Journal of Superconductivity and Novel Magnetism最新文献

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Superparamagnetic Behaviour and Magnetotransport in Mn-doped Ni/NiO Nanocomposites mn掺杂Ni/NiO纳米复合材料的超顺磁性和磁输运
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-12 DOI: 10.1007/s10948-026-07232-6
S. D. Kamble, C. D. Kamble, U. P. Gawai, N. B. Thakare, P. G. Chavan, D. Kumar, S. K. Gurav
{"title":"Superparamagnetic Behaviour and Magnetotransport in Mn-doped Ni/NiO Nanocomposites","authors":"S. D. Kamble,&nbsp;C. D. Kamble,&nbsp;U. P. Gawai,&nbsp;N. B. Thakare,&nbsp;P. G. Chavan,&nbsp;D. Kumar,&nbsp;S. K. Gurav","doi":"10.1007/s10948-026-07232-6","DOIUrl":"10.1007/s10948-026-07232-6","url":null,"abstract":"<div><p>In the present work, pure and Mn (0.00, 0.02) doped Ni/NiO nanocomposites were synthesized via a microwave-assisted sol-gel auto-combustion method. The synthesized samples were characterized using X-ray diffraction (XRD), Raman spectroscopy, atomic force microscopy (AFM), vibrating sample magnetometer (VSM), and magnetoresistance (MR) measurements. Raman analysis revealed the presence of 1LO mode for pure Ni/NiO and 2LO mode for Mn-doped Ni/NiO. AFM images confirmed uniform and densely packed grains with root-mean-square (RMS) roughness values ranging from 23 to 32 nm. The 2% Mn-doped Ni/NiO nanostructures exhibit enhanced ferromagnetism with a blocking temperature around 200 K, as revealed by ZFC-FC bifurcation. Magnetic hysteresis loops confirm zero coercivity and no remanence, indicating soft ferromagnetic behaviour with superparamagnetic-like relaxation. The MR of 2% Mn-doped Ni/NiO nanocomposites was investigated over a wide temperature range (2–300 K). All samples exhibited negative MR due to suppression of AFM domains and enhanced FM ordering, with a maximum value of -0.40% at 300 K, while pure Ni/NiO showed a higher MR of -0.6%. The observed negative magnetoresistance and butterfly-like hysteresis are directly correlated with the coexistence of ferromagnetic Ni and antiferromagnetic NiO phases, where spin-dependent scattering and domain wall dynamics govern the transport behavior. Fitting of the resistivity to a Bloch-Grüneisen and Fermi liquid (T<sup>2</sup>) model yields a nearly field-independent Debye temperature (<span>(:{{Theta:}}_{D})</span>≈303–320 K). Doping significantly enhances the residual resistivity and electron-phonon scattering coefficient, consistent with stronger disorder scattering.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148751489","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Half-metallic Ferromagnetism and Giant Magnetic Anisotropy in Vacancy-ordered Double Perovskite Rb2WBr6 空位有序双钙钛矿Rb2WBr6的半金属铁磁性和巨磁各向异性
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-12 DOI: 10.1007/s10948-026-07231-7
Haiming Huang, Yiyuan Xiao, Ziyu Liu, Cheng Liu, Xuejing Yang, Yonghong Hu, Amel Laref
{"title":"Half-metallic Ferromagnetism and Giant Magnetic Anisotropy in Vacancy-ordered Double Perovskite Rb2WBr6","authors":"Haiming Huang,&nbsp;Yiyuan Xiao,&nbsp;Ziyu Liu,&nbsp;Cheng Liu,&nbsp;Xuejing Yang,&nbsp;Yonghong Hu,&nbsp;Amel Laref","doi":"10.1007/s10948-026-07231-7","DOIUrl":"10.1007/s10948-026-07231-7","url":null,"abstract":"<div><p>We report a first-principles investigation on cubic double perovskite Rb<sub>2</sub>WBr<sub>6</sub>, which exhibits an exceptional combination of structural robustness, mechanical flexibility, perfect spin polarization, high Curie temperature, and giant magnetic anisotropy-key merits urgently demanded in advanced spintronics. This compound possesses excellent thermodynamic stability confirmed by tolerance factor, negative formation energy, and cohesive energy. Mechanical evaluations demonstrate its satisfied Born-Huang stability, superior ductility, and intrinsic flexibility, enabling facile integration into flexible devices. Remarkably, Rb<sub>2</sub>WBr<sub>6</sub> is identified as a robust half-metal with 100% spin polarization at the Fermi level, accompanied by a large half-metallic gap of 0.85 eV for high operational stability. The total magnetic moment is 2.0 μ<sub>B</sub> per unit cell, dominated by W atoms. Most prominently, it achieves a record-high three-dimensional magnetic anisotropy energy up to 2881.41 μeV/unit cell, far beyond most rare-earth-free magnets. These superior integrated properties make Rb<sub>2</sub>WBr<sub>6</sub> a highly promising candidate for next-generation spintronic devices, flexible magnetoelectronics, and high-density magnetic storage systems.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148751481","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A First-Principles Study of Structural, Electronic, Magnetic, Mechanical and Thermodynamic Properties of CeCrO3 Compound CeCrO3化合物结构、电子、磁性、力学和热力学性质的第一性原理研究
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-11 DOI: 10.1007/s10948-026-07226-4
Omer Kabi, Alae Samih, Hussein Sabbah, Rachid El Fdil, Zakaria Fadil, Mohammed S.S. Abu-Jafar, Mahmoud M.A. Farout, El Mehdi Salmani, Ahmad A.A. Mousa, Hala S. A Ghannam, Chaitany Jayprakash Raorane, Salah Saadaoui
{"title":"A First-Principles Study of Structural, Electronic, Magnetic, Mechanical and Thermodynamic Properties of CeCrO3 Compound","authors":"Omer Kabi,&nbsp;Alae Samih,&nbsp;Hussein Sabbah,&nbsp;Rachid El Fdil,&nbsp;Zakaria Fadil,&nbsp;Mohammed S.S. Abu-Jafar,&nbsp;Mahmoud M.A. Farout,&nbsp;El Mehdi Salmani,&nbsp;Ahmad A.A. Mousa,&nbsp;Hala S. A Ghannam,&nbsp;Chaitany Jayprakash Raorane,&nbsp;Salah Saadaoui","doi":"10.1007/s10948-026-07226-4","DOIUrl":"10.1007/s10948-026-07226-4","url":null,"abstract":"<div><p>A first-principles study of orthorhombic CeCrO<sub>3</sub> is carried out to investigate its structural, electronic, magnetic, elastic, and thermodynamic properties. The results confirm the stability of the orthorhombic perovskite structure. Electronic calculations indicate half-metallicity within the GGA and SCAN approximations with a magnetic moment of ~ 8 µB. A systematic GGA + U investigation reveals a transition to a semiconducting state with increasing electron correlation, yielding a band gap of 3.02 eV, in excellent agreement with the experimental optical gap of 3.04 eV. The material exhibits a robust ferromagnetic ground state dominated by Cr moments, with contributions from Ce and O through orbital hybridization. Elastic analysis reveals a stiff, moderately ductile with a poisson’s ratio of 0.266, and anisotropic material, while thermodynamic properties confirm strong bonding and thermal stability. These findings highlight CeCrO<sub>3</sub> as a promising candidate for spintronic, magnetoelectric, and multifunctional applications.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148751099","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermal Quantum Correlations in a Two-Qubit XXZ Heisenberg Chain with Dzyaloshinskii–Moriya, Kaplan–Shekhtman–Entin–Wohlman–Aharony, and Asymmetric In-Plane Anisotropy Interactions 具有Dzyaloshinskii-Moriya, Kaplan-Shekhtman-Entin-Wohlman-Aharony和不对称面内各向异性相互作用的二量子位XXZ海森堡链中的热量子相关
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-10 DOI: 10.1007/s10948-026-07233-5
Mounaim Hamdoune, Mohammed Daoud
{"title":"Thermal Quantum Correlations in a Two-Qubit XXZ Heisenberg Chain with Dzyaloshinskii–Moriya, Kaplan–Shekhtman–Entin–Wohlman–Aharony, and Asymmetric In-Plane Anisotropy Interactions","authors":"Mounaim Hamdoune,&nbsp;Mohammed Daoud","doi":"10.1007/s10948-026-07233-5","DOIUrl":"10.1007/s10948-026-07233-5","url":null,"abstract":"<div><p>This work investigates quantum correlations in a thermally equilibrated two-qubit Heisenberg XXZ spin chain extended with Dzyaloshinskii–Moriya (DM), Kaplan–Shekhtman–Entin–Wohlman–Aharony (KSEA) interactions, and a physically motivated asymmetric exchange anisotropy (<span>(delta )</span>) that breaks the symmetry within the <i>xy</i>-plane. We derive the exact thermal density matrix and analytically evaluate two measures of non-classicality: Local Quantum Uncertainty (LQU) and Trace Distance Discord (TDD). We complement this with an analysis of concurrence as a standard entanglement measure to provide a comprehensive comparative perspective. Our results show that the DM interaction significantly enhances and thermally stabilizes both LQU and TDD. In contrast, the asymmetric anisotropy <span>(delta )</span> plays a contrary role: it consistently suppresses these quantum correlations, a behavior not reported in previous generalized models. The KSEA interaction introduces a distinct effect that slows the thermal decay of TDD. We provide a spectral explanation for this behavior by examining the energy gap structure of the Hamiltonian. The results demonstrate how the competition between different types of spin–orbit couplings—antisymmetric DM, symmetric KSEA, and the new in-plane anisotropy <span>(delta )</span>—can be used to control the robustness of quantum correlations against temperature fluctuations. We also discuss how these coupling constants can be linked to experimentally accessible regimes in strained quantum dots or cold-atom lattices.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148751213","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Phase Transitions and Critical Behavior in the Two-Dimensional Weakly Diluted 4-State Potts Model 二维弱稀释四态波模型的相变和临界行为
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-10 DOI: 10.1007/s10948-026-07235-3
A. K. Murtazaev, A. B. Babaev, M. A. Babaev
{"title":"Phase Transitions and Critical Behavior in the Two-Dimensional Weakly Diluted 4-State Potts Model","authors":"A. K. Murtazaev,&nbsp;A. B. Babaev,&nbsp;M. A. Babaev","doi":"10.1007/s10948-026-07235-3","DOIUrl":"10.1007/s10948-026-07235-3","url":null,"abstract":"<div><p>Here, we introduce a high-precision Monte Carlo study examining the static critical behavior of the 4-state Potts model subjected to quenched disorder on a hexagonal lattice. The calculations are conducted for spin systems under periodic boundary conditions at spin concentrations of <i>p</i> = 1.0–0.80. Systems with linear sizes <i>L</i> in the range <i>L</i> = 21–180 are studied. The fourth-order Binder cumulant method is employed for determining the critical temperatures. The critical exponents <i>β</i>, <i>γ</i>, <i>α</i>, and <i>v</i>, describing magnetization, susceptibility, heat capacity, and correlation radius respectively, were determined using finite-size scaling theory for the dilution range <i>p</i> studied. Our findings affirm a second-order phase transition, exhibiting critical exponents consistent with the undiluted pure (<i>p</i> = 1.00) 2D 4-state Potts model’s universality class. For weak non-magnetic dilution (<i>p</i> = 0.90, 0.80), the addressed model exhibits a new set of critical exponents, defining a universality class different from the pure Potts model.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148751212","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Influence of Electric Field and Biaxial Strain on the Structural, Electronic, Magnetic, Phonon, and Optical Properties of Bulk and Monolayer VBi 电场和双轴应变对块体和单层VBi结构、电子、磁性、声子和光学性质的影响
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-08 DOI: 10.1007/s10948-026-07229-1
Muhammad Rashid Iqbal, Iqra Asif
{"title":"Influence of Electric Field and Biaxial Strain on the Structural, Electronic, Magnetic, Phonon, and Optical Properties of Bulk and Monolayer VBi","authors":"Muhammad Rashid Iqbal,&nbsp;Iqra Asif","doi":"10.1007/s10948-026-07229-1","DOIUrl":"10.1007/s10948-026-07229-1","url":null,"abstract":"<div><p>This study using the first-principles density functional theory (DFT) calculation within the CASTEP package, we systematically investigate the structural, electronic, magnetic and optical properties of bulk, monolayer VBi and effects of external electric field and the biaxial strain to the monolayer.The bulk phase crystallizes with a lattice constant of <span>(varvec{6.32})</span> <b><i>Å</i></b> and an indirect band gap of 0.65 eV (PBE-GGA) and 1.2 eV (HSE06), which is indicative of half-metallic behaviour.The band gap of GGA is 0.59 eV, and it is 0.98 eV for HSE06 in the spin-down channel, For the monolayer, the lattice constant is <span>(varvec{8.2})</span> <b><i>Å</i></b> and the total magnetic moment is <span>(varvec{2mu })</span> B, which is in accord with the Slater-Pauling rule (Zt = 8). The half-metallic character is maintained in the presence of biaxial strain (-6% to +6%) and perpendicular electric fields (up to ±0.8 V/nm), over a critical range of which a transition to semiconducting occurs. The optical dielectric function, refractive index and absorption coefficient are highly strain and field tunable. With its strong half-metallicity and external field tunability, our results suggest that monolayer VBi can be a good candidate for spintronics and optoelectronic applications.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148751315","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
First-Principles Investigation of the Electronic and Magnetic Properties of an Extended-Supercell Fe@Si-Doped SiC Nanotube 扩展型超级单体Fe@Si-Doped碳化硅纳米管的电子和磁性能第一性原理研究
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-06 DOI: 10.1007/s10948-026-07216-6
Sevda Rzayeva, Shovqiyya Amirova, Vafa Tarverdiyeva, Gulnara Guliyeva, Debarati Dey Roy, Maftun Aliyev
{"title":"First-Principles Investigation of the Electronic and Magnetic Properties of an Extended-Supercell Fe@Si-Doped SiC Nanotube","authors":"Sevda Rzayeva,&nbsp;Shovqiyya Amirova,&nbsp;Vafa Tarverdiyeva,&nbsp;Gulnara Guliyeva,&nbsp;Debarati Dey Roy,&nbsp;Maftun Aliyev","doi":"10.1007/s10948-026-07216-6","DOIUrl":"10.1007/s10948-026-07216-6","url":null,"abstract":"<div><p>The electronic and magnetic properties of an extended-supercell Fe@Si-doped SiC nanotube were investigated using spin-polarized density functional theory. First, the electronic structure of the pristine SiC nanotube was analyzed, revealing a direct band gap of approximately 1.67 eV, confirming its intrinsic semiconducting character with a non-magnetic ground state. Subsequently, the substitutional doping of Fe at the Si site was introduced to explore the modification of electronic and magnetic properties. The calculated band structure demonstrates that Fe incorporation significantly reduces the band gap to approximately 0.37 eV, indicating strong impurity-induced electronic states within the band gap region. The spin-polarized density of states reveals a pronounced asymmetry between spin-up and spin-down channels, confirming the emergence of magnetism in the doped nanotube. Orbital-projected density of states analysis indicates that the magnetic behavior mainly originates from the partially filled Fe-3d orbitals, which strongly hybridize with the p orbitals of neighboring Si and C atoms. Mulliken population analysis shows that the Fe dopant carries a dominant magnetic moment of 3.14 µ<sub>B</sub>, while smaller induced magnetic moments appear on surrounding atoms, leading to a total magnetic moment of 4.005 µ<sub>B</sub> for the supercell. Geometry optimization results confirm that the doped nanotube is structurally stable with small residual forces and negligible internal stress. The combined electronic and magnetic analyzes demonstrate that Fe substitution effectively tunes the electronic structure and induces stable spin polarization in SiC nanotubes, suggesting promising applications in spintronic and nanoelectronic devices.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148751117","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Topological Hall Behaviour Detected in Frustrated Shastry-Sutherland Magnet (text {HoB}_4) 受挫Shastry-Sutherland磁体的拓扑霍尔行为检测 (text {HoB}_4)
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-05 DOI: 10.1007/s10948-026-07227-3
Hongyu Xiao, Nan Zhou, Ming Cheng, Xiangyu Li, Yu Zhao, Yifan Deng, Ruihuan Lan, Wenhai Song, Xuan Luo, Yuping Sun
{"title":"Topological Hall Behaviour Detected in Frustrated Shastry-Sutherland Magnet (text {HoB}_4)","authors":"Hongyu Xiao,&nbsp;Nan Zhou,&nbsp;Ming Cheng,&nbsp;Xiangyu Li,&nbsp;Yu Zhao,&nbsp;Yifan Deng,&nbsp;Ruihuan Lan,&nbsp;Wenhai Song,&nbsp;Xuan Luo,&nbsp;Yuping Sun","doi":"10.1007/s10948-026-07227-3","DOIUrl":"10.1007/s10948-026-07227-3","url":null,"abstract":"<div><p>Geometrically frustrated systems exhibit intriguing physical phenomena under applied magnetic fields. The rare-earth tetraboride (<i>R</i>B<span>(_4)</span>, <i>R</i> is a magnetic rare-earth) family, a Shastry–Sutherland frustrated magnetic system, displays plateaus at fractional values of the saturation magnetization. Because of its metallic character, <span>(textit{R}text {B}_4)</span> could be an ideal platform for investigating the interplay between conduction electrons and fractional plateau phases. Here, we investigate the electrical transport of <span>(text {HoB}_4)</span>, which is a member of the <span>(textit{R}text {B}_4)</span> family that possesses fractional magnetization plateaus. We observe pronounced peak-like features and a violation of Kohler’s rule in the magnetoresistance associated with the complex magnetic phases. In addition, we identify a distinct hump-like anomaly in the Hall resistivity corresponding to the fractional plateau phases. We propose that the hump-like feature is most likely a manifestation of the topological Hall effect, arising from the real-space accumulation of Berry curvature due to non-coplanar spin textures. Our work provides new insights into the origin of the fractional magnetization plateaus in <span>(text {HoB}_4)</span> and serves as a useful reference for understanding frustrated magnetism in metallic systems.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148750809","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Low Temperature Complex Magnetic and Dielectric Studies on Al3+ substituted GaFeO3 Multiferroic Solid Solutions Al3+取代GaFeO3多铁质固溶体的低温复磁和介电研究
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-08-03 DOI: 10.1007/s10948-026-07228-2
Manjunatha T, Shidaling Matteppanavar, Sudhindra Rayaprol, Basavaraj Angadi
{"title":"Low Temperature Complex Magnetic and Dielectric Studies on Al3+ substituted GaFeO3 Multiferroic Solid Solutions","authors":"Manjunatha T,&nbsp;Shidaling Matteppanavar,&nbsp;Sudhindra Rayaprol,&nbsp;Basavaraj Angadi","doi":"10.1007/s10948-026-07228-2","DOIUrl":"10.1007/s10948-026-07228-2","url":null,"abstract":"<div><p>A series of Ga<sub>1-x</sub>Al<sub>x</sub>FeO<sub>3</sub> (x = 0, 0.2, 0.4 and 0.6) solid solutions were synthesized through the conventional solid-state reaction method to investigate the effect of Al<sup>3+</sup> substitution on their structural, microstructural, magnetic, and dielectric properties. Room temperature X-ray diffraction (XRD) and neutron diffraction (ND) analyses confirm the formation of the non-centrosymmetric <i>orthorhombic</i> structure across all compositions. Detailed Rietveld refinement of both XRD and ND patterns provided quantitative insights into lattice parameters, cation distribution, and structural distortions induced by Al<sup>3+</sup> substitution. Raman spectroscopy further corroborates the formation of the <i>orthorhombic</i> phase, revealing 15 Raman-active vibrational modes characteristic of GaFeO<sub>3</sub>. Scanning electron microscopy (SEM) micrographs exhibit well-defined grains and distinct grain boundaries, while progressive Al<sup>3+</sup> substitution results in systematic grain size reduction. Low-temperature (5–300 K) dc magnetization measurements, including zero-field-cooled (ZFC) and field-cooled (FC) protocols along with magnetic hysteresis (M-H) loops, reveal a clear paramagnetic-ferrimagnetic transition (<i>T</i><sub>N</sub>). Notably, <i>T</i><sub>N</sub> shifts toward higher temperatures with increasing Al<sup>3+</sup> concentration, approaching room temperature. The enhancement in magnetic transition temperature is attributed to structural distortion and modified Fe–O–Fe superexchange interactions induced by Al<sup>3+</sup> substitution. Temperature-dependent dielectric measurements exhibit anomalies near T<sub>N</sub>, indicating significant indirect magnetoelectric coupling in all solid solutions. Overall, Al<sup>3</sup>⁺ substitution in GaFeO<sub>3</sub> effectively modulates magnetic ordering and enhances magnetodielectric coupling, highlighting the potential of Ga<sub>1-x</sub>Al<sub>x</sub>FeO<sub>3</sub> solid solutions for multifunctional and spintronic device applications.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"39 4","pages":""},"PeriodicalIF":1.8,"publicationDate":"2026-08-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148750769","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Magnetic Properties Evaluation and Loss Simulation of FeNiMo/Ni₀.₆Zn₀.₄Fe₂O₄ Soft Magnetic Composites FeNiMo/Ni 0、₆Zn 0的磁性能评价及损耗模拟。₄Fe₂O₄软磁复合材料
IF 1.8 4区 物理与天体物理
Journal of Superconductivity and Novel Magnetism Pub Date : 2026-07-29 DOI: 10.1007/s10948-026-07225-5
Shen Wu, Jinliang Song, Xiaoran Sun, Haoyu Zhu, Jianglei Fan, Yaju Zhou
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