Advanced Optical Materials最新文献_第8页

Large Electrogyration Effect in Ferroaxial NiTiO3 at Near Infrared Wavelengths 近红外波段轴向铁NiTiO3的大电旋效应

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-11 DOI: 10.1002/adom.202500364

Takeshi Hayashida, Koei Matsumoto, Tsuyoshi Kimura

引用次数: 0

Long-Term Study of Optical Nanoparticles Doped With Yb3+/Er3+ and Transition Metal Ions and their Real Application for Imaging and Temperature Sensing on Triticum Aestivum L. 掺杂Yb3+/Er3+和过渡金属离子的光学纳米颗粒的长期研究及其在小麦成像和温度传感中的实际应用

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-08 DOI: 10.1002/adom.202500432

Dominika Przybylska, Kevin Soler-Carracedo, Anna Ekner-Grzyb, Natalia Jurga, Marjanossadat Hosseinifard

{"title":"Long-Term Study of Optical Nanoparticles Doped With Yb3+/Er3+ and Transition Metal Ions and their Real Application for Imaging and Temperature Sensing on Triticum Aestivum L.","authors":"Dominika Przybylska, Kevin Soler-Carracedo, Anna Ekner-Grzyb, Natalia Jurga, Marjanossadat Hosseinifard","doi":"10.1002/adom.202500432","DOIUrl":"https://doi.org/10.1002/adom.202500432","url":null,"abstract":"Upconverting nanoparticles (UCNPs) have incredible potential for countless applications, especially in biology and medicine. These NPs can be used to bioimaging animals and plants and analyze their physiology, metabolic pathways, or intercellular interactions in real-time. However, before reaching such an application, the UCNPs physicochemical properties during prolonged storage and their toxicity to a particular species must be studied. Herein, SrF2:Yb3+, Er3+ water colloid, additionally doped with transition metals (Sc3+ or Zn2+) to enhance observed emission, are tested during 22 weeks of storage in ambient conditions. The obtained compounds presented high stability throughout the entire duration of the experiment, with minor changes in their composition, emission intensity, and thermal sensitivity. After carefully investigating the phytotoxicity of UCNPs on wheat Triticum aestivum L., UC emission plant imaging is successfully observed under 975 nm excitation while overcoming laser heating that can harm the plant. The UC emission from the UCNPs in the plant is also calibrated to monitor temperature. Moreover, it is discovered that SrF2:Yb3+, Er3+, Zn2+ can positively influence wheat growth. These results indicate that presented UCNPs are among the most promising candidates for biological and agriculture studies and applications.","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 18","pages":""},"PeriodicalIF":8.0,"publicationDate":"2025-05-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adom.202500432","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144492839","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Fluorophore-Bridge-Fluorophore Architecture for Efficient Narrowband Pure Green Electroluminescence 高效窄带纯绿色电致发光的荧光团-桥-荧光团结构

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-06 DOI: 10.1002/adom.202500395

Xiao-Sheng Zhong, Jia-Qi Xi, Jia-Jun Hu, Li Yuan, You-Xuan Zheng

{"title":"Fluorophore-Bridge-Fluorophore Architecture for Efficient Narrowband Pure Green Electroluminescence","authors":"Xiao-Sheng Zhong, Jia-Qi Xi, Jia-Jun Hu, Li Yuan, You-Xuan Zheng","doi":"10.1002/adom.202500395","DOIUrl":"https://doi.org/10.1002/adom.202500395","url":null,"abstract":"Developing narrowband multiple resonance thermally activated delayed fluorescence (MR-TADF) materials for concentration-independent organic light-emitting diodes (OLEDs) with high efficiency and color purity is still a challenge. Herein, a fluorophore-bridge-fluorophore architecture is developed, resulting in two MR-TADF materials (BNCz-n-POABNCz and POABNCz-n-POABNCz) by “face-to-face” arrangement of BNCz (based on carbazole unit) and POABNCz (based on carbazole and phenoxazine groups) cores sterically on the naphthalene bridge. Two materials show green emissions peaking at 501/516 nm with full-width at half-maximum values of 30/33 nm in toluene and photoluminescence quantum yields of 94%/87% in doped films, respectively. Remarkably, the POABNCz-n-POABNCz exhibits high color purity with Commission Internationale de L'Eclairage coordinates of (0.19, 0.71), reaching the National Television System Committee standard for pure green emission. Furthermore, the OLEDs D1 and D2 composing BNCz-n-POABNCz and POABNCz-n-POABNCz illustrate maximum external quantum efficiencies (EQEmax) of 32.0% and 33.6%, respectively. Even at a doping ratio of 20 wt%, D2 still remains an EQEmax ≈28.5%.","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 18","pages":""},"PeriodicalIF":8.0,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144492802","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Optoelectrical Performance Enhancement by Integrating CsPbI3 Quantum Dots Layer with Bi2O2Se/Si Photodiodes CsPbI3量子点层与Bi2O2Se/Si光电二极管集成提高光电性能

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-06 DOI: 10.1002/adom.202403355

Heng Yang, Sizhe Chen, Yi Liu, Qian Zhao, Fangchao Lu, Fengrui Hu, Jing Zhang, Xiaolong Liu

{"title":"Optoelectrical Performance Enhancement by Integrating CsPbI3 Quantum Dots Layer with Bi2O2Se/Si Photodiodes","authors":"Heng Yang, Sizhe Chen, Yi Liu, Qian Zhao, Fangchao Lu, Fengrui Hu, Jing Zhang, Xiaolong Liu","doi":"10.1002/adom.202403355","DOIUrl":"https://doi.org/10.1002/adom.202403355","url":null,"abstract":"Benefiting from the versatile energy band structure design of 2D materials and effective modulation of dopant concentration in Si, 2D/Si hybrid heterostructures demonstrate desirable device performances. Bismuth oxychalcogenide material Bi2O2Se, exhibits high carrier mobility and ultrafast optoelectrical dynamics, when interfaced with Si, the device efficiencies will be improved in the aspects of photo-induced carrier separation and collection. However, due to the indirect bandgap features of Bi2O2Se and Si, the light absorption of the heterostructure is unsatisfactory, deteriorating the external quantum efficiency. To address this, additional light absorption enhancing materials (LAEMs) are incorporated, and boosted with the photo-gating effects generated from the residual carriers within the LAEMs, and photoconductive gain and photoresponsivity are improved at the cost of response speed. In this study, the CsPbI3 quantum dot layer is adopted to provide excess carriers, which are injected into Bi2O2Se/p-Si heterojunction in the form of excitonic energy transfer. The carrier multiplication effect is thus circumvented, leading to an improved photoresponsivity as high as 2078 A W−1, while specific time constants of the rising and falling edges of photocurrent are accelerated to 267 and 391 µs.","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 15","pages":""},"PeriodicalIF":8.0,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144148467","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Quantum Sensing of Lanthandie Binding Tags with Relaxometer of NV Center in Diamond 基于金刚石NV中心弛豫计的镧钛结合标签量子传感

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-06 DOI: 10.1002/adom.202500308

Zibo Gao, Zhengzhi Jiang, Qiyu Liang, Ruihua He, Van Cuong Mai, Yingwei Tang, Qirong Xiong, Wenting Zhao, Hongwei Duan, Hongliang Sun, Mo Li, Yansong Miao, Weibo Gao

{"title":"Quantum Sensing of Lanthandie Binding Tags with Relaxometer of NV Center in Diamond","authors":"Zibo Gao, Zhengzhi Jiang, Qiyu Liang, Ruihua He, Van Cuong Mai, Yingwei Tang, Qirong Xiong, Wenting Zhao, Hongwei Duan, Hongliang Sun, Mo Li, Yansong Miao, Weibo Gao","doi":"10.1002/adom.202500308","DOIUrl":"https://doi.org/10.1002/adom.202500308","url":null,"abstract":"Lanthanide binding tags (LBTs) stand out as a prominent group of fluorescent probes that are extensively utilized in biological detection. However, research on LBTs has predominantly emphasized their fluorescence properties, which frequently compromised by background fluorescence noise. Investigating magnetic properties could optimize detection methodologies that offer enhanced sensitivity and specificity. This study measures the response of a relaxometer based on ensemble nitrogen-vacancy (NV) centers in diamond to various amounts of LBTs with gadolinium ions, determining the detection limit of LBTs to be 25 fmol. A detection scheme employing the NV relaxometer to detect specific binding between LBTs and target is then proposed and demonstrated. Specifically, the study assesses the relaxometer's response to various concentrations of the interaction between the modified LBTs and Receptor-Binding Domain (RBD) of SARS-COVID-2 spike protein, with the detection threshold reaching ≈2 pmol. The research provides a potential application platform for biomarker detection under picomole concentration by using NV centers to detect the magnetism of LBTs.","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 18","pages":""},"PeriodicalIF":8.0,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144492801","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Rotatable Terahertz Vortex Field Based on Magneto-Optical Metasurface 基于磁光超表面的可旋转太赫兹涡旋场

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-06 DOI: 10.1002/adom.202500088

Hang Yin, Hao Wang, Fei Fan, Pengxuan Li, Huijun Zhao, Yunyun Ji, Jierong Cheng, Shengjiang Chang

{"title":"Rotatable Terahertz Vortex Field Based on Magneto-Optical Metasurface","authors":"Hang Yin, Hao Wang, Fei Fan, Pengxuan Li, Huijun Zhao, Yunyun Ji, Jierong Cheng, Shengjiang Chang","doi":"10.1002/adom.202500088","DOIUrl":"https://doi.org/10.1002/adom.202500088","url":null,"abstract":"Terahertz vortex fields hold immense potential for wideband, high-capacity wireless communication. However, existing functional devices face challenges such as the lack of multi-channel multiplexing and active control capabilities. Here, a magneto-optical dielectric spiral metasurface that enables the generation and active rotation of vortex fields with different functionalities is proposed: within the frequency band of a completely orthogonal polarization conversion, the vortex beams excited by the two spin photonic states exhibit distinct topological charges with the mode purity of over 80% and focusing characteristics with spatial separation between them. In addition, within the frequency band of half orthogonal polarization conversion, a spiral field distribution can be obtained resulting from interference between the conversion and the direct-through components. By adjusting the magnetic field, the device allows dynamic, nonreciprocal rotation of both local polarization states and vortex fields. The rotation angle is determined by magnetization and topological charge with a maximum rotation of up to 180°. The magneto-optical light field manipulation mechanism offers promising applications in high-capacity communications, information encryption, and particle manipulation.","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 16","pages":""},"PeriodicalIF":8.0,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144232187","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Quantum Dot-Enhanced Dual-Modality Heterojunction Optoelectronic Synapse for Neuromorphic Computing (Advanced Optical Materials 13/2025) 用于神经形态计算的量子点增强双模异质结光电突触（Advanced Optical Materials 13/2025）

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-05 DOI: 10.1002/adom.202570091

Junyan Li, Hao Lei, Kanghong Wang, Xianyao Li, Zhuo Chen, Sang Lam, Xin Tu, Ka Lok Man, Chun Zhao

引用次数: 0

Suppressed Trap Density and Reduced Energy Disorder for High-Performance Ultrathin Organic Near-Infrared Photodetectors 高性能超薄有机近红外光电探测器的抑制陷阱密度和降低能量紊乱

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-05 DOI: 10.1002/adom.202403173

Xuewu Li, Jiawei Qiao, Mingxu Zhou, Xue Shi, Yufeng Ge, Zhen Fu, Xiaotao Hao

{"title":"Suppressed Trap Density and Reduced Energy Disorder for High-Performance Ultrathin Organic Near-Infrared Photodetectors","authors":"Xuewu Li, Jiawei Qiao, Mingxu Zhou, Xue Shi, Yufeng Ge, Zhen Fu, Xiaotao Hao","doi":"10.1002/adom.202403173","DOIUrl":"https://doi.org/10.1002/adom.202403173","url":null,"abstract":"Ultrathin Organic Photodetectors (OPDs), renowned for their high miniaturization and energy efficiency, are increasingly integrated into everyday devices, including smartphones, tablet computers, and medical equipment. However, the inherent high trap density and energy disorder associated with organic materials (especially at ultrathin thickness) have posed significant challenges to their performance and efficiency. This study presents a strategy for controlling trap density and energy disorder of high-performance ultrathin near-infrared (NIR) OPDs by incorporating L8-BO into the active layer of PM6:BTP-eC9 blends. A notable increase in trap density is observed as the thickness decreases from 110 to 20 nm, which correlates with a diminished photoelectric response of ultrathin OPDs. The incorporation of L8-BO enhances the crystallinity of the blends, significantly suppressing the trap density and energy disorder. Additionally, the L8-BO strategic integration can mitigate exciton-phonon coupling and extend carrier recombination time. Subsequently, the optimized devices exhibit a responsivity exceeding 0.4 A W−1 and an outstanding specific detectivity (2.30 × 1013 Jones) at 850 nm, positioning them at the forefront of contemporary NIR photodetector technology. These advancements present a significant opportunity to enhance the performance of NIR OPDs, thereby facilitating their integration into the rapidly expanding field.","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 15","pages":""},"PeriodicalIF":8.0,"publicationDate":"2025-05-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144148480","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Laser-Induced Crystallization and Oxidation Phase Diagrams for High-Throughput Evaluation of MoS2/MoOx Optical Thin Films 激光诱导结晶和氧化相图用于高通量评价MoS2/MoOx光学薄膜

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-05 DOI: 10.1002/adom.202500190

Drake R. Austin, Brian Everhart, Michael Altvater, Arthur R. Woll, Christopher Muratore, Benjamin Robertson, Lirong Sun, Mario Hofmann, Michael E. McConney, Peter R. Stevenson, Nicholas R. Glavin

{"title":"Laser-Induced Crystallization and Oxidation Phase Diagrams for High-Throughput Evaluation of MoS2/MoOx Optical Thin Films","authors":"Drake R. Austin, Brian Everhart, Michael Altvater, Arthur R. Woll, Christopher Muratore, Benjamin Robertson, Lirong Sun, Mario Hofmann, Michael E. McConney, Peter R. Stevenson, Nicholas R. Glavin","doi":"10.1002/adom.202500190","DOIUrl":"https://doi.org/10.1002/adom.202500190","url":null,"abstract":"The development of thin film materials for optoelectronic and meta-optic applications requires the discovery of novel materials and reliable control over their optical constants during the growth process. In this work, localized laser oxidation and crystallization are used to tailor the optical constants of an amorphous MoS2 precursor thin film. By scanning focused laser light across multiple films with varying intensity and speed in a controlled oxygen environment, the transient heating associated with this technique is used to control the localized oxidation of each film. Characterization of the laser-processed regions results in synthesis phase diagrams indicating the laser conditions at which each oxide phase is formed. The optical constants of each phase are also measured, showing changes in refractive index Δn and extinction coefficient Δk as large as Δn = 0.43 and Δk = 0.35 for MoS2, Δn = 1.7 and Δk = 1.6 for MoO3, and Δn = 1.7 and Δk= 1.3 for MoO2. These changes are attributed to oxygen dopants, strain, improved crystallinity for MoS2, and oxygen vacancies and sulfur dopants for the oxide phases. These findings demonstrate the versatility of the laser processing approach for the highly controlled tailoring of thin film optical properties for high-throughput materials discovery.","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 17","pages":""},"PeriodicalIF":8.0,"publicationDate":"2025-05-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144299710","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Elucidating and Biomimicking the Coloration Mechanisms Responsible for the Vibrant Blue Hues of the Common Kingfisher (Advanced Optical Materials 13/2025) 普通翠鸟鲜艳的蓝色色调的着色机制的阐明和仿生（先进光学材料13/2025）

IF 8 2区材料科学

Advanced Optical Materials Pub Date : 2025-05-05 DOI: 10.1002/adom.202570089

Jihun Kang, Seunghwan Moon, Deok-Jin Jeon, Seungmuk Ji, Eunok Lee, Jong-Souk Yeo

引用次数: 0