{"title":"Distinct nucleation and growth kinetics of BaTiO3 on Ge (001) by RF magnetron sputtering","authors":"Ruyuan Ma, Wentao Yan, Mingliang Zhao, Xiaofei Liu, Yuanmao Pu, Yang Qiu, Xingyan Zhao, Shaonan Zheng, Qize Zhong, Yuan Dong, Ting Hu","doi":"10.1063/5.0275009","DOIUrl":"https://doi.org/10.1063/5.0275009","url":null,"abstract":"The integration of metal oxide films with conventional semiconductors like silicon (Si) and germanium (Ge) enables the introduction of functionalities in semiconductor devices. This work experimentally demonstrates the BaTiO3 (BTO) thin film with crystalline Amm2 structure grown directly on Ge(001) using RF magnetron sputtering. In addition, its nucleation and growth kinetics are analyzed in detail. A systematic investigation of the crystal structural, optical, and morphological properties of BTO grown under different chamber pressures is performed. This study presents a growth model related to 3D + 2D growth to improve the mobility of barium (Ba) and titanium (Ti) atoms, with a stoichiometric ratio of Ba:Ti approaching 1.1. Consequently, at a wavelength of 800 nm, the refractive index (n) of BTO was approximately 2.15, rivaling those grown by pulsed laser deposition in refractive index.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"92 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144603866","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Wanjiong Li, Jibin Li, Nai Jiang, Xinhao Guo, Mingyi Chen, Yunzhen Hu, Quanlin Ye, Xinman Chen, Shuxiang Wu, Chao Shen, Shuwei Li
{"title":"Spin-correlated optical transitions in room-temperature ferromagnetic Fe3GaTe2","authors":"Wanjiong Li, Jibin Li, Nai Jiang, Xinhao Guo, Mingyi Chen, Yunzhen Hu, Quanlin Ye, Xinman Chen, Shuxiang Wu, Chao Shen, Shuwei Li","doi":"10.1063/5.0259343","DOIUrl":"https://doi.org/10.1063/5.0259343","url":null,"abstract":"Fe3GaTe2 has been recently identified as a potential van der Waals (vdW) ferromagnetic material for spintronic devices, owing to long-range ferromagnetic order, strong perpendicular magnetic anisotropy, and high Curie temperature (TC) above room temperature. The band structure and electronic transitions are crucial for understanding magnetic properties of Fe3GaTe2, requiring a comprehensive investigation of the electronic behavior of Fe3GaTe2 under external magnetic fields. In this study, magnetic circular dichroism (MCD) spectroscopy was employed to examine the electronic transitions in Fe3GaTe2 at room temperature. Three distinct MCD peaks are clearly observed under the applied magnetic fields, which could correspond to three electronic transitions determined by first-principles density functional theory calculations of the band structure of Fe3GaTe2. Furthermore, the three transition bands would be correlated with the Fe d orbitals, as supported by the calculated orbital-resolved band structure of Fe3GaTe2. These findings offer insights into the electronic transitions and the underlying electronic structure in Fe3GaTe2, providing a basis for further fundamental research and potential applications in spintronic devices.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"706 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144603867","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
S. Nobel, X. Zhu, J. Wu, N. Peyghambarian, R. A. Norwood
{"title":"Optical refrigeration of Tm3+ doped indium fluoride glass from room temperature","authors":"S. Nobel, X. Zhu, J. Wu, N. Peyghambarian, R. A. Norwood","doi":"10.1063/5.0244229","DOIUrl":"https://doi.org/10.1063/5.0244229","url":null,"abstract":"Optical refrigeration has significant promise for vibration-free cryogenic cooling and radiation-balanced fiber lasers. In this paper, we report theoretical and experimental investigations of optical refrigeration in thulium (Tm3+) doped indium fluoride glass (Tm3+:InF3) from room temperature. Comprehensive spectroscopic studies of Tm3+:InF3 were conducted, and its cooling with 1875, 1900, and 1950 nm pump lasers at different power levels has been measured. Maximum cooling of 2.4 K was achieved with 4.4 W from a 1900 nm laser. The experimental results agree with our theoretical expectations. Our experiment has demonstrated that Tm3+:InF3 has better cooling efficiency than Tm3+ doped ZrF4-BaF2-LaF3-AlF3-NaF glass due to Tm3+:InF3's lower maximum phonon energy, which reduces non-radiative decay.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"71 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144603864","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"High-frequency spin transport in thin aluminum calculated by spin drift-diffusion equation","authors":"Runzi Hao, R. H. Victora","doi":"10.1063/5.0251897","DOIUrl":"https://doi.org/10.1063/5.0251897","url":null,"abstract":"Lateral spin valves (LSV) are an essential element in spintronics research and applications. The separation of spin injection and spin detection in the LSV makes it a useful platform for studying fundamental physics (e.g., spin relaxation) and building nanoscale devices (spin transistors, magnetic sensors, etc.). To drive many LSV-based prototypes closer to production, there is a need to evaluate the LSV performance under high-frequency (e.g., gigahertz) operations, especially with information spectra rather than single tones. Here we calculate gigahertz spin transport in a nonmagnetic channel of the LSV using a pseudo-random binary sequence as an input signal to mimic information. We solved the time-dependent spin drift-diffusion equation and provide an integral solution for the transmitted spin polarization. A frequency-dependent spin transport length is found that shows high-frequency spin signals transmit much less efficiently than low-frequency spin signals. An applied electric field consistent with the high resistance of thin films is shown to improve transmission. The transmitted signal strength and its signal-to-noise ratio (SNR) are analyzed with respect to the transmission distance, the diffusion coefficient, and an applied electric field along the channel; these effects can be explained in the frequency domain. Finally, we calculated gigahertz spin transport in a thin aluminum channel and obtained an SNR >20 dB, which is a value that exceeds the SNR of the input signal. This demonstrates the great potential of LSV-based miniaturized spintronic devices to transmit information in high-frequency regimes.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"47 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144603863","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Long Zhang, Zhongzhu Jiang, Yugang Zhang, Jing Zhang, Aifeng Wang, Mingquan He, Y. P. Sun, Xuan Luo, Yisheng Chai
{"title":"Magnetic phase diagram of Cr2Te3 revisited by ac magnetostrictive coefficient","authors":"Long Zhang, Zhongzhu Jiang, Yugang Zhang, Jing Zhang, Aifeng Wang, Mingquan He, Y. P. Sun, Xuan Luo, Yisheng Chai","doi":"10.1063/5.0271368","DOIUrl":"https://doi.org/10.1063/5.0271368","url":null,"abstract":"Two-dimensional (2D) magnetic materials have attracted considerable interest owing to their potential applications in spintronics and fundamental investigations into low-dimensional magnetism. Cr2Te3, a quasi-2D non-van der Waals magnet, exhibits a complex magnetic phase diagram due to competing magnetic interactions within and between layers. However, the precise nature and evolution of these magnetic phases remain unclear. Here, we utilize an ultrahigh-sensitive composite magnetoelectric technique, which probes the ac magnetostrictive coefficient, to systematically explore the temperature–magnetic field phase diagram of Cr2Te3 single crystals. Our results reveal the coexistence of multiple magnetic phases, including canted ferromagnetic, antiferromagnetic, and paramagnetic states. An additional canted ferromagnetic phase and a possible triple point are also proposed. The updated phase diagram provides deeper insights into the specific spin configurations associated with each phase. These findings further highlight the decoupled magnetic ordering between the Cr1/Cr3 layers and the Cr2 layer near the magnetic ordering temperatures.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"6 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144603865","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Efficient spin–orbit torque driven magnetization switching of GdFe using phosphorus-implanted platinum layers","authors":"Kazuki Shintaku, Arun Jacob Mathew, Akihisa Iwamoto, Mojtaba Mohammadi, Hiroyuki Awano, Hironori Asada, Yasuhiro Fukuma","doi":"10.1063/5.0271181","DOIUrl":"https://doi.org/10.1063/5.0271181","url":null,"abstract":"The capability of the spin–orbit torque (SOT) generated via phenomena such as the spin Hall effect in heavy metals, in switching the magnetization of an adjacent magnetic material, has been studied extensively over the last decade. The efficiency of SOT generation is commonly quantified in terms of the spin Hall angle (SHA). In this work, we demonstrate experimentally that implanting platinum (Pt) with phosphorus (P), resulting in Pt (P) with different implantation doses, increases SHA by a factor of 7, from 0.06 (dose of zero) to 0.43 (dose of 10 × 1016 ions/cm2). The enhanced SHA, along with factors such as perpendicular magnetic anisotropy and resistivity, leads to reduction of the critical current density for switching the perpendicular magnetization of ferrimagnetic rare earth-transition metal alloy Gd26Fe74, by a factor of nearly 27, from 4.0 × 1011 A/m2 (zero) to 1.5 × 1010 A/m2 (10 × 1016 ions/cm2). Furthermore, the switching current density at zero thermal fluctuations and thermal stability factor were evaluated and found to be 2.0 × 1010 A/m2 and 61.4 (10 × 1016 ions/cm2), with the latter being sufficiently above the required threshold for commercial memory applications. Our results suggest that Pt (P) could be a strong candidate in realizing efficient SOT driven magnetization switching, leading to the development of improved memory and logic devices in the future.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"3 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144594174","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Enhancement of long-term memory of IGZO synaptic transistors by the introduction of an Al2O3 charge trapping layer","authors":"Yuhui Wang, Guangtan Miao, Zezhong Yin, Ranran Ci, Guoxia Liu, Fukai Shan","doi":"10.1063/5.0282482","DOIUrl":"https://doi.org/10.1063/5.0282482","url":null,"abstract":"Brain-inspired neuromorphic computing has been widely considered a promising solution to overcome the limitations of traditional von Neumann architecture in the current computer system. As an essential component of the neuromorphic system, the artificial synaptic device exhibits great potential in adaptive learning. Due to their controllable channel conductance and CMOS compatibility, solid electrolyte-gated synaptic transistors (EGSTs) have garnered significant interest as next-generation neuromorphic devices. However, most of the existing EGSTs suffer from rapid self-diffusion of the ions, making it difficult to maintain the stable channel conductance states. In this work, the synaptic transistors were fabricated with indium–gallium–zinc oxide as the channel layer, Al2O3 as the charge trapping layer, and ZrO2 as the solid electrolyte layer. The self-diffusion of the hydrogen ions can be suppressed by the positive charges trapped in the Al2O3 layer, which significantly improves the long-term plasticity (LTP) of the devices. By adjusting the presynaptic spike scheme, the typical synaptic behaviors, including excitatory postsynaptic current, paired-pulse facilitation, and the transition from short-term memory to long-term memory, were simulated. Based on the conductance modulation properties of the channel in the synaptic transistor, an artificial neural network was constructed for pattern recognition, and a high accuracy of 95.4% was obtained. This work demonstrates an effective strategy for the enhancement of the LTP of the synaptic transistor.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"7 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144594176","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Rajeswari Roy Chowdhury, Daichi Kurebayashi, Jana Lustikova, Oleg A. Tretiakov, Shunsuke Fukami, Ravi Prakash Singh, Samik DuttaGupta
{"title":"Unraveling effects of competing interactions and frustration in vdW ferromagnetic Fe3GeTe2 nanoflake devices","authors":"Rajeswari Roy Chowdhury, Daichi Kurebayashi, Jana Lustikova, Oleg A. Tretiakov, Shunsuke Fukami, Ravi Prakash Singh, Samik DuttaGupta","doi":"10.1063/5.0262983","DOIUrl":"https://doi.org/10.1063/5.0262983","url":null,"abstract":"Two-dimensional (2D) van der Waals (vdW) magnets and devices have garnered significant attention owing to the stabilization of long-range magnetic order down to atomic limit, and the prospect for quantum devices with unique functionalities. To achieve this objective, clarification of magnetotransport properties and understanding of the relevant interactions with lowering of dimensions are of extreme importance. Here, the magnetotransport properties of few atomic layer Fe3GeTe2 and (Co0.25Fe0.75)3GeTe2 nanoflake devices have been investigated. Magnetotransport investigations with applied magnetic field along the easy-axis show anomalous Hall effect, while that for applied magnetic field along the hard-axis reveal an unusual behavior. Atomistic calculations considering the presence of antiferromagnetic, ferromagnetic, and local symmetry-breaking interactions reveal the critical role of magnetic frustration effect assisted by thermal fluctuations, leading to a non-zero scalar spin chirality manifesting in an unconventional Hall effect. The present result clarifies the underlying interactions in few-layer 2D vdW ferromagnetic material system, important for the understanding of non-collinear spin configurations in vdW magnets for 2D spintronic devices.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"21 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144594177","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Agnieszka Klimeczek, Maurizio De Santis, Aurélien Masseboeuf, Jan Vogel, Laurent Ranno, Anne Lamirand, Stefania Pizzini
{"title":"Large exchange bias field in Pt/Co bilayers with ultrathin native oxide","authors":"Agnieszka Klimeczek, Maurizio De Santis, Aurélien Masseboeuf, Jan Vogel, Laurent Ranno, Anne Lamirand, Stefania Pizzini","doi":"10.1063/5.0275288","DOIUrl":"https://doi.org/10.1063/5.0275288","url":null,"abstract":"We studied the magnetic properties of a Pt/Co bilayer sample with an ultrathin cobalt layer deposited as a wedge with a thickness between 0.7 and 1.4 nm. After exposure to air, the top 0.5 nm of Co oxidizes, leading to a 0.9 nm-thick CoO surface layer. The residual metallic cobalt is still ferromagnetic at room temperature, with a strong perpendicular magnetic anisotropy even down to ≈0.2–0.3 nm thickness. These properties are conserved for several months after deposition. Anomalous Hall effect measurements show the presence of an exchange bias field and a blocking temperature between 120 and 150 K, indicating that despite being ultrathin, the CoO layer acquires antiferromagnetic order at low temperatures. We attribute the large exchange bias field (up to 0.9 T at 4 K) to the ultralow thickness of the ferromagnetic Co layer. These results show that simply exposing an ultrathin Co layer to air in order to form a native CoO oxide layer allows obtaining functional properties competing with the best reported so far for optimized Co/CoO layers and core-shell nanoparticles.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144594175","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Enhancement of resistive switching properties in RRAM with AlN-Al2O3 bilayer structure","authors":"Jinshan He, Xiaoling Duan, Dong Wang, Jiangcheng Wu, Zhihong Liu, Tao Zhang, Yue Hao, Jincheng Zhang","doi":"10.1063/5.0262592","DOIUrl":"https://doi.org/10.1063/5.0262592","url":null,"abstract":"This study presents the fabrication process and bipolar resistive switching behavior of an Au/Al/AlN/Al2O3/Pt/Ti random-access memory device. The proposed device, incorporating a thin Al2O3 layer between the AlN resistive switching layer and the Pt bottom electrode, exhibits enhanced resistive switching performance. Specifically, the device demonstrates improved endurance, with the number of switching cycles increasing from 122 to 2791, and a higher switching resistance ratio, with the maximum on/off ratio rising from 105 to 108. The enhanced switching stability originates from the inserted Al2O3 layer enabling precise control over conductive filament rupture locations. This spatial regulation yields more stable resistive switching behavior, which is a critical requirement for nonvolatile memory applications.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"21 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144594178","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}