Kun Wang, Xue Chen, Zhiyu Zeng, Xi Su, Tao Guo, Zexin Tu, Jiaxian Wan, Liwei Ji, Hao Wu, Chang Liu
{"title":"High performance annealing-free thin-film transistors with 7-nm In0.72Ga0.28O/13-nm In0.46Ga0.54O homojunction channel","authors":"Kun Wang, Xue Chen, Zhiyu Zeng, Xi Su, Tao Guo, Zexin Tu, Jiaxian Wan, Liwei Ji, Hao Wu, Chang Liu","doi":"10.1063/5.0278333","DOIUrl":"https://doi.org/10.1063/5.0278333","url":null,"abstract":"Atomic layer deposition (ALD) enables the deposition of large-area, high-quality amorphous oxide semiconductor layers with precise control over film stoichiometry and thickness. In this study, homojunction thin-film transistors (TFTs) were fabricated using ALD. The homojunction structure consisted of a 7 nm thick In0.72Ga0.28O front channel layer and a 13 nm thick In0.46Ga0.54O back channel layer. By controlling In/Ga composition ratio and channel thickness, high performance field-effect transistors were fabricated at 200 °C without additional annealing. The transistor exhibited a mobility of 42.4 cm2 V−1 s−1, a conductive voltage near 0 V, a high Ion/Ioff ratio of 109, and a low subthreshold swing of 0.16 V/dec. Furthermore, compared to single-channel IGO devices, the homojunction dual-channel TFTs demonstrate superior performance in both bias stress stability and long-term stability.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"33 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983369","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Unusual Fermi-level pinning and Ohmic contact engineering for Janus TMD heterojunctions from an electronegativity perspective","authors":"Qian Liu, Zhen Zhu, Hai-Qing Xie, Zhi-Qiang Fan, Dan Wu, Ke-Qiu Chen","doi":"10.1063/5.0287304","DOIUrl":"https://doi.org/10.1063/5.0287304","url":null,"abstract":"Using density functional theory calculations, we systematically investigated the fat band structures and Schottky barriers of 72 van der Waals heterojunctions (vdWHs) formed by combining 1T-phase transition metal dichalcogenides (TMDs) (MX2, M = Mo, W; X = S, Se, Te) with 2H-phase Janus TMDs (MXY, M = Mo, W; X, Y = S, Se, Te). Unlike conventional TMDs, Janus TMDs lack mirror symmetry and exhibit a built-in in-plane dipole due to their asymmetric atomic configuration. A larger electronegativity gradient across the Janus TMDs leads to enhanced charge redistribution at the vdWH interface and a stronger in-plane dipole, resulting in unusual Fermi-level pinning (FLP). The calculated pinning factors for 1T-TMDs/MoSTe and 1T-TMDs/WSTe vdWHs are particularly low, reflecting a strong FLP effect. Despite the wide variation in work functions among the 1T-TMDs, their Fermi levels are consistently pinned near the band edges of MoSTe and WSTe, enabling quasi-Ohmic or Ohmic p-type and n-type contacts. Furthermore, the vdWHs exhibit low tunneling-specific resistivity, confirming their potential for ultra-low contact resistance applications in next-generation single-layer transistors.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"14 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983419","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Wanchun Yu, Ni Xiong, Tao Wen, Huihong Wu, Zhenzhi Cheng, Fei Gao, Guangsheng Luo, Weiping Zhou
{"title":"Large room temperature anomalous Hall effect in c axis oriented non-collinear antiferromagnetic Mn3Ga thin films with ferrimagnetic Mn3Ga inclusion","authors":"Wanchun Yu, Ni Xiong, Tao Wen, Huihong Wu, Zhenzhi Cheng, Fei Gao, Guangsheng Luo, Weiping Zhou","doi":"10.1063/5.0281636","DOIUrl":"https://doi.org/10.1063/5.0281636","url":null,"abstract":"Non-collinear antiferromagnets Mn3X (X = Sn, Ge, Ga) have recently attracted a lot of attention due to their fascinating properties with great application prospects in spintronics. Mn3Ga possesses the highest Néel temperature among this family, providing huge potential for realistic spintronic device application. However, the small anomalous Hall conductivity of Mn3Ga makes it lack competitiveness. In this paper, c axis oriented Mn3Ga thin films with D019 hexagonal structure were prepared by optimizing the MgO(111) substrate temperature. Large anomalous Hall resistivity up to 1.53 μΩ cm at 300 K is observed for (0002) oriented Mn3Ga film grown at 450 °C, corresponding to a Hall conductivity of about 30 Ω−1 cm−1. Further analysis indicates that the skew-scattering mechanism, which is attributable to the presence of a small amount of the D022-Mn3Ga phase, is the main source for the large Hall conductivity observed here. These results raise the intriguing prospect of Mn3Ga films as a key component in antiferromagnetic spintronic devices.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"162 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983347","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Al3+-mediated aggregation-induced enhancement of photosensitization performance of gold nanoclusters","authors":"Yuchi Cheng, Menghui Jia, Zhongwei Yu","doi":"10.1063/5.0284240","DOIUrl":"https://doi.org/10.1063/5.0284240","url":null,"abstract":"Photocatalytic oxidation driven by photosensitizers has demonstrated significant potential in the realm of green chemistry. In recent years, metal nanoclusters with well-defined atomic structures have garnered attention as promising photosensitizers owing to their distinctive photoelectronic properties. Nevertheless, enhancing the efficiency of photosensitization remains a critical challenge that impedes its practical implementation. This study reveals that the addition of Al3+ can concurrently augment both the luminescence and photosensitization abilities of glutathione-protected gold nanoclusters. Time-resolved spectroscopic investigations indicate that Al3+ induces intermolecular aggregation of gold nanoclusters, thereby promoting the radiative transition of the excited triplet state and enhancing the energy transfer efficiency to molecular oxygen. The strategy presented herein offers a convenient approach for developing high-performance metal nanocluster-based photosensitization systems.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"36 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983371","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Li-Tong Su, Cheng Peng, Zheng-Hao Guo, Chun-Ting Xu, Wei Hu
{"title":"Multi-order optical differentiator integrated with an omnidirectionally selective subtracter","authors":"Li-Tong Su, Cheng Peng, Zheng-Hao Guo, Chun-Ting Xu, Wei Hu","doi":"10.1063/5.0292585","DOIUrl":"https://doi.org/10.1063/5.0292585","url":null,"abstract":"Optical computing offers high-speed, low-power data processing, while optical differentiation enables instant edge detection for applications like autonomous driving, object recognition, and bio-detection. Introducing an extra algorithm to optical differentiation will further extend its functionality. Here, we integrate an omnidirectional subtracter with a multi-order optical differentiator via combining distinct spiral lens phases with deflection phases. With this design, zeroth-, first-, and second-order differentiations are spatially separated, and the local linear polarization always orients toward the normal of optical edges for linearly polarized incidence. Thereby, selective edge subtractions can be carried out through simply rotating a polarizer. The design is verified in a photopatterned liquid crystal, whose electro-optical tunability enables a broadband operation across the entire visible spectrum. Rotating a polarizer confirms omnidirectional edge extraction in first- and second-order differentiations while preserving the zeroth-order bright field imaging. The direction-selective defect suppression enhances applications like rainy-day autonomous driving and object recognition in directional noise. This work advances optical differentiation, enabling high-performance edge-sensitive imaging.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"47 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983374","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Thermal stress stabilized thick perovskite heterostructures for radiation detection","authors":"Xini Zhang, Yiping Li, Yuanxiao Chen, Yanshuang Li, Hongxing Tian, Rongrong Cheacharoen, Jingjing Zhao, Yehao Deng","doi":"10.1063/5.0283310","DOIUrl":"https://doi.org/10.1063/5.0283310","url":null,"abstract":"Integrating lead halide perovskite onto the standard readout circuit substrate is the path to the commercialization of perovskite-based radiation detection and imaging. However, due to the large thermal expansion coefficient difference between perovskite and inorganic substrate, such heterostructure faces the challenge of thermal stress induced mechanical instability. This problem will be extremely severe for the thick perovskite film for radiation detection because the thermal strain energy accumulates with film thickness. Here, first by theoretical analysis, we quantized the thermal stress instability and found that a temperature variation of only 20 °C around room temperature will suffice to delaminate a 100 µm thick perovskite film from the substrate, which prediction agrees with experiments. We then proposed to promote the heterostructure's mechanical stability by increasing the perovskite nucleation rate on inorganic substrate to enhance the interface adhesive energy. Based on a sacrificial seeding layer, we realized stable interface between the thick perovskite film and the typical inorganic substrate, including indium tin oxide, silicon, and gallium nitride that can withstand at least 100 cycles of temperature variation between 25 and 150 °C and then fabricated high performance radiation detectors based on such heterostructures.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983348","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pengshun Shan, Jie Su, Yong Liu, Ruowei Wang, Minghui Xu, Weijin Kong, Jinhua Zhao, Tao Liu
{"title":"Controlled filament stability in SrTiO3 memristors via swift Xe ion irradiation","authors":"Pengshun Shan, Jie Su, Yong Liu, Ruowei Wang, Minghui Xu, Weijin Kong, Jinhua Zhao, Tao Liu","doi":"10.1063/5.0276146","DOIUrl":"https://doi.org/10.1063/5.0276146","url":null,"abstract":"Due to uncontrolled conductive filament (CF) formation and rupture during operation, CF randomness in SrTiO3-based memristors severely limits their stability and retention. To address this challenge, we employ swift heavy ion (SHI) irradiation—516 MeV Xe ions—on Pt/SrTiO3/Nb:SrTiO3 devices, introducing controlled ion track defects that guide filament formation. The irradiated memristors demonstrate remarkable performance improvements, achieving a lower SET voltage of 0.65 V (compared to 0.85 V for unirradiated devices), extended retention (>106 s vs <105 s), and superior stability (σ/μ = 0.06/0.06 vs 0.14/0.04). Moreover, these devices reliably emulate synaptic plasticity with minimal cycle-to-cycle variations (<7.2%), enabling high-fidelity neuromorphic applications. When deployed in simulated neural networks for handwritten digit recognition, the irradiated memristors attain a recognition accuracy of 91.6%, showcasing their robustness in real-time computing tasks. These results highlight SHI irradiation as an effective strategy to engineer defect-guided pathways in oxide memristors, advancing their applicability in stable, high-performance neuromorphic systems.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"29 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983367","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pengfei Liu, Meng Zhang, Lanrong Zou, Zhendong Jiang, Lei Lu, Man Wong, Hoi-Sing Kwok
{"title":"Alleviation of self-heating degradation in polycrystalline silicon thin-film transistors via voltage pulse modulation","authors":"Pengfei Liu, Meng Zhang, Lanrong Zou, Zhendong Jiang, Lei Lu, Man Wong, Hoi-Sing Kwok","doi":"10.1063/5.0274914","DOIUrl":"https://doi.org/10.1063/5.0274914","url":null,"abstract":"This work presents a voltage pulse modulation strategy to effectively mitigate self-heating degradation in polycrystalline silicon thin-film transistors. By applying synchronized voltage stress (SVS) with optimized pulse parameters, the proposed method significantly suppresses channel temperature buildup and reduces device degradation. A predictive thermal model, rigorously validated through coupled simulations and experimental measurements, enables precise control of temperature dynamics under diverse operating conditions. Experimental demonstrations using light-emitting diode-integrated driver circuits reveal substantially improved operational stability under SVS, in sharp contrast to the rapid performance degradation observed with continuous stress. This purely electrical approach requires no structural modifications and offers a practical and cost-effective solution to enhance the reliability of advanced display technologies.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"47 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983365","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Xiaodong Qiu, Zhujuan Li, Can Wang, Yuyang Mu, Yaling Zhou, Zhenjie Fan, Lin Huang, Fan Yu, Qichao Tian, Qinghao Meng, Bin Yang, Di Wu, Junwei Liu, Fang-Sen Li, Yi Zhang
{"title":"Molecular beam epitaxy and electronic structures of rare-earth selenide EuSe thin films","authors":"Xiaodong Qiu, Zhujuan Li, Can Wang, Yuyang Mu, Yaling Zhou, Zhenjie Fan, Lin Huang, Fan Yu, Qichao Tian, Qinghao Meng, Bin Yang, Di Wu, Junwei Liu, Fang-Sen Li, Yi Zhang","doi":"10.1063/5.0278149","DOIUrl":"https://doi.org/10.1063/5.0278149","url":null,"abstract":"The rare-earth Eu-based compound EuSe has attracted widespread attention due to its unique half-filled 4f orbital with large orbital momentum and strong correlation effects. Here, we realize the molecular beam epitaxial (MBE) growth of high-quality EuSe thin films on SrTiO3(001) and bilayer graphene (BLG) substrates. The EuSe grown on SrTiO3 substrate forms an out-of-plane (001) facet single-crystalline film, with the in-plane orientation EuSe〈110〉 direction paralleled to the SrTiO3〈100〉 direction. In contrast, the EuSe film grown on the BLG substrate has various in-plane rotational domains. The electronic band structures of the EuSe films are experimentally characterized by in situ angle-resolved photoemission spectroscopy, showing a semiconductive nature with the Eu 4f band as the top of the valence band. The bandgap size of EuSe grown on BLG is further determined as about 2.8 eV via low-temperature scanning tunneling spectroscopy. The MBE growth and the electronic structure characterizations of the EuSe thin films would promote further research and applications on the half-filled 4f electrons of rare-earth Eu-based compounds.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"31 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983366","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Shuhao Xie, Shaohua Gao, Longchao Wang, Yang Li, Jie Dang, Xinzheng Zhang, Mingjiang Zhang
{"title":"Low-threshold lasing in cholesteric liquid crystals enabled by asymmetric defect layer positioning","authors":"Shuhao Xie, Shaohua Gao, Longchao Wang, Yang Li, Jie Dang, Xinzheng Zhang, Mingjiang Zhang","doi":"10.1063/5.0272422","DOIUrl":"https://doi.org/10.1063/5.0272422","url":null,"abstract":"Liquid crystal lasers are significant in photonics and applications, yet achieving low-threshold lasing remains challenging. Here, we investigate how defect positioning affects lasing performance in cholesteric liquid crystals (CLCs) with three defect layers. Simulations reveal that synchronously displacing the first two defect layers toward the third layer significantly enhances the central defect mode's density of states (DOS), particularly in asymmetric configurations near the third defect layer. This asymmetry-induced DOS enhancement boosts dye emission efficiency. Experimentally, we use wedge-shaped LC films to continuously tune defect positions and observe that asymmetric structures near the third defect layer exhibit higher lasing intensity and a lower threshold. The threshold of the asymmetric structure could be reduced by a factor of 3.4 compared to the symmetric structure. Our findings provide a strategy for low-threshold CLC lasers by leveraging defect positioning.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"61 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144983368","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}