Eco-Environment & Health最新文献

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COPD deaths attributable to ozone in 2019 and future projections using the WHO AQG 2021 in urban China 2019年臭氧导致的慢性阻塞性肺病死亡人数以及使用世卫组织2021年空气质量指标对中国城市未来的预测
Eco-Environment & Health Pub Date : 2022-12-01 DOI: 10.1016/j.eehl.2022.11.002
Mingyao Yao , Ying Hu , Ao Zhang , John S. Ji , Bin Zhao
{"title":"COPD deaths attributable to ozone in 2019 and future projections using the WHO AQG 2021 in urban China","authors":"Mingyao Yao ,&nbsp;Ying Hu ,&nbsp;Ao Zhang ,&nbsp;John S. Ji ,&nbsp;Bin Zhao","doi":"10.1016/j.eehl.2022.11.002","DOIUrl":"https://doi.org/10.1016/j.eehl.2022.11.002","url":null,"abstract":"<div><p>Chronic obstructive pulmonary disease (COPD) is an epidemic in China. Ozone is a possible risk factor of COPD, with ozone concentrations increasing in China, despite air pollution mitigation measures that reduced particulate matter. The WHO Air Quality Guidelines (AQG) recommendations in 2021 are a turning point that formally recognizes the crucial role of indoor air pollution. We aimed to investigate the premature COPD deaths attributable to ozone in 2019, taking the WHO AQG 2021 level into account to determine the gap to bridge ozone control in China. First, we assessed ozone exposures initiated from indoor and outdoor sources by gender and age groups in 344 cities under four scenarios: 2019 as a baseline, and outdoor ozone at WHO AQG 2021 level in 2019, 2030, and 2050, respectively. Subsequently, we estimated COPD deaths attributable to ozone. The results show that the COPD deaths attributable to ozone are 77,737 in 2019, and 527, 872, 1355 if the outdoor ozone concentration is reduced to the WHO AQG 2021 level in 2019 (counterfactual scenario), 2030, and 2050, respectively in urban China. The indoor ozone sources only contribute to less than 5% of COPD deaths. A gap of 68.5 μg/m<sup>3</sup> for the highest seasonal ozone concentration should be bridged to meet the WHO AQG 2021 and avoid over 76 thousand (98%) COPD deaths in 2019 in urban China.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000394/pdfft?md5=c6a76526d0d54ceeade87e8f9cdc712d&pid=1-s2.0-S2772985022000394-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"91618079","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Fight for carbon neutrality with state-of-the-art negative carbon emission technologies 用最先进的负碳排放技术争取碳中和
Eco-Environment & Health Pub Date : 2022-12-01 DOI: 10.1016/j.eehl.2022.11.005
Jiaju Fu , Pan Li , Yuan Lin , Huitong Du , Hongzhi Liu , Wenlei Zhu , Hongqiang Ren
{"title":"Fight for carbon neutrality with state-of-the-art negative carbon emission technologies","authors":"Jiaju Fu ,&nbsp;Pan Li ,&nbsp;Yuan Lin ,&nbsp;Huitong Du ,&nbsp;Hongzhi Liu ,&nbsp;Wenlei Zhu ,&nbsp;Hongqiang Ren","doi":"10.1016/j.eehl.2022.11.005","DOIUrl":"https://doi.org/10.1016/j.eehl.2022.11.005","url":null,"abstract":"<div><p>After the Industrial Revolution, the ever-increasing atmospheric CO<sub>2</sub> concentration has resulted in significant problems for human beings. Nearly all countries in the world are actively taking measures to fight for carbon neutrality. In recent years, negative carbon emission technologies have attracted much attention due to their ability to reduce or recycle excess CO<sub>2</sub> in the atmosphere. This review summarizes the state-of-the-art negative carbon emission technologies, from the artificial enhancement of natural carbon sink technology to the physical, chemical, or biological methods for carbon capture, as well as CO<sub>2</sub> utilization and conversion. Finally, we expound on the challenges and outlook for improving negative carbon emission technology to accelerate the pace of achieving carbon neutrality.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000424/pdfft?md5=69088ceeb580f4beea2accd1b6c4c098&pid=1-s2.0-S2772985022000424-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"91618081","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 11
China Biodiversity Observation Network for better global sustainability developments 中国生物多样性观测网,促进全球可持续发展
Eco-Environment & Health Pub Date : 2022-12-01 DOI: 10.1016/j.eehl.2022.11.001
Jianfeng Yi , Fangzhou Ma , Jiaqi Li , Wei Liu, Yun Cao, Yaqiong Wan, Chenbin Wang, Mengmeng Chen, Dandan Yu, Haigen Xu
{"title":"China Biodiversity Observation Network for better global sustainability developments","authors":"Jianfeng Yi ,&nbsp;Fangzhou Ma ,&nbsp;Jiaqi Li ,&nbsp;Wei Liu,&nbsp;Yun Cao,&nbsp;Yaqiong Wan,&nbsp;Chenbin Wang,&nbsp;Mengmeng Chen,&nbsp;Dandan Yu,&nbsp;Haigen Xu","doi":"10.1016/j.eehl.2022.11.001","DOIUrl":"https://doi.org/10.1016/j.eehl.2022.11.001","url":null,"abstract":"","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000370/pdfft?md5=96f95ced73ee4c0aaa52e8cd7460b7f0&pid=1-s2.0-S2772985022000370-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"91662666","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Molecular signature of soil organic matter under different land uses in the Lake Chaohu Basin 巢湖流域不同土地利用方式下土壤有机质分子特征
Eco-Environment & Health Pub Date : 2022-12-01 DOI: 10.1016/j.eehl.2022.10.003
Han Gao , Huixin Li , Chen Lin , Pedro J.J. Alvarez , Caroline A. Masiello , Dongqiang Zhu , Ao Kong , Xiaolei Qu
{"title":"Molecular signature of soil organic matter under different land uses in the Lake Chaohu Basin","authors":"Han Gao ,&nbsp;Huixin Li ,&nbsp;Chen Lin ,&nbsp;Pedro J.J. Alvarez ,&nbsp;Caroline A. Masiello ,&nbsp;Dongqiang Zhu ,&nbsp;Ao Kong ,&nbsp;Xiaolei Qu","doi":"10.1016/j.eehl.2022.10.003","DOIUrl":"https://doi.org/10.1016/j.eehl.2022.10.003","url":null,"abstract":"<div><p>The concentration and molecular composition of soil organic matter (SOM) are important factors in mitigation against climate change as well as providing other ecosystem services. Our quantitative understanding of how land use influences SOM molecular composition and associated turnover dynamics is limited, which underscores the need for high-throughput analytical approaches and molecular marker signatures to clarify this etiology. Combining a high-throughput untargeted mass spectrometry screening and molecular markers, we show that forest, farmland and urban land uses result in distinct molecular signatures of SOM in the Lake Chaohu Basin. Molecular markers indicate that forest SOM has abundant carbon contents from vegetation and condensed organic carbon, leading to high soil organic carbon (SOC) concentration. Farmland SOM has moderate carbon contents from vegetation, and limited content of condensed organic carbon, with SOC significantly lower than that of forest soils. Urban SOM has high abundance of condensed organic carbon markers due to anthropogenic activities but relatively low in markers from vegetation. Consistently, urban soils have the highest black carbon/SOC ratio among these land uses. Overall, our results suggested that the molecular signature of SOM varies significantly with land use in the Lake Chaohu Basin, influencing carbon dynamics. Our strategy of molecular fingerprinting and marker discovery is expected to enlighten further research on SOM molecular signatures and cycling dynamics.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000369/pdfft?md5=6de101cc0be0f5ad065836dde8ead850&pid=1-s2.0-S2772985022000369-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"91618078","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Environmental behavior, human health effect, and pollution control of heavy metal(loid)s toward full life cycle processes 重金属的环境行为、对人体健康的影响及污染控制——面向全生命周期过程
Eco-Environment & Health Pub Date : 2022-12-01 DOI: 10.1016/j.eehl.2022.11.003
Haoyu Deng , Yuling Tu , Han Wang , Ziyi Wang , Yanyu Li , Liyuan Chai , Wenchao Zhang , Zhang Lin
{"title":"Environmental behavior, human health effect, and pollution control of heavy metal(loid)s toward full life cycle processes","authors":"Haoyu Deng ,&nbsp;Yuling Tu ,&nbsp;Han Wang ,&nbsp;Ziyi Wang ,&nbsp;Yanyu Li ,&nbsp;Liyuan Chai ,&nbsp;Wenchao Zhang ,&nbsp;Zhang Lin","doi":"10.1016/j.eehl.2022.11.003","DOIUrl":"10.1016/j.eehl.2022.11.003","url":null,"abstract":"<div><p>Heavy metal(loid)s (HMs) have caused serious environmental pollution and health risks. Although the past few years have witnessed the achievements of studies on environmental behavior of HMs, the related toxicity mechanisms, and pollution control, their relationship remains a mystery. Researchers generally focused on one topic independently without comprehensive considerations due to the knowledge gap between environmental science and human health. Indeed, the full life cycle control of HMs is crucial and should be reconsidered with the combination of the occurrence, transport, and fate of HMs in the environment. Therefore, we started by reviewing the environmental behaviors of HMs which are affected by a variety of natural factors as well as their physicochemical properties. Furthermore, the related toxicity mechanisms were discussed according to exposure route, toxicity mechanism, and adverse consequences. In addition, the current state-of-the-art of available technologies for pollution control of HMs wastewater and solid wastes were summarized. Finally, based on the research trend, we proposed that advanced in-operando characterizations will help us better understand the fundamental reaction mechanisms, and big data analysis approaches will aid in establishing the prediction model for risk management.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000400/pdfft?md5=01613ed51475e5db4389ff73e3cda5a2&pid=1-s2.0-S2772985022000400-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"134368884","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 26
Heavy metals in agricultural soil in China: A systematic review and meta-analysis 中国农业土壤重金属:系统综述与荟萃分析
Eco-Environment & Health Pub Date : 2022-12-01 DOI: 10.1016/j.eehl.2022.10.004
Moyan Wen , Ziqi Ma , Daniel B. Gingerich , Xiao Zhao , Dongye Zhao
{"title":"Heavy metals in agricultural soil in China: A systematic review and meta-analysis","authors":"Moyan Wen ,&nbsp;Ziqi Ma ,&nbsp;Daniel B. Gingerich ,&nbsp;Xiao Zhao ,&nbsp;Dongye Zhao","doi":"10.1016/j.eehl.2022.10.004","DOIUrl":"10.1016/j.eehl.2022.10.004","url":null,"abstract":"<div><p>Research about farmland pollution by heavy metals/metalloids in China has drawn growing attention. However, there was rare information on spatiotemporal evolution and pollution levels of heavy metals in the major grain-producing areas. We extracted and examined data from 276 publications between 2010 and 2021 covering five major grain-producing regions in China from 2010 to 2021. Spatiotemporal evolution characteristics of main heavy metals/metalloids was obtained by meta-analysis. In addition, subgroup analyses were carried out to study preliminary correlations related to accumulation of the pollutants. Cadmium (Cd) was found to be the most prevailing pollutant in the regions in terms of both spatial distribution and temporal accumulation. The Huang-Huai-Hai Plain was the most severely polluted. Accumulation of Cd, mercury (Hg) and copper (Cu) increased from 2010 to 2015 when compared with the 1990 background data. Further, the levels of five key heavy metals (Cd, Cu, Hg, lead [Pb] and zinc [Zn]) showed increasing trends from 2016 to 2021 in all five regions. Soil pH and mean annual precipitation had variable influences on heavy metal accumulation. Alkaline soil and areas with less rainfall faced higher pollution levels. Farmlands cropped with mixed species showed smaller effect sizes of heavy metals than those with single upland crop, suggesting that mixed farmland use patterns could alleviate the levels of heavy metals in soil. Of various soil remediation efforts, farmland projects only held a small market share. The findings are important to support the research of risk assessment, regulatory development, pollution prevention, fund allocation and remediation actions.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000382/pdfft?md5=fd9df5d17ce7b3429003d123a645c568&pid=1-s2.0-S2772985022000382-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"129552929","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 19
Highly spatial and temporal bottom-up vehicle emission characterization and its control in a typical ecology-preservation area 典型生态保护区高时空自底向上机动车排放特征及其控制
Eco-Environment & Health Pub Date : 2022-09-01 DOI: 10.1016/j.eehl.2022.09.003
Pengju Bie , Fanyuan Deng , Bi Chen , Li Wang , Fan Yang , Jianguo Zhou , Huan Liu , Kebin He
{"title":"Highly spatial and temporal bottom-up vehicle emission characterization and its control in a typical ecology-preservation area","authors":"Pengju Bie ,&nbsp;Fanyuan Deng ,&nbsp;Bi Chen ,&nbsp;Li Wang ,&nbsp;Fan Yang ,&nbsp;Jianguo Zhou ,&nbsp;Huan Liu ,&nbsp;Kebin He","doi":"10.1016/j.eehl.2022.09.003","DOIUrl":"10.1016/j.eehl.2022.09.003","url":null,"abstract":"<div><p>The Chishui River Valley is a microscale ecology-preservation area with industrial clusters. The significance of evaluating vehicular emissions has been gradually highlighted with the rapid development of the local transportation and tourism sectors. This study provides the first estimates based on both bottom-up and top-down approaches. The annual total emissions of CO, NO<sub><em>x</em></sub>, hydrocarbons (HC), PM<sub>10,</sub> and PM<sub>2.5</sub> in 2019 were 347.8, 189.6, 46.3, 6.9, and 6.3 Mg, respectively. Trucks contributed the most (55%) to the NO<sub><em>x</em></sub> emissions, followed by heavy-duty passenger vehicles (26%). In contrast, light-duty passenger vehicles and motorcycles generated 75% of the HC emissions. The superior accuracy of highly spatial and temporal bottom-up estimates versus top-down estimates is validated by the similar variation trends of hourly emission intensities and enhanced concentrations relative to background observations for both NO<sub><em>x</em></sub> and CO, with Pearson correlation coefficients between the intensities and concentrations ranging from 0.79 to 0.85. Historical HC emissions peaked in 2013, followed by a sharp decline in 2014 and a continuous rise since then, whereas NO<sub><em>x</em></sub> emissions have kept increasing since 2010. These indicated the necessity and urgency of effective vehicular emission mitigations. Based on scenario analysis, traffic restrictions combined with upgrading the emission standards of admitted vehicles will possess huge emission reduction potentials. Future recommendations about establishing a low emission zone in the valley and supporting policies were introduced.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000321/pdfft?md5=37702a183dec4a60dc2cb2a8a3fe3b4f&pid=1-s2.0-S2772985022000321-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"124883703","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 7
Corrigendum to “Environmental pollution, a hidden culprit for health issues” [Eco-Environ. Health (2022) 31–45] “环境污染,健康问题的罪魁祸首”[生态环境]更正。健康(2022)31-45]
Eco-Environment & Health Pub Date : 2022-09-01 DOI: 10.1016/j.eehl.2022.08.001
Hanqing Xu , Yang Jia , Zhendong Sun , Jiahui Su , Qian S. Liu , Qunfang Zhou , Guibin Jiang
{"title":"Corrigendum to “Environmental pollution, a hidden culprit for health issues” [Eco-Environ. Health (2022) 31–45]","authors":"Hanqing Xu ,&nbsp;Yang Jia ,&nbsp;Zhendong Sun ,&nbsp;Jiahui Su ,&nbsp;Qian S. Liu ,&nbsp;Qunfang Zhou ,&nbsp;Guibin Jiang","doi":"10.1016/j.eehl.2022.08.001","DOIUrl":"10.1016/j.eehl.2022.08.001","url":null,"abstract":"","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000242/pdfft?md5=b56c6b4f9e2d6aba88d3de3138957f35&pid=1-s2.0-S2772985022000242-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"121718300","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Roadmap of environmental health research on emerging contaminants: Inspiration from the studies on engineered nanomaterials 新兴污染物的环境健康研究路线图:来自工程纳米材料研究的启示
Eco-Environment & Health Pub Date : 2022-09-01 DOI: 10.1016/j.eehl.2022.10.001
Xiaona Li , Feng He , Zhenyu Wang , Baoshan Xing
{"title":"Roadmap of environmental health research on emerging contaminants: Inspiration from the studies on engineered nanomaterials","authors":"Xiaona Li ,&nbsp;Feng He ,&nbsp;Zhenyu Wang ,&nbsp;Baoshan Xing","doi":"10.1016/j.eehl.2022.10.001","DOIUrl":"10.1016/j.eehl.2022.10.001","url":null,"abstract":"<div><p>Research on the environmental health of emerging contaminants is critical to understand their risks before causing severe harm. However, the low environmental concentrations, complex behaviors, and toxicology of emerging contaminants present enormous challenges for researchers. Here, we reviewed the research on the environmental health of engineered nanomaterials (ENMs), one of the typical emerging contaminants, to enlighten pathways for future research on emerging contaminants at their initial exploratory stage. To date, some developed pretreatment methods and detection technologies have been established for the determination of ENMs in natural environments. The mechanisms underlying the transfer and transformation of ENMs have been systematically explored in laboratory studies. The mechanisms of ENMs-induced toxicity have also been preliminarily clarified at genetic, cellular, individual, and short food chain levels, providing not only a theoretical basis for revealing the risk change and environmental health effects of ENMs in natural environments but also a methodological guidance for studying environmental health of other emerging contaminants. Nonetheless, due to the interaction of multiple environmental factors and the high diversity of organisms in natural environments, health effects observed in laboratory studies likely differ from those in natural environments. We propose a holistic approach and mesocosmic model ecosystems to systematically carry out environmental health research on emerging contaminants, obtaining data that determine the objectivity and accuracy of risk assessment.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000345/pdfft?md5=e194fbbd2135c20ea36790c9ae8f7e90&pid=1-s2.0-S2772985022000345-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"127390205","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 30
Monthly variations of unregulated brominated disinfection by-products in chlorinated water are correlated with total bromine 氯化水中无管制的溴化消毒副产物的月变化与总溴有关
Eco-Environment & Health Pub Date : 2022-09-01 DOI: 10.1016/j.eehl.2022.06.002
Christena Watts , Jianxian Sun , Paul D. Jones , Hui Peng , John P. Giesy
{"title":"Monthly variations of unregulated brominated disinfection by-products in chlorinated water are correlated with total bromine","authors":"Christena Watts ,&nbsp;Jianxian Sun ,&nbsp;Paul D. Jones ,&nbsp;Hui Peng ,&nbsp;John P. Giesy","doi":"10.1016/j.eehl.2022.06.002","DOIUrl":"10.1016/j.eehl.2022.06.002","url":null,"abstract":"<div><p>Brominated disinfection by-products (Br-DBPs) can form during the chlorination of drinking water in treatment plants (DWTP). Regulations exist for a small subset of Br-DBPs; however, hundreds of unregulated Br-DBPs have been detected, and limited information exists on their occurrence, concentrations, and seasonal trends. Here, a data-independent precursor isolation and characteristic fragment (DIPIC-Frag) method were optimized to screen chlorinated waters for Br-DBPs. There were 553 Br-DBPs detected with <em>m/z</em> values ranging from 170.884 to 497.0278 and chromatographic retention times from 2.4 to 26.2 min. With MS<sup>2</sup> information, structures for 40 of the 54 most abundant Br-DBPs were predicted. The method was then applied to a year-long study in which raw, clear well, and finished water were analyzed monthly. The 54 most abundant unregulated Br-DBPs were subjected to trend analysis. Br-DBPs with higher oxygen-to-carbon (O/C) and bromine-to-carbon (Br/C) ratios increased as water moved from the clear well to the finished stage, which indicated the dynamic formation of Br-DBPs. Monthly trends of unregulated Br-DBPs were compared to raw water parameters, such as natural organic matter, temperature, and total bromine, but no correlations were observed. It was found that total concentrations of bromine (TBr) in finished water (0.04–0.12 mg/L) were consistently and significantly greater than in raw water (0.013–0.038 mg/L, <em>P</em> &lt; 0.001), suggesting the introduction of bromine during the disinfection process. Concentrations of TBr in treatment units, rather than raw water, were significantly correlated to 34 of the Br-DBPs at α = 0.05. This study provides the first evidence that monthly trends of unregulated Br-DBPs can be associated with the concentration of TBr in treated waters.</p></div>","PeriodicalId":29813,"journal":{"name":"Eco-Environment & Health","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772985022000308/pdfft?md5=b05da5f6719e0fde3a9589382d9dbb27&pid=1-s2.0-S2772985022000308-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"116606308","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
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