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Leveraging MXenes for wearable bioelectronics 利用MXenes用于可穿戴生物电子产品
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-05-12 DOI: 10.1016/j.mattod.2025.04.017
Yu Song , Jing Xu , Xiao Xiao , Farid Manshaii , Yanxin Wang , Jianguo Tang , Linjun Huang , Jun Chen
{"title":"Leveraging MXenes for wearable bioelectronics","authors":"Yu Song ,&nbsp;Jing Xu ,&nbsp;Xiao Xiao ,&nbsp;Farid Manshaii ,&nbsp;Yanxin Wang ,&nbsp;Jianguo Tang ,&nbsp;Linjun Huang ,&nbsp;Jun Chen","doi":"10.1016/j.mattod.2025.04.017","DOIUrl":"10.1016/j.mattod.2025.04.017","url":null,"abstract":"<div><div>In light of the growing challenges in public health, exacerbated by global pandemics and the increasing demands of an aging population, intelligent wearables utilizing advanced materials such as MXenes are emerging as crucial solutions to providing fresh insights into the real-time health monitoring and responsiveness. This review examines the synthesis, properties, and varied applications of MXene-based intelligent materials, underscoring their essential contribution to the advancement of wearable bioelectronics. It discusses a range of synthesis techniques, such as etching methods, with a specific emphasis on the benefits and drawbacks of different processing techniques, including electrospinning, wet spinning, and coating. MXene-based functional materials exhibit exceptional efficiency in sensing applications, including pressure, temperature, and humidity detection. They are also crucial for electromagnetic shielding and facilitating human-computer interactions. MXenes' versatility has led to their widespread adoption in the development of diverse wearable bioelectronics. Furthermore, the review addresses environmental and stability challenges associated with MXene synthesis, while emphasizing the potential of novel synthesis methods, the development of hybrid structures, and the expansion of application areas. In conclusion, it underscores the promising future of MXene-based wearables in modern technologies. Overcoming current challenges will unlock their transformative potential in the wearable technology sector, ushering in a new era of healthcare monitoring and interactive solutions.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 304-328"},"PeriodicalIF":21.1,"publicationDate":"2025-05-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254254","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Electrocatalytic materials engineering: Towards the renaissance of electrochemical organic synthesis 电催化材料工程:走向电化学有机合成的复兴
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-05-12 DOI: 10.1016/j.mattod.2025.05.012
Gui Liu, Hongjie Zhang, Jianxin Kang, Lin Guo
{"title":"Electrocatalytic materials engineering: Towards the renaissance of electrochemical organic synthesis","authors":"Gui Liu,&nbsp;Hongjie Zhang,&nbsp;Jianxin Kang,&nbsp;Lin Guo","doi":"10.1016/j.mattod.2025.05.012","DOIUrl":"10.1016/j.mattod.2025.05.012","url":null,"abstract":"<div><div>The rapid evolution of electrochemical technology has propelled electrocatalytic organic synthesis (EOS) into the spotlight as a sustainable and selective alternative to classical organic synthesis. However, the ongoing development of EOS has been hindered by the limitations of electrode materials engineering. Therefore, there is an urgent need to comprehensively present the latest advancements in EOS and elucidate the pivotal role of electrocatalytic material engineering. In this review, we first picture the recent progress of commonly functional-group transformations in EOS, followed by a brief introduction to fundamental electrochemical setup and essential, laying the groundwork for understanding the key factors influencing EOS. This not only showcases the potential of EOS in diverse chemical transformations but also emphasizes the strong demand for improved electrocatalytic material. Most importantly, we propose a framework that deeply integrates electrocatalytic material engineering, with a particular focus on amorphization strategies, into EOS, for its broader applications. Benefiting from the efficiently tunable structure–activity relationship, electrocatalytic material engineering contributes EOS to widespread prosperity, in which the atomic economy, activity, and stability of the catalytic materials can be significantly improved, thereby promoting the cost-efficient large-scale industrialization of future electrocatalytic organic synthesis, and contributing to a more sustainable future energy and chemical industry.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 422-441"},"PeriodicalIF":21.1,"publicationDate":"2025-05-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254371","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
MXene quantum dots enable self-repairing and anti-corrosive interphase for high-performance zinc anode MXene量子点实现了高性能锌阳极的自修复和抗腐蚀界面
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-05-11 DOI: 10.1016/j.mattod.2025.05.015
Xinlong Liu, King Yan Chung, Qingjun Yang, Cuiqin Fang, Shenzhen Deng, Jing Han, Jian Lu, Bingang Xu
{"title":"MXene quantum dots enable self-repairing and anti-corrosive interphase for high-performance zinc anode","authors":"Xinlong Liu,&nbsp;King Yan Chung,&nbsp;Qingjun Yang,&nbsp;Cuiqin Fang,&nbsp;Shenzhen Deng,&nbsp;Jing Han,&nbsp;Jian Lu,&nbsp;Bingang Xu","doi":"10.1016/j.mattod.2025.05.015","DOIUrl":"10.1016/j.mattod.2025.05.015","url":null,"abstract":"<div><div>Zinc-ion batteries (ZIBs) hold great promise owing to their inherent safety and high energy density, yet their practical application is challenged by low Coulombic efficiency (CE), parasitic reactions, and dendrite growth of zinc anode. Herein, we introduce MXene quantum dots (MQDs) as a multifunctional colloid additive to construct a robust solid electrolyte interphase (SEI) and with dynamic self-repairing function. Particularly, MQDs can effectively modify the H-bond environment, provide anti-corrosion benefits, and eliminate dendrites. The strong bonding of MQDs with free water molecules and metallic Zn enhances interfacial stability via modifying localized H-bond network. Depth profile analysis shows that Zn<sup>2+</sup> plating coincides with SEI layer formation (ZHS/TiCO), resulting in uniform and dense deposition with mixed crystalline phases. Consequently, this additive strategy achieves dendrite-free deposition with a high Coulombic efficiency of 99.2 %, a reversible lifetime of 3,700 h in symmetric cells, anti-corrosion performance exceeding 4,000 h, along with 3,900 h of self-repairing cycling. Additionally, impressive full-cell cycling retention is further demonstrated with MnO<sub>2</sub>, I<sub>2</sub>, and PANI cathodes. This work paves a new way for more efficient metallic anode in aqueous rechargeable batteries.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 103-113"},"PeriodicalIF":21.1,"publicationDate":"2025-05-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254435","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Sequential hardening mechanisms in additive-manufactured NiTi shape memory alloys that can significantly delay compressive failure 增材制造的NiTi形状记忆合金的顺序硬化机制可以显著延缓压缩失效
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-05-07 DOI: 10.1016/j.mattod.2025.04.014
Huwen Ma , Yanchun Zhao , Junhui Luo , Yu Su , Tengfei Zheng , Zhiqi Yu , Yuan Wu , Yanfei Gao
{"title":"Sequential hardening mechanisms in additive-manufactured NiTi shape memory alloys that can significantly delay compressive failure","authors":"Huwen Ma ,&nbsp;Yanchun Zhao ,&nbsp;Junhui Luo ,&nbsp;Yu Su ,&nbsp;Tengfei Zheng ,&nbsp;Zhiqi Yu ,&nbsp;Yuan Wu ,&nbsp;Yanfei Gao","doi":"10.1016/j.mattod.2025.04.014","DOIUrl":"10.1016/j.mattod.2025.04.014","url":null,"abstract":"<div><div>Most material design strategies devoted to the strength-ductility synergy in tension are based on the delay of the necking instability. However, the counterpart investigations under compression remain elusive. Recent developments in simulating the failure process reveal that microscopic voids or cavities under compression/shear-dominated loadings will evolve sequentially as flattened to a micro-crack, rotating and elongating into kinks, and then interacting and coalescing with neighboring micro-cracks. This entire process can be significantly slowed down if the matrix material sustains a high work hardening exponent. Motivated by this novel micromechanical understanding, this work successfully realized hierarchically heterostructured microstructures in NiTi shape memory alloys (SMA) by using the selective laser melting (SLM) additive manufacturing technique. It is the sequential or progressive transition from the martensitic phase transformation, to heterogeneous deformation induced hardening, and then to amorphous lamellae hardening at later stage that sustains a high work hardening rate which results into an exceptionally high failure strain of the as-fabricated (without post-treatment) SMA under compression. The occurrence of amorphization at high strains is attributed to the high dislocation density and to the oxygen-assisted energy barrier reduction. This work thus offers an unprecedent design approach for the development of high performance SMAs.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 36-48"},"PeriodicalIF":21.1,"publicationDate":"2025-05-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254258","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Structure modifications of wood-based materials for water treatment applications: A review 木基水处理材料结构改性研究进展
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-05-07 DOI: 10.1016/j.mattod.2025.04.012
Yaqin Zhu , Shiyuan Wang , Yanbo Liu , Jingquan Han , Gaigai Duan , Qiliang Fu , Xiaoshuai Han , Chunmei Zhang , Shuijian He , Shaohua Jiang
{"title":"Structure modifications of wood-based materials for water treatment applications: A review","authors":"Yaqin Zhu ,&nbsp;Shiyuan Wang ,&nbsp;Yanbo Liu ,&nbsp;Jingquan Han ,&nbsp;Gaigai Duan ,&nbsp;Qiliang Fu ,&nbsp;Xiaoshuai Han ,&nbsp;Chunmei Zhang ,&nbsp;Shuijian He ,&nbsp;Shaohua Jiang","doi":"10.1016/j.mattod.2025.04.012","DOIUrl":"10.1016/j.mattod.2025.04.012","url":null,"abstract":"<div><div>With global freshwater scarcity and increasing water pollution due to industrial and agricultural activities, there is an urgent need for sustainable, high-performance water treatment materials. Conventional filtration and adsorption materials, such as polymer membranes and activated carbon, often suffer from high energy consumption, secondary pollution, and high production costs. In contrast, wood-based materials offer hierarchical porosity, natural adsorption sites, and tunable surface chemistry, making them a promising candidate for low-cost and environmentally friendly water treatment applications. In this review, we introduced the structure and properties of wood and described how these affect the preparation and water treatment properties of wood-based materials. We also summarized the structure design strategies for wood-based materials, mainly including delignification treatment, nanomaterials modification, functional group modification, and carbonation modification. In addition, we presented a comprehensive investigation of advances in the application of wood-based materials in water treatment with the aim of comparing, analyzing, and evaluating the practical functionality in sterilization, heavy metal ion removal, organic pollutants removal, oil/water separation, and desalination. Finally, we presented the serious challenges and new perspectives for wood-based materials in water treatment.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 252-286"},"PeriodicalIF":21.1,"publicationDate":"2025-05-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254442","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
In-situ traced intermediate dynamics and reaction mechanisms in heterogenous CO2 photoreduction systems 非均相CO2光还原体系的原位追踪中间动力学和反应机理
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-05-03 DOI: 10.1016/j.mattod.2025.04.011
Malik Zeeshan Shahid , Minghua Xu , Xiaowen Ruan , Lei Zhang , Xiaoqiang Cui
{"title":"In-situ traced intermediate dynamics and reaction mechanisms in heterogenous CO2 photoreduction systems","authors":"Malik Zeeshan Shahid ,&nbsp;Minghua Xu ,&nbsp;Xiaowen Ruan ,&nbsp;Lei Zhang ,&nbsp;Xiaoqiang Cui","doi":"10.1016/j.mattod.2025.04.011","DOIUrl":"10.1016/j.mattod.2025.04.011","url":null,"abstract":"<div><div>The in-situ tracking of redox intermediates during the photocatalytic CO<sub>2</sub> reduction process (PCRP) is pivotal in producing valued chemical energy. However, the co-existence and uncontrollability of these intermediates make elucidating the PCRP reaction mechanism extremely challenging. This review assesses the interplay between PCRP-derived intermediates and targeted active sites to achieve desired products via discrete reaction routes involving sequential proton-coupled electron transfers. More specifically, intermediates dynamics including adsorption, transition, stabilization, C<img>C coupling, and desorption are analyzed and thus clarified for producing CO, CH<sub>4</sub>, HCOOH, HCHO, CH<sub>3</sub>OH, CH<sub>3</sub>COOH, CH<sub>3</sub>CHO, CH<sub>3</sub>CH<sub>2</sub>OH, C<sub>2</sub>H<sub>4</sub>, C<sub>2</sub>H<sub>6</sub>, and C<sub>3</sub>H<sub>8</sub>, thereby offering a unique aspect for optimizing PCRP. Our review begins by highlighting the PCRP phenomenon, heterogeneous reactor setup, PCRP-derived products, and their reaction routes. Furthermore, it showcases in-situ challenges, proposes feasible solutions, furnishes notable considerations for upgrading PCRP to the industrial level and provides an outlook for robust PCRP. This work may offer directions for realizing sustainable energy and the environment through an in-depth understanding of PCRP intermediate dynamics and reaction mechanisms.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 231-251"},"PeriodicalIF":21.1,"publicationDate":"2025-05-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254440","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A transparent crystal with giant birefringence arising from π-electron anisotropy 由π电子各向异性引起的具有巨大双折射的透明晶体
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-04-29 DOI: 10.1016/j.mattod.2025.04.008
Yanqiang Li , Xianyu Song , Bin Chen , Yipeng Song , Weiqi Huang , Junhua Luo , Sangen Zhao
{"title":"A transparent crystal with giant birefringence arising from π-electron anisotropy","authors":"Yanqiang Li ,&nbsp;Xianyu Song ,&nbsp;Bin Chen ,&nbsp;Yipeng Song ,&nbsp;Weiqi Huang ,&nbsp;Junhua Luo ,&nbsp;Sangen Zhao","doi":"10.1016/j.mattod.2025.04.008","DOIUrl":"10.1016/j.mattod.2025.04.008","url":null,"abstract":"<div><div>Since researchers first observed the optical anisotropy phenomenon, i.e., birefringence, in a natural crystal, more than three centuries have passed. Known crystals either exhibit relatively small birefringence (e.g., commercial crystals with birefringence &lt;0.3) or do not allow for transmittance of visible light, which limits their significant applications in diverse photonics fields. Herein, by the solution method, we obtained a new crystal K<sub>2</sub>HC<sub>9</sub>N<sub>13</sub>·3H<sub>2</sub>O, which is not only transparent in the whole visible spectral region because of its wide bandgap of 3.52 eV, but also exhibits giant birefringence as large as 0.87. To the best of our knowledge, this birefringence is the largest among transparent crystals. First-principles calculations reveal that this giant birefringence mainly arises from the anisotropy of <em>π</em>-electron clouds in (H<sub>2</sub>C<sub>9</sub>N<sub>13</sub>)<sup>−</sup> with parallel spacing arrangement. We believe that this work would be insightful for the design and synthesis of birefringent crystals for transparent compact polarized optics.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 29-35"},"PeriodicalIF":21.1,"publicationDate":"2025-04-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254257","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
From Fundamentals to Mechanisms: Peroxyacetic acid catalysts in emerging pollutant degradation 从基本原理到机理:过氧乙酸催化剂在新兴污染物降解中的应用
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-04-28 DOI: 10.1016/j.mattod.2025.04.010
Qingtong Yuan , Linfeng Xiao , Sanshuang Gao , Abdukader Abdukayum , Qingquan Kong , Guangzhi Hu , Deepak Dubal , Yingtang Zhou
{"title":"From Fundamentals to Mechanisms: Peroxyacetic acid catalysts in emerging pollutant degradation","authors":"Qingtong Yuan ,&nbsp;Linfeng Xiao ,&nbsp;Sanshuang Gao ,&nbsp;Abdukader Abdukayum ,&nbsp;Qingquan Kong ,&nbsp;Guangzhi Hu ,&nbsp;Deepak Dubal ,&nbsp;Yingtang Zhou","doi":"10.1016/j.mattod.2025.04.010","DOIUrl":"10.1016/j.mattod.2025.04.010","url":null,"abstract":"<div><div>The growing research interest in advanced oxidation technologies has led to a focus on using reactive peroxyacetic acid (PAA), a strong oxidising agent capable of degrading emerging contaminants through both radical (e.g., hydroxyl, organic radicals) and non-radical (e.g., singlet oxygen, high-valent metal oxides) pathways, offering high resistance to environmental disturbances. Current PAA research faces significant challenges, particularly in unravelling complex degradation mechanisms to optimise catalytic efficiency and minimise environmental impacts. Previous reviews lack a focused exploration of specific oxidisers like PAA and provide less detailed mechanistic insights, practical application strategies, and environmental considerations compared to a more targeted, in-depth analysis. This study systematically investigates the role of catalyst-assisted activation of PAA in the degradation of emerging pollutants within advanced oxidation processes (AOPs). We focus on analysing the physicochemical properties of PAA and its activation mechanisms, with particular emphasis on the effects of different catalysts on the reactivity of PAA and the degradation mechanisms. Furthermore, we summarise the key factors influencing the degradation efficiency of pollutants, assess the applicability of the PAA system in environmental remediation, and explore the application of density functional theory (DFT) calculations in revealing interactions between catalysts and PAA, as well as in elucidating catalytic mechanisms. Finally, we discuss challenges and future directions for PAA in pollutant management, aiming to establish a theoretical foundation and support the development of environmentally friendly materials for pollution remediation.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 197-230"},"PeriodicalIF":21.1,"publicationDate":"2025-04-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254441","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The Resurrection of Fe in layered cathode materials for sodium-ion batteries 钠离子电池层状正极材料中铁的复活
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-04-27 DOI: 10.1016/j.mattod.2025.04.009
Zongyu Guan , Guoyao Pang , Meng Li , Haoxiang Zhuo , Kuan Wang , Jiangtao Hu , Biwei Xiao , Weidong Zhuang
{"title":"The Resurrection of Fe in layered cathode materials for sodium-ion batteries","authors":"Zongyu Guan ,&nbsp;Guoyao Pang ,&nbsp;Meng Li ,&nbsp;Haoxiang Zhuo ,&nbsp;Kuan Wang ,&nbsp;Jiangtao Hu ,&nbsp;Biwei Xiao ,&nbsp;Weidong Zhuang","doi":"10.1016/j.mattod.2025.04.009","DOIUrl":"10.1016/j.mattod.2025.04.009","url":null,"abstract":"<div><div>Sodium-ion batteries (SIBs) have attracted renewed attention due to their cost-effectiveness and dynamic capabilities. Layered cathodes in SIBs are regarded as having the most potential for practical applications, attributed to their high energy density and straightforward synthesis methods. However, akin to lithium-ion batteries (LIBs), the utilization of Ni and Co for capacity enhancement significantly undermines the resource and cost advantages inherent in SIBs. It is noteworthy that the Fe<sup>3+</sup>/Fe<sup>4+</sup> redox couple cannot be realized in layered lithium oxide cathodes, yet it can provide high voltage and capacity in layered sodium oxide cathodes. Nevertheless, the incorporation of Fe into layered sodium oxide cathodes presents several challenges, including material preparation issue, Fe migration, Fe dissolution, and the instability of Fe<sup>4+</sup>. In this review, the reasons why Fe<sup>3+</sup>/Fe<sup>4+</sup> redox couple is unsuitable for LIBs applications yet viable for SIBs is thoroughly examined. Furthermore, we delve into the benefits associated with employing Fe in layered sodium oxide cathodes along with current research efforts aimed at overcoming challenges linked to its application. We hope that this review can inspire future designs and developments of high-performance and low-cost iron-based layered oxide cathode materials for SIBs.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 176-196"},"PeriodicalIF":21.1,"publicationDate":"2025-04-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254439","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Additive manufacturing of immiscible/incompatible systems 不混相/不相容系统的增材制造
IF 21.1 1区 材料科学
Materials Today Pub Date : 2025-04-24 DOI: 10.1016/j.mattod.2025.04.003
Rakesh Das , Sameehan S. Joshi , Peter Samora Owuor , Abdullah Khan , Sandra Ike , Pankaj Kumar , Narendra B. Dahotre , Chandra Sekhar Tiwary
{"title":"Additive manufacturing of immiscible/incompatible systems","authors":"Rakesh Das ,&nbsp;Sameehan S. Joshi ,&nbsp;Peter Samora Owuor ,&nbsp;Abdullah Khan ,&nbsp;Sandra Ike ,&nbsp;Pankaj Kumar ,&nbsp;Narendra B. Dahotre ,&nbsp;Chandra Sekhar Tiwary","doi":"10.1016/j.mattod.2025.04.003","DOIUrl":"10.1016/j.mattod.2025.04.003","url":null,"abstract":"<div><div>The advent of additive manufacturing (AM) has propelled significant innovation in industries due to its capacity for technological advancement as a sustainable, adaptable, and personalized manufacturing method. Exploring the (AM) of immiscible systems is a critical area that requires exploration to achieve both multifunctionalities of different elements or phases and stability during the service period. The review commences with an overview of the fundamental AM processes followed by an in-depth case study of the innovation in this immiscible alloy and composite development. We have also systematically illustrated AM of immiscible systems and development in design and material innovations. A framework is provided to computationally model various AM processes tailored for immiscible/incompatible systems. In the end, the current obstacles with limitations of AM techniques in manufacturing immiscible systems are highlighted, followed by their prospects for possible future innovations. AM can precisely control the microstructure of immiscible systems through tailored processing parameters and has the ability to create functionally graded materials where immiscible phases serve specific roles.</div></div>","PeriodicalId":387,"journal":{"name":"Materials Today","volume":"87 ","pages":"Pages 125-150"},"PeriodicalIF":21.1,"publicationDate":"2025-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144254437","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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