{"title":"Near room-temperature large negative electrocaloric effect accompanied by giant thermal switching ratio in Zr-rich lead zirconate titanate","authors":"Jian Guo, Haoran Yu, Mingqian Yuan, Xue-Jun Yan, Shan-Tao Zhang","doi":"10.1063/5.0228865","DOIUrl":"https://doi.org/10.1063/5.0228865","url":null,"abstract":"Materials with electrocaloric effect (ECE) and/or thermal switching ratio λ are desirable for developing various heat management devices, but developing high-performance candidates, especially those that simultaneously possess large near room-temperature ECE and λ is actually absent. The Zr-rich PbZr1−xTixO3 (PZT) displays a composition-induced antiferroelectric-ferroelectric (AFE-FE) phase boundary, where an unusual negative ECE is expected. Meanwhile, the electric field-sensitive dipole orientation during the AFE-FE phase transition can be employed to modulate λ. In this work, the Zr-rich PZT with coexisting AFE and FE phases was developed and the AFE-FE phase transition temperature is tuned toward room temperature by changing the Ti content to achieve large negative ECE and λ. A large adiabatic temperature change ΔT of −3.3 K accompanied by a giant λ of 1.84 near 60 °C is captured in optimal PbZr0.95Ti0.05O3 ceramics, demonstrating a prominent application prospect in solid-state refrigeration.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142144428","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Two-dimensional ferroelectric semiconductor floating-gate transistor with light-tunable field effect for memory and photo-synapse","authors":"Yurong Jiang, Rui Wang, Yuting Peng, Hongzhi Li, Xueping Li, Yiduo Shao, Xiaobing Yan, Liangzhi Kou, Congxin Xia","doi":"10.1063/5.0197542","DOIUrl":"https://doi.org/10.1063/5.0197542","url":null,"abstract":"Ferroelectric field effect transistors (Fe-FETs) offer promising candidates for neuromorphic computing. However, it is still challenging to achieve a light-tunable field effect, which limits the function of photo-synapse. In this work, a ferroelectric semiconductor floating-gate transistor (FSF-FET) is proposed based on MoS2/h-BN/α-In2Se3 van der Waals heterojunctions (vdWHs), in which the two-dimensional ferroelectric semiconducting α-In2Se3 and dielectric h-BN serve as the trapped layer of charges and prevent layer, respectively. The excellent memory performances are exhibited, including a high programming/erasing ratio of over 107, a large memory window ratio of 74.69%, and good non-volatility. Moreover, the FSF-FETs also possess the light-tunable synapse behaviors, including the high paired-pulse facilitation of 236% and an obvious transition from short-term plasticity to long-term plasticity. The high recognition rate of 93.9% is achieved with dual-mode modulation of light and electrical pulses. The ferroelectric semiconductor floating-gate design opens up a strategy to realize the light-tunable field effect of Fe-FETs for photo-synapse.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142144429","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Haris Naeem Abbasi, Seunghyun Lee, Hyemin Jung, Nathan Gajowski, Yi Lu, Yifan Wang, Donghyeok Kim, Jie Zhou, Jiarui Gong, Chris Chae, Jinwoo Hwang, Manisha Muduli, Subramanya Nookala, Zhenqiang Ma, Sanjay Krishna
{"title":"Structural and electrical properties of grafted Si/GaAsSb heterojunction","authors":"Haris Naeem Abbasi, Seunghyun Lee, Hyemin Jung, Nathan Gajowski, Yi Lu, Yifan Wang, Donghyeok Kim, Jie Zhou, Jiarui Gong, Chris Chae, Jinwoo Hwang, Manisha Muduli, Subramanya Nookala, Zhenqiang Ma, Sanjay Krishna","doi":"10.1063/5.0225069","DOIUrl":"https://doi.org/10.1063/5.0225069","url":null,"abstract":"The short-wave infrared (SWIR) wavelength, especially 1.55 μm, has attracted significant attention in various areas such as high-speed optical communication and LiDAR systems. Avalanche photodiodes (APDs) are a critical component as a receiver in these systems due to their internal gain, which enhances the system performance. Silicon-based APDs are promising since they are CMOS compatible, but they are limited in detecting 1.55 μm light detection. This study proposes a p-type Si on n-type GaAs0.51Sb0.49 (GaAsSb) lattice matched to InP substrates heterojunction formed using a grafting technique for future GaAsSb/Si APD technology. A p+Si nanomembrane is transferred onto the GaAsSb/AlInAs/InP substrate, with an ultrathin ALD-Al2O3 oxide at the interface, which behaves as both double-side passivation and quantum tunneling layers. The devices exhibit excellent surface morphology and interface quality, confirmed by atomic force microscope and transmission electron microscope. Also, the current–voltage (I–V) of the p+Si/n−GaAsSb heterojunction shows the rectifying characteristics with an ideality factor of 1.8. The I–V tests across multiple devices confirm high consistency and yield. Furthermore, the x-ray photoelectron spectroscopy measurement reveals that GaAsSb and Si are found to have type-II band alignment with a conduction band offset of 50 meV, which is favorable for the high-bandwidth APD application. The demonstration of the GaAsSb/Si heterojunction highlights the potential to advance current SWIR PD technologies.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142144427","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Enhanced all-optical vector atomic magnetometer enabled by artificial neural network","authors":"Jianan Qin, Jinxin Xu, Zhiyuan Jiang, Jifeng Qu","doi":"10.1063/5.0218065","DOIUrl":"https://doi.org/10.1063/5.0218065","url":null,"abstract":"This paper reports an all-optical vector magnetometer enhanced by a machine learning model. Using a dual probing beam setup, spin projections in both probe directions are simultaneously detected. Vector information is directly obtained from the measured phases of spin projection signals. To enhance the measurement accuracy and mitigate the dead zone effect, we introduce an artificial neural network (ANN) to link the phase signals to the field direction. With the addition of amplitude information to the ANN input, the average angle error is reduced to less than 0.3° within a hemisphere. Furthermore, this configuration demonstrates a field angle sensitivity of better than 30 μ rad/Hz1/2.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142144426","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Malathi Nagaraja, Ullattuparambil Anagha, Saswat Subhankar, Rajeev N. Kini
{"title":"Thermally driven resistive switching in a charge density wave compound","authors":"Malathi Nagaraja, Ullattuparambil Anagha, Saswat Subhankar, Rajeev N. Kini","doi":"10.1063/5.0218725","DOIUrl":"https://doi.org/10.1063/5.0218725","url":null,"abstract":"This study delves into the nonlinear transport phenomena exhibited by the telephone number compound Sr14Cu24O41 (SCO), shedding light on the underlying mechanisms driving resistive switching behavior. Through a comprehensive investigation utilizing various measurement techniques, including continuous and pulsed I–V sweeps, terahertz time-domain spectroscopy, and numerical simulations, we unravel the intricate interplay between charge density wave (CDW) dynamics and Joule heating. Our findings reveal that while CDW-related effects contribute to the nonlinear conductivity observed in SCO at moderate electric fields, Joule heating emerges as the primary driving force behind the observed negative differential resistance and hysteresis at high electric fields/current densities. This conclusion is corroborated by the disappearance of nonlinear behavior under pulsed excitation, as well as the agreement between the numerical simulations and the experimental observations. Simulations underscore the pivotal role of Joule heating in inducing resistive switching. These insights deepen our understanding of the complex interplay between CDW physics and thermal effects in correlated electron systems, offering avenues for the design and optimization of functional electronic devices.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142142818","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Chubin Lin, Jiandong Chen, Huihui Wang, Yangyang Fu
{"title":"Unification of the breakdown criterion for thermal field emission-driven microdischarges","authors":"Chubin Lin, Jiandong Chen, Huihui Wang, Yangyang Fu","doi":"10.1063/5.0227666","DOIUrl":"https://doi.org/10.1063/5.0227666","url":null,"abstract":"Determining the characteristics of thermal field emission-induced breakdown is essential for various electron emission devices, such as thermionic energy converters. In previous studies, several mathematical models were developed to determine the breakdown voltages driven by field emission under different conditions; however, complicated computations were required to solve the numerical equations. There is still no consensus on the breakdown criterion when the thermal field emission comes into play. In this work, a unified breakdown criterion for the thermal field emission-induced microdischarge is proposed based on the definition of the thermal field emission coefficient γTFE (combined with the thermionic emission coefficient γTE and field emission coefficient γFE) from the emission current. The breakdown voltages scaling with the cathode temperature and gap distance are quantified. Distinct regimes corresponding to different electron emissions and their transitions are examined with the cathode temperature and gap distance tuned across a range of values. The results from this study provide an evaluation of thermal field emission-induced breakdowns and the dominant electron emission mechanisms in distinct regimes can be straightforwardly determined from the present model.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142142840","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Limits of high-frequency polarization switching in BaTiO3","authors":"Hasin Tamim, Rajan Khadka, Pawel Keblinski","doi":"10.1063/5.0218240","DOIUrl":"https://doi.org/10.1063/5.0218240","url":null,"abstract":"In this work, we use molecular dynamics simulations to investigate the switching behavior of BaTiO3 ferroelectric under the application of a high-amplitude high-frequency oscillatory electric field. While at lower frequencies, we observe a standard square-shaped hysteresis loop behavior, at frequencies approaching 1 THz, the hysteresis loop has an ellipsoidal shape. As the frequency increases, the average polarization oscillates without switching direction. To elucidate the origin of the ∼1 THz limit for the polarization switching, we analyzed unit-cell-level polarization vector maps. In this context, the analysis of the low-frequency switching events revealed that in addition to the majority of the polarization vectors exhibiting rapid switching, some “metastable” aligned polarization vectors persist longer with an average lifetime of ∼1 ps. As the frequency increases to the THz range, several polarization vector lines remain unswitched, thus preventing the polarization switching at the simulation domain level. Furthermore, we observe that with the increase in the amplitude of the applied electric field, one can increase the frequency at which switching is observed.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142142835","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Xun Ji, Qin Liu, Shan Huang, Andi Chen, Shengjun Wu
{"title":"Quantum sparse coding and decoding based on quantum network","authors":"Xun Ji, Qin Liu, Shan Huang, Andi Chen, Shengjun Wu","doi":"10.1063/5.0226021","DOIUrl":"https://doi.org/10.1063/5.0226021","url":null,"abstract":"Sparse coding provides a versatile framework for efficiently capturing and representing crucial data (information) concisely, which plays an essential role in various computer science fields, including data compression, feature extraction, and general signal processing. Here, we propose symmetric quantum neural networks for realizing sparse coding and decoding algorithms. Our networks consist of multi-layer, two-level unitary transformations that are naturally suited for optical circuits. Specifically, the two networks we propose can be efficiently trained together or separately via a quantum natural gradient descent algorithm. Utilizing the trained model, we achieve coding and decoding of sparse data including sparse classical data of binary and grayscale images, as well as sparse quantum data that are quantum states in a certain smaller subspace. The results demonstrate an accuracy of 98.77% for image reconstruction and a fidelity of 97.68% for quantum state revivification. Our quantum sparse coding and decoding model offers improved generalization and robustness compared to the classical model, giving insights to further research on quantum advantages in artificial neural networks.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142142806","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Zhongtao Shen, Zhaoyue Lü, Zhehao Chen, Junling Wang, Haichuan Mu
{"title":"Achievement and mechanism of large-scale color tunable OLEDs based on interfacial charge transfer complexes with dual donors","authors":"Zhongtao Shen, Zhaoyue Lü, Zhehao Chen, Junling Wang, Haichuan Mu","doi":"10.1063/5.0226298","DOIUrl":"https://doi.org/10.1063/5.0226298","url":null,"abstract":"Color tunable organic light-emitting diodes have intrigued many application fields, such as smart lighting and information encryption. In this study, we propose a simple structure based on interfacial charge transfer complexes (CTCs) with double donors and single acceptors for achieving color tunability. Through embedding a second donor between the primary donor and the acceptor, the emission of devices can be well-tuned by simply controlling the applied voltage. The calculated frontier molecular orbitals of constituted monomers and heterodimers via density function theory confirm the formation of CTCs between the donors and acceptor. Importantly, the highest occupied molecular orbital level and charge carrier mobility of the second donor are crucial to realize widely adjustable spectra with the voltage. With this strategy, the device incorporating 1,3-di(9H-carbazol-9-yl)benzene as the second donor and 4,4′,4″-tris[(3-methylphenyl)phenylamino] triphenylamine as the primary donor exhibits the largest color shift. The CIE coordinates span from (0.52, 0.46) at 4 V to (0.29, 0.26) at 10 V. These findings shed light on the fact that the double-donor-strategy is feasible for fulfilling large-scale color tunability of CTC-based organic light-emitting diodes and is beneficial to simplify the fabrication process.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142142833","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Oded Katz, Gilad Robert Barir, Barak Hadad, Daniel Marima, Alon Bahabad
{"title":"Optical inference using nonlinear optical diffraction","authors":"Oded Katz, Gilad Robert Barir, Barak Hadad, Daniel Marima, Alon Bahabad","doi":"10.1063/5.0212880","DOIUrl":"https://doi.org/10.1063/5.0212880","url":null,"abstract":"We present an optical inference platform based on the nonlinear interaction of a spatially modulated optical waveform in a second-harmonic-generation nonlinear crystal. Tuning the phase-matching condition allows for both efficient nonlinearity, required for general all-optical computing, and for optimizing the system performance, matching it to the spectral distribution of the input data to be processed.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142142839","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}