ACS Omega最新文献

{"title":"Kombucha–Proteinoid Crystal Bioelectric Circuits","authors":"Panagiotis Mougkogiannis*,&nbsp;Anna Nikolaidou and Andrew Adamatzky,&nbsp;","doi":"10.1021/acsomega.4c0731910.1021/acsomega.4c07319","DOIUrl":"https://doi.org/10.1021/acsomega.4c07319https://doi.org/10.1021/acsomega.4c07319","url":null,"abstract":"<p >We propose “kombucha–proteinoid crystal bioelectric circuits” as a sustainable bio-computing platform. These circuits are hybrid biological-inorganic devices that utilize crystal growth dynamics as the physical substrate to convert information. Microfluidic prototypes couple custom-synthesized thermal proteinoids within kombucha cellulose matrices and metastable calcium carbonate solutions. This bio-mineral configuration examines if precision modulation of crystal growth rates could instantiate reconfigurable logic gates for unconventional computing applications. Programming organic acid secretions allows for the adjustment of biotic-mineral polarity, thereby establishing microbial-synthetic pairings that consistently regulate the crystal growth rate of calcite deposition. By coordinating intrinsic physicochemical phenomena, accrued mineral densities literally crystallize additive/multiplicative operations via Boolean AND/OR logics. An additional way to generate structured logics similar of neural assemblies is by chaining modular crystallizer units. Proteinoid-guided carbonate crystallization may prove to be a viable material platform for unconventional computing-green, self-organizing, scalable architectures grown directly from solution-pending definitive affirmation of proof-of-concept.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c07319","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142609255","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Role of the Polymer in the Emulsion Stability of an Amphoteric Polyacrylamide in Different Flooding Systems","authors":"Jin Huang,&nbsp;Xinxin Xia,&nbsp;Huai Jiang,&nbsp;Yanjia Huo,&nbsp;Jinling Li,&nbsp;Wei Li,&nbsp;Xiaorong Ma,&nbsp;Feng Li and Cuiqin Li*,&nbsp;","doi":"10.1021/acsomega.4c0323610.1021/acsomega.4c03236","DOIUrl":"https://doi.org/10.1021/acsomega.4c03236https://doi.org/10.1021/acsomega.4c03236","url":null,"abstract":"<p >Polymers with high viscosity and good viscosity–temperature property have attracted attention as chemical agents for enhanced oil recovery. The role of polymers in the emulsifying stability of an amphoteric polyacrylamide (TSPAM) with good viscosity–temperature property in different flooding systems was investigated by means of a new emulsion stability model and molecular simulations. The results indicated that TSPAM exhibited superior emulsion stability compared to hydrolyzed polyacrylamide (HPAM). The half-life of emulsions containing TSPAM was 1–7 min longer than that of emulsions containing HPAM. The results of molecular simulation revealed that the HPAM molecules adsorbed at the oil–water interface in a “point adsorption” mode, whereas the TSPAM molecules adsorbed in a “surface adsorption” mode, resulting in higher interfacial adsorption efficiency and more stable interfacial film. The polymer flooding systems containing TSPAM showed a larger interfacial thickness of 1.029 nm and higher emulsification efficiency compared to the polymer flooding systems containing HPAM. The addition of Na₂CO₃ or surfactants further improved the stability of emulsions in the binary systems containing TSPAM. The stability of emulsions containing all three oil displacement agents was the strongest, with the half-life extended by 3.8–13.6 min. Amphoteric polyacrylamide significantly enhanced the stability of the emulsions. Through the integration of experimental and molecular simulation techniques, the molecular structure of polyacrylamide can be optimized, facilitating the development of more efficient oil recovery formulations for enhanced oil recovery applications.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c03236","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577712","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Transparent X-ray Shielding Solutions with Various Metal Ions","authors":"Ryoma Tokonami,&nbsp;Minoru Osanai,&nbsp;Masahiro Hosoda,&nbsp;Shinji Tokonami and Tatsuhiro Takahashi*,&nbsp;","doi":"10.1021/acsomega.4c0790410.1021/acsomega.4c07904","DOIUrl":"https://doi.org/10.1021/acsomega.4c07904https://doi.org/10.1021/acsomega.4c07904","url":null,"abstract":"<p >We fabricated transparent, Pb-free X-ray shielding materials using solvated ions in a polar solvent. Previous materials have been based on dispersions of metal-containing particles such as barium sulfate (BaSO₄) in a matrix. Comparisons of suspensions of metal-based particles and solutions of metal ions in a solvent enable better understanding of interactions such as reflection, scattering, and absorption between X-rays and substances. The X-ray shielding properties of a solution of solvated metal ions were similar to or better than those of suspensions of metal-containing particles. In addition, the metal-ion solutions exhibited high transparency. The most effective material among those investigated for X-ray shielding was barium bromide (BaBr₂), which exhibits high solubility in polar solvents. X-ray shielding of 92% was confirmed at a tube voltage of 120 kV, along with ∼90% UV transmittance at a visible-light wavelength of 400 nm. Thus, both high X-ray shielding performance and high transparency were achieved.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c07904","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577701","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A Comprehensive Review of Multifunctional Proppants","authors":"Guang Wang,&nbsp;Qinyue Ma,&nbsp;Longqiang Ren and Jirui Hou*,&nbsp;","doi":"10.1021/acsomega.4c0694110.1021/acsomega.4c06941","DOIUrl":"https://doi.org/10.1021/acsomega.4c06941https://doi.org/10.1021/acsomega.4c06941","url":null,"abstract":"<p >Hydraulic fracturing technology is a crucial method for enhancing the production and recovery rates of unconventional oil and gas wells. In this process, proppants, as key materials, directly influence the effectiveness of the fracturing operation, thus attracting widespread attention. With the continuous development of hydraulic fracturing technology, researchers have designed and prepared a series of multifunctional proppants, such as surface-modified proppants, self-suspending proppants, and slow-release proppants, to effectively address issues like water production, sand production, and scaling in reservoirs. This paper aims to systematically review the research progress on multifunctional proppants, analyze their application potential in fracturing operations, and forecast the development direction of proppants. It is hoped that this review will provide valuable references for researchers and promote the further development of proppant-related technologies in hydraulic fracturing.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c06941","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577624","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Structural and Solution Speciation Studies on fac-Tricarbonylrhenium(I) Complexes of 2,2′-Bipyridine Analogues","authors":"Tamás Pivarcsik,&nbsp;Jakob Kljun,&nbsp;Sergio Clemente Rodriguez,&nbsp;David Cortéz Alcaraz,&nbsp;Uroš Rapuš,&nbsp;Márta Nové,&nbsp;Egon F Várkonyi,&nbsp;József Nyári,&nbsp;Anita Bogdanov,&nbsp;Gabriella Spengler,&nbsp;Iztok Turel* and Éva A. Enyedy*,&nbsp;","doi":"10.1021/acsomega.4c0711710.1021/acsomega.4c07117","DOIUrl":"https://doi.org/10.1021/acsomega.4c07117https://doi.org/10.1021/acsomega.4c07117","url":null,"abstract":"<p >In this study, we report the synthesis and characterization of 12 novel rhenium(I) complexes with the general formula <i>fac</i>-[Re(CO)₃(NN)X]ⁿ⁺ where (NN) is a 2,2′-bipyridine analogue ligand, X = Cl^–, Br^–, or H₂O, and <i>n</i> = 0 or 1, focusing on their speciation in an aqueous solution. The prepared organorhenium complexes are stable in a wide pH range in an aqueous solution, and no release of the bidentate ligands or the carbonyl ligands was observed. The stability of the complexes in various biologically relevant matrices (cell culture medium and real blood serum) was also demonstrated. However, the simultaneous substitution of the halido ligand by water and slow hydrolysis of the ester bonds in the ligands were observed, affecting both the solubility and the lipophilicity of the compounds. The aqua complexes became more lipophilic in the presence of chloride ions, while the hydrophilicity increased significantly with time due to the hydrolysis of the ester bonds, which probably contributed to their weak pharmacological activity. The results also showed kinetically hindered aqueous solvation of the halido complexes and low chloride ion affinity of the aqua complexes. The deprotonation of the coordinated aqua ligand in the complexes occurs in the pH = 7–10 range, leading to significant formation (18–30%) of hydroxido species at pH = 7.4. The halido complexes showed somewhat higher cytotoxicity (IC₅₀ = 60–99 μM) on human colon adenocarcinoma cancer cells (Colo205 and Colo320) than the corresponding aqua complexes (IC₅₀ &gt; 100 μM). In all cases, no antibacterial effect was observed (MIC &gt; 100 μM), but some of the complexes showed moderate antiviral activity (IC₅₀ ∼ 50 μM) on Herpes simplex virus 2.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c07117","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577625","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Eco-Friendly Jute-Based Hybrid Nonwoven Fabric for Packaging Applications","authors":"Md. Abdus Shahid*,&nbsp;Md. Ahasan Habib,&nbsp;Imam Hossain,&nbsp;Md. Golam Mortuza Limon,&nbsp;Tarikul Islam* and Gajanan Bhat,&nbsp;","doi":"10.1021/acsomega.4c0725510.1021/acsomega.4c07255","DOIUrl":"https://doi.org/10.1021/acsomega.4c07255https://doi.org/10.1021/acsomega.4c07255","url":null,"abstract":"<p >Eco-friendly materials must replace pure synthetic materials to protect the environment and improve human welfare. This study uses a blow room-integrated carding machine to create a filmy web by properly mixing modified jute and polyester fibers. Jute-polyester fiber blended carded webs have been utilized to produce jute-based hybrid nonwoven fabrics (JHNFs), which are subsequently given an antibacterial treatment by spraying a solution of silver nitrate, ethanol, and ammonia. The performance of the developed JHNF is evaluated by its morphological, FTIR, antibacterial, mechanical, and thermal properties. The fiber distribution of jute and polyester fibers is shown in SEM micrographs. The JHNF showed 29 and 27.8 mm ZOI against <i>Staphylococcus aureus</i> bacteria and <i>Escherichia coli</i>, respectively. The developed sample exhibited a 2.3% extension at the break and 170.8 N of breaking force. The sample confirmed itself as a water-repellent material as water could not penetrate from one surface to another when it was tested by a moisture management tester. The thermal conductivity of the produced sample was measured at 0.0839 W/m K. The lower thermal conductivity signifies a good thermally insulative packaging material. The developed jute polyester nonwoven fabric also demonstrated higher radiative heat resistance, providing a thermal barrier of 22 °C. The porosity, thickness, and density were determined at 49.59%, 0.22 mm, and 0.40 g/cm³, respectively. The sample exhibited significant thermal stability, with polymer degradation initiating at temperatures above 280 °C. The developed nonwoven fabric proves its practical utility as a packaging material, offering a viable alternative to pure synthetic packaging materials.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c07255","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577504","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A Convenient Route to Large-Scale Chemical Synthesis of p-Hydroxyphenylacetaldehyde Oxime and Its p-β-d-Glucopyranoside: Key Intermediates and Products in Plant Specialized Metabolism","authors":"Birger Lindberg Møller,&nbsp;Carl Erik Olsen,&nbsp;Yong Zhao and Mohammed Saddik Motawie*,&nbsp;","doi":"10.1021/acsomega.4c0501410.1021/acsomega.4c05014","DOIUrl":"https://doi.org/10.1021/acsomega.4c05014https://doi.org/10.1021/acsomega.4c05014","url":null,"abstract":"<p >Oximes are unrecognized chameleons in general and specialized plant metabolism. <i>E-</i> and <i>Z-p</i>-hydroxyphenylacetaldehyde oxime are key intermediates in the biosynthesis of the cyanogenic glucoside dhurrin produced in sorghum. Nevertheless, none of the geometrical oxime isomers accumulate in the plant. Herein, we report a convenient route to the chemical synthesis of <i>E-</i> and <i>Z-p</i>-hydroxyphenylacetaldehyde oxime and its biologically produced <i>p</i>-β-<span>d</span>-glucopyranoside using <i>p</i>-hydroxyphenylacetic acid as a starting material. This starting material is also available in radiolabeled forms. All reaction steps proceeded with excellent yield under mild conditions, operational facility, and scalability.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c05014","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577610","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Pressure Analysis of Vertical-Wells with the Hydraulic Fracturing Assisted Water Injection in Low-Permeability Hydrogen and Carbon Reservoirs","authors":"Zhaodong Yu,&nbsp;Shuangxi Liu,&nbsp;Jun Tang,&nbsp;Baohua Zhu,&nbsp;Shuangping Dong,&nbsp;Jianshen Du and Zhongwei Wu*,&nbsp;","doi":"10.1021/acsomega.4c0655510.1021/acsomega.4c06555","DOIUrl":"https://doi.org/10.1021/acsomega.4c06555https://doi.org/10.1021/acsomega.4c06555","url":null,"abstract":"<p >Enhancing the energy of hydrogen and carbon reservoirs is crucial for the extraction of these resources. Currently, the conventional water-flooding technology faces challenges in replenishing the energy of hydrogen and carbon reservoirs due to the low injection rates caused by their low-permeability properties. To address this, hydraulic fracturing-assisted water injection technology has been employed to enhance the energy of these reservoirs. However, there has been a lack of research on pressure analysis for vertical wells using this technology. Existing studies on pressure analysis are not applicable to this scenario due to the unique behavior of dynamic fracture propagation. In this article, we present a pressure analysis model for vertical wells with hydraulic fracturing-assisted water injection in low-permeability hydrogen and carbon reservoirs, considering dynamic fracture propagation. The model examines the effects of key parameters on the pressure and fluid flow fronts, and it is applied to field wells for validation. Our findings include the following: the typical pressure response curve for vertical wells with hydraulic fracturing-assisted water injection in low-permeability hydrogen and carbon reservoirs can be divided into six stages: dynamic fracture propagation region, linear flow region in hydrogen and carbon reservoirs, bilinear flow region, radial flow region, transition flow region, and boundary control flow region. The production rate affects the pressure and pressure derivatives in the later stages of the process. However, reservoir permeability influences all flow regions, causing the pressure and pressure derivative curves to shift left with increasing permeability. Increases in both the injection rate and production rate result in a rise in the position of fluid fronts. The impact of permeability on fluid fronts is more significant in the early stages than in later stages. This work is of great significance for the development of low-permeability hydrogen and carbon reservoirs, providing a deeper understanding of the pressure dynamics involved in hydraulic fracturing-assisted water injection.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c06555","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577634","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A Systematic Review of the Contribution of Additive Manufacturing toward Orthopedic Applications","authors":"Alphonsa Joseph,&nbsp; and ,&nbsp;Vijayalakshmi Uthirapathy*,&nbsp;","doi":"10.1021/acsomega.4c0487010.1021/acsomega.4c04870","DOIUrl":"https://doi.org/10.1021/acsomega.4c04870https://doi.org/10.1021/acsomega.4c04870","url":null,"abstract":"<p >Human bone holds an inherent capacity for repairing itself from trauma and damage, but concerning the severity of the defect, the choice of implant placement is a must. Additive manufacturing has become an elite option due to its various specifications such as patient-specific custom development of implants and its easy fabrication rather than the conventional methods used over the years. Additive manufacturing allows customization of the pore size, porosity, various mechanical properties, and complex structure design and formulation. Selective laser melting, powder bed fusion, electron beam melting, and fused deposition modeling are the various AM methods used extensively for implant fabrication. Metals, polymers, biocrystals, composites, and bio-HEA materials are used for implant fabrication for various applications. A wide variety of polymer implants are fabricated using additive manufacturing for nonload-bearing applications, and β-tricalcium phosphate, hydroxyapatite, bioactive glass, etc. are mainly used as ceramic materials in additive manufacturing due to the biological properties that could be imparted by the latter. For decades metals have played a major role in implant fabrication, and additive manufacturing of metals provides an easy approach to implant fabrication with augmented qualities. Various challenges and setbacks faced in the fabrication need postprocessing such as sintering, coating, surface polishing, etc. The emergence of bio-HEA materials, printing of shape memory implants, and five-dimensional printing are the trends of the era in additive manufacturing.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c04870","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577694","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Targeting the Plasmodium falciparum IspE Enzyme","authors":"Eleonora Diamanti,&nbsp;Annina M. Steinbach,&nbsp;Lais P. de Carvalho,&nbsp;Henni-Karoliina Ropponen,&nbsp;Antoine Lacour,&nbsp;Rawia Hamid,&nbsp;Sidra Eisa,&nbsp;Patricia Bravo,&nbsp;Spyridon Bousis,&nbsp;Boris Illarionov,&nbsp;Markus Fischer,&nbsp;Mostafa M. Hamed,&nbsp;Nina C. Bach,&nbsp;Matthias Rottmann,&nbsp;Jana Held,&nbsp;Matthias Witschel,&nbsp;Stephan A. Sieber and Anna K. H. Hirsch*,&nbsp;","doi":"10.1021/acsomega.4c0603810.1021/acsomega.4c06038","DOIUrl":"https://doi.org/10.1021/acsomega.4c06038https://doi.org/10.1021/acsomega.4c06038","url":null,"abstract":"<p >The enzyme IspE in <i>Plasmodium falciparum</i> is considered an attractive drug target, as it is essential for parasite survival and is absent in the human proteome. Yet it still has not been addressed by a small-molecule inhibitor. In this study, we conducted a high-throughput screening campaign against the <i>Pf</i>IspE enzyme. Our approach toward a <i>Pf</i>IspE inhibitor comprises <i>in vitro</i> screening, structure–activity relationship studies, examining the docking position using an AlphaFold model, and finally target verification through probe binding and sodium dodecyl sulfate-polyacrylamide gel electrophoresis (SDS-PAGE) analysis. The newly synthesized probe containing a diazirine and an alkyne moiety (<b>23</b>) allowed us to demonstrate its binding to IspE in the presence of a lysate of human cells (HEK293 cells) and to get evidence that both probe <b>23</b> and the best inhibitor of the series (<b>19</b>) compete for the same IspE binding site.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":null,"pages":null},"PeriodicalIF":3.7,"publicationDate":"2024-10-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsomega.4c06038","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142577682","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}