Advanced Optical Materials最新文献

{"title":"Versatile Metamaterial: Exploring the Resonances of Symmetry-Protected Modes for Multitasking Functionality (Advanced Optical Materials 35/2024)","authors":"Souhaïla Boublouh,&nbsp;Miguel Suarez,&nbsp;Feng Gao,&nbsp;Abderrahmane Belkhir,&nbsp;Abdelkrim Khelif,&nbsp;Fadi Baida","doi":"10.1002/adom.202470114","DOIUrl":"https://doi.org/10.1002/adom.202470114","url":null,"abstract":"<p><b>Exploring the Resonances of Symmetry-Protected Modes for Multitasking</b></p><p>Fadi Baida and co-workers have designed a sub-wavelength meta-device to excite multiple continuum-integrated states (BICs) under varying illumination conditions and wavelengths (see article number 2401558). These resonances enable a range of applications, including acousto-optic modulation by coupling with surface acoustic waves, second harmonic generation (SHG) exploiting the nonlinear properties of lithium niobate, electro-optic modulation and pyroelectric applications, both enhanced by strong electric field confinement associated with the electro-optic and pyroelectric properties of lithium niobate.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"12 35","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adom.202470114","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142860826","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Abnormal Response of Indirect Excitons to Non-Uniform Elastic Strain in MoS2 Flakes (Advanced Optical Materials 35/2024)","authors":"Xinxin Yue,&nbsp;Lifu Zhang,&nbsp;Xiang Chen,&nbsp;Shaozheng Ji,&nbsp;Fang Liu,&nbsp;Min Feng,&nbsp;Shibin Deng,&nbsp;Zhenpeng Hu,&nbsp;Yuan Yan,&nbsp;Xuewen Fu","doi":"10.1002/adom.202470117","DOIUrl":"https://doi.org/10.1002/adom.202470117","url":null,"abstract":"<p><b>Response of Indirect Excitons to Non-Uniform Elastic Strain in MoS₂ Flakes</b></p><p>In article number 2401728, Lifu Zhang, Zhenpeng Hu, Yuan Yan, Xuewen Fu, and co-workers report the abnormal response of indirect excitons to non-uniform elastic strain in MoS₂ flakes, fundamentally distinct from the linear energy-shift behavior of direct excitons. Such abnormal phenomenon arises from the strain-induced competition between two indirect bandgap transitions and the spatial exciton funnel effect in the non-uniform strain field.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"12 35","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adom.202470117","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142861006","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Masthead: (Advanced Optical Materials 35/2024)","authors":"","doi":"10.1002/adom.202470115","DOIUrl":"https://doi.org/10.1002/adom.202470115","url":null,"abstract":"","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"12 35","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adom.202470115","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142860827","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Synergistic Effects of Defects and Strain on Photoluminescence in Van der Waals Layered Crystal AgScP2S6 (Advanced Optical Materials 35/2024)","authors":"Abhishek Mukherjee,&nbsp;Damian Wlodarczyk,&nbsp;Ajeesh K. Somakumar,&nbsp;Piotr Sybilski,&nbsp;Ryan Siebenaller,&nbsp;Rahul Rao,&nbsp;Michael A. Susner,&nbsp;Andrzej Suchocki,&nbsp;Svetlana V. Boriskina","doi":"10.1002/adom.202470116","DOIUrl":"https://doi.org/10.1002/adom.202470116","url":null,"abstract":"<p><b>Effect of Defects and Strain on Photoluminescence in Metal Thiophosphates</b></p><p>This cover image displays the surface topography of 2D AgScP₂S₆, where sulfur vacancies act as color centers (depicted by the bottom right figure). Structural ‘crater-like’ defects on the surface enhance and modulate light emission originating from these vacancies, resulting in broadband visible light. For further details, see article number 2400481 by Abhishek Mukherjee, Svetlana V. Boriskina, and co-workers.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"12 35","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adom.202470116","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142861005","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Photoluminescent Sol-Gel Glass Constructed via Highly Efficient Förster Resonance Energy Transfer","authors":"Longyue Yu,&nbsp;Wenwen Fu,&nbsp;Mengdie Li,&nbsp;Hailong Liu,&nbsp;Xionghui Huang,&nbsp;Xia Xin,&nbsp;Lei Feng,&nbsp;Hongguang Li","doi":"10.1002/adom.202402123","DOIUrl":"https://doi.org/10.1002/adom.202402123","url":null,"abstract":"<p>Photoluminescent (PL) solid with color tunability are in high demand for the development of large-area display and illumination devices. With high transparency, high chemical stability, and mature fabrication, sol-gel glass is an ideal solid matrix to obtain such materials by chromophore doping. However, it remains a big challenge to obtain sol-gel glass with high luminous efficiency under a single excitation wavelength. Herein, the construction of highly luminescent sol-gel glass enabled by Förster resonance energy transfer (FRET) is reported. Branched siloxane is used to modify naphthalene and BODIPY, which led to the formation of blue-emitting donor (denoted as Si-Nap) and green-emitting acceptor (denoted as Si-BODIPY), respectively. Efficient FRET occurs between Si-Nap and Si-BODIPY proved by spectral titration and lifetime measurements, with an energy transfer efficiency (<i>Φ</i>_ET) up to 97.9%. When RhB is added, it acts as a final acceptor that enables the occurrence of a sequential FRET from Si-Nap to Si-BODIPY and further to RhB. The overall energy transfer efficiency reaches 94%, and the fluorescence quantum yield exceeds 88%. By adjustment of the composition, color-tunable sol-gel glass is obtained with emergence of white-emitting samples, opening potential applications in a variety of fields.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 2","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143112730","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Preparing Smaller InP Quantum Dots by Suppressing Over-Etch Using Core Protective Layer and Ammonium Fluoride as Alternative Etchant","authors":"Hsueh-Shih Chen,&nbsp;Chang-Wei Yeh,&nbsp;Hsuan-Yu Lee,&nbsp;Yi-Jui Ho","doi":"10.1002/adom.202402051","DOIUrl":"https://doi.org/10.1002/adom.202402051","url":null,"abstract":"<p>Indium phosphide (InP) is emerging as a viable and environmentally friendly alternative to toxic cadmium-based quantum dots (QDs), especially in the fields of lighting and display. This is owing to similar material properties of InP to those of commercial Cd-based QDs. Nonetheless, the surface quality of InP needs enhancement through a post-treatment process to eliminate surface oxides, typically with hydrofluoric acid (HF). The challenge arises with smaller, such as green InP QDs, as HF easily over-etch the InP cores, thus leading to an unpredictable size distribution and reduced production consistency. This research introduces a refined synthetic strategy that circumvents this over-etching phenomenon and offers a more precise control over the etching process of smaller InP QDs. By applying an additional protective layer to the InP cores prior to etching and employing ammonium fluoride (NH₄F) as an alternative to the conventional HF, the over-etching incidence can be markedly mitigated. The results reveal that smaller InP/ZnSeS QDs with photoluminescence quantum yield (QY) &gt;90% can be consistently produced, thereby proposing a more efficient and safer method for the fabrication of smaller InP QDs.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 2","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143112368","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Tunable Optical High-Order Differential Microscopy for Cell Structure Detection","authors":"Shuoqing Liu,&nbsp;Yongqi Zhao,&nbsp;Dandan Zheng,&nbsp;Shizhen Chen,&nbsp;Shuangchun Wen,&nbsp;Hailu Luo","doi":"10.1002/adom.202402186","DOIUrl":"https://doi.org/10.1002/adom.202402186","url":null,"abstract":"<p>Optical differential microscopy is an important tool for the detection and recognition of transparent biological objects. Among it, the first-order optical differentiation is commonly utilized to aid in fast, label-free, and contactless detection. However, the characterization of detailed contours for some smooth object areas may be limited, and a higher order operation needs to be executed. A tunable optical high-order differential microscopy is proposed and implemented, in virtue of electric-driven liquid crystal (LC). By electrically switching the working state of LC, the differential operation can be flexibly tuned in desired order, such as from zero-order to first-order and second-order differentiations. Using this scheme, clear edge-enhanced images of different-contrast objects even transparent biological cells are experimentally acquired under multi-wavelength cases. Specifically, based on the connection between high-order differential results and edge features, further gained in-depth information in the size of light spot and structure of plant cells. The beam waist radius of a laser is determined as 0.35 ± 0.002 mm, and the cell wall thickness is estimated about 3 to 5 microns. These results may open the avenue for biological imaging and microscopic measurement.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 3","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143112729","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Biomimetically Inspired Micro-Nano Hierarchical Structures of Rose Petals for Efficient SERS Sensing Applications","authors":"Yunjie Xia,&nbsp;Mengnan Sun,&nbsp;Li Zhang,&nbsp;Shuyan Qi,&nbsp;Yaru Jia,&nbsp;Zihou Li,&nbsp;Mingkun Wang,&nbsp;Shunxiang Li,&nbsp;Aiguo Wu,&nbsp;Bo Chen","doi":"10.1002/adom.202401657","DOIUrl":"https://doi.org/10.1002/adom.202401657","url":null,"abstract":"<p>Surface-enhanced Raman spectroscopy (SERS) detection is a crucial technology for rapid sensing and “fingerprinting”, achieved through the combination of Raman spectroscopy and arrays of noble metal nanoparticles (NPs). This study introduces a low-cost biomimetic-inspired approach to fabricate rose petal structured micro/nano hierarchical structures with silver (Ag) film, serving as a reliable SERS substrate. These substrates are thoroughly compared by replicating the upper surface of rose petals of different colors into a transparent polydimethylsiloxane (PDMS) mixture and subsequently sputtering Ag film of varying thicknesses. Ultimately, the white negative rose PDMS replica is chosen, demonstrating a high enhancement factor, good batch-to-batch reproducibility, high stability, and high sensitivity for crystal violet (CV), an organic contaminant with mutagenic and toxigenic properties. In a proof-of-concept experiment, the multiplex detection capability of this SERS substrate is demonstrated by analyzing a combination of two sets of analytes (CV and methylene blue as well as CV and Nile blue A). Furthermore, this SERS substrate is utilized to test tau protein and amyloid β peptides, both recognized biomarkers of Alzheimer's disease. This study illustrates that the proposed 3D SERS substrate exhibits significant potential for the highly sensitive and rapid detection of biomolecules in practical applications.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"12 36","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142868123","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Tunable Single-Phase White Light Emission from Complex Perovskite Sr3CaNb2O9: Dy3+/Eu3+ Phosphors","authors":"Noor Zamin Khan,&nbsp;Sayed Ali Khan,&nbsp;Nisar Muhammad,&nbsp;Weilong Chen,&nbsp;Jahangeer Ahmed,&nbsp;Muhammad Amin Padhiar,&nbsp;Mei Chen,&nbsp;Marcin Runowski,&nbsp;Saad M. Alshehri,&nbsp;Baohua Zhang,&nbsp;Shu-Sheng Pan,&nbsp;Ren-Kui Zheng","doi":"10.1002/adom.202401938","DOIUrl":"https://doi.org/10.1002/adom.202401938","url":null,"abstract":"<p>Sr₃CaNb₂O₉:Dy³⁺/Eu³⁺ phosphors with a complex perovskite structure are prepared using a high-temperature solid- state reaction technique. These phosphors are doped either singly or in combination with Dy³⁺/Eu³⁺ ions, resulting in efficient energy transfer from Dy³⁺ to Eu³⁺ and thus tunable-color emission. Under 353 nm excitation, the Sr₃CaNb₂O₉:Dy³⁺ phosphor emits blue (492 nm), yellow (583 nm), and red (682 nm) light, with the optimal doping concentration of Dy³⁺ of 0.04%. When excited by 394 nm (⁷F₀ → ⁵L₆), the Sr₃CaNb₂O₉:Eu³⁺ phosphor exhibits two most intense emissions centered at 593 nm (⁵D₀ → ⁷F₁) and 614 nm (⁵D₀ → ⁷F₂). The decrease in luminescence intensity with increasing doping concentration of Dy³⁺ and Eu³⁺ is due to the cross-relaxation associated with electric dipole–dipole interaction. Photoluminescence emission measurements under excitations of 353 and 365 nm indicate that the Sr₃CaNb₂O₉:0.04Dy³⁺/0.05Eu³⁺ phosphor shows excellent thermal stability, even at a temperature of 150 °C, where the luminescence intensity preserves 79% of its initial value at room temperature. The electroluminescence performance of the Sr₃CaNb₂O₉:0.04Dy³⁺/0.05Eu³⁺ phosphor is tested with 365 nm LED chips for potential use in white LEDs. The results confirm that Sr₃CaNb₂O₉:0.04Dy³⁺/0.05Eu³⁺ phosphor has great potential for use in high-power white LED applications as a single matrix.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 1","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143112369","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Singularities of Radial Gradient Perfect Vortex Beams Generated by Pancharatnam-Berry Metasurfaces","authors":"Shuyan Zhang,&nbsp;Weijie Shi,&nbsp;Lili Tang,&nbsp;Zheng-Gao Dong","doi":"10.1002/adom.202402091","DOIUrl":"https://doi.org/10.1002/adom.202402091","url":null,"abstract":"<p>Perfect vortex beams (PVBs) have recently attracted much attention because they can maintain donut-like intensity profiles with sizes that do not depend on topological charges (TCs). The superposition of them can further expand the potential applications. However, the conventional superposition method is limited to PVBs with identical donut sizes and discrete TCs, which reduces the degrees of freedom for flexible manipulation of light. A compact metasurface approach for superposed PVBs with radial gradient sequential integer TCs and numerical aperture is proposed in this paper. This method achieves radial gradient PVBs (RGPVBs) with asymmetric intensity singularity distribution, and the singularity positions can be further modulated by introducing an initial phase in the metasurface design. Additionally, an array of RGPVBs can be realized. This kind of singularity beams of RGPVBs is expected to be used in optical trapping, optical communications, and quantum information.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 2","pages":""},"PeriodicalIF":8.0,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143112681","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}