Composites Part B: Engineering最新文献

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Orthogonal orientation incorporated gradient-sandwich structure for enhanced energy storage performance of all-inorganic nanocomposites 正交取向结合梯度夹层结构增强了全无机纳米复合材料的储能性能
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-08 DOI: 10.1016/j.compositesb.2025.112673
Yang Liu , Bingzhong Shen , Bo Xie , Zaiying Li , Jianhong Kang , Yueqing Jiang , Rui Zhang
{"title":"Orthogonal orientation incorporated gradient-sandwich structure for enhanced energy storage performance of all-inorganic nanocomposites","authors":"Yang Liu ,&nbsp;Bingzhong Shen ,&nbsp;Bo Xie ,&nbsp;Zaiying Li ,&nbsp;Jianhong Kang ,&nbsp;Yueqing Jiang ,&nbsp;Rui Zhang","doi":"10.1016/j.compositesb.2025.112673","DOIUrl":"10.1016/j.compositesb.2025.112673","url":null,"abstract":"<div><div>Dielectric energy storage capacitors, widely used in advanced domains of electronics and power, play a crucial role in electronic systems. However, current challenges stem from the coupled limitations of polarization and breakdown field strength in dielectric capacitors, which present significant obstacles to achieving a breakthrough in energy storage performance. Here, we propose an orthogonal design for all-inorganic nanocomposite using innovative composite molding techniques. The increased path tortuosity is tailored during the electrical treeing process through the orthogonal distribution of ferroelectric nanofillers, ensuring the preservation of high breakdown strength and polarization. Meanwhile, a gradient-sandwich multilayer configuration is developed to leverage the interfacial polarization effect and interface barrier effect between adjacent layers. Hence, integrating a gradient electric field distribution enhances both the polarization and breakdown strength of the nanocomposites, ultimately resulting in a significant improvement in energy storage performance. The ultrahigh energy density of 24.5 J cm<sup>−3</sup> at a low electric field of 1700 kV cm<sup>−1</sup> is obtained in orthogonal orientation gradient-sandwich structure ≈1.8 times that of the parallel filler orientations nanocomposites. Incorporating the orthogonal orientation and gradient-sandwich structure strategy significantly enhances energy output, making it suitable for a wide range of electronic devices.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"305 ","pages":"Article 112673"},"PeriodicalIF":12.7,"publicationDate":"2025-06-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144279934","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Tackling data scarcity in machine learning-based CFRP drilling performance prediction through a broad learning system with virtual sample generation (BLS-VSG) 基于虚拟样本生成(BLS-VSG)的广义学习系统解决基于机器学习的CFRP钻井性能预测中的数据稀缺性问题
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-07 DOI: 10.1016/j.compositesb.2025.112701
Jia Ge , Zequan Yao , Ming Wu , José Humberto S. Almeida Jr , Yan Jin , Dan Sun
{"title":"Tackling data scarcity in machine learning-based CFRP drilling performance prediction through a broad learning system with virtual sample generation (BLS-VSG)","authors":"Jia Ge ,&nbsp;Zequan Yao ,&nbsp;Ming Wu ,&nbsp;José Humberto S. Almeida Jr ,&nbsp;Yan Jin ,&nbsp;Dan Sun","doi":"10.1016/j.compositesb.2025.112701","DOIUrl":"10.1016/j.compositesb.2025.112701","url":null,"abstract":"<div><div>Machine learning (ML)-based data-driven method has emerged as a powerful tool for predicting the manufacturing performance of carbon fibre reinforced plastic (CFRP), particularly in CFRP machining, where physics-based models are computationally expensive. However, the effectiveness of ML models are often constrained by limited datasets, due to the high cost and time required for experimental data acquisition. To address this, this paper presents the first study to apply virtual sample generation (VSG) techniques to enlarge the training dataset and mitigate data scarcity in the prediction of CFRP drilling performance. A novel hybrid ML framework integrating Broad Learning System (BLS) and VSG (BLS-VSG) is proposed to combine the capability of BLS in small dataset prediction with the enlarged dataset generated by VSG. The model has been employed to predict the drilling thrust force and delamination damage under various drilling conditions (spindle speed, feed rate, point angle). Three different VSG methods (SMOTE, MD-MTD and CVT) and the number of virtual samples were evaluated in detail. Results show that VSG can effectively enlarge the training dataset and improve the prediction performance of the ML model. Specifically, VSG reduced the mean square error (MSE) and mean absolute percentage error (MAPE) for thrust force prediction by 39.0 % and 12.9 %, respectively, compared to the benchmark without VSG. For delamination factor F<sub>da</sub> prediction, MSE and MAPE were reduced by 22.6 % and 16.5 %, respectively. The proposed BLS-VSG model outperforms other conventional ML models (BPNN, ELM, SVR and RT) for both scenarios (with/without VSG), providing a robust and data-efficient solution for CFRP drilling performance prediction.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"305 ","pages":"Article 112701"},"PeriodicalIF":12.7,"publicationDate":"2025-06-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144314318","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Compression resistance of CFRP/mater fractal nested structures based on self-similar fractal strategy 基于自相似分形策略的CFRP/mater分形嵌套结构抗压性能
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-07 DOI: 10.1016/j.compositesb.2025.112698
Xiaoli Xu , Wenzhen Huang , Jianxing Yang , Sipei Cai , Jiacheng Wu , Yong Zhang
{"title":"Compression resistance of CFRP/mater fractal nested structures based on self-similar fractal strategy","authors":"Xiaoli Xu ,&nbsp;Wenzhen Huang ,&nbsp;Jianxing Yang ,&nbsp;Sipei Cai ,&nbsp;Jiacheng Wu ,&nbsp;Yong Zhang","doi":"10.1016/j.compositesb.2025.112698","DOIUrl":"10.1016/j.compositesb.2025.112698","url":null,"abstract":"<div><div>The plastic deformation of metallic structures is promising to improving the load-bearing instability of carbon fiber-reinforced polymer (CFRP) thin-walled structures. Therefore, this study proposes a novel self-similar fractal strategy of CFRP/stainless steel nested structure to fully exploit the mechanical advantages of distinct materials. The structure consists of an outer quadrilateral CFRP tube nested with an internal stainless-steel fractal substructure, named the Quadrilateral Fractal Nested Structure (QFNS). Through the compression test, it is found that the CFRP/stainless steel nested structure has more stable mechanical loading behavior compared with the pure metal structure. Numerical simulations further explored the energy contribution mechanism, which reveals that the load-bearing capacity of QFNS surpasses the combined performance of its individual components, emphasizing the significant interaction effect between internal and external structures. In addition, the fractal order, the number of paving layers and the fractal wall thickness significantly affect its crashworthiness. In particular, when the fractal order increases from 0 to 2, the specific absorption energy increases (SEA) by 122.97 %. Moreover, compared to typical CFRP/metal structures, the self-similar fractal design elevates SEA by 110.39 %. This study provides a cost-effective, lightweight solution with simplified assembly for designing high-performance protective structures.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"304 ","pages":"Article 112698"},"PeriodicalIF":12.7,"publicationDate":"2025-06-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144242878","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of non-uniform roving-matrix-CSM architecture on the flange-web interface behavior of pultruded GFRP composite members 非均匀粗纱-基体- csm结构对拉挤GFRP复合材料法兰-腹板界面性能的影响
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-06 DOI: 10.1016/j.compositesb.2025.112684
TianQiao Liu , Shilong Zhen , Zhengfu Wang , Peng Feng , Kent A. Harries , Yejun Luo , Ke Tang , Youkun Gong
{"title":"Effect of non-uniform roving-matrix-CSM architecture on the flange-web interface behavior of pultruded GFRP composite members","authors":"TianQiao Liu ,&nbsp;Shilong Zhen ,&nbsp;Zhengfu Wang ,&nbsp;Peng Feng ,&nbsp;Kent A. Harries ,&nbsp;Yejun Luo ,&nbsp;Ke Tang ,&nbsp;Youkun Gong","doi":"10.1016/j.compositesb.2025.112684","DOIUrl":"10.1016/j.compositesb.2025.112684","url":null,"abstract":"<div><div>Pultruded glass fiber reinforced polymer (PGFRP) composites are heterogenous compositions of glass roving, continuous strand mat (CSM) and resin matrix. Nonetheless, PGFRPs are considered to be idealized homogeneous materials for structural design. Unintended variation of roving-matrix-CSM (RMC) architecture can result in a reduction in PGFRP flexural member capacity. The objective of this study is to investigate the effect of non-uniform RMC architecture on the performance of PGFRP members subject to flexure, focusing on the failure mode characterized by cracking at the flange-web junctions of such members. This study considers five PGFRP shapes – box, I, C, T and L – and quantifies non-unform RMC architecture for 18 sections. A robust FE model capturing the individual roving and CSM layers of the PGFRP was developed, and both non-uniform and idealized uniform RMC architectures were modeled in every case allowing the effect of RMC architecture variation to be investigated. Three-dimensional Hashin damage criterion was implemented to predict the progressive failure of PGFRP materials in an accurate and repeatable manner. A parametric study varying fiber volume ratio, CSM proportion and shear span resulted in 360 separate FE models. Study conclusions demonstrate the increased sensitivity of box shapes to variations in RMC architecture with reductions in capacity compared to idealized RMC architecture exceeding 20% in some cases.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"305 ","pages":"Article 112684"},"PeriodicalIF":12.7,"publicationDate":"2025-06-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144263713","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A review of recent research on bionic structural characteristics and performance mechanisms of biomimetic materials 综述了仿生材料的仿生结构特征及性能机理
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-05 DOI: 10.1016/j.compositesb.2025.112681
Wang Haipeng , Li Shaomin , Zhou Qijie , Peng Haichun , Liu Xiaolin , Shao Zhenyu , Song Peng
{"title":"A review of recent research on bionic structural characteristics and performance mechanisms of biomimetic materials","authors":"Wang Haipeng ,&nbsp;Li Shaomin ,&nbsp;Zhou Qijie ,&nbsp;Peng Haichun ,&nbsp;Liu Xiaolin ,&nbsp;Shao Zhenyu ,&nbsp;Song Peng","doi":"10.1016/j.compositesb.2025.112681","DOIUrl":"10.1016/j.compositesb.2025.112681","url":null,"abstract":"<div><div>Lightweight structures with high energy absorption (EA) performance are of great significance in many crucial fields. Biomimetic structural design has demonstrated an effective strategy to improve the performance of both materials and structures by incorporating the unique structural characteristics of natural organisms. This review paper provides an in-depth and comprehensive overview of some important advances in structural design to obtain novel bio-inspired structures with improved energy absorption properties. The structural designs are categorized and summarized based on the common characteristics of biomimetic structures and their bio-inspired sources, and detailedly introduced in terms of the structural configurations, manufacturing processes, analysis methods and energy absorption properties as well as the comparative analysis of performance indicators. Moreover, the application investigations of biomimetic lightweight structures across diverse engineering domains are explored. The introduction of biomimetic structural characteristics indeed significantly improved the structural energy absorption performance and crashworthiness while maintaining the similar overall weight. This phenomenon drives many researchers to devote themselves to this investigations, and continuously achieve new research results. Meanwhile, the endless variety of biological species in nature provides inexhaustible sources for biomimetic structural designs. However, most of these investigations stop at laboratory and are difficult to achieve actual applications due to their various limitations such as manufacturing processes, serviceability in specific environments, the cost of innovative materials and production, product maturity, and the feasibility and cost of mass production. In short, the biomimetic lightweight structures present great potential and broad application prospects, but there are still many challenges to the practical applications.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"304 ","pages":"Article 112681"},"PeriodicalIF":12.7,"publicationDate":"2025-06-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144231677","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Development of self-healing composite membranes with enhanced conductivity for wearable electronics 可穿戴电子产品导电性增强的自修复复合膜的研制
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-05 DOI: 10.1016/j.compositesb.2025.112676
Md Ikram Hossen , Yaqing Wang , Hao Zhang , Na Li , Xin Hu , Danish Iqbal , Naveed Iqbal , Yan He , Yuanyuan Shang , Kelvin Fu , Baohui Shi
{"title":"Development of self-healing composite membranes with enhanced conductivity for wearable electronics","authors":"Md Ikram Hossen ,&nbsp;Yaqing Wang ,&nbsp;Hao Zhang ,&nbsp;Na Li ,&nbsp;Xin Hu ,&nbsp;Danish Iqbal ,&nbsp;Naveed Iqbal ,&nbsp;Yan He ,&nbsp;Yuanyuan Shang ,&nbsp;Kelvin Fu ,&nbsp;Baohui Shi","doi":"10.1016/j.compositesb.2025.112676","DOIUrl":"10.1016/j.compositesb.2025.112676","url":null,"abstract":"<div><div>Flexible and conductive electronics are transforming wearable technologies, yet achieving a balance between high conductivity and self-healing capabilities remains a critical challenge. In this study, we present a conductive self-healing membrane (CSHM) fabricated through electrospinning polyurethane and coated it with liquid metal. This approach integrates mechanical stretchability, electrical conductivity, and self-repair properties into a single material system, addressing key limitations in flexible electronics. The membrane exhibits exceptional performance, with tensile strength recovering to 97 % after 24 h of healing at 40 °C. Its durability is further validated through cyclic tensile tests, where the resistance showed only a slight increase after 10,000 stretching cycles at 100 % strain, indicating excellent electrical stability. The membrane's ability to restore conductivity after damage was confirmed through resistance-time analysis and practical applications, including powering LED circuits.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"305 ","pages":"Article 112676"},"PeriodicalIF":12.7,"publicationDate":"2025-06-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144279939","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Buckling and fracture analysis of three-dimensional four-directional braided composite tubes with cutouts under axial compression 三维四向带切口编织复合材料管轴压屈曲与断裂分析
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-04 DOI: 10.1016/j.compositesb.2025.112680
Hao Song , Haojie Xu , Yutao Wang , Kangmei Li , Jun Hu
{"title":"Buckling and fracture analysis of three-dimensional four-directional braided composite tubes with cutouts under axial compression","authors":"Hao Song ,&nbsp;Haojie Xu ,&nbsp;Yutao Wang ,&nbsp;Kangmei Li ,&nbsp;Jun Hu","doi":"10.1016/j.compositesb.2025.112680","DOIUrl":"10.1016/j.compositesb.2025.112680","url":null,"abstract":"<div><div>The mechanical properties of cutouts are a key issue in the engineering application of three-dimensional four-directional(3D4D) braided composite tubes. In this study, numerical and experimental methods were used to investigate the effect of different hole diameters on the buckling properties of 3D4D braided composite tubes under axial loading. In the numerical part, microscale RVE model and mesoscale RVE model were established to predict the elastic properties by applying the multiscale finite element method, and the accuracy of them was verified by theoretical calculations. A macroscale-mesoscale coupling model was established to perform linear buckling and nonlinear analysis of braided tubes with different hole sizes to predict the buckling behavior of 3D4D braided composite tubes. The simulation results show that the buckling load decreases with the increase of the hole sizes. In the experimental part, specimens were prepared by braiding process, axial compression experiments were carried out until failure and full-field displacements and strain distribution were recorded by digital image correlation(DIC) technique. Smaller holes enable fiber-dominated strain transfer networks, medium-sized holes trigger matrix-fiber cooperative failure, whereas larger holes induce strain localization and premature failure through interface debonding.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"305 ","pages":"Article 112680"},"PeriodicalIF":12.7,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144270122","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Getting in line: Filler alignment strategies for anisotropic composite fabrication 排队:各向异性复合材料制造的填料对齐策略
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-04 DOI: 10.1016/j.compositesb.2025.112626
Dong Hae Ho , Yoon Young Choi , Seung Yeon Ki , Dong-Hwan Kim , Jeong Ho Cho
{"title":"Getting in line: Filler alignment strategies for anisotropic composite fabrication","authors":"Dong Hae Ho ,&nbsp;Yoon Young Choi ,&nbsp;Seung Yeon Ki ,&nbsp;Dong-Hwan Kim ,&nbsp;Jeong Ho Cho","doi":"10.1016/j.compositesb.2025.112626","DOIUrl":"10.1016/j.compositesb.2025.112626","url":null,"abstract":"<div><div>The growing demand for high-performance materials in cutting-edge technologies has prompted intensive research into anisotropic composites, which exhibit properties that vary with direction. By aligning fillers within a matrix, it is possible to harness the distinct advantages of each filler with minimal loading, allowing for the production of lightweight, highly functional polymeric composites at a fraction of the cost of conventional engineering materials. This review examines fabrication techniques that induce anisotropy through controlled filler orientation and concentration. We categorize these methods by their principal alignment mechanisms: mechanically induced, field-induced, template-/scaffold-based, and self-assembly-driven, along with hybrid approaches. Each category offers unique benefits and faces distinct challenges in achieving targeted filler orientation and, consequently, in tuning the resultant anisotropic properties. This review also discusses the factors influencing filler alignment and how they enhance the mechanical and conductive performance of anisotropic composites.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"305 ","pages":"Article 112626"},"PeriodicalIF":12.7,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144255373","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High-performance, eco-friendly calcium carbonate cement via alginate-mediated biomimetic mineralisation 高性能,环保碳酸钙水泥通过海藻酸介导的仿生矿化
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-04 DOI: 10.1016/j.compositesb.2025.112696
Olivia de Souza Heleno Santos , Wendy Tian , Kwong Ming Tse , Yali Li
{"title":"High-performance, eco-friendly calcium carbonate cement via alginate-mediated biomimetic mineralisation","authors":"Olivia de Souza Heleno Santos ,&nbsp;Wendy Tian ,&nbsp;Kwong Ming Tse ,&nbsp;Yali Li","doi":"10.1016/j.compositesb.2025.112696","DOIUrl":"10.1016/j.compositesb.2025.112696","url":null,"abstract":"<div><div>Calcium carbonate-based binders offer significant environmental advantages, particularly in carbon capture and sustainable construction. Inspired by the organic matrix in biomineralisation, this study investigates sodium alginate as a functional additive and matrix to enhance calcium carbonate cement. Incorporating 1.5 wt% sodium alginate within the mineralisation system yielded a lightweight composite with a compressive strength of 46 MPa and an elastic modulus of 800 MPa after 28 days of curing – improvements of 1084 % and 155 %, respectively, compared to alginate-free samples. The phase evolution and structural development influenced by alginate were extensively characterised using X-ray diffraction, thermogravimetric analysis, attenuated total reflection infrared analysis, scanning electron microscopy, and transmission electron microscopy. Alginate was pivotal in nucleating and stabilising amorphous calcium carbonate, orienting its subsequent transformation into spherulitic calcite. Micro-computed tomography analysis under compression revealed the exceptional elasticity and toughness of the alginate composites. It further elucidated the defects distribution of different features of the stabilisation and crystallisation within the composites before, during, and after compression. These findings underscore the critical role of biopolymer-mediated mineralisation in engineering high-performance, cementitious calcium carbonate composites. Beyond CO<sub>2</sub> sequestration, this environmentally friendly material offers promising applications in sustainable construction and advanced composite systems.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"304 ","pages":"Article 112696"},"PeriodicalIF":12.7,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144231676","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Durable and temperature-adapted flexible rechargeable zinc-air batteries enabled by in-situ encapsulated FeMo alloy nanoparticles within nitrogen-doped carbon particles cathode 在氮掺杂碳颗粒阴极内原位封装FeMo合金纳米颗粒,实现了耐用且适应温度的柔性可充电锌空气电池
IF 12.7 1区 材料科学
Composites Part B: Engineering Pub Date : 2025-06-04 DOI: 10.1016/j.compositesb.2025.112695
Jicai Hu , Shengcui Pang , Shulin Gao, Hang Yu, Nan Duan, Sujuan Hu
{"title":"Durable and temperature-adapted flexible rechargeable zinc-air batteries enabled by in-situ encapsulated FeMo alloy nanoparticles within nitrogen-doped carbon particles cathode","authors":"Jicai Hu ,&nbsp;Shengcui Pang ,&nbsp;Shulin Gao,&nbsp;Hang Yu,&nbsp;Nan Duan,&nbsp;Sujuan Hu","doi":"10.1016/j.compositesb.2025.112695","DOIUrl":"10.1016/j.compositesb.2025.112695","url":null,"abstract":"<div><div>Flexible rechargeable zinc-air batteries (FRZABs) are highly desirable for portable and wearable electronics due to their high energy density and safety. However, achieving reliable performance of FRZABs across a broad temperature range remains challenging due to inherent cathode limitations. These challenges include not only insufficient oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) kinetics at high and low temperatures but also poor structural and interfacial stability across temperature. Herein, we report a novel self-growth strategy to synthesize a composite cathode catalyst comprising FeMo alloy nanoparticles embedded on nitrogen-doped porous carbon particles (FeMo/NCPs). Notably, benefiting from rapid electron transfer, a protective structural framework of the carbon matrix, and abundant active sites of the FeMo/NCPs, the FRZABs exhibit excellent ORR performance with an <em>E</em><sub><em>1/2</em></sub> as high as 0.85 V, and an OER overpotential of 390 mV at a current density of 10 mA cm<sup>−2</sup>, as well as good structural stability and flexibility in a wide temperature range. As a proof of concept, FeMo/NCPs-based aqueous RZABs exhibit a cycling life exceeding 2720 h with a peak power density of 139 mW cm<sup>−2</sup>. FRZABs exhibit a low charge-discharge voltage gap and a discharge lifespan of 170 h at 5 mA cm<sup>−2</sup>, and remarkable tolerance to both high and low temperatures, showcasing immense application potential in wearable and portable electronic devices.</div></div>","PeriodicalId":10660,"journal":{"name":"Composites Part B: Engineering","volume":"304 ","pages":"Article 112695"},"PeriodicalIF":12.7,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144242888","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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