Reports on progress in physics. Physical Society (Great Britain)最新文献

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Strong field physics in open quantum systems. 开放量子系统中的强场物理。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-07-11 DOI: 10.1088/1361-6633/adeebb
Neda Boroumand, Adam Thorpe, Graeme Bart, Andrew M Parks, Mohamad Toutounji, Giulio Vampa, Thomas Brabec, Lu Wang
{"title":"Strong field physics in open quantum systems.","authors":"Neda Boroumand, Adam Thorpe, Graeme Bart, Andrew M Parks, Mohamad Toutounji, Giulio Vampa, Thomas Brabec, Lu Wang","doi":"10.1088/1361-6633/adeebb","DOIUrl":"https://doi.org/10.1088/1361-6633/adeebb","url":null,"abstract":"<p><p>Dephasing is the loss of phase coherence due to the interaction of an electron with the environment. The most common approach to model dephasing in light-matter interaction is the relaxation time approximation. Surprisingly, its use in intense laser physics results in a pronounced failure, because ionization is highly overestimated. Here, this shortcoming is corrected by developing a strong field model in which the many-body environment is represented by a heat bath. Our model reveals that ionization enhancement and suppression by several orders of magnitude are still possible, however only in more extreme parameter regimes. Our approach allows the integration of many-body physics into intense laser dynamics with minimal computational and mathematical complexity, thus facilitating the identification of novel effects in strong-field physics and attosecond science.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144621450","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The Dean-Kawasaki equation and stochastic density functional theory. Dean-Kawasaki方程与随机密度泛函理论。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-07-10 DOI: 10.1088/1361-6633/adee2e
Pierre Illien
{"title":"The Dean-Kawasaki equation and stochastic density functional theory.","authors":"Pierre Illien","doi":"10.1088/1361-6633/adee2e","DOIUrl":"https://doi.org/10.1088/1361-6633/adee2e","url":null,"abstract":"<p><p>The Dean-Kawasaki (DK) equation, which is at the basis of stochastic density functional theory (SDFT), was proposed in the mid-nineties to describe the evolution of the density of interacting Brownian particles, which can represent a large number of systems such as colloidal suspensions, supercooled liquids, polymer melts, biological molecules, active or chemotactic particles, or ions in solution. This theoretical framework, which can be summarized as a mathematical reformulation of the coupled overdamped Langevin equations that govern the dynamics of the particles, has attracted a significant amount of attention during the past thirty years. In this review, I present the context in which this framework was introduced, and I recall the main assumptions and calculation techniques that are employed to derive the DK equation. Then, in the broader context of statistical mechanics, I show how SDFT is connected to other theories, such fluctuating hydrodynamics, macroscopic fluctuation theory, or mode-coupling theory. The mathematical questions that are raised by the DK equation are presented in a non-specialist language. In the last parts of the review, I show how the original result was extended in several directions, I present the different strategies and approximations that have been employed to solve the DK equation, both analytically and numerically. I finally list the different situations where SDFT was employed to describe the fluctuations of Brownian suspensions, from the physics of active matter to the description of charged particles and electrolytes.&#xD;&#xD.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144610564","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Laser-induced plasma formation and cavitation in water: from nanoeffects to extreme states of matter. 激光诱导等离子体形成和水中空化:从纳米效应到物质的极端状态。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-07-09 DOI: 10.1088/1361-6633/adedb3
Norbert Linz, Sebastian Freidank, Xiao-Xuan Liang, Alfred Vogel
{"title":"Laser-induced plasma formation and cavitation in water: from nanoeffects to extreme states of matter.","authors":"Norbert Linz, Sebastian Freidank, Xiao-Xuan Liang, Alfred Vogel","doi":"10.1088/1361-6633/adedb3","DOIUrl":"https://doi.org/10.1088/1361-6633/adedb3","url":null,"abstract":"<p><p>We present an in-depth analysis of the energy dependence of optical breakdown in water by tightly focused laser pulses, from plasma formation to shock waves and cavitation. Laser pulses of fs to ns durations and UV to IR wavelengths are aberration-free focused through microscope objectives. Photography captures luminescent plasmas with submicrometer resolution, and bubble threshold and size are determined via probe beam scattering. The energy dependence of mechanical effects is quantified through the maximum bubble radius R<sub>max</sub>. We find three key scenarios depicting the interaction between multiphoton and avalanche ionization, recombination, and thermal ionization from nanoeffects near threshold to extreme energy densities. They include a previously unknown scenario that emerges with single-longitudinal-mode UV ns pulses from compact lasers. It enables cost-effective creation of nanoeffects, as demonstrated on corneal tissue and glass. High-resolution colour photography revealed new insights in the spatiotemporal dynamics of plasma formation, with an interplay of breakdown waves, string formation by local instabilities of avalanche ionization, and radiative energy transport. Plasma volume data from photographs together with absorption measurements show that the average energy density of luminescent fs and ns plasmas is similar, ranging between 10 and 40 kJ/cm<sup>3</sup>. However, small hot regions with up to 400 kJ/cm<sup>3</sup>are formed in ns breakdown. From the hot regions, energy is spread out via X-ray bremsstrahlung, forming a luminescent halo. Well above threshold, R<sub>max</sub>scales with E<sup>1/3</sup>across all scenarios, with 15% - 20% conversion of laser energy into bubble energy. With increasing plasma energy density, an ever-larger energy fraction is converted into shock wave energy (75% at 40 kJ/cm<sup>3</sup>). We discuss guidelines for parameter selection in laser surgery and material processing in bulk media as well as for laser ablation and breakdown spectroscopy in liquids. Finally, we suggest roadmaps for future experimental and modeling work, and for broadening applications.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144602492","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fluctuations and the limit of predictability in protein evolution. 蛋白质进化中的波动和可预测性的限制。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-07-09 DOI: 10.1088/1361-6633/adea92
Saverio Rossi, Leonardo Di Bari, Martin Weigt, Francesco Zamponi
{"title":"Fluctuations and the limit of predictability in protein evolution.","authors":"Saverio Rossi, Leonardo Di Bari, Martin Weigt, Francesco Zamponi","doi":"10.1088/1361-6633/adea92","DOIUrl":"10.1088/1361-6633/adea92","url":null,"abstract":"<p><p>Protein evolution involves mutations occurring across a wide range of time scales. In analogy with disordered systems in statistical physics, this dynamical heterogeneity suggests strong correlations between mutations happening at distinct sites and times. To quantify these correlations, we examine the role of various fluctuation sources in protein evolution, simulated using a data-driven energy landscape as a proxy for protein fitness. By applying spatio-temporal correlation functions developed in the context of disordered physical systems, we disentangle fluctuations originating from the initial condition, i.e. the ancestral sequence from which the evolutionary process originated, from those driven by stochastic mutations along independent evolutionary paths. Our analysis shows that, in diverse protein families, fluctuations from the ancestral sequence predominate at shorter time scales. This allows us to identify a time scale over which ancestral sequence information persists, enabling its reconstruction. We link this persistence to the strength of epistatic interactions: ancestral sequences with stronger epistatic signatures impact evolutionary trajectories over extended periods. At longer time scales, however, ancestral influence fades as epistatically constrained sites evolve collectively. To confirm this idea, we apply a standard ancestral sequence reconstruction (ASR) algorithm and verify that the time-dependent recovery error is influenced by the properties of the ancestor itself. Overall, our results reveal that the properties of ancestral sequences-particularly their epistatic constraints-influence the initial evolutionary dynamics and the performance of standard ASR algorithms.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144546516","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Quantum Fisher information and its dynamical nature. 量子费雪信息及其动力学性质。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-07-07 DOI: 10.1088/1361-6633/ade453
Matteo Scandi, Paolo Abiuso, Jacopo Surace, Dario De Santis
{"title":"Quantum Fisher information and its dynamical nature.","authors":"Matteo Scandi, Paolo Abiuso, Jacopo Surace, Dario De Santis","doi":"10.1088/1361-6633/ade453","DOIUrl":"10.1088/1361-6633/ade453","url":null,"abstract":"<p><p>The importance of the Fisher information metrics and its quantum generalisations is testified by the number of applications that this has in very different fields, ranging from hypothesis testing to metrology, passing through thermodynamics. Still, from the rich range of possible quantum Fisher informations, only a handful are typically used and studied. This review aims at collecting a number of results scattered in the literature and provide a cohesive treatment to people who begin the study of Fisher information and to those who are already working on it to have a more organic understanding of the topic. Moreover, we complement the review with new results about the relation between Fisher information and physical evolutions. Extending previous works, we show that dynamical properties such as (complete) positivity, Markovianity, detailed balance, retrodictive power of evolution maps can be characterised in terms of their relation with respect to the Fisher information metrics. These results show a fact that was partially overseen in the literature, namely the inherently dynamical nature of Fisher information.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144295458","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Many-body quantum resources of graph states. 图态的多体量子资源。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-07-07 DOI: 10.1088/1361-6633/adecc0
Marcin Płodzień, Maciej Lewenstein, Jan Chwedenczuk
{"title":"Many-body quantum resources of graph states.","authors":"Marcin Płodzień, Maciej Lewenstein, Jan Chwedenczuk","doi":"10.1088/1361-6633/adecc0","DOIUrl":"https://doi.org/10.1088/1361-6633/adecc0","url":null,"abstract":"<p><p>Characterizing the non-classical correlations of a complex many-body system is an important part of quantum technologies. A versatile tool for such a task is one that scales well with the size of the &#xD; system and which can be both easily computed and measured. In this work we focus on graph states, that are promising platforms for quantum computation, simulation and metrology. We consider four topologies, namely the star graph states with edges, Tur'an graphs, $r$-ary tree graphs, and square grid cluster states, &#xD; and provide a method to characterise their quantum content: the &#xD; many-body Bell correlations, non-separability and entanglement depth for an arbitrary number of qubits. &#xD; We also relate the strength of these many-body correlations to the usefulness of graph states for quantum sensing. Finally, we characterize many-body entanglement depth in graph states with up &#xD; to $8$ qubits in $146$ classes non-equivalent under local transformations and graph isomorphisms. &#xD; The technique presented is simple and does not make any assumptions about the multi-qubit state, so it could find applications wherever precise knowledge of many-body quantum correlations is required.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144585832","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A review of the fraction of four-coordinated boron in binary borate glasses and melts. 二元硼酸玻璃中四配位硼组分的研究进展。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-07-03 DOI: 10.1088/1361-6633/adc69c
Oliver L G Alderman, Nagia S Tagiara, Ian Slagle, Rebecca M Gabrielsson, Piper Boggs, Molly Wagner, Aaron Rossini, Sophia John, Leilani Rocha, Robert M Wilson, Harry Hawbaker, Steve W Martin, Alex C Hannon, Efstratios I Kamitsos, Steve A Feller
{"title":"A review of the fraction of four-coordinated boron in binary borate glasses and melts.","authors":"Oliver L G Alderman, Nagia S Tagiara, Ian Slagle, Rebecca M Gabrielsson, Piper Boggs, Molly Wagner, Aaron Rossini, Sophia John, Leilani Rocha, Robert M Wilson, Harry Hawbaker, Steve W Martin, Alex C Hannon, Efstratios I Kamitsos, Steve A Feller","doi":"10.1088/1361-6633/adc69c","DOIUrl":"10.1088/1361-6633/adc69c","url":null,"abstract":"<p><p>In borate materials, boron is found predominantly in either trigonal planar, or tetrahedral coordination states with oxygen, which are the two most ubiquitous building blocks of borate glasses. The fraction of tetrahedral boron,<i>N</i><sub>4</sub>, is found to vary considerably with both glass composition and applied pressure, as well as with fictive temperature - a result of its underlying dependence on temperature in the molten and supercooled liquid states. As such, the parameter<i>N</i><sub>4</sub>is of fundamental structural importance, along with the mechanisms driving its evolution and its strong influence on thermophysical material properties.<i>N</i><sub>4</sub>in glasses has been experimentally determined using a variety of means including nuclear magnetic resonance (NMR) spectroscopy, vibrational spectroscopy, and x-ray and neutron diffraction. In this review, we discuss how the techniques for the measurement of<i>N</i><sub>4</sub>have evolved and improved since the pioneering x-ray diffraction measurements of the 1930s, up to the present day. A database is compiled of the available<i>high-quality</i>numerical experimental data for<i>N</i><sub>4</sub>, with a non-exclusive focus on binary borate glasses of the form<i>RM</i><sub>2</sub>O<sub><i>z</i></sub>-B<sub>2</sub>O<sub>3</sub>where<i>R</i>is the molar ratio of modifier to boron oxide and<i>M</i>is a metal cation of formal charge<i>z+</i>, other than boron. In addition, we report new<i>N</i><sub>4</sub>values for a series of strontium borate glasses, measured by<sup>11</sup>B magic angle spinning NMR, where a disparity in the literature is found. Based on the findings of the review, we are able to point to the gaps in our knowledge where future resources could best be focused, as well as summarizing overarching trends, the present state-of-the-art, and making recommendations for best practices.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-07-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143744571","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Revealing quantum geometry in nonlinear quantum materials. 揭示非线性量子材料中的量子几何。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-07-03 DOI: 10.1088/1361-6633/ade454
Yiyang Jiang, Tobias Holder, Binghai Yan
{"title":"Revealing quantum geometry in nonlinear quantum materials.","authors":"Yiyang Jiang, Tobias Holder, Binghai Yan","doi":"10.1088/1361-6633/ade454","DOIUrl":"10.1088/1361-6633/ade454","url":null,"abstract":"<p><p>Berry curvature-related topological phenomena have been a central topic in condensed matter physics. Yet, until recently other quantum geometric quantities such as the metric and connection received only little attention due to the relatively few effects which have been documented for them. This review gives a modern perspective how quantum geometric quantities naturally enter the nonlinear responses of quantum materials and demonstrate their deep connection with excitation energy, lifetimes, symmetry, and corresponding physical processes. The multitude of nonlinear responses can be subdivided into nonlinear optical effects, subgap responses, and nonlinear transport phenomena. Such a distinction by energy scales facilitates an intuitive understanding of the underlying electronic transitions, giving rise to a unified picture of the electron motion beyond linear order. The well-known injection and shift currents constitute the main resonances in the optical regime. Exploiting their respective lifetime and symmetry dependencies, this review elucidates how these resonances can be distinguished by a corresponding quantum geometric quantity that shares the same symmetry. This is followed by a brief exposition of the role of quasiparticle lifetimes for nonlinear subgap responses, which presents a window into the microscopic short-term dynamics as well as the ground state correlation and localization. We conclude with an account of the anomalous motion due to the Berry curvature dipole and quantum metric dipole in nonlinear transport, clarifying the correspondence between physical observables and the underlying mechanisms. This review highlights the close relationship between quantum geometry and nonlinear response, showing the way towards promising probes of quantum geometry and enabling novel avenues to characterize complex materials.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-07-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144295459","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Temporal solitons in hybrid-driven active resonators. 混合驱动有源谐振器中的时间孤子。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-06-13 DOI: 10.1088/1361-6633/addfe9
D Kazakov, F Capasso, M Piccardo
{"title":"Temporal solitons in hybrid-driven active resonators.","authors":"D Kazakov, F Capasso, M Piccardo","doi":"10.1088/1361-6633/addfe9","DOIUrl":"10.1088/1361-6633/addfe9","url":null,"abstract":"<p><p>Solitons, as coherent structures that maintain their shape while traveling at constant velocity, are ubiquitous across various branches of physics, from fluid dynamics to quantum fields. However, it is within the realm of optics where solitons have not only served as a primary testbed for understanding solitary wave phenomena but have also transitioned into applications ranging from telecommunications to metrology. In the optical domain, temporal solitons are localized light pulses, self-reinforcing via a delicate balance between nonlinearity and dispersion. Among the many systems hosting temporal solitons, active optical resonators stand out due to their inherent gain medium, enabling to actively sustain solitons. Unlike conventional mode-locked lasers, active resonators offer a richer landscape for soliton dynamics through hybrid driving schemes, such as coupling to passive cavities or under external optical injection, affording them unparalleled control and versatility. We discuss key advantages of these systems, with a particular focus on quantum cascade lasers as a promising soliton technology within the class of active resonators. By exploring diverse architectures from traditional Fabry-Perot cavities to racetrack devices operated under external injection, we present the current state-of-the-art and future directions for soliton-based sources in the realm of semiconductor lasers and hybrid integrated photonic systems.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144217766","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A homogenous polymer design with widely tunable work functions for high-performance two-dimensional photodetectors. 一种具有广泛可调工作功能的高性能二维光电探测器的均匀聚合物设计。
Reports on progress in physics. Physical Society (Great Britain) Pub Date : 2025-06-12 DOI: 10.1088/1361-6633/ade006
Youchen Chen, Nan Cui, Xiaoru Li, Yang Li, Zhenhe Zhao, Yu Wang, Miaomiao Yang, Haoran Mu, Nianqing Fu, Guangyu Zhang, Shenghuang Lin
{"title":"A homogenous polymer design with widely tunable work functions for high-performance two-dimensional photodetectors.","authors":"Youchen Chen, Nan Cui, Xiaoru Li, Yang Li, Zhenhe Zhao, Yu Wang, Miaomiao Yang, Haoran Mu, Nianqing Fu, Guangyu Zhang, Shenghuang Lin","doi":"10.1088/1361-6633/ade006","DOIUrl":"10.1088/1361-6633/ade006","url":null,"abstract":"<p><p>Contact electrodes, which significantly influence the Schottky barrier and interfacial quality with two-dimensional (2D) materials, are key to boosting the performance of 2D photodetectors. However, it is challenging to fabricate electrically conducting films with sufficiently high or low work functions (WF<sub>2</sub>) in homogenous electrodes for 2D devices due to the fixed WF of traditional metallic and semi-metallic electrodes, which restricts their adaptability for 2D metal-semiconductor-metal (MSM) structured photodetectors. Here, we utilize a homogenous PEDOT:PSS electrode designed with adjustable WF ranging from 5.1 to 3.2 eV in 2D MSM photodetectors, achieving a high rectification ratio of ∼10<sup>5</sup>and superior performance metrics: responsivity up to 1.8 A W<sup>-1</sup>, an<i>I</i><sub>light</sub>/<i>I</i><sub>dark</sub>of 10<sup>8</sup>, and an ultrafast response time of 3.2 μs. Meanwhile, the excellent transparency of PEDOT:PSS electrode extends the 2D device's response to the near-infrared (NIR) region, overcoming the semiconductor bandgap limitation. The universality of polymer electrode is proven across various 2D photodetectors, and its flexibility enables the creation of durable, wearable 2D devices. This work paves the way for the development of flexible, self-powered photodetectors, heralding a new era of next-generation intelligent interactive systems.</p>","PeriodicalId":74666,"journal":{"name":"Reports on progress in physics. Physical Society (Great Britain)","volume":" ","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144217765","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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