Te-Huan Liu, Tianyu Wang, Jun Zhou, Xin Qian, Ronggui Yang
{"title":"Thermal-driven multi-carrier transport in electronic and energy materials","authors":"Te-Huan Liu, Tianyu Wang, Jun Zhou, Xin Qian, Ronggui Yang","doi":"10.1063/5.0265763","DOIUrl":"https://doi.org/10.1063/5.0265763","url":null,"abstract":"Thermal-driven multi-carrier transport is essential for both scientific research and technological applications in electronic, spintronic, and energy conversion devices. This article reviews the fundamentals of phonon, electron, spin, and ion transport driven by temperature gradients in solid-state and soft condensed matter, and the microscopic interactions between energy/charge carriers that can be leveraged for manipulating electrical and thermal transport in energy conversion devices, such as electron–phonon coupling, spin–phonon interaction, and ion–solvent interactions. In coupled electron–phonon transport, we discuss the basics of electron–phonon interactions and their effects on phonon dynamics, thermalization, and nonequilibrium thermal transport. For the phonon–spin interaction, nonequilibrium transport formulation is introduced first, followed by the physics of spin thermoelectric effect and strategies to manipulate them. Contributions to thermal conductivity from magnons as heat carriers are also reviewed. For coupled transport of heat and ions/molecules, we highlight the importance of local molecular configurations that determine the magnitude of the electrochemical gradient, which is the key to improving the efficiency of low-grade heat energy conversion.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"232 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144629486","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Deterministic switching between flux-closure and center-type polar topological structures via modulation of oxygen vacancies","authors":"Luyong Zhang, Xiangping Zhang, Jianbiao Xian, Ruifeng Chen, Guo Tian, Changjian Li, Jun-ming Liu, Xingsen Gao","doi":"10.1063/5.0268812","DOIUrl":"https://doi.org/10.1063/5.0268812","url":null,"abstract":"Deterministic control of polar topological structures has attracted considerable attention due to its potential applications in post-Moore electronics. While manipulation techniques such as strain (via substrates), electric fields, and temperature are commonly employed, switching induced by charged defects between different polar topological structures remains a rarely observed phenomenon. In this study, we demonstrate that oxygen vacancies can effectively enable the switching between flux-closure and center-type topological structures in PbTiO3 (PTO) nano-island arrays. Supported by evidence from x-ray photoelectron spectroscopy, scanning Kelvin probe microscopy, and piezoresponse force microscopy, we demonstrate that a high concentration of oxygen vacancies favors the formation of center-type domains, while the topological structure transitions to the flux-closure configuration following elimination of oxygen vacancies via in situ annealing under various gas atmospheres. This deterministic switching between the two polar topological structures highlights the critical role of charged defects and opens new avenues for the manipulation of polar topological structures in future applications.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"107 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144603868","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Achieving high-performance organic photodetectors with novel interpenetrated heterojunction architectures","authors":"Zhenqi Gong, Yiwei Zhang, Ping-An Chen, Zhaojing Xiao, Kaixin Niu, Jiangnan Xia, Huan Wei, Jiaqi Ding, Yu Zhang, Chengyuan Peng, Xi Zeng, Wenpei Shi, Chen Chen, Yuanyuan Hu","doi":"10.1063/5.0273823","DOIUrl":"https://doi.org/10.1063/5.0273823","url":null,"abstract":"Heterojunctions are indispensable for fabricating high-performance organic photodetectors. However, traditional structures—such as planar heterojunctions (PHJs) and bulk heterojunctions (BHJs)—face significant challenges. PHJs often suffer from limited exciton dissociation in thick films, while BHJs experience considerable charge transport barriers. Although quasi-planar heterojunctions have been proposed to address these issues, controlling their nanoscale interface remains complex and material-dependent, limiting their applications. Herein, we introduce novel interpenetrated heterojunctions (IPHJs), formed by penetrating a secondary organic semiconductor layer into a porous bottom layer during annealing. This innovative structure is revealed to possess efficient exciton dissociation and charge transport. Remarkably, organic photodiodes (OPDs) featuring PM6:N2200 IPHJs demonstrate exceptional performance, achieving a responsivity (R) of 36.5 A/W, a specific detectivity (D*) of 8.6 × 1012 Jones, and a response time (τ) of 30 μs, representing state-of-the-art performance for OPDs. Furthermore, extending the IPHJ concept to tri-layer interpenetrated heterojunctions (T-IPHJs) shows significant promise for organic phototransistor applications. The PM6:N2200 T-IPHJ devices exhibit a responsivity exceeding 44.7 A/W, a D* value reaching 5.23 × 1014 Jones, and a τ of 70 ms. These results show the potential of IPHJs to advance the field of high-performance organic photodetectors and related devices.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"11 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144593843","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Ultralow cyclic and device variability memristors via deterministic resistive switching in phase segregated nickel nanofilaments","authors":"Jiahao Song, Yanghe Wang, Linkun Wang, Zhenghao Liu, Yihan Lei, Mingqiang Cheng, Yingli Zhang, Weikun Zhou, Zengxu Xu, Xianglong Li, Muhammad Shahrukh Saleem, Lang Chen, Boyuan Huang, Wei Wang, Changjian Li","doi":"10.1063/5.0269546","DOIUrl":"https://doi.org/10.1063/5.0269546","url":null,"abstract":"Memristor crossbar arrays, mimicking the human brain, hold immense potential for energy-efficient data-intensive computations in artificial intelligence applications such as image recognition and natural language processing. However, the stochastic nature of resistive switching (RS) in memristors often leads to poor device stability and uniformity, hindering the scalability required for real-world applications. Here, we present a novel phase segregation strategy to achieve uniformly distributed self-assembled Ni nanofilaments within a BaTiO3 matrix, enabling local deterministic redox reactions for RS, as confirmed by comprehensive structural, local, and macroscopic RS studies. This approach yields drastic enhancement in cyclic performance and device uniformity, with the average cyclic variances of Set voltage and low resistance state down to 1.4% and 9.6%, respectively. The devices also exhibit excellent endurance (109 cycles) and ultrafast programming speed (down to 100 ns) and achieve over 5-bit level long-term memory states. The enhanced cyclic stability and device uniformity translate to high training and learning accuracies (95%) in a three-level deep neural network, with 1-bit inputs. Our phase segregation strategy provides a generic pathway to overcome the long-standing challenge of device variability in neuromorphic computing.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"18 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144577862","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Siying Gao, Zhuoqun Wang, Ning Lu, Lei Xu, Zhanghua Han, Mohsen Rahmani, Yuechen Jia, Feng Chen
{"title":"Lithium tantalate resonant metasurfaces for highly efficient ultraviolet harmonic generation","authors":"Siying Gao, Zhuoqun Wang, Ning Lu, Lei Xu, Zhanghua Han, Mohsen Rahmani, Yuechen Jia, Feng Chen","doi":"10.1063/5.0258436","DOIUrl":"https://doi.org/10.1063/5.0258436","url":null,"abstract":"Lithium tantalate (LiTaO3, LT), structurally similar to lithium niobate, possesses a broad spectrum of optoelectronic properties that hold significant promise for integrated photonics applications. Due to its larger bandgap and higher optical damage threshold, LT can be employed for efficient nonlinear optical frequency conversion in the ultraviolet (UV) wavelength range. Here, we report on fabrication of monolithic, high-quality LT metasurfaces, composed of periodic arrays of LT truncated square pyramids, created by partially etching of a LT thin film layer using a focused ion beam milling process. These pyramidal structures introduce discrete translational symmetry, which allows for the folding of guided-mode dispersion into the first Brillouin zone, leading to the formation of guided mode resonances with Q-factors that can be easily controlled by the height of LT pyramids. The measurements show a Q-factor up to approximately 640 at 786 nm. By leveraging the strong field localization of these high-Q resonances, we demonstrate enhanced second-harmonic generation at 393 nm with an absolute conversion efficiency of 0.042%, establishing a new benchmark for the UV harmonic generation in dielectric metasurfaces. Moreover, our fabrication technique can be readily adapted to a wide range of other material platforms, opening new avenues for the development of high-quality UV metasurfaces and advanced nonlinear photonic meta-devices.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"51 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144577861","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Muzaffar Ahmad Boda, Chen Chen, Xiang He, Zhiguo Yi
{"title":"Photostriction in emerging inorganic materials for next-generation micro-optomechanical devices","authors":"Muzaffar Ahmad Boda, Chen Chen, Xiang He, Zhiguo Yi","doi":"10.1063/5.0249005","DOIUrl":"https://doi.org/10.1063/5.0249005","url":null,"abstract":"Photostrictive effect exhibits a high potential to realize the smart micro-optomechanical devices, which can be operated at a simple principle of direct conversion of light energy into mechanical strain. Unlike electrostrictive and magnetostrictive effects, it does not involve complex circuits, therefore offering a promising prospect of accomplishing the advanced, compact, and remote-control devices. The key step to produce the light-induced strain of practical value is to design highly efficient photostrictive materials. Based upon the nature of the material systems to be explored for micro-optomechanical devices, the photostriction in inorganic–materials-based systems, including semiconductors, transition metal oxides, halide perovskites, and ferroelectrics in bulk and two-dimensions, are summarized herein. For each material, the feasible strategies of compositional engineering, processing conditions, and sample sculpturing, with a special focus on the meticulous tailoring of multiple phase boundaries in representative ferroelectric systems to produce significant photostriction, are given. Since ferroelectric photostriction is accounted as the superposition effect of photovoltaic and inverse piezoelectric effects, both effects are introduced and discussed. Finally, perspectives on future research of photostrictive materials are added. We believe that this review will bring new insights in producing highly efficient photostrictive materials for the commercial production of upcoming state-of-the-art micro optomechanical devices.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"8 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144577871","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Daeyeon Won, HyeongJun Kim, Taek-Soo Kim, Seung Hwan Ko
{"title":"Hydrogel electronic materials and microfabrication processes for soft electronic applications","authors":"Daeyeon Won, HyeongJun Kim, Taek-Soo Kim, Seung Hwan Ko","doi":"10.1063/5.0261387","DOIUrl":"https://doi.org/10.1063/5.0261387","url":null,"abstract":"Hydrogel electronic materials (HEMs) have emerged as strong candidates for various applications in soft electronics based on their unique softness and exceptional ability to retain water. Central to the advancement of these materials are conjugated polymers, such as conducting and semiconducting polymers, which have been the focus of extensive materials science and engineering. Despite this progress, the practical application of HEMs necessitates the development of microfabrication techniques that allow for effective fabrication methodologies and precise patterning at a micro-scale. By reducing HEMs to micro-sized devices, various innovative technologies such as implantable electronics and imperceptible soft robots can be realized. In this review, we present the latest advancements in the design methods and microfabrication strategies for HEMs. Then, we also discuss the physical properties of fabricated HEMs and the methodologies to precisely measure them. Finally, we will introduce potential applications of soft electronics and conclude with the future direction of research in this exciting field.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"19 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144533211","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yu Zhou, Junhua Tan, HaiBo Hu, Sikai Hua, Chunhui Jiang, Bo Liang, Tongyuan Bao, Xinfang Nie, Shumin Xiao, Dawei Lu, Junfeng Wang, Qinghai Song
{"title":"Silicon carbide: A promising platform for scalable quantum networks","authors":"Yu Zhou, Junhua Tan, HaiBo Hu, Sikai Hua, Chunhui Jiang, Bo Liang, Tongyuan Bao, Xinfang Nie, Shumin Xiao, Dawei Lu, Junfeng Wang, Qinghai Song","doi":"10.1063/5.0262377","DOIUrl":"https://doi.org/10.1063/5.0262377","url":null,"abstract":"Quantum networks based on solid-state spin defects present a transformative approach to secure communication and distributed quantum computing, utilizing quantum entanglement and coherent spin–photon interfaces. Silicon carbide (SiC) stands out as a compelling material platform due to its unique combination of a wide bandgap, high optical nonlinearity, CMOS-compatible fabrication, and controllable spin-active defects. These intrinsic properties facilitate efficient photon emission, robust spin coherence at both room and cryogenic temperatures, and integration with photonic nanostructures. Recent advancements in defect engineering and micro-nanophotonics have unlocked the potential of SiC quantum nodes, which feature electron-nuclear spin systems for high-fidelity quantum operations and long-lived quantum memories. Key steps such as single-shot readout and spin-photon entanglement have been successfully demonstrated, bringing SiC closer to a real quantum network platform. This review offers a comprehensive overview of the advancements in SiC-based quantum networks, encompassing key aspects such as defect fabrication methodologies, optimization of spin-photon interfaces, and strategies for photonic integration. Additionally, it examines the existing challenges and outlines promising future directions in this rapidly evolving field.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"41 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144533212","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"From bubble dynamics to acoustic control: Underwater bubble-based metamaterials for marine sustainability","authors":"Qibo Deng, Tianying Du, Cuihua An, Zhandong Huang","doi":"10.1063/5.0256788","DOIUrl":"https://doi.org/10.1063/5.0256788","url":null,"abstract":"Marine acoustics is crucial for the sustainable utilization of ocean resources. Researchers have discovered that underwater bubbles can serve as highly efficient acoustic resonators, enabling precise manipulation of sound waves in water. However, understanding the complex dynamics of bubble evolution in fluids is essential to optimize their acoustic characteristics. This review provides theoretical forecasts and practical approaches for studying bubble evolution, along with an overview of recent advancements in underwater bubble metamaterials. It covers classical and modified theoretical equations and explores strategies for modifying acoustic environments through resonant coupling in bubbles. Techniques, such as applying external forces, introducing surfactants, and creating micropatterned designs for structuring bubbles, are discussed. This review evaluates the superior acoustic properties of underwater bubble metamaterials, including their reflection, absorption, and transmission capabilities and their potential applications in marine environments. Finally, this study outlines the challenges that need to be addressed to manage bubble dynamics and enhance acoustic metamaterial technologies for underwater applications. These insights are expected to contribute to the sustainable development of the ocean.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"652 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144533255","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
M. Gersemann, A. Rajagopalan, M. Abidi, P. Barbey, A. Sabu, X. Chen, N. B. Weddig, B. Tennstedt, J. Petring, N. Droese, A. Kassner, C. Künzler, L. Keinert, X. Xiao, F. Dencker, M. C. Wurz, A. Löwer, E. von Hinüber, D. Schlippert, E. M. Rasel, S. Schön, S. Abend
{"title":"Developments for quantum inertial navigation systems employing Bose–Einstein condensates","authors":"M. Gersemann, A. Rajagopalan, M. Abidi, P. Barbey, A. Sabu, X. Chen, N. B. Weddig, B. Tennstedt, J. Petring, N. Droese, A. Kassner, C. Künzler, L. Keinert, X. Xiao, F. Dencker, M. C. Wurz, A. Löwer, E. von Hinüber, D. Schlippert, E. M. Rasel, S. Schön, S. Abend","doi":"10.1063/5.0250666","DOIUrl":"https://doi.org/10.1063/5.0250666","url":null,"abstract":"Quantum technology became a new tool for navigation based on measuring accelerations and rotations. However, the full potential of atom interferometers that operate with ultracold atoms has not yet been exploited. This paper presents current developments in the field of generation and application of Bose–Einstein condensates for inertial navigation. It covers the advancements in the form of atom chip and compact vacuum technology, classical sensor hybridization, and a multi-axis atom interferometry technique. In addition, the synergies of combining quantum sensors with classical inertial measurement units and their implications for navigation trajectories are discussed.","PeriodicalId":8200,"journal":{"name":"Applied physics reviews","volume":"2 1","pages":""},"PeriodicalIF":15.0,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144533215","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}