Carbohydrate Polymers最新文献_第3页

Homogeneous synthesis of cationic celluloses with broad-spectrum antibacterial activities for the treatment of vaginitis in mice 均相合成具有广谱抗菌活性的阳离子纤维素，用于治疗小鼠阴道炎

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-05 DOI: 10.1016/j.carbpol.2024.122950

Lian Yang , Lujie Wang , Zihui Zhang , Shufei Zhang , Yong He , Ying Wang , Bingshu Li , Jinping Zhou , Li Hong

{"title":"Homogeneous synthesis of cationic celluloses with broad-spectrum antibacterial activities for the treatment of vaginitis in mice","authors":"Lian Yang , Lujie Wang , Zihui Zhang , Shufei Zhang , Yong He , Ying Wang , Bingshu Li , Jinping Zhou , Li Hong","doi":"10.1016/j.carbpol.2024.122950","DOIUrl":"10.1016/j.carbpol.2024.122950","url":null,"abstract":"<div><div>Microbial infection is a significant health issue for humans. Despite the development of numerous antibiotics, the continuous rise of drug-resistant bacteria highlights the urgent need for new materials to combat these problems. In this study, four water-soluble quaternized cellulose (QC) derivatives with degrees of substitution (DS) ranging from 0.23 to 0.45 were synthesized homogeneously from cellulose carbamate (CC) in NaOH/ZnO aqueous solution. The QC derivatives exhibited broad-spectrum antibacterial activity against gram-negative/positive bacteria, fungi and drug-resistance bacteria. Models of bacterial vaginitis (BV) and vulvovaginal candidiasis (VVC) were used to evaluate the application of QC derivatives visually. Secretion smears and tissue section staining revealed that treatment with QC derivatives led to a reduction in mycelia and spores in the vagina and secretions in the VVC model, along with improved inflammation. In the BV model, vaginal secretions were reduced, clue cells in smears significantly decreased, and inflammation markedly improved. Additionally, cell experiments and staining of mouse organ tissue sections demonstrated that QC derivatives exhibited good biocompatibility. Therefore, using QC derivatives in flushing douches represents a novel approach for treating vaginitis and could serve as a benchmark for addressing other infectious diseases.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"349 ","pages":"Article 122950"},"PeriodicalIF":10.7,"publicationDate":"2024-11-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654981","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Deferoxamine functionalized alginate-based collagen composite material enhances the integration of metal implant and bone interface 去铁胺功能化藻酸盐胶原蛋白复合材料可增强金属植入物与骨界面的整合性

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-05 DOI: 10.1016/j.carbpol.2024.122944

Zhenjia Che , Xiao Sheng , Qi Sun , Yanglin Wu , Kaihang Song , Aopan Chen , Jing Chen , Qiyun Chen , Ming Cai

{"title":"Deferoxamine functionalized alginate-based collagen composite material enhances the integration of metal implant and bone interface","authors":"Zhenjia Che , Xiao Sheng , Qi Sun , Yanglin Wu , Kaihang Song , Aopan Chen , Jing Chen , Qiyun Chen , Ming Cai","doi":"10.1016/j.carbpol.2024.122944","DOIUrl":"10.1016/j.carbpol.2024.122944","url":null,"abstract":"<div><div>Poor osseointegration markedly compromises the longevity of prostheses. To enhance the stability of titanium implants, surface functionalization is a proven strategy to promote prosthesis-bone integration. This study developed a hydrogel coating capable of simultaneous osteoangiogenesis and vascularization by incorporating deferoxamine (DFO) into a sodium alginate mineralized collagen composite hydrogel. The physicochemical properties of this hydrogel were thoroughly analyzed. <em>In vivo</em> and <em>in vitro</em> experiments confirmed the hydrogel scaffold's osteogenic and angiogenic capabilities. Results indicated that sodium alginate notably enhanced the mechanical characteristics of the mineralized collagen, allowing it to fully infiltrate the interstices of the 3D-printed titanium scaffold. Furthermore, as the hydrogel degraded, collagen, calcium ion, phosphate ion, and DFO were gradually released around the scaffolds, altering the local osteogenic microenvironment and strongly inducing new bone tissue growth. These findings offer novel perspectives for the creation and utilization of functionalized bone implant materials.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"349 ","pages":"Article 122944"},"PeriodicalIF":10.7,"publicationDate":"2024-11-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654978","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Temperature-responsive gating chitosan-based microcapsules for controlled release of urea fertilizers 用于控制尿素肥料释放的温度响应门控壳聚糖基微胶囊

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-04 DOI: 10.1016/j.carbpol.2024.122929

Nian Xiang , Yuming Lin , Zuzeng Qin , Tongming Su , Xinling Xie , Hongbing Ji

{"title":"Temperature-responsive gating chitosan-based microcapsules for controlled release of urea fertilizers","authors":"Nian Xiang , Yuming Lin , Zuzeng Qin , Tongming Su , Xinling Xie , Hongbing Ji","doi":"10.1016/j.carbpol.2024.122929","DOIUrl":"10.1016/j.carbpol.2024.122929","url":null,"abstract":"<div><div>Polysaccharides-based smart fertilizers are essential for promoting plant growth, yet significant challenges exist in achieving stable structures and synchronizing nutrient release and plant growth. This study developed a temperature-responsive gating chitosan-based microcapsule (CTSMC-g-PNIPAM) by grafting N-isopropyl acrylamide (NIPAM) onto chitosan microcapsules (CTSMC) via atom transfer radical polymerization (ATRP). The interfacial crosslinking of chitosan (CTS) and terephthalendehyde (TPA) formed the CTSMC matrix with a hollow chamber structure and ensured stability. CTSMC-g-PNIPAM exhibited reversible temperature-responsive gating properties and sustained release behavior, and the PNIPAM chains acted like gating switches. Below the low critical solution temperature (LCST) (25 °C), the PNIPAM chains stretched and the gating switch closed, slowing down the release rate. Above the LCST (40 °C), the PNIPAM chains contracted and the gating switch opened, accelerating the release rate. The release behaviors of CTSMC-g-PNIPAM in soil indicated that the gating microcapsule effectively prolonged the release of urea. Moreover, the cumulative release of CTSMC-g-PNIPAM at 40 °C was significantly higher than at 25 °C. The first-order kinetic and Korsmeyer-Peppas model indicate that the urea release involves concentration gradient diffusion and skeleton dissolution. Compared with pure urea, urea@(CTSMC-g-PNIPAM) increased the growth status of maize, suggesting a promising strategy for smart fertilizers.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"348 ","pages":"Article 122929"},"PeriodicalIF":10.7,"publicationDate":"2024-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654231","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Chitosan nanoparticles of imatinib mesylate coated with TPGS for the treatment of colon cancer: In-vivo & in-vitro studies 涂有 TPGS 的甲磺酸伊马替尼壳聚糖纳米粒子用于治疗结肠癌：体内和体外研究

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-04 DOI: 10.1016/j.carbpol.2024.122935

Darshan Bhirud , Sankha Bhattacharya , Harshvardhan Raval , Preeti Chidambar Sangave , Girdhari Lal Gupta , Gaurav Paraskar , Megha Jha , Satyam Sharma , Sateesh Belemkar , Devendra Kumar , Rahul Maheshwari , Mayank Sharma

{"title":"Chitosan nanoparticles of imatinib mesylate coated with TPGS for the treatment of colon cancer: In-vivo & in-vitro studies","authors":"Darshan Bhirud , Sankha Bhattacharya , Harshvardhan Raval , Preeti Chidambar Sangave , Girdhari Lal Gupta , Gaurav Paraskar , Megha Jha , Satyam Sharma , Sateesh Belemkar , Devendra Kumar , Rahul Maheshwari , Mayank Sharma","doi":"10.1016/j.carbpol.2024.122935","DOIUrl":"10.1016/j.carbpol.2024.122935","url":null,"abstract":"<div><div>The study aimed to develop and evaluate chitosan-based nanoparticles coated with TPGS for the targeted delivery of imatinib mesylate to colon cancer cells. Particle size and zeta potential analysis were within the acceptable range for targeting colon cancer. CS-IMT-TPGS-NPs had a significant positive zeta potential of 30.4 mV, suggesting improved cellular intake. FE-SEM and TEM demonstrated that the nanoparticles appeared spherical, smooth, and did not aggregate, with a visible TPGS coating. XRD confirmed that crystalline imatinib transitioned to an amorphous state during nano formulation. In-vitro tests on HCT-116 cells demonstrated that CS-IMT-TPGS-NPs outperformed free IMT regarding cytotoxicity, apoptosis induction, cellular uptake, and cell migration inhibition. Additionally, the nanoparticles were examined in vitro using mitochondrial membrane potential, DNA fragmentation, GAPDH relative gene expression, ROS estimation, and cell cycle analysis. The effect of therapy on expected colon-associated bacterial strains was also investigated. The biocompatibility of nanoparticles was assessed by hemolysis and platelet aggregation experiments. The anti-inflammatory impact was determined using the HET-CAM test. Non-Fickian diffusion at pH 5.5 resulted in sustained in-vitro drug release, with no initial burst. In-vivo investigations using albino Wistar rats suggest pharmacokinetic properties for produced nanoparticles, whereas histopathological examinations assess acute toxicity.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"348 ","pages":"Article 122935"},"PeriodicalIF":10.7,"publicationDate":"2024-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654230","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Novel food-grade water-in-water emulsion fabricated by amylopectin and tara gum: Property evaluation and stability analysis 由直链淀粉和塔拉胶制成的新型食品级水包水乳液：性能评估和稳定性分析

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-04 DOI: 10.1016/j.carbpol.2024.122937

Tian Luo, Zihao Wei, Changhu Xue

{"title":"Novel food-grade water-in-water emulsion fabricated by amylopectin and tara gum: Property evaluation and stability analysis","authors":"Tian Luo, Zihao Wei, Changhu Xue","doi":"10.1016/j.carbpol.2024.122937","DOIUrl":"10.1016/j.carbpol.2024.122937","url":null,"abstract":"<div><div>To surmount the limitation of the instability of the currently reported water-in-water (<em>W</em>/W) emulsions, novel W/W emulsionss were constructed using amylopectin (AMP) and tara gum (TG) as the phases, and differently shaped ovalbumin (OVA) particles were used as stabilizers to improve the stability of <em>W</em>/W emulsions. Experiments displayed that the conformation of OVA could be changed by heating treatment, thus forming fibrous or spherical OVA particles that had the potential to stabilize TG-in-AMP (TG/AMP) emulsions. The emulsions had the best stability when the pH was 4 and the concentration of OVA particles was 3 %. Moreover, since ovalbumin fibril (OVAF) had better adsorption at the water-water interface than ovalbumin sphere (OVAS), OVAF-stabilized TG/AMP emulsion (OF-TE) had a relatively denser interfacial layer and exhibited more satisfactory ionic stability and physical stability than OVAS-stabilized TG/AMP emulsion (OS-TE). The rheological results demonstrated that OVAF and OVAS had little effect on the viscosity of TG/AMP emulsions. In brief, OVAF was more effective in improving the stability of TG/AMP emulsions than OVAS, and OF-TE did not show phase separation for at least 5 days. This study may be of great significance in improving the stability of food-grade <em>W</em>/W emulsions.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"348 ","pages":"Article 122937"},"PeriodicalIF":10.7,"publicationDate":"2024-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654242","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Natural cellulose reinforced multifunctional eutectogels for wearable sensors and epidermal electrodes 用于可穿戴传感器和表皮电极的天然纤维素增强多功能共晶凝胶

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-04 DOI: 10.1016/j.carbpol.2024.122939

Qianwen Lu , Hengfeng Li , Zhijian Tan

{"title":"Natural cellulose reinforced multifunctional eutectogels for wearable sensors and epidermal electrodes","authors":"Qianwen Lu , Hengfeng Li , Zhijian Tan","doi":"10.1016/j.carbpol.2024.122939","DOIUrl":"10.1016/j.carbpol.2024.122939","url":null,"abstract":"<div><div>Wearable electronics significantly impact health monitoring, clinical care, and human-machine interfaces. Eutectogels, which utilize deep eutectic solvents (DES) address the drawbacks of hydrogels, such as weight loss and poor temperature tolerance, as well as the high costs and toxicities associated with ionogels. Despite these advances, most eutectogels serve only as sensors or epidermal electrodes and rarely fulfill both functions simultaneously. In this study, we present a multifunctional eutectogel designed to function in both ways. Incorporating natural cotton cellulose nanofibers as nanofillers reinforced the tensile strength of the resultant eutectogel by 7.47 times compared to that of the pure eutectogel, reaching 4.93 MPa. This eutectogel exhibited high ionic conductivity (1.22 S m<sup>−1</sup>), strong adhesion (1562.2 kPa to iron), self-healing ability (80.37% strain recovery and 80.53% tensile strength recovery), a broad temperature tolerance (−40 to 80 °C), and antibacterial properties. It demonstrates high sensitivity for the real-time strain detection of human activities and accurately captures electrophysiological signals, enabling the control of a small car. This versatile eutectogel has excellent potential for use in flexible wearable electronics.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"348 ","pages":"Article 122939"},"PeriodicalIF":10.7,"publicationDate":"2024-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654232","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Potential of natural polysaccharide for ovarian cancer therapy 天然多糖治疗卵巢癌的潜力

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-04 DOI: 10.1016/j.carbpol.2024.122946

Miaomiao Xiao , Siwen Chen , Yaochen Yang , Ke Hu , Yantao Song , Zhipeng Hou , Siyu Sun , Liqun Yang

引用次数: 0

A deep eutectic solvent with bifunctional acid sites treatment to upgrade a bamboo kraft pulp into a cellulose-acetate grade dissolving pulp 双官能团酸场所处理的深共晶溶剂将竹牛皮浆升级为纤维素-醋酸盐级溶解浆

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-02 DOI: 10.1016/j.carbpol.2024.122942

Chaochao Tian , Chao Duan , Yuchen Bie , Xiaoshuang Liu , Bingxu Zhou , Ruoteng Ma , Qi Fan , Zengyin Xie , Yonghao Ni

{"title":"A deep eutectic solvent with bifunctional acid sites treatment to upgrade a bamboo kraft pulp into a cellulose-acetate grade dissolving pulp","authors":"Chaochao Tian , Chao Duan , Yuchen Bie , Xiaoshuang Liu , Bingxu Zhou , Ruoteng Ma , Qi Fan , Zengyin Xie , Yonghao Ni","doi":"10.1016/j.carbpol.2024.122942","DOIUrl":"10.1016/j.carbpol.2024.122942","url":null,"abstract":"<div><div>Valorization of non-wood pulp, such as bamboo bleached kraft pulp into high-purity cellulose acetate (CA)-grade dissolving pulp is crucial but challenging in China. Herein, a series of metal salt-based deep eutectic solvents (MSDESs) involving various ZnCl<sub>2</sub>-urea (U), ZnCl<sub>2</sub>-glycerol (G), and ZnCl<sub>2</sub>-lactic acid (LA) are comparatively investigated for this purpose. Thanks to the bifunctional acid sites of Lewis acid ZnCl<sub>2</sub> and Brønsted acid LA, the ZnCl<sub>2</sub>-LA MSDES has the highest acidity (2.62) and interaction affinity to bamboo fibers, leading to the highest efficiency in simultaneous pulp purification and activation. As a result, the resultant upgraded pulp from ZnCl<sub>2</sub>-LA (DES3-F) features remarkable improvements in purity (from 80.8 % to 93.1 %), intrinsic viscosity (from 897 to 419 mg/L), and reactivity (from 18.1 % to 80.8 %). Moreover, the modified acetate product has a high degree of substitution of 2.84 and a yield of 75.5 %. In short, such a proposed MSDES treatment can offer a promising and alternative approach for the manufacture of high-quality dissolving pulp and its derivatives.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"348 ","pages":"Article 122942"},"PeriodicalIF":10.7,"publicationDate":"2024-11-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654226","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Application of natural materials containing carbohydrate polymers in rheological modification and fluid loss control of water-based drilling fluids: A review 含碳水化合物聚合物的天然材料在水基钻井液流变改性和流体损失控制中的应用：综述

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-11-01 DOI: 10.1016/j.carbpol.2024.122928

Yu Wu , Fuchang You , Shanshan Hou

{"title":"Application of natural materials containing carbohydrate polymers in rheological modification and fluid loss control of water-based drilling fluids: A review","authors":"Yu Wu , Fuchang You , Shanshan Hou","doi":"10.1016/j.carbpol.2024.122928","DOIUrl":"10.1016/j.carbpol.2024.122928","url":null,"abstract":"<div><div>As the concept of green and sustainable development gains widespread acceptance, the demand for non-toxic, biodegradable, renewable, and widely sourced natural materials (NMs) is increasing across various fields. In oil and gas well drilling operations, water-based drilling fluids (WBDFs) are at the forefront of eco-friendly practices. Their rheological modification and fluid loss control properties are two fundamental and crucial aspects ensuring safe drilling. This review explores the research progress in enhancing these key properties of WBDFs using NMs, primarily focusing on polysaccharide polymers. It analyzes the sources, effective components, and potential functions of these NMs, and introduces three clean production methods: mechanical processing, extraction, and fermentation. Furthermore, the review focuses on the contributions of NMs obtained through these methods to the rheological and fluid loss control properties of WBDFs, highlighting their advantages and disadvantages. Despite challenges such as raw material supply stability, material synergy, compatibility, process scalability, field application, resistance to complex geological conditions, and economic feasibility, NMs, due to their outstanding environmental benefits, remain strong candidates for sustainable drilling fluid additives. Future research should focus on optimizing the performance of these materials and addressing existing issues to promote green and sustainable development in the drilling industry.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"348 ","pages":"Article 122928"},"PeriodicalIF":10.7,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654227","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Bioinspired mineralization of ultra-small ceria on cellulose nanofiber enables biocompatible and efficient nanozyme 纤维素纳米纤维上超小型铈的生物启发矿化技术实现了生物兼容的高效纳米酶

IF 10.7 1区化学

Carbohydrate Polymers Pub Date : 2024-10-31 DOI: 10.1016/j.carbpol.2024.122938

Jiahua Zhou, Dongjian Shi, Tatsuo Kaneko, Weifu Dong, Mingqing Chen

{"title":"Bioinspired mineralization of ultra-small ceria on cellulose nanofiber enables biocompatible and efficient nanozyme","authors":"Jiahua Zhou, Dongjian Shi, Tatsuo Kaneko, Weifu Dong, Mingqing Chen","doi":"10.1016/j.carbpol.2024.122938","DOIUrl":"10.1016/j.carbpol.2024.122938","url":null,"abstract":"<div><div>The escalating threat of antibiotic-resistant bacteria necessitates the exploration of alternative therapeutic strategies. Mimicking natural enzymes with artificial nanomaterials to release reactive oxygen species offers an attractive approach but is still challenged by limited catalytic activity, high production costs, and compromised biocompatibility. This work develops a bioinspired mineralization strategy for immobilizing high-density and ultra-small ceria nanoparticles onto cellulose nanofibers. The high surface-to-volume ratio of as-prepared nanoceria coupled with the aqueous processing environment facilitates the incorporation of a high Ce<sup>3+</sup> content, significantly enhancing the peroxidase-like activity. The resulting ceria nanozyme demonstrates efficient antibacterial activity with negligible cytotoxicity. The utilization of bio-based resources and a sustainable mineralization procedure allows for the cost-effective, facile preparation of eco-friendly nanozyme products under mild conditions. This study presents a promising strategy for the rational design and large-scale fabrication of high-performance and low-cost bio-based catalysts applicable to diverse targeted catalytic applications.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"348 ","pages":"Article 122938"},"PeriodicalIF":10.7,"publicationDate":"2024-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142654325","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0