Advanced Composites and Hybrid Materials最新文献

{"title":"Unveiling the latent potential: Ni/CoFe2O4-loaded electrospun PVDF hybrid composite-based triboelectric nanogenerator for mechanical energy harvesting applications","authors":"Hema Malini Venkatesan,&nbsp;Insun Woo,&nbsp;Jae Uk Yoon,&nbsp;Prasad Gajula,&nbsp;Anand Prabu Arun,&nbsp;Jin Woo Bae","doi":"10.1007/s42114-025-01296-z","DOIUrl":"10.1007/s42114-025-01296-z","url":null,"abstract":"<div><p>This study investigates the potential of Ni-doped cobalt ferrite (CoFe₂O₄, N-CF) nanoparticles (NPs)-loaded electrospun poly(vinylidene fluoride) (PVDF) composites for triboelectric nanogenerators (TENGs) to efficiently harness electrical energy from low-frequency mechanical vibrations. PVDF was chosen for its strong electroactive polar phase and inherent tribo-negative properties. Cobalt ferrite (CF) NPs exhibit exceptional charge-trapping capabilities, while nickel’s metallic nature minimizes triboelectric losses due to its conductivity. The synergistic effects of Ni-doped CF (N-CF) fillers enhance charge-trapping efficiency and reduce triboelectric losses, significantly boosting TENG performance. Nickel oxide (NiO), CF, and N-CF NPs were synthesized using a facile co-precipitation method, and PVDF composites were fabricated through electrospinning. The physical and crystalline properties of the composites were characterized using various spectroscopic techniques. Results indicated that incorporating 3 wt% N-CF into PVDF optimized the <i>β</i>-crystalline phase content, crucial for improved output performance. Electrospun PVDF/N-CF (PNC) nanocomposite mats served as the tribo-negative (TN) layer, while aluminum (Al) electrode acted as the tribo-positive (TP) layer in TENG device fabrication. Electrical measurements showed that pristine PVDF/Al TENG devices exhibited lower performance (open-circuit potential—<i>V</i>_oc = 22 V, short-circuit current—<i>I</i>_sc = 0.61 µA) compared to the optimized Al/PNC3 TENG devices (<i>V</i>_oc = 421 V, <i>I</i>_sc = 1.0 µA). The importance of a spacer gap was emphasized, with devices incorporating a spacer gap demonstrating superior performance. The optimized TENG device successfully powered over 30 light-emitting diodes and a stopwatch in real-time applications. This study highlights the exceptional output performance of Al/PNC3-based TENGs and provides valuable insights into the development of next-generation sustainable energy harvesting materials.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01296-z.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143698581","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Influence of TiC particles on the properties of AA2017 friction surfaced coatings","authors":"Mariane Chludzinski,&nbsp;Javier Vivas,&nbsp;Juan Manuel Vázquez-Martínez,&nbsp;Irene Del Sol,&nbsp;Egoitz Aldanondo Begiristain","doi":"10.1007/s42114-025-01231-2","DOIUrl":"10.1007/s42114-025-01231-2","url":null,"abstract":"<div><p>Friction surfacing (FS) is a solid-state process employed for coatings that has demonstrated significant advancements in the manufacturing of aluminium matrix composites reinforced with ceramic particles. This study explores the effect of AA2017 aluminium consumable rods packed with titanium carbide (TiC) in the FS process applied to an AA6082 substrate. A subsequent post-processing friction stir process (FSP) was performed to further refine the distribution of ceramic particles. Analyses were conducted using light optical and scanning electron microscopy, X-ray diffractometer (XRD), microhardness, and pin-on-flat wear testing. The results demonstrated that the incorporation of TiC reinforcement significantly enhanced the FS deposition efficiency and rate by approximately 31%, without affecting rod consumption. Initially, the TiC particles were distributed in layers parallel to the substrate surface, but the FSP technique dispersed them throughout the aluminium matrix. In terms of mechanical properties, the reinforcement increased microhardness by 13.6% and reduced wear resistance (wear volume) by 13%. Notably, the FSP process enhanced wear resistance, reducing wear volume by 48% compared to the TiC-free coating, while also mitigating the hardness increase caused by the FS process. Additionally, XRD analysis indicated that neither FS nor FSP generated new phases, indicating no interaction between the aluminium matrix and the ceramic reinforcements.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01231-2.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143698579","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A novel disposable dual-sensing platform based on DNA-aptamer amplified with gold nanoparticles/Nb4C3-MXene for simultaneous detection of lead and cadmium","authors":"Hassan Karimi-Maleh,&nbsp;Zhouxiang Zhang,&nbsp;Najmeh Zare,&nbsp;Onur Karaman,&nbsp;Yangpin Wen,&nbsp;Tao Wu,&nbsp;Nianbing Zhong,&nbsp;Li Fu","doi":"10.1007/s42114-025-01216-1","DOIUrl":"10.1007/s42114-025-01216-1","url":null,"abstract":"<div><p>Herein, we designed a special screen-printing carbon electrode system with two independent zones to realize the immobilization of two kinds of aptamers on electrode surface. Nb₄C₃-MXene is a remarkable member from MX₃ MXene with many excellent properties. In this study, Nb₄C₃-MXene nanosheets were firstly modified onto the screen-printing carbon electrode surface as the substrate materials to offer big surface area and then gold nanoparticles were loaded onto the surface of Nb₄C₃-MXene nanosheets through electrodeposition. Afterward, the aptamer-containing double-stranded DNA was spontaneously assembled onto the modified electrode surface through the Au–S bond. Owing to high affinity of aptamers towards the heavy metal ions (Cd²⁺ and Pb²⁺ in this case), the aptamers tagged with methylene blue and ferrocene would specifically bond with heavy metal ions to form folded structures and competed off from the electrode surface, and then the change of electrochemical signals can be detected by square wave voltammetry. The aptasensor exhibits a good linear response towards Cd²⁺ and Pb²⁺ from 1 × 10⁻¹⁰ to 1 × 10⁻⁷ M, and their detection limits are 59.8 pM of Pb²⁺ and Cd²⁺ of 146.2 pM; LOQ are 93.7 pM of Pb²⁺ and 164.8 pM of Cd²⁺, respectively.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01216-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143688595","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Aromatic polyamine-grafted and nitrogen-doped graphene anodes boosting surface-dominated sodium storage","authors":"Di Wu,&nbsp;Qingzhi Song,&nbsp;Deliang Cui,&nbsp;Yanlu Li,&nbsp;Qilong Wang,&nbsp;Haohai Yu,&nbsp;Gang Lian","doi":"10.1007/s42114-025-01274-5","DOIUrl":"10.1007/s42114-025-01274-5","url":null,"abstract":"<div><p>The development of high-capacity and long-cycled carbon anodes for sodium-ion batteries is limited by the sluggish kinetics of surface capacitive adsorption that dominates the rate capability. Covalently grafted functionalization and heteroatom doping have emerged as promising strategies to overcome these issues. Herein, a one-step hydrothermal strategy is proposed to simultaneously achieve 1,2,4-Triaminobenzene (Tri) grafting and nitrogen doping of reduced graphene oxide (Tri-N-rGO). The formation of an amide bond between Tri and rGO enables structural stability and enriches additional adsorption sites around Tri. A high edge-nitrogen ratio of 82.5% facilitates the enhancement of surface-dominated sodium adsorption. Consequently, the Tri-N-rGO electrode delivers a high discharge specific capacity of 340.3 mAh g⁻¹ at 0.1 A g⁻¹ and a superior rate capability of 180.3 mAh g⁻¹ at 5 A g⁻¹. More importantly, it displays excellent long-term cycling stability and delivers a reversible capacity of 175.1 mAh g⁻¹ after 5000 cycles even at 5 A g⁻¹. The enhanced surface-controlled adsorption mechanism is further demonstrated by multiple measurements and theoretical calculations. The corresponding full cell can still deliver a high specific capacity of 172.7 mAh g⁻¹ after 500 cycles at 0.5 A g⁻¹. This study opens a new avenue for designing high-performance carbon for high-rate sodium-ion batteries and confers the extension to other secondary batteries.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01274-5.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143688571","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Enhanced electrochemical performance of zinc-ion batteries using functionalized nano-chitin separators","authors":"Chengwei Lin,&nbsp;Sainan Ou,&nbsp;Baobin Liu,&nbsp;Yao Niu,&nbsp;Xian Wang,&nbsp;Huiping Lin,&nbsp;Ran Li,&nbsp;Meng An,&nbsp;Xinxiang Zhang,&nbsp;Zhanhui Yuan","doi":"10.1007/s42114-025-01211-6","DOIUrl":"10.1007/s42114-025-01211-6","url":null,"abstract":"<div><p>The development and evaluation of a novel separator material for aqueous zinc-ion batteries (ZIBs) are discussed, which are promising for energy storage due to their use of abundant zinc metal, eco-friendly electrolytes, and high safety. The main challenges in ZIBs are the formation of zinc dendrites and the hydrogen evolution reaction (HER), which can lead to short circuits and reduced battery life. To address these issues, the authors have functionalized chitin separators through a process involving alkaline treatment and mechanical grinding, resulting in nano-chitin fibers with varying degrees of deacetylation (D-x-ChNF). The D-4-ChNF separator, in particular, has been shown to have uniformly distributed nanochannels, high mechanical strength, and excellent electrochemical stability. It also exhibits a strong affinity for aqueous ZnSO₄ electrolytes and enhances the electrochemical reversibility of zinc through increased coordination with Zn²⁺ ions. This leads to a significant improvement in the battery’s cycle life, with the D-4-ChNF separator outperforming traditional glass fiber (GF) separators by more than six times in cycle life at 5 mA cm⁻² and 5 mAh cm⁻². The D-4-ChNF separator also demonstrates superior rate performance and long-term cycling stability, with capacity retention rates of 90.46% and 96.68% after 1000 cycles at 5 A g⁻¹ and 10 A g⁻¹, respectively. The separator’s ability to suppress dendrite growth and improve the uniformity of zinc deposition is attributed to its ability to reduce nucleation overpotential and promote uniform zinc deposition along the (002) crystal plane. The D-4-ChNF separator, with its low cost and high stability, offers a promising solution for enhancing the performance and practical application of ZIBs, providing new insights into the development of efficient and sustainable energy storage technologies.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01211-6.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143667978","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Robust superhydrophobic ORMOSIL hybrid coating via chemical-assembly engineering for wood protection","authors":"Xinxiang Zhang,&nbsp;Sainan Ou,&nbsp;Linxin Zhang,&nbsp;Jiaxin Tan,&nbsp;Wensheng Lin,&nbsp;Ran Li,&nbsp;Zhanhui Yuan","doi":"10.1007/s42114-025-01223-2","DOIUrl":"10.1007/s42114-025-01223-2","url":null,"abstract":"<div><p>Poor mechanical stability of superhydrophobic coating limits its practical application. In this work, robust superhydrophobic organically modified silicate (ORMOSIL) hybrid coatings were fabricated on wood surface by a chemical-assembly engineering induced by click reaction of PMHS. The superhydrophobic ORMOSIL coating was hybridized from poly(methylhydrogen)siloxane (PMHS), tetravinyltetramethylcyclotetrasiloxane (V4), and silica nanoparticles (SNPs). The click reaction between PMHS and SNPs built a chemically bonded rough surface with very low surface energy, while click reaction between PMHS and V4 resulted in a strong glue of adjacent SNPs, endowing ORMOSIL hybrid coatings with good mechanical stability. Chemical-assembly engineering afforded ORMOSIL coatings superhydrophobicity, self-cleaning property, and good robustness, and the unique physical characteristic of ORMOSIL also gave superhydrophobic coatings excellent resistance to UV light, high and low temperature, and humid and salt mist environments. Finally, chemical-assembly engineering had been demonstrated to be applicable in fabrication of superhydrophobic coating on various substrates containing hydroxyl groups and various nanoparticles could be applied to replace SNPs.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01223-2.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143667975","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Unleashing potential: engineering advancements in two-dimensional MoS2 for improved energy applications","authors":"Shalmali R. Burse,&nbsp;Harshitha B. Tyagaraj,&nbsp;Moein Safarkhani,&nbsp;Supriya J. Marje,&nbsp;Gagankumar S. K,&nbsp;Amal Al Ghaferi,&nbsp;Ebrahim Alhajri,&nbsp;Nilesh R. Chodankar,&nbsp;Yun Suk Huh,&nbsp;Young-Kyu Han","doi":"10.1007/s42114-025-01289-y","DOIUrl":"10.1007/s42114-025-01289-y","url":null,"abstract":"<div><p>Molybdenum disulfide (MoS₂) has emerged as a promising material in the search for sustainable energy solutions due to its exceptional properties. This article comprehensively explores the potential of MoS₂ in energy-related applications, focusing on its structure, synthesis methods, and engineering strategies. The unique structural features of MoS₂, such as its monolayer and hierarchical architecture, are examined in detail, highlighting their significant impact on energy conversion and storage phenomena. Additionally, various synthesis techniques, including both top-down and bottom-up approaches, are discussed, along with how these methods can be tailored to control the morphology and properties of MoS₂ for specific applications. Engineering strategies to optimize MoS₂ for energy technologies are also explored. These include nanostructure tuning, heteroatom doping, heterostructure integration, and manipulation of interlayer spaces, all of which can enhance the material’s performance in energy generation and storage devices. The importance of these strategies in improving the efficiency, stability, and scalability of MoS₂-based technologies is emphasized. Overall, this work underscores the immense potential of MoS₂ for propelling energy technologies toward sustainability and efficiency, instilling hope and optimism for the future of the energy field.</p><h3>Graphical Abstract</h3>\u0000<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01289-y.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143667863","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Polyvinyl alcohol modified plant fiber hydrogel pressure and strain dual-model sensors for biomedical signal detection","authors":"Zhiheng Gu,&nbsp;Ruikang Ma,&nbsp;Xia Chen,&nbsp;Zhaoxing Lin,&nbsp;Yu Yang,&nbsp;Bin Tan,&nbsp;Jiaji Sun,&nbsp;Tingjie Chen","doi":"10.1007/s42114-024-01165-1","DOIUrl":"10.1007/s42114-024-01165-1","url":null,"abstract":"<div><p>Flexible and stretchable hydrogels have become promising materials for wearable biomedical devices used in continuous health monitoring. A simple and effective ball-milling method is proposed to create conductive, biocompatible polyvinyl alcohol (PVA) hydrogels modified with plant fibers and carbon nanotubes (CNTs) for dual-model wearable devices. The plant fibers and CNTs disperse within the PVA network, providing excellent stretchability (up to 4200% tensile strain), self-healing, and conductivity. These hydrogels can be used for assembling and repairing electrical circuits and serve as sensing elastomers for capacitive strain sensors with high sensitivity, durability, and wide strain range. After high temperature treatment, a conductive and compressible porous PVA/PF@CNT sponge can be obtained from PVA/PF@CNT hydrogel, which can be assembled as piezoresistive pressure sensors with a sensitivity of 0.89 kPa⁻¹. These sensors enable real-time monitoring of human biological signals, including joint movements, facial expressions, and throat activity.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-024-01165-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143667800","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Rational synthesis of sea urchin-like NiCo-LDH/tannin carbon microsphere composites using microwave hydrothermal technique for high-performance asymmetric supercapacitor","authors":"Weigang Zhao,&nbsp;Jianping Deng,&nbsp;Menghan Li,&nbsp;Guanben Du,&nbsp;Mizi Fan,&nbsp;Haili Gao,&nbsp;Zhanhui Yuan","doi":"10.1007/s42114-025-01220-5","DOIUrl":"10.1007/s42114-025-01220-5","url":null,"abstract":"<div><p>In this study, tannin-derived porous carbon (TAC) with different microstructures was prepared via a microwave hydrothermal method, followed by KOH activation. Subsequently, the sea urchin–like NiCo-LDH/Tannin-derived carbon-based microsphere composite materials were rationally synthesized through a single-step microwave hydrothermal co-assembly process. The physicochemical characteristics and supercapacitive performance were systematically analyzed. TAC with a microspherical structure promoted and controlled the growth of LDHs, resulting in a more regular sea urchin–like structure, improved dispersibility, reduced resistance, and increased active sites. NiCo-LDH@TAC600-0 (without KOH activation) as an electrode material delivered a specific capacitance (Cs) of 1250 F g⁻¹ at 1 A g⁻¹ and 1035 F g⁻¹ at 10 A g⁻¹, with a rate performance of 82.8%. The asymmetric supercapacitor device using NiCo-LDH@TAC600-0 and TAC provided an energy density of 30.8 Wh kg⁻¹ at 800 W kg⁻¹ and a capacitance retention rate of 72.5% after 5000 cycles. This study offers a novel approach to enhancing NiCo-LDH properties for efficient energy storage.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01220-5.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143667799","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Halide perovskite-polymer composite film for bright and stable light-emitting devices","authors":"Maoding Cheng,&nbsp;Brooke Robinson,&nbsp;Manoj Shah,&nbsp;Emad Omar Badradeen,&nbsp;Araceli Herrera Mondragon,&nbsp;Roberto Gonzalez Rodriguez,&nbsp;Jingbiao Cui,&nbsp;Yuankun Lin,&nbsp;Anupama B. Kaul,&nbsp;Fumiya Watanabe,&nbsp;Grant Wangila,&nbsp;Mansour Mortazavi,&nbsp;Chao Yan,&nbsp;Zhanhu Guo,&nbsp;Qinglong Jiang","doi":"10.1007/s42114-025-01294-1","DOIUrl":"10.1007/s42114-025-01294-1","url":null,"abstract":"<div><p>Stability is the primary hindrance for the application of halide perovskite material in light-emitting devices, solar cells, and other devices. In this work, halide perovskite and polymer composite film have been prepared for stable and bright light-emitting devices. Pure-phase Cs₄PbBr₆ crystals have been synthesized, and their photoluminescence (PL) properties and fluorescence lifetimes have been investigated. The Cs₄PbBr₆ crystals exhibited high uniformity but underwent rapid photodegradation under light irradiation. To address this issue, we prepared bright light-emitting devices using composite of Cs₄PbBr₆ crystals and polyethylene oxide (PEO) as the emission layer. The aim was to improve the optical and physical properties of halide perovskites, such as photodegradation and stability. PEO, with its excellent film-forming ability, created a uniform and dense film on the halide perovskite surface, filling microscopic defects and providing a protective barrier. FTIR, morphology, and PL analyses confirmed the protective role of the halide perovskite and polymer composite film. The composite film light-emitting devices demonstrated improved stability and higher PL brightness, with a peak brightness approaching 3 × 10⁸ cd/m², which was approximately 75% higher than the pure halide perovskite devices.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 2","pages":""},"PeriodicalIF":23.2,"publicationDate":"2025-03-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s42114-025-01294-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143655289","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}