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Harnessing Fe(II)/α-ketoglutarate-dependent oxygenases for sustainable synthesis 利用铁(II)/α-酮戊二酸依赖的加氧酶进行可持续合成
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2026-04-01 Epub Date: 2026-02-13 DOI: 10.1016/j.cogsc.2026.101059
Huibin Wang , Takahiro Mori , Ikuro Abe
{"title":"Harnessing Fe(II)/α-ketoglutarate-dependent oxygenases for sustainable synthesis","authors":"Huibin Wang ,&nbsp;Takahiro Mori ,&nbsp;Ikuro Abe","doi":"10.1016/j.cogsc.2026.101059","DOIUrl":"10.1016/j.cogsc.2026.101059","url":null,"abstract":"<div><div>Fe(II)/α-ketoglutarate-dependent oxygenases (αKG OXs) have emerged as versatile biocatalysts for selective C–H functionalization, offering sustainable routes to complex molecules under mild conditions. Recent advances in data-driven enzyme discovery, machine learning (ML)-guided enzyme engineering, and computational design have significantly improved their substrate scope, stability, and scalability for pharmaceutical synthesis. Beyond native oxidative modifications, repurposed αKG OXs mediate new-to-nature transformations, including site-selective azidation, Mukaiyama hydration, Conia-ene cyclization, and photoenzymatic cross-coupling. Their integration into chemoenzymatic cascades has enabled concise and green syntheses of complex natural products and drug intermediates. This review highlights recent advances in studies that establish αKG OXs as key enzymes for sustainable biocatalytic synthesis.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"58 ","pages":"Article 101059"},"PeriodicalIF":9.4,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147388178","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Water-enabled organometallic and enzymatic catalysis: Sustainable technologies supporting API manufacturing 水催化有机金属和酶催化：支持原料药制造的可持续技术
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2026-02-01 Epub Date: 2026-01-07 DOI: 10.1016/j.cogsc.2025.101058
Alessandra Tolomelli, Tommaso Fantoni, Davide Carboni, Lucia Ferrazzano, Walter Cabri
{"title":"Water-enabled organometallic and enzymatic catalysis: Sustainable technologies supporting API manufacturing","authors":"Alessandra Tolomelli,&nbsp;Tommaso Fantoni,&nbsp;Davide Carboni,&nbsp;Lucia Ferrazzano,&nbsp;Walter Cabri","doi":"10.1016/j.cogsc.2025.101058","DOIUrl":"10.1016/j.cogsc.2025.101058","url":null,"abstract":"<div><div>Aqueous chemistry is a key platform for advancing sustainable organometallic and enzymatic catalytic technologies relevant to API manufacturing. Effective implementation requires minimizing process mass intensity (PMI), increasing reaction mass efficiency, ensuring final product quality, and managing the impact of water-waste contaminants. Recent advances in palladium cross-coupling show how water or aqueous cosolvents can deliver highly efficient transformations: micellar water/sodium dodecyl sulfate/cyclopentylmethyl ether systems with new monodentate basic phosphines enable 0.125–0.5 mol% Pd and PMIs near 20 on complex architecture, while bidentate nitrogen ligands in hydroxyethyl pyrrolidone/water achieve 0.1–0.005 mol% Pd, turnover numbers up to 17,800, and &gt;90% Pd recovery. Enzymatic innovations, including Merck’s free-enzyme cascade for islatravir and subtilisin-engineered peptide ligation for liraglutide, demonstrate how aqueous biocatalysis can provide selective, scalable, and greener API-relevant processes.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"57 ","pages":"Article 101058"},"PeriodicalIF":9.4,"publicationDate":"2026-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146070962","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Recycling and reuse of olefinic separators in lithium-ion batteries: A mini review 锂离子电池中烯烃分离器的回收和再利用：综述
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2025-12-01 Epub Date: 2025-10-25 DOI: 10.1016/j.cogsc.2025.101054
Himanshu Gupta, N. Raveendran Shiju
{"title":"Recycling and reuse of olefinic separators in lithium-ion batteries: A mini review","authors":"Himanshu Gupta,&nbsp;N. Raveendran Shiju","doi":"10.1016/j.cogsc.2025.101054","DOIUrl":"10.1016/j.cogsc.2025.101054","url":null,"abstract":"<div><div>The rapid expansion of lithium-ion battery (LIB) applications over the past decade—driven by the rise in portable electronics and electric vehicles—has led to a significant increase in battery waste. While the recovery of valuable metals such as lithium and cobalt from spent LIBs has received considerable attention, the recycling of separator materials remains largely neglected. These separators, typically made from polyethylene (PE) and polypropylene (PP), are critical to battery function yet are often discarded through landfilling, raising environmental concerns due to their non-biodegradable nature. This mini-review highlights the emerging need to address the end-of-life management of LIB separators, discusses recent advances in their reuse and recycling, and outlines potential pathways to incorporate these materials into circular economy models. Greater focus on separator recovery could enhance the overall sustainability and resource efficiency of LIB recycling processes.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"56 ","pages":"Article 101054"},"PeriodicalIF":9.4,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145571722","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Recent advancements in solid-state ammonia sorbents 固态氨吸附剂的最新进展
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2025-12-01 Epub Date: 2025-10-24 DOI: 10.1016/j.cogsc.2025.101050
Janna Attari , Valentina Mendoza Martinez , Farid Akhtar , Anastasiia Karabanova
{"title":"Recent advancements in solid-state ammonia sorbents","authors":"Janna Attari ,&nbsp;Valentina Mendoza Martinez ,&nbsp;Farid Akhtar ,&nbsp;Anastasiia Karabanova","doi":"10.1016/j.cogsc.2025.101050","DOIUrl":"10.1016/j.cogsc.2025.101050","url":null,"abstract":"<div><div>The growing ammonia demand and the need to mitigate its toxicity have raised interest in solid-state ammonia sorbents as a safe alternative to conventional storage systems. This review paper focuses on the development of ammonia storage and thermochemical energy storage, based on research published from 2022 to 2024. Results demonstrate that the two applications have reached different technologies’ maturity. For ammonia storage, the aim was to enhance the sorbent’s performance by novel synthesis routes, whereas a recent shift toward the optimization of systems has been observed for energy storage applications. In our opinion, one should aim for a simplification of the sorbent synthesis route while keeping a look at novel developments to combine the enhancement of both efficiency and stability.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"56 ","pages":"Article 101050"},"PeriodicalIF":9.4,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145571721","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Regeneration and sustainable chemistry: Current dynamics, interconnections, and perspectives 再生和可持续化学：当前动态，相互联系和观点
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2025-12-01 Epub Date: 2025-11-04 DOI: 10.1016/j.cogsc.2025.101055
Vânia G. Zuin Zeidler , Caroindes J. Corrêa Gomes
{"title":"Regeneration and sustainable chemistry: Current dynamics, interconnections, and perspectives","authors":"Vânia G. Zuin Zeidler ,&nbsp;Caroindes J. Corrêa Gomes","doi":"10.1016/j.cogsc.2025.101055","DOIUrl":"10.1016/j.cogsc.2025.101055","url":null,"abstract":"<div><div>This paper aims at exploring the role of sustainable chemistry to address regenerative practices, dynamics, and systems as the ones related to agriculture, food production, and processing, including topics such as valorization of agro-industrial waste, biorefinery, biomass, bio-based materials and related flows or processes, renewable resources and energy, considering the links to the United Nations Sustainable Development Goals.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"56 ","pages":"Article 101055"},"PeriodicalIF":9.4,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145618198","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
CO2 mitigation via seaweed and microalgae farming for sustainable biofuel production in the blue bioeconomy 通过海藻和微藻养殖，在蓝色生物经济中实现可持续生物燃料生产，减少二氧化碳排放
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2025-12-01 Epub Date: 2025-10-23 DOI: 10.1016/j.cogsc.2025.101053
Yaleeni Kanna Dasan , Uganeeswary Suparmaniam , Man Kee Lam , Inn Shi Tan , Sie Yon Lau , Fui Chin Bridgid Lai
{"title":"CO2 mitigation via seaweed and microalgae farming for sustainable biofuel production in the blue bioeconomy","authors":"Yaleeni Kanna Dasan ,&nbsp;Uganeeswary Suparmaniam ,&nbsp;Man Kee Lam ,&nbsp;Inn Shi Tan ,&nbsp;Sie Yon Lau ,&nbsp;Fui Chin Bridgid Lai","doi":"10.1016/j.cogsc.2025.101053","DOIUrl":"10.1016/j.cogsc.2025.101053","url":null,"abstract":"<div><div>Rising carbon dioxide (CO<sub>2</sub>) levels demand urgent, scalable solutions that decarbonize the energy sector without compromising sustainability. Algae-based carbon capture stands at the frontier of innovation, offering rapid CO<sub>2</sub> fixation, low resource input, and versatile biofuel applications. This short review explores recent advances in seaweed and microalgae cultivation for CO<sub>2</sub> mitigation, emphasizing their role in the emerging blue bioeconomy. Evaluation of energy use, greenhouse gas emissions, and cost trade-offs from both life cycle and techno-economic perspectives demonstrate the potential of algae as a viable climate solution and a sustainable renewable resource. A harmonized life cycle assessment framework is proposed to guide commercialization of marine biomass for biofuel and successful integration into coastal carbon strategies. The review concludes by identifying key challenges and future directions to scale algae technologies as nature-based carbon sinks for a net-zero future.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"56 ","pages":"Article 101053"},"PeriodicalIF":9.4,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145520869","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Recycling-privileged plastic polymers 具有回收优势的塑料聚合物
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2025-12-01 Epub Date: 2025-10-21 DOI: 10.1016/j.cogsc.2025.101049
Jules Armand Wilhelmina Harings , Hendrik Ballerstedt , Lars Mathias Blank
{"title":"Recycling-privileged plastic polymers","authors":"Jules Armand Wilhelmina Harings ,&nbsp;Hendrik Ballerstedt ,&nbsp;Lars Mathias Blank","doi":"10.1016/j.cogsc.2025.101049","DOIUrl":"10.1016/j.cogsc.2025.101049","url":null,"abstract":"<div><div>The plastic crisis is in full swing, requiring our collective attention to limit its adverse impact on the environment and human health. Here in, we argue that the high recycling quota required can be more easily achieved when using recycling-privileged plastics, for examplem i.e., plastics that, at the end of their life, are in a technological environment readily depolymerized into their monomers or building blocks of higher, but controlled order (chemistry). Incidentally, recycling rates or recycling quotas are mandated targets, expressed as a percentage, for the amount of waste that must be collected and recycled, often by governments and regulatory bodies. These quotas, such as the EU's overall 65% packaging recycling goal by 2025, aim to promote a circular economy, reduce landfill waste, conserve resources, and decrease pollution. They are calculated as an output-oriented rate, meaning only waste that is successfully reused is counted towards the target. Once degradation pathways are understood, this can be achieved by crossing multiple length scales down to the molecular level to intercept them on time. These recycling-privileged plastics typically contain heteroatomic bonds and are classified as polycondensates, such as polyesters or polyamides. These plastics can consist of novel monomers and/or of modified material, tailored not only for the application but also for recycling. It goes without saying that any future plastic economy relies on alternative carbon sources (biomass, CO<sub>2</sub>, plastic waste). We state the challenges, present the state-of-the-art of recycling-privileged polymers, and discuss the many possibilities at the end-of-life when polymer physics is used to tailor material properties during and after the utilization phase.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"56 ","pages":"Article 101049"},"PeriodicalIF":9.4,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145335168","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Special issue on green sorbent materials 绿色吸附材料特刊
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2025-10-01 Epub Date: 2025-07-18 DOI: 10.1016/j.cogsc.2025.101042
Mohamed Chaker Necibi, Borhane Mahjoub
{"title":"Special issue on green sorbent materials","authors":"Mohamed Chaker Necibi,&nbsp;Borhane Mahjoub","doi":"10.1016/j.cogsc.2025.101042","DOIUrl":"10.1016/j.cogsc.2025.101042","url":null,"abstract":"","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"55 ","pages":"Article 101042"},"PeriodicalIF":9.4,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144860802","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Comment to ‘Plasma catalysis for gas conversion—Impact of catalyst on the plasma behavior’ 评《气体转化的等离子体催化——催化剂对等离子体行为的影响》
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2025-10-01 Epub Date: 2025-08-11 DOI: 10.1016/j.cogsc.2025.101043
G. Akay , A.R. González-Elipe , A. Gómez-Ramírez
{"title":"Comment to ‘Plasma catalysis for gas conversion—Impact of catalyst on the plasma behavior’","authors":"G. Akay ,&nbsp;A.R. González-Elipe ,&nbsp;A. Gómez-Ramírez","doi":"10.1016/j.cogsc.2025.101043","DOIUrl":"10.1016/j.cogsc.2025.101043","url":null,"abstract":"","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"55 ","pages":"Article 101043"},"PeriodicalIF":9.4,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145049268","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Integrating sustainability in atmospheric chemistry analysis 将可持续性纳入大气化学分析
IF 9.4 2区 化学
Current Opinion in Green and Sustainable Chemistry Pub Date : 2025-10-01 Epub Date: 2025-09-04 DOI: 10.1016/j.cogsc.2025.101048
Regina M.B.O. Duarte, Armando C. Duarte
{"title":"Integrating sustainability in atmospheric chemistry analysis","authors":"Regina M.B.O. Duarte,&nbsp;Armando C. Duarte","doi":"10.1016/j.cogsc.2025.101048","DOIUrl":"10.1016/j.cogsc.2025.101048","url":null,"abstract":"<div><div>The concepts that help us to better understand the atmospheric chemistry, including the composition and dynamics of air particles and gaseous species, and their impact on climate and human health, rely on the development of sensitive and selective analytical methods that allow one to measure an ever-increasing range of analytes, whose physicochemical features vary both in time and space. Motivated by the ongoing awareness of the need to adopt eco-friendly practices, this perspective highlights analytical practices with the potential to meet green and sustainable requirements and that have offered an almost unexplored playground for deciphering and mapping the intricacies of atmospheric chemistry. The most promising green metrics currently available to estimate the environmental impact and efficiency of analytical methods are also highlighted. Rather than presenting new quantitative data, this perspective offers a critical and conceptual discussion aimed at advancing the adoption of sustainable analytical solutions in the highly challenging field of atmospheric chemistry analysis.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"55 ","pages":"Article 101048"},"PeriodicalIF":9.4,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145121198","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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