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Investigating the Balance between Power Conversion Efficiency and Average Visible Transmittance for Semitransparent Perovskite Solar Cells
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-24 DOI: 10.1002/ente.202401452
Muhammad Noman, Azmat Ullah, Shayan Tariq Jan, Adnan Daud Khan
{"title":"Investigating the Balance between Power Conversion Efficiency and Average Visible Transmittance for Semitransparent Perovskite Solar Cells","authors":"Muhammad Noman,&nbsp;Azmat Ullah,&nbsp;Shayan Tariq Jan,&nbsp;Adnan Daud Khan","doi":"10.1002/ente.202401452","DOIUrl":"https://doi.org/10.1002/ente.202401452","url":null,"abstract":"<p>The raising demand for sustainable energy in architecture has increased interest in building-integrated photovoltaics (BIPV), with semi-transparent perovskite cells (PSCs) emerging as an option. This research focuses on the critical balance between efficiency (PCE) and average visible transmittance (AVT) necessary for the development of semi-transparent PSCs. Through comprehensive investigation, two perovskites, MAPbI<sub>3</sub> and MAPbBr<sub>3</sub>, are examined for their respective advantages of high PCE and transparency. A series of simulations are conducted to analyze the impact of perovskite thickness on the properties of the PSC. The study analyzes the compatibility of different charge transport layers with perovskites to enhance carrier flow and reduce recombination at heterojunction. Furthermore, the effect of the work-function of transparent conductive oxide electrode on the performance of the PSCs is investigated. The findings show that an optimal range of perovskite thickness that achieves PCE of over 10% while maintaining an AVT above 20% offers a viable solution for BIPV. For applications where visual transparency is crucial, the SnO<sub>2</sub>/MAPbBr<sub>3</sub>/CuSCN presents a compelling choice with AVT of 29.2% along with PCE of 10.72% at 440 nm thickness. In contrast, for applications requiring higher PCE, the SnO<sub>2</sub>/MAPbI<sub>3</sub>/CuSCN stands out with the PCE of 19.22% and AVT of 20% at 250 nm thickness.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 3","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143565443","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Lattice Distortion Creates Enhancements in Photocatalytic and Electrocapacitive Performance of Sol–Gel-Derived Cu-Doped NiTiO3
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-23 DOI: 10.1002/ente.202401138
Sakshi Chaudhary, Kanak Pal Singh Parmar, Ranjeet Brajpuriya, Bhupendra Singh Rawat, Ankush Vij
{"title":"Lattice Distortion Creates Enhancements in Photocatalytic and Electrocapacitive Performance of Sol–Gel-Derived Cu-Doped NiTiO3","authors":"Sakshi Chaudhary,&nbsp;Kanak Pal Singh Parmar,&nbsp;Ranjeet Brajpuriya,&nbsp;Bhupendra Singh Rawat,&nbsp;Ankush Vij","doi":"10.1002/ente.202401138","DOIUrl":"https://doi.org/10.1002/ente.202401138","url":null,"abstract":"<p>A remarkable 35% enhancement in the photocatalytic and electrocatalytic abilities of an ilmenite nickel titanate (NiTiO<sub>3</sub>) material is reported. This boost in catalytic performance is achieved by simply creating a static distortion in the rhombohedral unit cell by replacing a small proportion of a small-size nondegenerate Ni (69 pm) with a large-size degenerate Cu (73 pm). The materials are synthesized by using a simple sol–gel method. The appropriate doping amount of Cu facilitates the better separation of intrinsic charge carrier pairs by inhibiting their recombination. The photocatalytic and electrochemical activities of durable materials in aqueous MB dye (10 ppm) and KOH (1 molar) electrolyte solutions are found to be directly associated with this improvement in inherent charge carrier transfer characteristics. The enhanced photodissociation of MB dye (42–56%) and specific capacitance (381–450 F g<sup>−1</sup>) in a KOH (1 molar) electrolyte are in full accord with the investigations carried out using crystallographic and optoelectronic analysis, charging–discharging measurements, and electrochemical impedance (EIS) spectroscopy investigations. Same material with high textural surface areas or controllable particle morphologies might show a far better photo/electrocatalytic performance in a variety of practical applications.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 3","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143565388","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Navigating the Frontier Role of Electrolyte Interfaces in Dye-Sensitized Solar Cell Technology
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-22 DOI: 10.1002/ente.202401345
Santhosh Kamaraj, Ganesan Shanmugam, Balamurugan Selvaraj
{"title":"Navigating the Frontier Role of Electrolyte Interfaces in Dye-Sensitized Solar Cell Technology","authors":"Santhosh Kamaraj,&nbsp;Ganesan Shanmugam,&nbsp;Balamurugan Selvaraj","doi":"10.1002/ente.202401345","DOIUrl":"https://doi.org/10.1002/ente.202401345","url":null,"abstract":"<p>Recent advances in solar cell technology have been motivated by new materials and inventive engineering techniques. Dye-sensitized solar cells (DSSCs) are becoming more widely recognized as a possible alternative for sustainable energy. Optimizing electrolytes is one of the most important variables impacting their effectiveness and durability. The electrolyte interface is critical to optimize charge separation, ion transport, and diffusion ensuring device stability and efficiency. The present investigation focuses on enhancing interface stability and investigating innovative electrolyte compositions to improve DSSC performance for sustainability in solar energy applications. Despite progress, obstacles remain in presenting core principles and research approaches in DSSC technology. Continued research is required to overcome these limitations and fully realize the potential of DSSCs in sustainable energy solutions.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 1","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143118051","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dual Metal Sites Coengineered Graphitic Carbon Nitride as Green Electrocatalyst for Highly Selective Overall Water Splitting—A Sustainable Approach
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-22 DOI: 10.1002/ente.202401577
Satya Lakshmi Pasarakonda, Srikanth Ponnada, Maryam Sadat Kiai, Velu Duraisamy, Hima Bindu G, Annapurna Nowduri, Sakkarapalayam Murugesan Senthil Kumar, Rakesh K Sharma
{"title":"Dual Metal Sites Coengineered Graphitic Carbon Nitride as Green Electrocatalyst for Highly Selective Overall Water Splitting—A Sustainable Approach","authors":"Satya Lakshmi Pasarakonda,&nbsp;Srikanth Ponnada,&nbsp;Maryam Sadat Kiai,&nbsp;Velu Duraisamy,&nbsp;Hima Bindu G,&nbsp;Annapurna Nowduri,&nbsp;Sakkarapalayam Murugesan Senthil Kumar,&nbsp;Rakesh K Sharma","doi":"10.1002/ente.202401577","DOIUrl":"https://doi.org/10.1002/ente.202401577","url":null,"abstract":"<p>The development of efficient, low-cost, non-noble metal-oxide-based nanohybrid materials for overall water splitting is a critical strategy for enhancing clean energy use and addressing environmental issues. In this study, an interfacial engineering strategy for the development of bimetallic Co–Ni nanoparticles on graphitic carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) using ultrasonication followed by coprecipitation is conveyed. These nanoparticles demonstrate high efficacy as bifunctional electrocatalysts for the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) in alkaline conditions. Co–Ni nanoparticles on graphitic carbon nitride demonstrate an increased surface area via ultrasonication and subsequent coprecipitation. The g-C<sub>3</sub>N<sub>4</sub> combined with Co–Ni nanoparticles leads to the development of bifunctional catalysts that exhibit significant efficiency in both HER and OER, and their interfacial properties are investigated for the first time. The chemical composition and morphology of g-C<sub>3</sub>N<sub>4</sub> integrated with Co–Ni nanoparticles significantly influence the modulation of redox-active sites and the facilitation of electron transfer, resulting in improved splitting efficiency. The interactions between the Co–Ni bimetal and g-C<sub>3</sub>N<sub>4</sub> demonstrate exceptional electrochemical performance for water splitting. Consequently, the 20% 20–Co–Ni–graphitic carbon nitride electrode demonstrated superior HER performance, comparable to the other electrodes. In the results, it is indicated that an increased molar ratio of Co and Ni incorporated in graphitic carbon nitride significantly improves HER performance.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 1","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143118050","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Investigating the Impact of Hydrogen Bonding on Silicon Nitride (SiNx) Film
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-22 DOI: 10.1002/ente.202400761
Hasnain Yousuf, Alamgeer Khan, Muhammad Quddamah Khokhar, Rafi ur Rahman, Polgampola Chamani Madara, Jaljalalul Abedin Jony, Muhammad Aleem Zahid, Youngkuk Kim, Junsin Yi
{"title":"Investigating the Impact of Hydrogen Bonding on Silicon Nitride (SiNx) Film","authors":"Hasnain Yousuf,&nbsp;Alamgeer Khan,&nbsp;Muhammad Quddamah Khokhar,&nbsp;Rafi ur Rahman,&nbsp;Polgampola Chamani Madara,&nbsp;Jaljalalul Abedin Jony,&nbsp;Muhammad Aleem Zahid,&nbsp;Youngkuk Kim,&nbsp;Junsin Yi","doi":"10.1002/ente.202400761","DOIUrl":"https://doi.org/10.1002/ente.202400761","url":null,"abstract":"<p>The deposition of amorphous hydrogenated silicon nitride (a-SiN<sub><i>x</i></sub>:H) via plasma-enhanced chemical vapor deposition is critical for optimizing the performance of crystalline silicon (c-Si) solar cells. This study investigates the impact of varying gas ratios (GR = NH<sub>3</sub>/SiH<sub>4</sub>) on the optical and physical properties of deposited SiN<sub><i>x</i></sub> films. Results show that the refractive index (RI) ranges from 1.8 to 2.3 with changing gas compositions. Fourier transform infrared Spectroscopy reveals shifts in [SiN<span></span>H] and [Si<span></span>H] stretching modes, indicating changes in hydrogen passivation and nitrogen incorporation. Hydrogen bonding densities of [Si<span></span>H] and [SiN<span></span>H] correlate positively with the RI. For example, the hydrogen bonding density [N<sub>H</sub>] ranges from 4.53 × 10<sup>23</sup> to 6.32 × 10<sup>23</sup> cm<sup>−3</sup> for [SiN<span></span>H] bonds while [Si-H] varies from 6.93 × 10<sup>23</sup> to 1.06 × 10<sup>24</sup> cm<sup>−3</sup>. Secondary ion mass spectrometry (SIMS) analysis shows stable hydrogen intensity, contrasting with a decrease in nitrogen<span></span>hydrogen bonds. These findings highlight the key role of hydrogen bonding in determining SiN<sub><i>x</i></sub> film properties, with significant implications for semiconductor and photovoltaic applications.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 1","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143118225","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
An Experimental Investigation on Synthesis, Characterization, and Photothermal Conversion Efficiency of Stable Aqueous Nanofluids Containing Multiwalled Carbon Nanotubes for Direct Absorption Solar Collectors
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-21 DOI: 10.1002/ente.202400784
John George, Meledath Sadanandan Sreekanth
{"title":"An Experimental Investigation on Synthesis, Characterization, and Photothermal Conversion Efficiency of Stable Aqueous Nanofluids Containing Multiwalled Carbon Nanotubes for Direct Absorption Solar Collectors","authors":"John George,&nbsp;Meledath Sadanandan Sreekanth","doi":"10.1002/ente.202400784","DOIUrl":"https://doi.org/10.1002/ente.202400784","url":null,"abstract":"<p>The nanofluids are the potential substitute in solar collectors as working fluids for better photothermal conversion efficiency. The present investigation focuses on the development of aqueous-based nanofluids comprising multiwalled carbon nanotubes (MWCNTs) with and without surfactants to enhance the capacity of photothermal conversion in direct absorption solar collectors. To improve the stability of the nanofluid, the gum Arabic (GA) and polyvinyl alcohol (PVA) are used as the surfactants. The stable nanofluid was characterized using UV-visible spectroscopy, zeta potential, fourier-transform infrared spectroscopy, field emission scanning electron microscopy, and energy dispersive X-ray spectroscopy (EDS) analysis. The results indicated that the thermal conductivity was enhanced by 94.57% and 91.19% for the MWCNT/GA/deionized (DI) water and MWCNTs/PVA/DI water based nanofluids in presence of surfactants at 90 °C and 0.02 wt%. The presence of surfactant in MWCNTs/DI water nanofluids exhibit excellent stability and enhanced MWCNTs dispersion. In the photothermal response analysis, the highest temperature of 62.8 °C, which is 16 °C higher than the base fluid, is obtained from 0.02wt% MWCNT/GA nanofluid. The highest efficiency of 27.94% is recorded when 0.02wt% MWCNT/GA nanofluid is used, which shows 71.24% enhancement as compared to the DI water after exposure of 30 minutes under solar irradiation. The use of MWCNTs/GA nanofluid as light-absorbing working fluids in solar collectors is encouraged in the present investigation.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 1","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143117674","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Convenient Aqueous-Phase Synthesis of Covalent Organic Frameworks for Anhydrous Proton Conduction
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-21 DOI: 10.1002/ente.202400381
Haiyan Tao, Shuping Jia, Weixiong Dong, Abdukader Abdukayum, Lifeng Zhao
{"title":"Convenient Aqueous-Phase Synthesis of Covalent Organic Frameworks for Anhydrous Proton Conduction","authors":"Haiyan Tao,&nbsp;Shuping Jia,&nbsp;Weixiong Dong,&nbsp;Abdukader Abdukayum,&nbsp;Lifeng Zhao","doi":"10.1002/ente.202400381","DOIUrl":"https://doi.org/10.1002/ente.202400381","url":null,"abstract":"<p>Covalent organic frameworks (COFs) as a kind of emerging materials has been widely concerned. Developing and recovering new COF materials is of great importance for anhydrous proton conduction, most of the synthesis methods are not organic solvent phase or convenient enough, which would inevitably lead to solvent waste and increase environmental burden. Herein, a method of COF synthesis in aqueous phase is developed, which is used for nonpolluting and sustainable fabrication. Benefits from the suitable channels and stability of HCOF-1, the composite material H<sub>3</sub>PO<sub>4</sub>@HCOF-1 exhibit high proton conductivity (1.29 × 10<sup>−4</sup> S cm<sup>−1</sup>) at 413 K and the crystallinity of HCOF-1 is maintained well after measurements. This work broadens the scope of COF synthesis and promotes the development of anhydrous proton conduction.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 1","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143117676","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Summary, Future, and Challenges of Fluoride-Ion Batteries
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-16 DOI: 10.1002/ente.202401374
Jingwen Li, Mingqiang Li, Haochen Weng, Shuailiang Xu
{"title":"Summary, Future, and Challenges of Fluoride-Ion Batteries","authors":"Jingwen Li,&nbsp;Mingqiang Li,&nbsp;Haochen Weng,&nbsp;Shuailiang Xu","doi":"10.1002/ente.202401374","DOIUrl":"https://doi.org/10.1002/ente.202401374","url":null,"abstract":"<p>Due to the limitations of lithium-ion batteries (LIBs), there is an urgent need to explore alternative energy storage technologies. However, the high-energy density of fluoride-ion batteries (FIBs) has attracted widespread attention as a potential successor to LIBs. FIBs are emerging as a low-cost, safe, and versatile energy storage solution, with a broad operating temperature range. With continuous efforts from researchers, significant progress has been made in the field of FIBs. Nevertheless, compared to traditional batteries, research on FIBs remains limited, and many challenges and unexplored avenues persist. This article elucidates the principles of FIBs, summarizes the materials for both cathodes and anodes, discusses electrolytes, and addresses existing issues. It also outlines future directions and potential applications of FIBs. As it is continued to innovate and explore, FIBs hold promise for revolutionizing energy storage technology, offering enhanced performance, safety, and sustainability.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 1","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143115684","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hybrid Wind-Solar Self-Powered Detector System Using a Triboelectric-Photovoltaic Generator for Smart Agriculture 使用三电-光伏发电机的风能-太阳能混合自供电探测器系统,用于智能农业
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-15 DOI: 10.1002/ente.202401281
Jing Zhao, Xinrui Li, Xiaolei Lu, Mingxing Cui, Wendong Qi, Dongming Wang, Ruifang Zheng, Xin Yu
{"title":"Hybrid Wind-Solar Self-Powered Detector System Using a Triboelectric-Photovoltaic Generator for Smart Agriculture","authors":"Jing Zhao,&nbsp;Xinrui Li,&nbsp;Xiaolei Lu,&nbsp;Mingxing Cui,&nbsp;Wendong Qi,&nbsp;Dongming Wang,&nbsp;Ruifang Zheng,&nbsp;Xin Yu","doi":"10.1002/ente.202401281","DOIUrl":"https://doi.org/10.1002/ente.202401281","url":null,"abstract":"<p>The growth of crops is affected by factors such as temperature, humidity, and salinity, so it is critical to monitor these indicators through detectors in smart agriculture. Collecting renewable energy in the farmland environment to power the detector will provide a feasible approach. Therefore, a triboelectric-photovoltaic hybrid generator (WS-TPHG) is proposed to collect solar and wind energy efficiently. The generator structure includes a photovoltaic panel (PV) and a wind-driven triboelectric nanogenerator (W-TENG). The switching function of the power supply can be realized through the power management circuit. In the case of sufficient light, the detector is powered by PV steadily, and in the case of insufficient light, the detector is powered by W-TENG via the switching function. The PV can supply a stable voltage of 8.1 V, and the open-circuit voltage (<i>V</i><sub>OC</sub>) of W-TENG can reach 478.6 V at 180 rpm. The results verify that the detection of temperature, humidity, and salinity can be successfully achieved through the detector which is powered by WS-TPHG. In this article, the potential application of WS-TPHG is demonstrated in farmland to provide a solution for the sustainable development of agriculture.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 3","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143565432","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Doping Strategies for Improving Performance of Li-Argyrodite Solid-State Electrolyte
IF 3.6 4区 工程技术
Energy technology Pub Date : 2024-10-15 DOI: 10.1002/ente.202401420
Qianjin Huang, Yinglei Wu, Zhongyi He, Sirui Wang, Jinhui Zhu, Xiaodong Zhuang
{"title":"Doping Strategies for Improving Performance of Li-Argyrodite Solid-State Electrolyte","authors":"Qianjin Huang,&nbsp;Yinglei Wu,&nbsp;Zhongyi He,&nbsp;Sirui Wang,&nbsp;Jinhui Zhu,&nbsp;Xiaodong Zhuang","doi":"10.1002/ente.202401420","DOIUrl":"https://doi.org/10.1002/ente.202401420","url":null,"abstract":"<p>Li-argyrodite solid-state electrolyte (SSE) holds promise for all-solid-state lithium batteries (ASSLB) but faces limitations in room-temperature ionic conductivity, electrode/electrolyte interface compatibility, and air stability. Doping strategies offer a viable approach to address these challenges. This article provides a comprehensive review of the structure–property relationships and recent doping strategies for Li-argyrodite electrolytes. First, the crystal structural features are analyzed to elucidate the intrinsic relationship between the structure and key properties, including ionic conductivity and the electrochemical window. Second, the mechanisms by different dopants affecting the performance of Li-argyrodite electrolytes are investigated, focusing on ionic conductivity, air stability, thermal stability, electrochemical performance, and interfacial stability. Finally, the current status and future development trends of Li-argyrodite SSE are summarized, and targeted strategies are proposed to enhance the application in ASSLB.</p>","PeriodicalId":11573,"journal":{"name":"Energy technology","volume":"13 1","pages":""},"PeriodicalIF":3.6,"publicationDate":"2024-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143115534","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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