V. Oliviero, I. Gilmutdinov, D. Vignolles, S. Benhabib, N. Bruyant, A. Forget, D. Colson, W. A. Atkinson, C. Proust
{"title":"Charge order near the antiferromagnetic quantum critical point in the trilayer high Tc cuprate HgBa2Ca2Cu3O8+δ","authors":"V. Oliviero, I. Gilmutdinov, D. Vignolles, S. Benhabib, N. Bruyant, A. Forget, D. Colson, W. A. Atkinson, C. Proust","doi":"10.1038/s41535-024-00688-6","DOIUrl":"https://doi.org/10.1038/s41535-024-00688-6","url":null,"abstract":"<p>We study the transport properties of underdoped trilayer cuprate HgBa<sub>2</sub>Ca<sub>2</sub>Cu<sub>3</sub>O<sub>8+<i>δ</i></sub> with doping level <i>p</i> = 0.10–0.12 in magnetic field up to 88 T. We report for the first time in a cuprate superconductor a dramatic change of the quantum oscillation spectrum versus temperature, which is accompanied by a sign change of the Hall effect below <i>T</i> ≈10 K. Based on numerical simulations, we infer a Fermi surface reconstruction in the inner plane from an antiferromagnetic state (hole pockets) to a biaxial charge density wave state (electron pockets). We show that both orders compete and share the same hotspots of the Fermi surface, and we discuss our result in the context of spin-fermion models.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-10-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142374121","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Interorbital antisymmetric hopping generated flat bands on kagome and pyrochlore Lattices","authors":"Keyu Zeng, Ziqiang Wang","doi":"10.1038/s41535-024-00685-9","DOIUrl":"https://doi.org/10.1038/s41535-024-00685-9","url":null,"abstract":"<p>Flat bands are intriguing platforms for correlated and topological physics. Various methods have been developed to create flat bands utilizing lattice geometry, but the investigation of orbital symmetry in multiorbital materials is a new area of focus. Here, we introduce a site symmetry-based approach to emerging multiorbital 2D and 3D flat bands on the kagome and pyrochlore lattices. As a conceptual advance, the one-orbital flat bands are shown to originate as mutual eigenstates of isolated molecular motifs. Further developing the mutual eigenstate method for multiple orbitals transforming differently under the site symmetries, we derive interorbital hopping generated flat bands from the antisymmetric interorbital Hamiltonian and introduce group-theoretic descriptions of the flat band wavefunctions. Realizations of multiorbital flat bands in realistic materials are shown to be possible in the Slater-Koster formalism. Our findings provide new directions for exploring flat-band electronic structures for novel correlated and topological quantum states.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142330329","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pascal Reiss, Alix McCollam, Zachary Zajicek, Amir A. Haghighirad, Amalia I. Coldea
{"title":"Collapse of metallicity and high-Tc superconductivity in the high-pressure phase of FeSe0.89S0.11","authors":"Pascal Reiss, Alix McCollam, Zachary Zajicek, Amir A. Haghighirad, Amalia I. Coldea","doi":"10.1038/s41535-024-00677-9","DOIUrl":"https://doi.org/10.1038/s41535-024-00677-9","url":null,"abstract":"<p>We investigate the high-pressure phase of the iron-based superconductor FeSe<sub>0.89</sub>S<sub>0.11</sub> using transport and tunnel diode oscillator studies using diamond anvil cells. We construct detailed pressure-temperature phase diagrams that indicate that the superconducting critical temperature is strongly enhanced by more than a factor of four towards 40 K above 4 GPa. The resistivity data reveal signatures of a fan-like structure of non-Fermi liquid behaviour which could indicate the existence of a putative quantum critical point buried underneath the superconducting dome around 4.3 GPa. With further increasing the pressure, the zero-field electrical resistivity develops a non-metallic temperature dependence and the superconducting transition broadens significantly. Eventually, the system fails to reach a fully zero-resistance state, and the finite resistance at low temperatures becomes strongly current-dependent. Our results suggest that the high-pressure, high-<i>T</i><sub>c</sub> phase of iron chalcogenides is very fragile and sensitive to uniaxial effects of the pressure medium, cell design and sample thickness. This high-pressure region could be understood assuming a real-space phase separation caused by nearly concomitant electronic and structural instabilities.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142330328","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Y. Alexanian, J. Saugnier, C. Decorse, J. Robert, R. Ballou, E. Lhotel, J. Debray, F. Gay, V. Simonet, S. de Brion
{"title":"Exploring possible magnetic monopoles-induced magneto-electricity in spin ices","authors":"Y. Alexanian, J. Saugnier, C. Decorse, J. Robert, R. Ballou, E. Lhotel, J. Debray, F. Gay, V. Simonet, S. de Brion","doi":"10.1038/s41535-024-00676-w","DOIUrl":"https://doi.org/10.1038/s41535-024-00676-w","url":null,"abstract":"<p>The possibilities of combining several degrees of freedom inside a unique material have recently been highlighted in their dynamics and proposed as information carriers in quantum devices where their cross-manipulation by external parameters such as electric and magnetic fields could enhance their functionalities. An emblematic example is that of electromagnons, spin-waves dressed with electric dipoles, that are fingerprints of multiferroics. Point-like objects have also been identified, which may take the form of excited quasiparticles. This is the case for magnetic monopoles, the exotic excitations of spin ices, that have been recently proposed to carry an electric dipole, although experimental evidences remain elusive. Presently, we investigate the electrical signature of a classical spin ice and a related compound that supports quantum fluctuations. Our in-depth study clearly attributes magneto-electricity to the correlated spin ice phase distinguishing it from extrinsic and single-ion effects. Our calculations show that the proposed model conferring magneto-electricity to monopoles is not sufficient, calling for higher-order contributions.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142276080","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Jianwei Huang, Chandan Setty, Liangzi Deng, Jing-Yang You, Hongxiong Liu, Sen Shao, Ji Seop Oh, Yucheng Guo, Yichen Zhang, Ziqin Yue, Jia-Xin Yin, Makoto Hashimoto, Donghui Lu, Sergey Gorovikov, Pengcheng Dai, Jonathan D. Denlinger, J. W. Allen, M. Zahid Hasan, Yuan-Ping Feng, Robert J. Birgeneau, Youguo Shi, Ching-Wu Chu, Guoqing Chang, Qimiao Si, Ming Yi
{"title":"Observation of flat bands and Dirac cones in a pyrochlore lattice superconductor","authors":"Jianwei Huang, Chandan Setty, Liangzi Deng, Jing-Yang You, Hongxiong Liu, Sen Shao, Ji Seop Oh, Yucheng Guo, Yichen Zhang, Ziqin Yue, Jia-Xin Yin, Makoto Hashimoto, Donghui Lu, Sergey Gorovikov, Pengcheng Dai, Jonathan D. Denlinger, J. W. Allen, M. Zahid Hasan, Yuan-Ping Feng, Robert J. Birgeneau, Youguo Shi, Ching-Wu Chu, Guoqing Chang, Qimiao Si, Ming Yi","doi":"10.1038/s41535-024-00683-x","DOIUrl":"https://doi.org/10.1038/s41535-024-00683-x","url":null,"abstract":"<p>Emergent phases often appear when the electronic kinetic energy is comparable to the Coulomb interactions. One approach to seek material systems as hosts of such emergent phases is to realize localization of electronic wavefunctions due to the geometric frustration inherent in the crystal structure, resulting in flat electronic bands. Recently, such efforts have found a wide range of exotic phases in the two-dimensional kagome lattice, including magnetic order, time-reversal symmetry breaking charge order, nematicity, and superconductivity. However, the interlayer coupling of the kagome layers disrupts the destructive interference needed to completely quench the kinetic energy. Here we demonstrate that an interwoven kagome network—a pyrochlore lattice—can host a three dimensional (3D) localization of electron wavefunctions. Meanwhile, the nonsymmorphic symmetry of the pyrochlore lattice guarantees all band crossings at the Brillouin zone X point to be 3D gapless Dirac points, which was predicted theoretically but never yet observed experimentally. Through a combination of angle-resolved photoemission spectroscopy, fundamental lattice model and density functional theory calculations, we investigate the novel electronic structure of a Laves phase superconductor with a pyrochlore sublattice, CeRu<sub>2</sub>. We observe evidence of flat bands originating from the Ce 4<i>f</i> orbitals as well as flat bands from the 3D destructive interference of the Ru 4<i>d</i> orbitals. We further observe the nonsymmorphic symmetry-protected 3D gapless Dirac cone at the X point. Our work establishes the pyrochlore structure as a promising lattice platform to realize and tune novel emergent phases intertwining topology and many-body interactions.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142245186","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Arman Rashidi, William Huynh, Binghao Guo, Sina Ahadi, Susanne Stemmer
{"title":"Vortex-induced anomalies in the superconducting quantum interference patterns of topological insulator Josephson junctions","authors":"Arman Rashidi, William Huynh, Binghao Guo, Sina Ahadi, Susanne Stemmer","doi":"10.1038/s41535-024-00684-w","DOIUrl":"https://doi.org/10.1038/s41535-024-00684-w","url":null,"abstract":"<p>The superconducting quantum interference (SQI) patterns of Josephson junctions fabricated from hybrid structures that interface an s-wave superconductor with a topological insulator can be used to detect signatures of novel quasiparticle states. Here, we compare calculated and experimental SQI patterns obtained from hybrid junctions fabricated on cadmium arsenide, a two-dimensional topological insulator. The calculations account for the effects of Abrikosov (anti-) vortices in the superconducting contacts. They describe the experimentally observed deviations of the SQI from an ideal Fraunhofer pattern, including anomalous phase shifts, node lifting, even/odd modulations of the lobes, irregular lobe spacing, and an asymmetry in the positive/negative magnetic field. We also show that under a current bias, these vortices enter the electrodes even if there is no intentionally applied external magnetic field. The results show that Abrikosov vortices in the electrodes of the junctions can explain many of the observed anomalies in the SQI patterns of topological insulator Josephson junctions.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142235244","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Unconventional spin textures emerging from a universal symmetry theory of spin-momentum locking","authors":"Yuntian Liu, Jiayu Li, Pengfei Liu, Qihang Liu","doi":"10.1038/s41535-024-00682-y","DOIUrl":"https://doi.org/10.1038/s41535-024-00682-y","url":null,"abstract":"<p>Spin textures, i.e., the distribution of spin polarization vectors in reciprocal space, exhibit diverse patterns determined by symmetry constraints, resulting in a variety of spintronic phenomena. Here, we propose a universal theory to comprehensively describe the nature of spin textures by incorporating three symmetry flavors of reciprocal wavevector, atomic orbital, and atomic site. Such an approach enables us to establish a complete classification of spin textures constrained by the little co-group and predict some exotic spin texture types, such as Zeeman-type spin splitting in antiferromagnets and quadratic spin texture. To illustrate the influence of atomic orbitals and sites on spin textures, we predict orbital-dependent spin texture and anisotropic spin-momentum-site locking effects, and corresponding material candidates validated through first-principles calculations. The comprehensive classification and the predicted new spin textures in realistic materials are expected to trigger future spin-based functionalities in electronics.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142231513","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Incommensurate magnetic order in an axion insulator candidate EuIn2As2 investigated by NMR measurement","authors":"Hikaru Takeda, Jian Yan, Zhongzhu Jiang, Xuan Luo, Yuping Sun, Minoru Yamashita","doi":"10.1038/s41535-024-00680-0","DOIUrl":"https://doi.org/10.1038/s41535-024-00680-0","url":null,"abstract":"<p>Magnetic topological insulators exhibit unique electronic states due to the interplay between the electronic topology and the spin structure. The antiferromagnetic metal EuIn<sub>2</sub>As<sub>2</sub> is a prominent candidate material in which exotic topological phases, including an axion insulating state, are theoretically predicted depending on the magnetic structure of the Eu<sup>2+</sup> moments. Here, we report experimental results of the nuclear magnetic resonance (NMR) measurements of all the nuclei in EuIn<sub>2</sub>As<sub>2</sub> to investigate the coupling between the magnetic moments in the Eu ions and the conduction electrons in In<sub>2</sub>As<sub>2</sub> layers and the magnetic structure. The <sup>75</sup>As and <sup>115</sup>In NMR spectra observed at zero external magnetic fields reveal the appearance of internal fields of 4.9 and 3.6 T, respectively, at the lowest temperature, suggesting a strong coupling between the conduction electrons in the In<sub>2</sub>As<sub>2</sub> layer and the ordered magnetic moments in the Eu ions. The <sup>75</sup>As NMR spectra under in-plane external magnetic fields show broad distributions of the internal fields produced by an incommensurate fan-like spin structure which turns into a forced ferromagnetic state above 0.7 T. We propose a spin reorientation process that an incommensurate helical state at zero external magnetic field quickly changes into a fan state by applying a slight magnetic field.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142170842","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"d-wave charge-4e superconductivity from fluctuating pair density waves","authors":"Yi-Ming Wu, Yuxuan Wang","doi":"10.1038/s41535-024-00674-y","DOIUrl":"https://doi.org/10.1038/s41535-024-00674-y","url":null,"abstract":"<p>We present a theory for charge-4<i>e</i> superconductivity as a leading low-temperature instability with a nontrivial <i>d</i>-wave symmetry. We show that in several microscopic models for the pair-density-wave (PDW) state, when the PDW wave vectors connect special parts of the Fermi surface, the predominant interaction is in the bosonic pairing channel mediated by exchanging low-energy fermions. This bosonic pairing interaction is repulsive in the <i>s</i>-wave channel but attractive in the <i>d</i>-wave one, leading to a <i>d</i>-wave charge-4<i>e</i> superconductor. By analyzing the Ginzburg-Landau free energy including higher-order fluctuation effects of PDW, we find that the charge-4<i>e</i> superconductivity emerges as a vestigial order of PDW, and sets in via a first-order transition. Both the gap amplitude and the transition temperature decay monotonically with increasing superfluid stiffness of the PDW order. Our work provides a microscopic mechanism of higher-charge condensates with unconventional ordering symmetry in strongly-correlated materials.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142138107","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Hui-Ke Jin, Wilhelm Kadow, Michael Knap, Johannes Knolle
{"title":"Kinetic ferromagnetism and topological magnons of the hole-doped Kitaev spin liquid","authors":"Hui-Ke Jin, Wilhelm Kadow, Michael Knap, Johannes Knolle","doi":"10.1038/s41535-024-00678-8","DOIUrl":"https://doi.org/10.1038/s41535-024-00678-8","url":null,"abstract":"<p>We study the effect of hole doping on the Kitaev spin liquid (KSL) and find that for ferromagnetic (FM) Kitaev exchange <i>K</i> the system is very susceptible to the formation of a FM spin polarization. Through density matrix renormalization group simulations on finite systems, we uncover that the introduction of a single hole, corresponding to ≈1% hole doping for the system size we consider, with a hopping strength of just <i>t</i> ~ 0.28<i>K</i> is enough to disrupt fractionalization and polarize the spins in the [001] direction due to an order-by-disorder mechanism. Taking into account a material relevant FM anisotropic exchange <i>Γ</i> drives the polarization towards the [111] direction via a transition into a topological FM state with chiral magnon excitations. We develop a parton mean-field theory incorporating fermionic holons and bosonic magnons, which accounts for the doping induced FM phases and topological magnon excitations. We discuss experimental implications for Kitaev candidate materials.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":null,"pages":null},"PeriodicalIF":5.7,"publicationDate":"2024-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142138108","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}