{"title":"Field-free spin–orbit torque magnetization switching in Pt/CoTb devices grown on flexible substrates for neuromorphic computing","authors":"Wei Wang, Chuanwei Feng, Yiheng Wang, Qikun Huang, Dong Wang, Yibo Fan, Xiang Han, Lihui Bai, Yanxue Chen, Yufeng Tian, Shishen Yan","doi":"10.1063/5.0231869","DOIUrl":"https://doi.org/10.1063/5.0231869","url":null,"abstract":"Flexible spintronic devices based on spin–orbit torque (SOT)-induced perpendicular magnetization switching (PMS) have attracted increasing attention due to their high storage intensity and good programming capability. However, to achieve deterministic PMS, an in-plane auxiliary magnetic field is required, which greatly limits its application. Here, we show that “robust” magnetic field-free SOT-driven PMS is realized in the oblique sputtered Pt/CoTb multilayers grown on a flexible polyimide substrate. “Robust” means the magnetic field-free SOT switching is highly repeatable and stable after 100 bending cycles under various bending conditions. Additionally, the fabricated flexible multilayers exhibit nearly linear and nonvolatile multistate plasticity as synapses and a nonlinear sigmoid activation function when acting as neurons. We construct a fully connected neural network for handwritten digit recognition, achieving an over 96.27% recognition rate. Our findings may spur further investigations on the SOT-based flexible spintronic devices for wearable artificial intelligence applications.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541752","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
E. Negri, W. Fuscaldo, D. González-Ovejero, P. Burghignoli, A. Galli
{"title":"TE-polarized leaky-wave beam launchers: Generation of Bessel and Bessel–Gauss beams","authors":"E. Negri, W. Fuscaldo, D. González-Ovejero, P. Burghignoli, A. Galli","doi":"10.1063/5.0234371","DOIUrl":"https://doi.org/10.1063/5.0234371","url":null,"abstract":"The generation of focused beams in the millimeter- and submillimeter-wave ranges, with transverse-electric (TE) polarization, is investigated in the radiative near-field region. The desired field distribution is achieved through a leaky-wave beam launcher consisting of a grounded dielectric slab with an annular strip grating on top excited by a circular slot on the bottom ground plane. The latter is fed by a Marié transducer, which converts the input, fundamental TE10 mode of a standard rectangular waveguide into the higher-order TE01 mode propagating in the circular waveguide connected to the device. The generation of TE-polarized diffraction-limited Bessel and Bessel–Gauss distributions is achieved by suitably synthesizing the annular strip grating. Simulated results are in excellent agreement with those predicted by leaky-wave analysis providing a proof-of-concept for the generation of TE-polarized Bessel and Bessel–Gauss beams at 300 GHz with a beam size of 1.7 and 1.9 mm up to the nondiffractive range of about 25 and 15 mm from an aperture plane with radius of 12.75 mm, respectively.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541750","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Low-cost green antisolvent with an ultrawide processing window for efficient and stable perovskite solar cells","authors":"Hui Li, Junhui Han, Qimin Lan, Zhe Wu, Cong Shao, Xing'ao Li, Jizheng Wang","doi":"10.1063/5.0235360","DOIUrl":"https://doi.org/10.1063/5.0235360","url":null,"abstract":"Antisolvent engineering is one of the most useful strategies to get high-efficiency perovskite solar cells (PSCs). Nevertheless, the most present commonly used effective antisolvents, such as chlorobenzene and diethyl ether, are toxic and expensive. Moreover, these antisolvents applied in PSCs are rather restricted due to their narrow processing window. Herein, we report a low-cost green antisolvent isopropanol (IPA) that displays ultrawide processing window, which dramatically enhances the reproducibility of PSCs. The highest power conversation efficiency of PSCs treated by IPA can reach as high as 24.8%. The origin of IPA effects is further disclosed by the intermolecular hydrogen-bonding force between IPA and DMF/DMSO, and the force can effectively remove DMF/DMSO in the spinning perovskite precursor film and helpfully enhance perovskite crystal growth with less carrier recombination as demonstrated by using various techniques. Our results here demonstrate a cheap green antisolvent for reproducible, high-efficient, stable PSCs and also provide an in-depth understanding the significant role of antisolvent in the fabrication of PSCs.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541749","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"High-efficiency and easy-processing thin-film lithium niobate edge coupler","authors":"Di Jia, Qiang Luo, Chen Yang, Rui Ma, Xuanyi Yu, Feng Gao, Qifan Yang, Fang Bo, Guoquan Zhang, Jingjun Xu","doi":"10.1063/5.0233467","DOIUrl":"https://doi.org/10.1063/5.0233467","url":null,"abstract":"Fiber-to-chip coupling with ultralow loss and broadband operation wavelength range is essential in the practical applications of thin-film lithium niobate (TFLN) integrated photonic devices. However, the existing edge couplers often require electron beam lithography overlaying and multiple etching processes, which are expensive and complex. In this Letter, we demonstrate an edge coupler that includes only a vertically tapered TFLN waveguide and silicon dioxide cladding. The coupling efficiency between a lensed fiber and an on-chip LN waveguide is down to 1.43 dB/facet, while the 3-dB bandwidth exceeds the range from 1510 to 1630 nm. These edge couplers also show reliable fiber misalignment tolerance. Furthermore, the fabrication complexity is greatly reduced since only a single etching step for the TFLN waveguide is needed. The minimum waveguide width of 1.3 μm guarantees compatibility with i-line photolithography, providing a potential for massive production of TFLN devices.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541751","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Investigating the correlation between flow dynamics and flow-induced voltage generation","authors":"Hikaru Takeda, Naoya Iwamoto, Mitsuhiro Honda, Masaki Tanemura, Ichiro Yamashita, Atsuki Komiya, Takeru Okada","doi":"10.1063/5.0230115","DOIUrl":"https://doi.org/10.1063/5.0230115","url":null,"abstract":"The conversion of water current to voltage generation through graphene has gained interest in both basic physics and applications such as sensors and electricity generation systems. However, many aspects of the mechanism remain unclear. Recently, quantum-based momentum transfer theories have been reported, but these often do not account for flow conditions. In this study, we investigated the correlation between the flow conditions of a liquid medium and the electrical conduction of graphene through experiments and numerical calculations. Our results suggest that the necessary condition is that the flow must be neither irregular nor purely laminar; instead, graphene responds to the transition process of the fluid. This finding supports the extension of current theories and presents valuable insights for both basic science and industrial applications.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541520","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Shizai Chu, Yifei Hao, Shaopeng Feng, Xia Hong, Keji Lai
{"title":"Room-temperature modulation of microwave conductivity in ferroelectric-gated correlated oxides","authors":"Shizai Chu, Yifei Hao, Shaopeng Feng, Xia Hong, Keji Lai","doi":"10.1063/5.0231424","DOIUrl":"https://doi.org/10.1063/5.0231424","url":null,"abstract":"We report the nonvolatile modulation of microwave conductivity in ferroelectric PbZr0.2Ti0.8O3-gated ultrathin LaNiO3/La0.67Sr0.33MnO3 correlated oxide channel visualized by microwave impedance microscopy. Polarization switching is obtained by applying a tip bias above the coercive voltage of the ferroelectric layer. The microwave conductivity of the correlated channel underneath the up- and down-polarized domains has been quantified by finite-element analysis of the tip-sample admittance. At room temperature, a resistance on/off ratio above 100 between the two polarization states is sustained at frequencies up to 1 GHz, which starts to drop at higher frequencies. The frequence-dependence suggests that the conductance modulation originates from ferroelectric field-effect control of carrier density. The modulation is nonvolatile, remaining stable after 6 months of domain writing. Our work is significant for potential applications of oxide-based ferroelectric field-effect transistors in high-frequency nanoelectronics and spintronics.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541746","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Hongru Zhao, Xinkong Wei, Ruiyin Gu, Mingzheng Xie, Weihua Han
{"title":"Enhanced water splitting on (010) facet-exposed BiVO4 photoanode with improved carrier injection efficiency","authors":"Hongru Zhao, Xinkong Wei, Ruiyin Gu, Mingzheng Xie, Weihua Han","doi":"10.1063/5.0231098","DOIUrl":"https://doi.org/10.1063/5.0231098","url":null,"abstract":"Transition metal oxide semiconductors, noted for their stability and suitable bandgap, are promising photoanodes for water splitting. Surface engineering is critical to tackle issues like low carrier mobility and charge recombination, stemming from atomic arrangement and Fermi level differences. While exposing dominant crystal facets boosts photocatalytic capability, it can hinder carrier injection into the electrolyte. In this study, BiVO4 films with various facet exposures were synthesized and characterized using scanning electron microscopy and x-ray diffraction to confirm their morphology and crystalline structure. Mott–Schottky analysis was employed to investigate changes in the band structure near the semiconductor–electrolyte interface, revealing that high (010)-BiVO4 facet exposure enhances carrier separation but reduces injection efficiency. The results from photoconductive atomic force microscopy tests demonstrated that enhanced band bending at the semiconductor interface improves hole transfer. Coating the (010)-BiVO4 photoanode with MoS2 and an amorphous ZrO2 interlayer yielded a photocurrent density of 0.6 mA cm−2 at 1.2 V (vs RHE) under AM 1.5 G illumination, tripling the pristine photoanode's performance and nearly tripling water splitting efficiency. Mechanism revealing the improved photoelectrochemical performance is attributed to a greater band bending on the BiVO4 surface, enhancing hole injection dynamics. This work provides a feasible strategy for a deeper understanding of the intrinsic mechanisms of facet engineering and improving the activity of photoanodes.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541748","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Coupling light into a guided Bloch surface wave using an inversely designed nanophotonic cavity","authors":"Zongyuan Tang, Tian-Long Guo, Yannick Augenstein, Adriano Troia, Yanjun Liu, Matthieu Roussey, Carsten Rockstuhl, Emiliano Descrovi","doi":"10.1063/5.0232450","DOIUrl":"https://doi.org/10.1063/5.0232450","url":null,"abstract":"Controlling the propagation of light in the form of surface modes on miniaturized platforms is crucial for multiple applications. For dielectric multilayers that sustain Bloch surface waves at their interface to an isotropic dielectric medium, a conventional approach to manipulate them exploits shallow surface topographies fabricated on top of the truncated stack. However, such structures typically exhibit low index contrasts, making it challenging to confine, steer, and guide the Bloch surface waves. Here, we theoretically and experimentally demonstrate a device for a Bloch surface wave platform that resonantly couples light from a cavity to a straight waveguide. The structure is designed using topology optimization in a 2D geometry under the effective index approximation. In particular, the cavity–waveguide coupling efficiency of the radiation emitted by an individual source in the cavity center is optimized. The cavity is experimentally found to exhibit a narrow resonant peak that can be tuned by scaling the structure. The waveguide is shown to guide only light that resonates in the cavity. Fully three-dimensional simulations of the entire device validate the experimental observations.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142536657","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Estimation of the friction coefficient by identifying the evolution of rough surface topography","authors":"Dafei Huang, Wurui Ta, Youhe Zhou","doi":"10.1063/5.0230431","DOIUrl":"https://doi.org/10.1063/5.0230431","url":null,"abstract":"The complexity and randomness of surface roughness make the origin of friction always puzzling. Is there a potential correlation mechanism between the evolution of friction force and surface topography, and is it possible to estimate the friction coefficient from the topography evolution? Here, we explore the evolution of surface topography in metallic materials during friction by defining the characteristic orientation of the surface and analyzing its changes over time, which closely mirrors the behavior of friction forces. Then, we propose a simple relationship that relates the characteristic orientation and friction force via the friction coefficient. Therefore, the friction coefficient can be evaluated based on topography evolution without relying on any theoretical modeling assumptions. These results reveal the mechanism between complex surface topography and friction force through a simple formula and provide a method to estimate the friction coefficient. This method has promising applications when the friction coefficient is difficult to measure, such as in large-scale landslides and geologic faults.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142536695","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Songqi Jia, Félix Beaudoin, Pericles Philippopoulos, Hong Guo
{"title":"Atomistic first-principles modeling of single donor spin-qubit","authors":"Songqi Jia, Félix Beaudoin, Pericles Philippopoulos, Hong Guo","doi":"10.1063/5.0221229","DOIUrl":"https://doi.org/10.1063/5.0221229","url":null,"abstract":"Using an impurity atom in crystal silicon as a spin-1/2 qubit has been made experimentally possible recently where the impurity atom acts as a quantum dot (QD). Quantum transport in and out of such a donor QD occurs in the sequential tunneling regime where a physical quantity of importance is the charging (addition) energy, which measures the energy necessary for adding an electron into the donor QD. In this work, we present a first-principles method to quantitatively predict the addition energy of the donor QD. Using density functional theory (DFT), we determine the impurity states that serve as the basis set for subsequent exact diagonalization calculation of the many-body states and energies of the donor QD. Due to the large effective Bohr radius of the conduction electrons in Si, very large supercells containing more than 10 000 atoms must be used to obtain accurate results. For the donor QD of a phosphorus impurity in bulk Si, the combined DFT and exact diagonalization predicts the first addition energy to be 53 meV, in good agreement with the corresponding experimental value. For the donor QD of an arsenic impurity in Si, the first addition energy is predicted to be 44.2 meV. The calculated many-body wave functions provide a vivid electronic picture of the donor QD.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":null,"pages":null},"PeriodicalIF":4.0,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142536689","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}