effect transistors 用于场效应晶体管的二维层状卤化物过氧化物
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-21 DOI: 10.1063/5.0206658
Tufan Paul, Silvia Colella, Emanuele Orgiu
{"title":"2D layered halide perovskite for field-effect transistors","authors":"Tufan Paul, Silvia Colella, Emanuele Orgiu","doi":"10.1063/5.0206658","DOIUrl":"https://doi.org/10.1063/5.0206658","url":null,"abstract":"Field-effect transistors are crucial components for modern electronics, generating significant research and profitable interest. Metal halide perovskites have recently emerged as a pioneering active material in solar cells, generating interest in their potential use in other electronic and (opto)electronic devices, including field-effect transistors and phototransistors. However, before they can be commercialized, they still face significant challenges owing to their immanent instabilities with respect to heat, moisture, and light. In contrast, due to their exceptional environmental stability, the newly emerging two-dimensional Ruddlesden–Popper type perovskites have garnered significant recognition. The current state of the field is covered in this review article, as are the problems, and a perspective for the scenarios of perovskite field-effect transistors. The effects of temperature, light, and measurement conditions are taken into account, as well as the physics of the device and the fundamental mechanisms that drive these devices, such as ion migration and ionic defects. Subsequently, the performance of perovskite transistors and phototransistors described so far is analyzed and critically evaluated. Finally, the major roadblocks to perovskite transistor advancement are identified and explored. The lessons learned from other perovskite optoelectronic devices are investigated in order to address these obstacles and bring these devices closer to industrial implementation.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142486504","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
On the study of proximity magnetism in van der Waals graphene/CuCrP2S6 heterostructure via the anomalous Hall effect 通过反常霍尔效应研究范德华石墨烯/CuCrP2S6 异质结构中的近程磁性
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-18 DOI: 10.1063/5.0223563
Yuriy Dedkov, Elena Voloshina
{"title":"On the study of proximity magnetism in van der Waals graphene/CuCrP2S6 heterostructure via the anomalous Hall effect","authors":"Yuriy Dedkov, Elena Voloshina","doi":"10.1063/5.0223563","DOIUrl":"https://doi.org/10.1063/5.0223563","url":null,"abstract":"Recently, several experimental works have appeared in the literature where induced magnetism in single- and few-layer graphene (SL-gr and FL-gr) interfaced with layered van der Waals materials was investigated via the application of the anomalous Hall effect (AHE). In most of these works, it is suggested that the observation of the AHE in such systems can be explained by a magnetic exchange interaction appearing at the interface between graphene and the underlying magnetic insulator. Considering the recently studied FL-graphene/bulk-CuCrP2S6 system as an example, our careful and rigorous analysis of recent experimental and theoretical data presented in the literature shows that the claimed observation of the AHE and magnetic proximity effect in this system is not supported. Moreover, the theoretically calculated electronic structures of the studied system contain serious errors and flaws that cannot be considered as an accurate description of such an interface and cannot be taken as solid support for the proposed proximity effect.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142448458","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Photonic Ising machines for combinatorial optimization problems 用于组合优化问题的光子伊辛机
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-14 DOI: 10.1063/5.0216656
Yuan Gao, Guanyu Chen, Luo Qi, Wujie Fu, Zifeng Yuan, Aaron J. Danner
{"title":"Photonic Ising machines for combinatorial optimization problems","authors":"Yuan Gao, Guanyu Chen, Luo Qi, Wujie Fu, Zifeng Yuan, Aaron J. Danner","doi":"10.1063/5.0216656","DOIUrl":"https://doi.org/10.1063/5.0216656","url":null,"abstract":"The demand for efficient solvers of complicated combinatorial optimization problems, especially those classified as NP-complete or NP-hard, has recently led to increased exploration of novel computing architectures. One prominent collective state computing paradigm embodied in the so-called Ising machines has recently attracted considerable research attention due to its ability to optimize complex problems with large numbers of interacting variables. Ising model-inspired solvers, thus named due to mathematical similarities to the well-known model from solid-state physics, represent a promising alternative to traditional von Neumann computer architectures due to their high degree of inherent parallelism. While there are many possible physical realizations of Ising solvers, just as there are many possible implementations of any binary computer, photonic Ising machines (PIMs) use primarily optical components for computation, taking advantage of features like lower power consumption, fast calculation speeds, the leveraging of physical optics to perform the calculations themselves, possessing decent scalability and noise tolerance. Photonic computing in the form of PIMs may offer certain computational advantages that are not easily achieved with non-photonic approaches and is nonetheless an altogether fascinating application of photonics to computing. In this review, we provide an overview of Ising machines generally, introducing why they are useful, what types of problems they can tackle, and how different Ising solvers can be compared and benchmarked. We delineate their various operational mechanisms, advantages, and limitations vis-à-vis non-photonic Ising machines. We describe their scalability, interconnectivity, performance, and physical dimensions. As research in PIMs continues to progress, there is a potential that photonic computing could well emerge as a way to handle large and challenging optimization problems across diverse domains. This review serves as a comprehensive resource for researchers and practitioners interested in understanding capabilities and potential of PIMs in addressing such complex optimization problems.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142436309","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Novel dopant-free ferromagnetic Mott-like insulator and high-energy correlated-plasmons in unconventional strongly correlated s band of low-dimensional gold 低维金的非传统强相关 S 波段中的新型无掺杂铁磁性莫特样绝缘体和高能相关等离子体
IF 15 1区 物理与天体物理
Applied physics reviews Pub Date : 2024-10-14 DOI: 10.1063/5.0177314
Muhammad Avicenna Naradipa, Angga Dito Fauzi, Bin Leong Ong, Muhammad Aziz Majidi, Caozheng Diao, Ganesh Ji Omar, Ariando Ariando, Mark B. H. Breese, Eng Soon Tok, Andrivo Rusydi
{"title":"Novel dopant-free ferromagnetic Mott-like insulator and high-energy correlated-plasmons in unconventional strongly correlated s band of low-dimensional gold","authors":"Muhammad Avicenna Naradipa, Angga Dito Fauzi, Bin Leong Ong, Muhammad Aziz Majidi, Caozheng Diao, Ganesh Ji Omar, Ariando Ariando, Mark B. H. Breese, Eng Soon Tok, Andrivo Rusydi","doi":"10.1063/5.0177314","DOIUrl":"https://doi.org/10.1063/5.0177314","url":null,"abstract":"Ferromagnetic insulators and plasmons have attracted a lot of interest due to their rich fundamental science and applications. Recent research efforts have been made to find dopant-free ferromagnetic insulators and unconventional plasmons independently both in strongly correlated electron systems. However, our understanding of them is still lacking. Existing dopant-free ferromagnetic insulator materials are mostly limited to complex d- or f-systems with extremely low Curie temperature, low-symmetry structure, and strict growth conditions on specific substrates, limiting their compatibility with industrial applications. Unconventional plasmon is, on the other hand, a quasiparticle that originates from the collective excitation of correlated-charges, yet they are rarely explored, particularly in ferromagnetic insulator materials. Herewith, we present a novel, room temperature dopant-free ferromagnetic Mott-like insulator with a high-symmetry structure in unconventional strongly correlated s band of low-dimensional highly oriented single-crystal gold quantum dots (HOSG-QDs) on MgO(001). Interestingly, HOSG-QDs show new high-energy correlated-plasmons with low-plasmonics-loss. With a series of state-of-the-art experimental techniques, we find that the Mott-insulating state is tunable with surprisingly strong spin-splitting and spin polarization accompanied by strong s–s transitions, disappearance of Drude response, and generating new Mott-like gap. Supported with a series of theoretical calculations, the interplay of quantum confinement, many-body electronic correlations, and hybridizations tunes electron–electron correlations in s band and determines the ferromagnetism, Mott-like insulator, and high-energy correlated-plasmons. Our result shows a new class of room temperature dopant-free ferromagnetic Mott-like insulator and high-energy correlated-plasmons with low-loss in strongly correlated s band and opens unexplored applications of low-dimensional gold in spin field-effect transistors and plasmonics.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":null,"pages":null},"PeriodicalIF":15.0,"publicationDate":"2024-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142436310","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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