ACS Photonics最新文献

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Inverse Designof the Topology–Bandwidth Trade-Offin Valley Photonic Crystals 拓扑带宽权衡谷光子晶体的反设计
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-10-05 DOI: 10.1021/acsphotonics.6c00268
Devansh Satra,Abhishek Kumar,Anshuman Kumar
{"title":"Inverse Design\u0000of the Topology–Bandwidth Trade-Off\u0000in Valley Photonic Crystals","authors":"Devansh Satra,Abhishek Kumar,Anshuman Kumar","doi":"10.1021/acsphotonics.6c00268","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c00268","url":null,"abstract":"Abstract Valley photonic crystals provide a route to broadband domain-wall guiding, but increasing the bulk gap can delocalize Berry curvature and reduce the nonquantized valley-Chern number. We introduce a mixed-integer particle-swarm framework that searches polygonal VPC unit cells and maps the Pareto trade-off between normalized bandgap and valley topology using the bulk objectiveT=(Δf/f0)2|Cv|. The selected designs are then evaluated independently using full-wave transport simulations through disorder-averaged propagation-length extraction in 200a domain-wall waveguides with positional disorder σ = 0.01a. Across the studied design ensemble, the extracted propagation length exhibits a positive empirical association with |Cv|, providing a direct multidesign connection between the patch-integrated valley-Chern number and quantified disorder-limited transport in this VPC family. The framework therefore treats bandwidth, valley topology, and device robustness as distinct but connected quantities, enabling balanced inverse design rather than optimization of a single transport metric alone.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"7 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149091324","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dual-Mode Electro-OpticModulation Based on BaTiO 3 Guided-Mode ResonancesAssisted by Spatial Filtering 空间滤波辅助下基于batio3导模共振的双模电光调制
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-10-05 DOI: 10.1021/acsphotonics.6c01544
Hongda Ren,Yixiao Zhang,Yiyang Wen,Xiaona Du,Zhenping Wu,Xu Li,Jiangbing Du,Weiwei Liu,Yang Zhang
{"title":"Dual-Mode Electro-Optic\u0000Modulation Based on BaTiO\u0000 3\u0000 Guided-Mode Resonances\u0000Assisted by Spatial Filtering","authors":"Hongda Ren,Yixiao Zhang,Yiyang Wen,Xiaona Du,Zhenping Wu,Xu Li,Jiangbing Du,Weiwei Liu,Yang Zhang","doi":"10.1021/acsphotonics.6c01544","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c01544","url":null,"abstract":"Abstract Liquid crystal spatial light modulators suffer from slow response, while conventional electro-optic (EO) thin-film devices exhibit limited modulation depth, hindering high-speed programmable optical systems. Here, we numerically propose a dual-mode EO spatial modulation scheme enabled by barium titanate guided-mode resonance (BaTiO3-GMR) combined with spatial filtering. A SiN photonic crystal structure integrated with a continuous BaTiO3 thin film uses GMR to convert weak electrically induced refractive index perturbations into pronounced complex reflection changes. To overcome the intrinsic amplitude-phase (AP) coupling of single resonant pixels, a two-pixel coherent field synthesis strategy expands the accessible complex field state space, enabling programmable joint AP encoding. Amplitude-type and phase-type trajectories are then selected as two representative constrained modes via 4f spatial-filtering readout. The numerical model yields a broad range near amplitude-only modulation (0 to 0.668) and phase modulation exceeding 2.443 rad. Simulations using MNIST handwritten digits further evaluate 2D amplitude and phase pattern reconstruction. These results establish a simulation-based proof of concept for dual-mode amplitude and phase modulation and provide a numerical basis for future development of programmable optical modulation systems.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"484 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149091326","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Single-ObjectiveLight-Sheet Microscopy Allows Long-Term,High-Resolution In Vivo Brain Imaging of Drosophila 单物镜薄层显微镜允许长期,高分辨率的果蝇体内脑成像
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-10-05 DOI: 10.1021/acsphotonics.6c01278
Francisco J. Tassara,Mariano Barella,Tomás Sebastián Fernández Troncoso,Lourdes Simó,M. Mailén Folgueira Serrao,Micaela Rodriguez-Caron,Juan Ignacio Ispizua,Mark H. Ellisman,Horacio O. de la Iglesia,M. Fernanda Ceriani,Julián Gargiulo
{"title":"Single-Objective\u0000Light-Sheet Microscopy Allows Long-Term,\u0000High-Resolution\u0000 In Vivo\u0000 Brain Imaging of\u0000 Drosophila","authors":"Francisco J. Tassara,Mariano Barella,Tomás Sebastián Fernández Troncoso,Lourdes Simó,M. Mailén Folgueira Serrao,Micaela Rodriguez-Caron,Juan Ignacio Ispizua,Mark H. Ellisman,Horacio O. de la Iglesia,M. Fernanda Ceriani,Julián Gargiulo","doi":"10.1021/acsphotonics.6c01278","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c01278","url":null,"abstract":"Abstract In vivo imaging of dynamic subcellular brain structures is key to understanding several phenomena in neuroscience. However, in the fruit fly, its implementation has been hindered by a trade-off among spatial resolution, speed, photobleaching, phototoxicity, and setup complexity required to access specific target regions of the small brain of Drosophila. Here, we present DrosoScope: a single-objective light-sheet microscope customized for in vivo imaging of adult flies and optimized for maximum resolution. With it, we imaged the axonal projections of small lateral ventral neurons (s-LNvs) in intact adult flies. We imaged the plasma membrane, cytoplasm, mitochondria, and dense-core vesicles with high spatial resolution of up to 310 nm, lower photobleaching than confocal microscopy, lower invasiveness and reduced sample-mounting complexity than alternative light-sheet technologies, and without relying on potentially phototoxic pulsed infrared lasers. Furthermore, we implemented active focus stabilization and sample-drift correction. Combined, these features enabled time-lapse brain imaging in living flies for up to 5 h, revealing neuronal plasticity and dynamic mitochondrial transport.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"54 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149092349","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Few-Layer GrapheneHeater Enabled High-Precision Phase-ChangePhotonic Devices 少层石墨烯加热器实现的高精度相变光子器件
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-10-05 DOI: 10.1021/acsphotonics.6c00755
Bing Song,Ganlin Xiong,Zhiyu Guo,Yuan Tian,MengJian Zhu,Hengyu Zhang,Xuan Li
{"title":"Few-Layer Graphene\u0000Heater Enabled High-Precision Phase-Change\u0000Photonic Devices","authors":"Bing Song,Ganlin Xiong,Zhiyu Guo,Yuan Tian,MengJian Zhu,Hengyu Zhang,Xuan Li","doi":"10.1021/acsphotonics.6c00755","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c00755","url":null,"abstract":"Abstract Photonic computing overcomes the power and interconnect bottlenecks of conventional electronics through its high bandwidth, low latency, and parallel processing capability, making it ideal for next-generation AI and data-intensive applications. However, current photonic computing devices still face challenges in modulation efficiency, precision, and state retention. Here, we demonstrate a few-layer graphene (FLG) heater enabled high precision nonvolatile photonic device based on Sb2Se3 phase-change material. By investigating the modulation mechanism of the FLG heater, we achieve precise control over the phase-change photonic device. Combined with a strip-segmented device structure, 101 highly uniform and distinct optical states are realized. Benefiting from the more efficient modulation of phase-change photonic devices by the FLG heater, a total phase shift of 4.5π is achieved over a 30 μm length of Sb2Se3, corresponding to a phase modulation efficiency of 0.15π/μm. This work provides a feasible solution to achieve high precision and high phase modulation efficiency in photonic devices, lays a foundation for more accurate and highly integrated photonic computing systems.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"55 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149091267","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nonlocal ReflectarrayMetasurfaces with High-EfficiencySpin-Dependent Deflection 具有高效自旋相关偏转的非局部反射元表面
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-10-02 DOI: 10.1021/acsphotonics.6c00612
Chandra Shakya,Kaleem Ullah,Adam Overvig
{"title":"Nonlocal Reflectarray\u0000Metasurfaces with High-Efficiency\u0000Spin-Dependent Deflection","authors":"Chandra Shakya,Kaleem Ullah,Adam Overvig","doi":"10.1021/acsphotonics.6c00612","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c00612","url":null,"abstract":"Abstract We report a nonlocal reflectarray metasurface that resolves a trade-off between efficiency and spectral selectivity in nonlocal flat optics. Local reflectarrays achieve high reflection efficiency but lack spectral control, while nonlocal metasurfaces support high-Q quasi–bound states in the continuum (q-BICs) with tailorable narrowband responses but suffer from an intrinsic 25% efficiency limit. By combining nonlocal resonances with a mirror-backed cavity, our design achieves narrowband, spin-dependent beam steering with efficiencies above 93% and tailorable resonant frequency, Q-factor, and deflection direction. We demonstrate with coupled mode theory that, by leveraging a self-coupling mechanism of the resonant metasurface through the reflection of the mirror, we achieve control over the amplitude and phase of reflected light at a fixed frequency. We extend these results to show nonlocal metalenses with resonant-exclusive and spin-dependent focusing. These results position hybrid nonlocal reflectarray metasurfaces as a multifunctional platform for efficient, spin-multiplexed imaging, secure optical communication, and quantum photonics.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"7 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-10-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149091325","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Sub-PoissonianElectroluminescence from Resonant InelasticTunneling in One-Dimensional Gold Atomic Chains 一维金原子链共振非弹性隧穿的亚泊松电致发光
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-10-02 DOI: 10.1021/acsphotonics.6c01563
Hongyi Yang,Haipeng Zhu,Shiyu Feng,Zexi Lu,Xiyao Peng,Hongsheng Chen,Sihan Zhao,Dexin Ye,Haoliang Qian
{"title":"Sub-Poissonian\u0000Electroluminescence from Resonant Inelastic\u0000Tunneling in One-Dimensional Gold Atomic Chains","authors":"Hongyi Yang,Haipeng Zhu,Shiyu Feng,Zexi Lu,Xiyao Peng,Hongsheng Chen,Sihan Zhao,Dexin Ye,Haoliang Qian","doi":"10.1021/acsphotonics.6c01563","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c01563","url":null,"abstract":"Abstract Electrically driven single-photon sources are central to integrated quantum photonics, but Poissonian carrier injection usually transfers electrical shot noise into classical photon statistics. Here we propose to suppress this bottleneck at its origin by using a one-dimensional (1D) gold atomic chain as an atomic-scale quantum conductor. Density-functional-theory-parameterized nonequilibrium Green’s function calculations show that resonant tunneling through a dz2-dominated ballistic channel suppresses electronic partition noise and generates a sub-Poissonian current. The same 1D spectrum, through discrete molecular levels and van Hove singularities, suppresses elastic tunneling while opening a resonant inelastic channel, yielding an intrinsic plasmon-excitation efficiency ηinel of about 80%. Coupling this quiet, high-yield electron flow to a nanometer-scale plasmonic antenna enables antibunched electroluminescence with a projected external photon-generation efficiency ηEQE ≈ 60% and a high photon purity (g(2)(0) ≈ 0). These results identify quantum-statistical engineering of electron transport as a route to electrically driven nonclassical light at the atomic limit.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"165 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-10-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149091327","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Electron Modulationand Ultrafast Near-Field Imagingwith Vectorial Laser Fields 矢量激光场的电子调制和超快近场成像
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-10-01 DOI: 10.1021/acsphotonics.6c01451
J. Kuttruff,L. Möhrle,L. Ciorciaro,L. Schmidt-Mende,P. Baum
{"title":"Electron Modulation\u0000and Ultrafast Near-Field Imaging\u0000with Vectorial Laser Fields","authors":"J. Kuttruff,L. Möhrle,L. Ciorciaro,L. Schmidt-Mende,P. Baum","doi":"10.1021/acsphotonics.6c01451","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c01451","url":null,"abstract":"Abstract Controlled interaction of laser light with electron beams is fundamental for ultrafast electron microscopy and electron-based quantum optics, yet their direct coupling is forbidden in free space. Here, we use longitudinally polarized light on a thin membrane and show that the emerging focal fields can modulate the electron beam in a direct, coherent, and linear way, without the need for nanostructured materials or slanted interaction geometries. Also, we use vectorial polarizations to excite and probe three-dimensional nanophotonic near fields in metallic mesocrystals by coherent electron energy gain and loss. We find that longitudinal electric fields excite axial near fields in a direct way, while longitudinal magnetic fields excite oscillating ring currents via azimuthal electric fields. These possibilities enable the tilt-free, collinear generation of attosecond electron pulses or free-electron qubits and provide novel imaging modes in ultrafast electron microscopy and metamaterial tomography.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"6 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149091044","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Excitation-Energy-DependentEnhancement of Hot-CarrierLifetimes in Graphene 石墨烯中热载子寿命的激发能依赖性增强
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-10-01 DOI: 10.1021/acsphotonics.6c01679
Sachin Sharma,Elliott Walker,Rachael Myers-Ward,Jenifer Hajzus,Yijing Liu,Paola Barbara,Ioannis Chatzakis
{"title":"Excitation-Energy-Dependent\u0000Enhancement of Hot-Carrier\u0000Lifetimes in Graphene","authors":"Sachin Sharma,Elliott Walker,Rachael Myers-Ward,Jenifer Hajzus,Yijing Liu,Paola Barbara,Ioannis Chatzakis","doi":"10.1021/acsphotonics.6c01679","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c01679","url":null,"abstract":"Abstract Understanding hot-carrier relaxation in graphene is important for ultrafast optoelectronic and terahertz technologies. Here, we investigate carrier cooling dynamics in mono- and bilayer graphene using mid-infrared pump pulses (0.22 to 0.73 eV) and terahertz probe pulses. We uncover a pronounced, reproducible, and nonmonotonic dependence of the carrier relaxation time on excitation photon energy. Within a narrow spectral window from 0.42 to 0.48 eV, the carrier lifetime increases by nearly an order of magnitude compared to the few-picosecond cooling observed at lower and higher excitation energies. The observed excitation-energy dependence is consistent with a hot-phonon bottleneck scenario in which the accumulation and reabsorption of nonequilibrium optical phonons suppress the energy transfer to the lattice. A phenomenological coupled carrier–phonon model supports this interpretation. These findings reveal a previously unreported excitation-energy dependence of hot-carrier cooling in graphene and provide new insight into nonequilibrium carrier–phonon interactions near the optical-phonon bottleneck.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"20 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149091045","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inkjet-PrintedMoS2 D-Shaped Fiberfor Resonance-Enhanced Optical Sensing 用于共振增强光传感的喷墨打印mos2 d形光纤
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-09-30 DOI: 10.1021/acsphotonics.6c01158
Amar N. Ghosh,Mingfei Xiao,Jinrui Chen,Victor Pacheco-Peña,Meng Huang,Noel Healy,Tawfique Hasan,Anna C. Peacock
{"title":"Inkjet-Printed\u0000MoS2 D-Shaped Fiber\u0000for Resonance-Enhanced Optical Sensing","authors":"Amar N. Ghosh,Mingfei Xiao,Jinrui Chen,Victor Pacheco-Peña,Meng Huang,Noel Healy,Tawfique Hasan,Anna C. Peacock","doi":"10.1021/acsphotonics.6c01158","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c01158","url":null,"abstract":"Abstract Two-dimensional (2D) materials have shown great potential for applications in environmental monitoring and sensing due to their unique physical and chemical properties. In particular, molybdenum disulfide (MoS2) has emerged as a versatile 2D material platform for many optical and optoelectronic applications due to its high refractive index, large surface-to-volume ratio, and tunable bandgap. In this work, the integration of MoS2 layers on a side-polished optical fiber with a D-shaped cross-section has been demonstrated using a low-cost and scalable inkjet printing technique. The MoS2-integrated optical fibers are shown to offer strong wavelength-dependent light-matter interactions that can be controlled by the thickness of the 2D material, allowing for tuning of their operation across the entire telecom band. Using a printed device with a MoS2 layer thickness of 30 nm, designed to exhibit a resonance-enhanced transmission dip at wavelengths of ∼1.50 μm, a refractive index sensor has been demonstrated using saline solutions. The experimental results have been verified via numerical simulations, confirming the sensitivity and flexibility offered by the 2D material structures. These results indicate that inkjet-printed MoS2 optical fiber devices are suitable for the development of large-scale sensing networks.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"42 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149090744","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Long Range Coherent Valley Pseudospin Transport viaBloch Surface Wave Polaritons in Monolayer Transition Metal Dichalcogenides 单层过渡金属二硫族化合物表面波极化子的长距离相干谷伪自旋输运
IF 7 1区 物理与天体物理
ACS Photonics Pub Date : 2026-09-30 DOI: 10.1021/acsphotonics.6c00182
Zhengyang Lyu,Haonan Zhao,Bin Liu,Claire E. Arneson,Lingxiao Zhou,Chenxi Liu,Yuhan Zhang,Stephen R. Forrest,Parag B. Deotare
{"title":"Long Range Coherent Valley Pseudospin Transport via\u0000Bloch Surface Wave Polaritons in Monolayer Transition Metal Dichalcogenides","authors":"Zhengyang Lyu,Haonan Zhao,Bin Liu,Claire E. Arneson,Lingxiao Zhou,Chenxi Liu,Yuhan Zhang,Stephen R. Forrest,Parag B. Deotare","doi":"10.1021/acsphotonics.6c00182","DOIUrl":"https://doi.org/10.1021/acsphotonics.6c00182","url":null,"abstract":"Abstract The feasibility of low-dimensional transition metal dichalcogenides (TMDs) as a platform for valleytronics relies on the ability to control the dynamics of the valley pseudospins. Here, we present long-range coherent valley pseudospin transport assisted by Bloch surface wave exciton-polaritons (BSWPs). We resolve the BSWP transport in exfoliated WS2 over distances exceeding 10 μm in both spatial and polarization spaces via momentum-selected circular dichroism spectroscopy at cryogenic temperatures. We show that the trajectories on the Poincaré sphere reflect hybrid light–matter polarization dynamics. Furthermore, we show that the BSWP transport can be optically or magnetically controlled through the photonic or the excitonic component. Our work demonstrates the ability to coherently transport valley pseudospin information over long distances and establishes the feasibility of an all-axis controllable quantum system in the spatial, spectral, momentum, and polarization domains.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"41 1","pages":""},"PeriodicalIF":7.0,"publicationDate":"2026-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149090746","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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