Environmental Pollution最新文献

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Physiological and behavioural responses of aquatic organisms to microplastics and experimental warming
IF 8.9 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-04 DOI: 10.1016/j.envpol.2025.126182
Danielle J. Marchant, Daniel M. Perkins, J. Iwan Jones, Pavel Kratina
{"title":"Physiological and behavioural responses of aquatic organisms to microplastics and experimental warming","authors":"Danielle J. Marchant, Daniel M. Perkins, J. Iwan Jones, Pavel Kratina","doi":"10.1016/j.envpol.2025.126182","DOIUrl":"https://doi.org/10.1016/j.envpol.2025.126182","url":null,"abstract":"Microplastics are an emerging contaminant of concern because of their potential to cause harm to aquatic biota, such as reproduction, growth, and survival, and there is a lack of knowledge about how microplastics can affect other sub-lethal responses, such as movement behaviour and respiration rates, which may have consequences for species interactions. Additionally, there is little evidence for the effects of microplastics under different climate warming scenarios. To address this knowledge gap, the effects of high-density polyethylene (HDPE) microplastics, in combination with different constant temperature regimes (10°C, 15°C, and 20°C) and a fluctuating regime (10 - 20°C over a 24h diel cycle) on the respiration rates, feeding rates, and movement speeds of <em>Gammarus pulex</em> and <em>Asellus aquaticus</em> were assessed. Respiration rates of <em>G. pulex</em> increased with temperature according to metabolic theory, but there was no evidence for increased respiration rates of <em>A. aquaticus</em> at higher temperatures. Overall, the respiration rates and movement speeds of <em>G. pulex</em> were higher than <em>A. aquaticus</em> but there was no evidence that microplastics independently, or in combination with experimental warming, influenced any of the responses tested. There is increasing evidence that some microplastic particles may not be harmful to aquatic biota, and the findings presented in this study indicated that further evidence about the effects of different microplastic types, in combination with other human-induced pressures, is required to better understand the hazards and risks associated with microplastic particles in the environment.","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"29 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2025-04-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143776081","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The role of atmospheric volatile organic compounds (VOCs) in ozone formation around China's largest plywood manufacturer
IF 7.6 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-04 DOI: 10.1016/j.envpol.2025.126197
Ningjie Li , Ting Sun , Stephen Mudge , Yuanxun Zhang , Zhenhui Gao , Lihui Huang , Jianing Lin
{"title":"The role of atmospheric volatile organic compounds (VOCs) in ozone formation around China's largest plywood manufacturer","authors":"Ningjie Li ,&nbsp;Ting Sun ,&nbsp;Stephen Mudge ,&nbsp;Yuanxun Zhang ,&nbsp;Zhenhui Gao ,&nbsp;Lihui Huang ,&nbsp;Jianing Lin","doi":"10.1016/j.envpol.2025.126197","DOIUrl":"10.1016/j.envpol.2025.126197","url":null,"abstract":"<div><div>The volatile organic compounds (VOCs) are a dominant contributor to the formation of ozone (O<sub>3</sub>) in Linyi, the plywood capital of China. However, the temporal variations and source origins of VOCs in Linyi remain unclear. This study gathered ambient air samples (n = 214) from the urban center of Linyi during the period April to October of 2021–2023. The total volatile organic compounds (TVOCs) concentrations ranged from 28 ppbv to 32 ppbv with oxygenated volatile organic compounds (OVOCs) taking the large portion (50.76 %) of TVOCs, followed by alkanes (28.11 %), aromatics (13.71 %), alkenes (6.66 %), and alkynes (0.76 %). The OVOCs (44.10 %) were the dominant contributors to ozone formation potential (OFP). Formaldehyde, an OVOC and particular pollutant from plywood industries contributed the most to OFP (∼21.60 %). The average concentration of TVOCs in 2022 was the lowest (28.61 ± 10.76 ppbv), with VOCs species, such as isobutane and propane having the lowest concentrations in 2022 (p &lt; 0.05), reflecting a decrease in transportation activity due to the impacts of pandemic lockdowns. Concentrations of OVOCs were annually increasing because of the annual growth of plywood yield. The TVOCs and OVOCs levels were significantly correlated to O<sub>3</sub> levels (p &lt; 0.01). The concentrations of TVOCs and OVOCs as well as O<sub>3</sub> were highest in June and September (p &lt; 0.05), when the temperature and the degree of photochemical reactions were high. The source apportionment analysis found that plywood industries were the main source (32.90 %) of TVOCs, followed by liquefied petroleum gas (LPG, 21.32 %). Trajectory statistical models (TSM) analysis suggested that Linyi is greatly affected by regional transport from the southwest (31.63 %). This study provides new insights into the mitigation and management of VOCs and O<sub>3</sub> pollution in plywood industry cities.</div></div>","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"373 ","pages":"Article 126197"},"PeriodicalIF":7.6,"publicationDate":"2025-04-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143776083","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Modelling Escherichia coli concentrations: 45.6% to 78.1% of China’s rivers show poor microbial water quality
IF 8.9 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-03 DOI: 10.1016/j.envpol.2025.126184
Songtao Mei, Kai Wang, Heike Schmitt, Nynke Hofstra
{"title":"Modelling Escherichia coli concentrations: 45.6% to 78.1% of China’s rivers show poor microbial water quality","authors":"Songtao Mei, Kai Wang, Heike Schmitt, Nynke Hofstra","doi":"10.1016/j.envpol.2025.126184","DOIUrl":"https://doi.org/10.1016/j.envpol.2025.126184","url":null,"abstract":"Water quality is under threat due to the presence of pathogenic and antibiotic-resistant bacteria. <em>Escherichia coli</em> (<em>E. coli</em>) serves as an indicator of faecal contamination and the potential presence of other harmful pathogens. Understanding <em>E. coli</em> concentrations helps in assessing the overall health risks associated with waterborne diseases and developing effective water management strategies. Therefore, we developed the first large-scale model, GloWPa-Ecoli C1 to simulate <em>E. coli</em> loads and concentrations in rivers and apply this model to China. The model provides the first comprehensive overview of microbial water quality across China’s rivers. The model simulates <em>E. coli</em> concentrations in 2020 to range from 10<sup>-1.2</sup> to 10<sup>6.3</sup> CFU/L, with 45.6% to 78.1% of rivers exhibiting poor microbial water quality. Major hotspots of <em>E. coli</em> pollution are Haihe, Huaihe and Pearl River Basins. Direct discharge of human faecal waste contributes 80.2% of the total <em>E. coli</em> load, while directly discharged livestock waste accounts for 13.1%. To mitigate <em>E. coli</em> pollution in rivers in China, we recommend increasing human waste collection rates, expanding wastewater treatment plant (WWTP) coverage, phasing out primary treatment WWTPs and eliminating direct livestock waste discharge, particularly from smallholder farms. The study underscores the urgent need to improve microbial water quality in China's rivers. The findings provide actionable insights to inform policy development aimed at safeguarding water quality and public health. Furthermore, the modelling approach is applicable to other regions and microorganisms, offering a foundation for developing models to address antibiotic-resistant bacteria and other emerging water quality challenges.","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"108 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143776043","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Antagonism or synergism? Contrasting toxicity mechanisms of combined antibiotic and metal pollution on Eisenia Fetida 拮抗还是协同?抗生素和金属联合污染对胎生伊蚊的不同毒性机制
IF 8.9 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-03 DOI: 10.1016/j.envpol.2025.126166
Qiuyun Xu, Xin Xiong, Yajuan Shi, Li Qian, Xuan Zhou, Xueli Tian, Jinyang Yu, Liuxuan Fang
{"title":"Antagonism or synergism? Contrasting toxicity mechanisms of combined antibiotic and metal pollution on Eisenia Fetida","authors":"Qiuyun Xu, Xin Xiong, Yajuan Shi, Li Qian, Xuan Zhou, Xueli Tian, Jinyang Yu, Liuxuan Fang","doi":"10.1016/j.envpol.2025.126166","DOIUrl":"https://doi.org/10.1016/j.envpol.2025.126166","url":null,"abstract":"The pervasive occurrence of combined metal and antibiotic pollution (CMAP) in agricultural soils is increasingly being recognized as a novel threat to ecosystems. However, the toxicity variations of CMAP compared to single pollution and the mechanisms underlying these changes remain poorly understood. Herein in this study, the toxicities of copper (Cu)/erythromycin (ERY) and lead (Pb)/norfloxacin (NOR) to earthworms (<em>Eisenia Fetida</em>) were investigated. These results indicated that a single exposure to ERY and NOR at environmental concentrations had negligible effects on physiological processes. Combined Cu/ERY exposure induced more significant oxidative stress, disrupted energy metabolism, and caused cellular damage than Cu alone, as indicated by altered antioxidant enzyme activities, malondialdehyde and adenosine triphosphate content, elevated reactive oxygen species levels, and apoptosis rates in coelomocytes. Conversely, these adverse effects were mitigated by Pb/NOR exposure compared to Pb treatment alone. Further analysis of the gut microbiota revealed that Cu/Pb-tolerant <em>Bacillus</em> spp. play a critical mediating role in the contrasting toxicity profiles. ERY reduced the abundance of <em>Bacillus</em> spp., diminishing their ability to secrete soluble phosphate to immobilize Cu in the gut and leading to increased Cu absorption and toxicity. NOR enriches <em>Bacillus</em> spp. in the gut, facilitating Pb immobilization and reducing Pb bioavailability and toxicity. The contrast toxicity profile revealed the response of the gut microbiota taxa is the primary determinant of the variation in CMAP toxicity. These findings advance our understanding of the impact of CMAP on soil organisms and highlight the need for comprehensive ecological risk assessments to inform regulatory strategies.","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"16 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143766551","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Sulfidated zero-valent iron bimetals for passive remediation of chlorinated vapors in the subsurface
IF 8.9 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-03 DOI: 10.1016/j.envpol.2025.126202
Clarissa Settimi, Daniela Zingaretti, Iason Verginelli, Renato Baciocchi
{"title":"Sulfidated zero-valent iron bimetals for passive remediation of chlorinated vapors in the subsurface","authors":"Clarissa Settimi, Daniela Zingaretti, Iason Verginelli, Renato Baciocchi","doi":"10.1016/j.envpol.2025.126202","DOIUrl":"https://doi.org/10.1016/j.envpol.2025.126202","url":null,"abstract":"This study explores a novel application of sulfidated zero-valent iron (S-ZVI) bimetals for the treatment of chlorinated solvents in the vapor phase. The potential of these reactive materials was investigated through batch, column, and modeling tests. The materials were produced by disc milling of ZVI, sulfur (S), copper (Cu), and nickel (Ni) with molar ratios of 0.05 and 0.2. The reactivity of the materials was assessed through vapor degradation batch tests conducted under partially saturated conditions using trichloroethylene (TCE) as a model compound. Sulfidated materials with a 0.05 S/ZVI molar ratio were the most reactive, achieving up to 99% degradation of TCE vapors within 18 hours and first-order degradation constants of 5-5.7 d<sup>-1</sup>. Compared to the non-sulfidated materials, sulfidated ones remained reactive even after aging by exposure to air for 30 days. In all tests, C<sub>3</sub>-C<sub>6</sub> hydrocarbons were detected as main byproducts, indicating β-elimination as the dominant TCE degradation pathway, with minor dichloroethylene and vinyl chloride amounts from the hydrogenolysis pathway. To evaluate the use of sulfidated bimetals as Horizontal Permeable Reactive Barriers (HPRBs) for treating chlorinated vapors in the subsurface, TCE diffusion column tests were performed using a 5 cm thick reactive layer of S-ZVI-Ni. These tests demonstrated up to 70% degradation over 25 days. By integrating the column test results into an analytical model, it was estimated that an 18 cm HPRB could ensure up to 99% degradation of TCE vapors. These findings highlight the potential of S-ZVI bimetals as an effective passive mitigation system for reducing chlorinated solvent vapor emissions from the subsurface.","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"58 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143776084","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effects of polystyrene microparticles exposures on spermatogenic cell differentiation and reproductive endpoints in male mice
IF 7.6 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-03 DOI: 10.1016/j.envpol.2025.126200
Rong Shen , Peng Xia , Yanan Guo , Pengfei Ji , Xinyi Yuan , Lu Wang , Si Shuang , Liwei Zhou , Ruizhi Tong , Lijuan Zhang , Disheng Liu , Degui Wang
{"title":"Effects of polystyrene microparticles exposures on spermatogenic cell differentiation and reproductive endpoints in male mice","authors":"Rong Shen ,&nbsp;Peng Xia ,&nbsp;Yanan Guo ,&nbsp;Pengfei Ji ,&nbsp;Xinyi Yuan ,&nbsp;Lu Wang ,&nbsp;Si Shuang ,&nbsp;Liwei Zhou ,&nbsp;Ruizhi Tong ,&nbsp;Lijuan Zhang ,&nbsp;Disheng Liu ,&nbsp;Degui Wang","doi":"10.1016/j.envpol.2025.126200","DOIUrl":"10.1016/j.envpol.2025.126200","url":null,"abstract":"<div><div>The widespread distribution of microplastics in the environment has raised concerns about their potential implications for human health. Microplastics accumulate in animals and humans, but the risks associated with these pollutants are not fully understood. This study aimed to investigate the effects of polystyrene microplastics on the male reproductive system. The 0.1 μm polystyrene (PS) could accumulate in the testicular tissue and spermatogonia GC-1, while 1 μm PS was not easy to enter and accumulate in the testicular tissue and cells. Mice continuously exposed for 3-months to 0.1 μm PS demonstrated lower fertility and inhibited spermatogonium differentiation compared to control mice. The 0.1 μm PS were dispersed throughout the seminiferous tubule of the testis. Metabolic reprogramming was found to be involved in these processes. Histone methylation and autophagy-related pathways showed significant differences following PS treatment in testis tissue and GC-1 cells. Our findings suggest that chronic exposure to 0.1 μm PS inhibited spermatogenic cell differentiation and impaired fertility in male mice. We propose that abnormal epigenetic modifications in 0.1 μm PS exposed mice contributed to the dysregulation of glycolytic enzymes, and that the impaired autophagic pathway exacerbated the accumulation of glycolytic enzymes further. Glycolysis plays a critical role in the regulation of spermatogenic cell differentiation, and its regulation partially alleviated the impairments associated with PS exposure. In conclusion, our findings suggest that chronic exposure to nanoplastics PS inhibited spermatogenic cell differentiation and impaired fertility in male mice via disrupted epigenetic modification and metabolic dysregulation.</div></div>","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"373 ","pages":"Article 126200"},"PeriodicalIF":7.6,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143766601","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Distribution and Characteristics of Microplastics in Fluvial Sediments from the Koshi River Basin, Nepal 尼泊尔甲西河流域冲积沉积物中微塑料的分布与特征
IF 8.9 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-03 DOI: 10.1016/j.envpol.2025.126189
Alisha Dahal, Bishal Dahal, Sagar Sitaula, Rupesh Bohara, Ramesh Raj Pant, Yukti Acharya, Khaga Raj Sharma, Basant Giri, Bhanu Bhakta Neupane
{"title":"Distribution and Characteristics of Microplastics in Fluvial Sediments from the Koshi River Basin, Nepal","authors":"Alisha Dahal, Bishal Dahal, Sagar Sitaula, Rupesh Bohara, Ramesh Raj Pant, Yukti Acharya, Khaga Raj Sharma, Basant Giri, Bhanu Bhakta Neupane","doi":"10.1016/j.envpol.2025.126189","DOIUrl":"https://doi.org/10.1016/j.envpol.2025.126189","url":null,"abstract":"Microplastics (MPs) are emerging contaminants found in various ecosystems including oceans, lakes, rivers, sediment air, and soil. Mapping of MPs in different deposition zones in fresh water sediment is important to identify their potential sources, sink, and transport mechanism. In this study, MPs were analyzed in sediment samples from Arun, Tamor, and Koshi Rivers in eastern Nepal. A total of 78 samples from 26 sites were collected from three independent deposition regions i.e. recent deposition (R0), recent past deposition (R1), and past deposition (R2) during monsoon season in 2023. All samples were analyzed following standard methods involving drying, peroxidation, density separation, microscopic examination and chemical identification by FTIR. In all the river basins differences in MPs count, color, and morphology were observed in three deposition regions. In Tamor basin the MPs count ranged from 3140-9500 MPKg<sup>-1</sup>, 3800-9420 MPKg<sup>-1</sup>, and 3180-9700 MPKg<sup>-1</sup> in R2, R1 and R0 regions, respectively. The mean abundance was found higher in downstream especially in Koshi River. The predominant shapes, sizes, and colors found in all three river basins were fragment (52.5%), 20-100 μm (58.86%), and black (33.76%). The particles were identified as polyamide, polypropylene, polyvinyl chloride, polysulfone, nylon, and, polyether ether ketone. The pollution risk assessment indicated minimal MPs contamination upstream and moderate contamination downstream. Finally, principal component analysis (PCA) and land use and land cover change (LULC) data were utilized to identify the potential sources of MPs. Agricultural and anthropogenic sources were identified as major contributors to the MPs load. This study provided baseline data for MP concentrations and their potential sources in Arun, Tamor, and Koshi river sediments. This information could be important for future MPs mitigation strategies.","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"27 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143766550","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Corrigendum to ‘What are exposure biomarkers of rare earth elements for the ionic rare earth occupational population?’ [Environ. Pollut. 345 (2024) 123499]
IF 7.6 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-03 DOI: 10.1016/j.envpol.2025.126079
Qingfeng Chen , Jun Hong , Guowen Lai , Xiaobo Yang , Guoliang Chen , Na Xu , Xuewei Li , Kaibo Hu , Tianci Chen , Yang Song , Yinhua Wan
{"title":"Corrigendum to ‘What are exposure biomarkers of rare earth elements for the ionic rare earth occupational population?’ [Environ. Pollut. 345 (2024) 123499]","authors":"Qingfeng Chen ,&nbsp;Jun Hong ,&nbsp;Guowen Lai ,&nbsp;Xiaobo Yang ,&nbsp;Guoliang Chen ,&nbsp;Na Xu ,&nbsp;Xuewei Li ,&nbsp;Kaibo Hu ,&nbsp;Tianci Chen ,&nbsp;Yang Song ,&nbsp;Yinhua Wan","doi":"10.1016/j.envpol.2025.126079","DOIUrl":"10.1016/j.envpol.2025.126079","url":null,"abstract":"","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"373 ","pages":"Article 126079"},"PeriodicalIF":7.6,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143759975","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Associations of non-essential metal/metalloids and their mixture with liver function in Chinese older adults: the mediating roles of lipid profiles
IF 7.6 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-03 DOI: 10.1016/j.envpol.2025.126207
Xuqiu Cheng , Wenyuan Liu , Ziwei Tian , Jinqi Yan , Xianglong Liu , Qiang Liu , Yan Zhang , Yuan Wang , Bing Hu , Jun Wang , Fangbiao Tao , Linsheng Yang
{"title":"Associations of non-essential metal/metalloids and their mixture with liver function in Chinese older adults: the mediating roles of lipid profiles","authors":"Xuqiu Cheng ,&nbsp;Wenyuan Liu ,&nbsp;Ziwei Tian ,&nbsp;Jinqi Yan ,&nbsp;Xianglong Liu ,&nbsp;Qiang Liu ,&nbsp;Yan Zhang ,&nbsp;Yuan Wang ,&nbsp;Bing Hu ,&nbsp;Jun Wang ,&nbsp;Fangbiao Tao ,&nbsp;Linsheng Yang","doi":"10.1016/j.envpol.2025.126207","DOIUrl":"10.1016/j.envpol.2025.126207","url":null,"abstract":"<div><div>The liver is vulnerable to damage from environmental pollutants, but evidence on the effects of non-essential metal/metalloid (NEM) mixture on liver function and their mechanisms remains limited. The study aimed to explore the correlations between individual NEMs and their combinations with liver function, and the mediating roles of lipid profiles. The research involved 2642 individuals aged 60 and older in China. Urine concentrations of arsenic (As), cesium (Cs), barium (Ba), thallium (Tl), and cadmium (Cd) were analyzed using ICP-MS. Liver function was assessed based on the levels of alanine aminotransferase (ALT), aspartate aminotransferase (AST), and albumin (ALB). To evaluate the individual and combined effects of these NEMs on liver function, linear regression, restricted cubic splines (RCS), weighted quantile sum (WQS), quantile g-computation (QGC), and Bayesian kernel machine regression (BKMR) models were utilized. Mediation analyses were conducted to explore the potential role of lipid profiles in NEM-liver function relations. Adjusted linear regression revealed positive associations of Tl with ALT (<em>β</em> = 0.044, 95 % <em>CI</em>: 0.022 to 0.066) and AST (<em>β</em> = 0.019, 95 % <em>CI</em>: 0.004 to 0.035), and negative associations of Cs (<em>β</em> = −0.015, 95 % <em>CI</em>: −0.020 to −0.010), Tl (<em>β</em> = −0.010, 95 % <em>CI</em>: −0.015 to −0.005), and Cd (<em>β</em> = −0.019, 95 % <em>CI</em>: −0.024 to −0.014) with ALB. The RCS model confirmed these linear relationships. Mixture models consistently demonstrated a positive association between the NEM mixture and ALT/AST, primarily driven by Tl, and a negative association with ALB, predominantly influenced by Cd. Mediation analyses suggested triglycerides and total cholesterol partially mediated the associations between Tl, the NEM mixture, and liver function. In conclusion, the NEM mixture, mainly driven by Tl and Cd, is linked to liver function impairment, with lipid profiles potentially mediating these effects. More research is needed to confirm these findings and clarify the mechanisms.</div></div>","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"373 ","pages":"Article 126207"},"PeriodicalIF":7.6,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143776042","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Environmental and Health Impacts of Heat Transfer Fluids (HTFs)
IF 8.9 2区 环境科学与生态学
Environmental Pollution Pub Date : 2025-04-03 DOI: 10.1016/j.envpol.2025.126201
R.P. Martínez-Esteban, V. López-Rodas, J. García, E. Costas, C. García-Balboa
{"title":"Environmental and Health Impacts of Heat Transfer Fluids (HTFs)","authors":"R.P. Martínez-Esteban, V. López-Rodas, J. García, E. Costas, C. García-Balboa","doi":"10.1016/j.envpol.2025.126201","DOIUrl":"https://doi.org/10.1016/j.envpol.2025.126201","url":null,"abstract":"Thermo Solar Systems are growing significantly around the world. Although they are thought to be clean, the analysis of its life cycle evidence a negative impact on the environment, due to unvoluntary spillages of heat fluid transfer (HTF). To know the risk of HTF spills for human health and environment, we selected human cell lines and toxicological model organisms to evaluate both aspects. In concrete, we selected two non-transformed human cell lines of fibroblasts and hepatocytes; Allivibrio fisherii, Dictyosphaerium chlorelloides, Emiliana huxleyi and Artemia salina. Using standardized toxicological tests, we studied the effect of HTF under two scenarios: 1) exposure cells to concentrations on the range from 0.1 to 15 μg/L for short periods (from 30 minutes to 72 hours) and 2) the same concentrations for 20 days. Additionally, we explored the toxic effect of two different HTF samples: commercial and thermal degraded HTF (used). Results proved that commercial is less toxic than used and that microalgae was extremely sensitive (IC50 around 3.5 μg/L) following of Allivibrio fisherii (IC50 around 200 μg/L), human cell lines (IC50 around 1,000 μg/L) and crustaceans (IC50 2,000 μg/L). The particularities of cell wall composition and the metabolic specialization justify the differences. Furthermore, a very interesting result was that exposure for 20 days produced greater damage than the same dose for periods of 72 hours in all the cell types studied. Our results suggest that HTF spillages have a bigger environmental impact than expected, which thermosolar plants are not as environmentally friendly as previously thought.","PeriodicalId":311,"journal":{"name":"Environmental Pollution","volume":"18 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143766909","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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