Resources Chemicals and Materials最新文献_第7页

Synthesis and applications of low dielectric polyimide 低介电聚酰亚胺的合成及应用

Resources Chemicals and Materials Pub Date : 2023-03-01 DOI: 10.1016/j.recm.2022.08.001

Yu Liu , Xiao-Yu Zhao , Ya-Guang Sun , Wen-Ze Li , Xiao-Sa Zhang , Jian Luan

{"title":"Synthesis and applications of low dielectric polyimide","authors":"Yu Liu , Xiao-Yu Zhao , Ya-Guang Sun , Wen-Ze Li , Xiao-Sa Zhang , Jian Luan","doi":"10.1016/j.recm.2022.08.001","DOIUrl":"https://doi.org/10.1016/j.recm.2022.08.001","url":null,"abstract":"<div><p>With the advent of the 5 G era, advanced packaging applications such as wafer-level fan-out packaging have emerged thanks to efforts to reduce signal loss and increase signal transmission rates. As one of the key materials employed in telecommunication devices, the interlayer dielectric material directly affects signal transmission and device reliability. Among them, polyimide (PI) has become an important interlayer dielectric material because of its excellent comprehensive properties. However, in order to meet the needs high-frequency and high-speed circuits for 5 G networks, it will be necessary to further reduce the dielectric constant and dielectric loss of PI. PI is widely used as a flexible dielectric material due to its excellent electrical insulation properties (dielectric constant ≈ 3.0–4.0, dielectric loss ≈ 0.02), mechanical properties, and thermal resistance. However, further reduction in the dielectric constant will be needed in order for PI-based materials to better meet the current high integration development needs of the microelectronics industry. This article starts from strategies to prepare low dielectric PI that have been developed in the last decade, based on a more systematic and inductive analysis, and prospects the development potential of low dielectric PI.</p></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"2 1","pages":"Pages 49-62"},"PeriodicalIF":0.0,"publicationDate":"2023-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49724549","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 6

Crystal structure and catalytic performance for direst oxidation of propylene to acrylic acid of MoVTeNbOx prepared by high-pressure hydrothermal synthesis 高压水热合成MoVTeNbOx的晶体结构及丙烯直接氧化制丙烯酸的催化性能

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/j.recm.2022.07.004

Yiwen Wang , Yaoxin Fan , Shuangming Li , Yujiao Wang , Yanan Chen , Dongqi Liu , Wenhui Wei , Sansan Yu

{"title":"Crystal structure and catalytic performance for direst oxidation of propylene to acrylic acid of MoVTeNbOx prepared by high-pressure hydrothermal synthesis","authors":"Yiwen Wang , Yaoxin Fan , Shuangming Li , Yujiao Wang , Yanan Chen , Dongqi Liu , Wenhui Wei , Sansan Yu","doi":"10.1016/j.recm.2022.07.004","DOIUrl":"https://doi.org/10.1016/j.recm.2022.07.004","url":null,"abstract":"<div><p>MoVTeNbO<sub>x</sub> catalysts were prepared through a high-pressure hydrothermal method, in which the crystalline structure and properties of the catalysts were tuned by varying the system pressure (0-12.0 MPa). Results showed that the system pressure had a significant influence on the structure and catalytic performance of MoVTeNbO<sub>x</sub>. Under 3.0 MPa, MoVTeNbO<sub>x</sub> prepared possessed the highest content of M1 phase (90.6%) and V<sup>5+</sup> content (60.7%), exhibiting a uniform short and thick needle-like morphology. Also, it showed excellent selectivity (79.1%) and yield (52.8%) to acrylic acid at the catalytic temperature of 380°C. However, under 4.4 and 11.6 MPa, the characteristic peaks of M1 shifted to a certain extent and the morphology changed from short and thick to slender. As a result, the V<sup>5+</sup> content of M1 (001) plane decreased, resulting in a remarkable decline of the selectivity to acrylic acid. Moreover, DFT simulation results showed that the anti-bond orbital energy of V-O bond is the highest under 3.0 MPa, while further increase of pressure leads to obvious extrusion between atoms in the internal structure of MoVTeNbO<sub>x</sub>. Moreover, it was clear that the lower the anti-bond orbital energy of V-O bond, the lower the selectivity to acrylic acid.</p></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"1 3","pages":"Pages 211-221"},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772443322000393/pdfft?md5=c37ffb318303fcf75b9b0e9b5420ddcd&pid=1-s2.0-S2772443322000393-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"91758413","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 1

Microwave vs conventional heating in hydrogen production via catalytic dry reforming of methane 微波与传统加热在甲烷催化干重整制氢中的比较

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/j.recm.2022.08.003

Seyyedmajid Sharifvaghefi , Ying Zheng

{"title":"Microwave vs conventional heating in hydrogen production via catalytic dry reforming of methane","authors":"Seyyedmajid Sharifvaghefi , Ying Zheng","doi":"10.1016/j.recm.2022.08.003","DOIUrl":"10.1016/j.recm.2022.08.003","url":null,"abstract":"<div><p>The world's energy systems are undergoing radical change driven by the commitments to achieve net zero emissions and energy independence. Development of clean hydrogen economy is of paramount importance and hydrogen is expected to play a more important role in the future energy market. An interesting way to produce hydrogen is via dry reforming reaction which uses two green house gasses (CH<sub>4</sub> and CO<sub>2</sub>) as feedstock. Dry reforming is a challenging reaction to scale-up due to its high endothermic and coke formation nature. Microwave has gained interest in the past years as a superior heating mechanism in catalytic reactions due to its capacity in enhancing conversions of reactants and selectivity of products, and suppression of coke formation. Such characteristics has made microwave an excellent alternative to conventional heating in dry reforming reaction. In this study, we aim to discuss different aspects of microwave heating technology and its application in the catalytic dry reforming of methane. The advantages of microwave-assisted methane reforming are discussed via the comparison to the conventional heating.</p></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"1 3","pages":"Pages 290-307"},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772443322000423/pdfft?md5=baee39ee9e26e206d87b9a365d2a090a&pid=1-s2.0-S2772443322000423-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77205364","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 8

Adsorptive removal and catalytic performance of metal-organic frameworks containing mixed azolium-bipyridine ligand 含混合偶氮-联吡啶配体的金属-有机骨架的吸附去除及催化性能

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/j.recm.2022.07.003

Nadia Gholampour , Chizoba I. Ezugwu , Shima Rahmdele , Ali Ghanadzadeh Gilanie , Francis Verpoort

{"title":"Adsorptive removal and catalytic performance of metal-organic frameworks containing mixed azolium-bipyridine ligand","authors":"Nadia Gholampour , Chizoba I. Ezugwu , Shima Rahmdele , Ali Ghanadzadeh Gilanie , Francis Verpoort","doi":"10.1016/j.recm.2022.07.003","DOIUrl":"https://doi.org/10.1016/j.recm.2022.07.003","url":null,"abstract":"<div><p>Two ligands, 1, 3-bis(4-carboxyphenyl)imidazolium chloride and 4, 4-bipyridine, were employed to prepare nickel and zinc azolium based MOFs, Ni-MOF and Zn-MOF by the mixed ligand solvothermal approach. The positively charged azolium moieties in the imidazolium linker resulted in a charged environment in the as-synthesized frameworks. As a result, Ni-MOF and Zn-MOF demonstrated preferential adsorption of CO<sub>2</sub> over methane molecules in the gas phase adsorption due to the higher quadruple moment of CO<sub>2</sub>, which interacts more with the positively charged frameworks. Besides, in aqueous media, Ni-MOF and Zn-MOF exhibited incredible adsorption efficiency for anionic dyes. In the following, Ni-MOF was metallated at the carbene site of the azolium linker to generate the novel heterogeneous catalyst Pd/Ni-MOF, which was successfully applied for Sonogashira and Suzuki-Miyaura coupling reactions without losing its activity after three cycles.</p></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"1 3","pages":"Pages 201-210"},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S277244332200037X/pdfft?md5=2cf78dd3705f1a9c49eb173dcc80ed4e&pid=1-s2.0-S277244332200037X-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"91773613","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 3

Dielectric elastomer actuators for artificial muscles: A comprehensive review of soft robot explorations 人造肌肉用介电弹性体作动器:软体机器人研究的综合综述

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/j.recm.2022.09.001

Yuhao Wang , Xuzhi Ma , Yingjie Jiang , Wenpeng Zang , Pengfei Cao , Ming Tian , Nanying Ning , Liqun Zhang

{"title":"Dielectric elastomer actuators for artificial muscles: A comprehensive review of soft robot explorations","authors":"Yuhao Wang , Xuzhi Ma , Yingjie Jiang , Wenpeng Zang , Pengfei Cao , Ming Tian , Nanying Ning , Liqun Zhang","doi":"10.1016/j.recm.2022.09.001","DOIUrl":"10.1016/j.recm.2022.09.001","url":null,"abstract":"<div><p>Dielectric elastomer actuators (DEAs) artificial muscle is a typical interdisciplinary research category, which has developed by leaps and bounds in the past 20 years, showing great application prospects in various fields. Upon external electrical stimulation, dielectric elastomers (DEs) display large deformation, high energy density and fast response, affording a promising material candidate for soft robotics. Herein, the working mechanisms, commonly used materials as well as the concepts for improving the performance of DEA materials are introduced. Various DEA driven soft robots, including soft grippers, bioinspired artificial arms, crawling/walking/underwater/flying/jumping soft robots and tunable lenses, are then described in detail. Finally, the main challenges of DEA driven soft robots are summarized, and some perspectives for promoting the practical application of DEAs are also proposed.</p></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"1 3","pages":"Pages 308-324"},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772443322000447/pdfft?md5=ba57ec05836153c774d48cde383a43e0&pid=1-s2.0-S2772443322000447-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77987066","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 5

Outside Back Cover 外封底

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/S2772-4433(22)00053-8

引用次数: 0

Introduction of ZnO, Sn, and P promoters in CuO/CeO2 catalysts for improved production of dimethyldichlorosilane in the Rochow-Müller reaction 在rochow - m<s:1> ller反应中引入ZnO、Sn和P促进剂以提高二甲二氯硅烷的产量

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/j.recm.2022.07.001

Xinyang Li , Yongxia Zhu , Baofang Jin , Yongjun Ji , Lei Shi , Dongxing Fu , Dingrong Bai , Fabing Su

引用次数: 1

A mini review on recent advances in thermocatalytic hydrogenation of carbon dioxide to value-added chemicals and fuels 综述了二氧化碳热催化加氢制取增值化学品和燃料的最新进展

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/j.recm.2022.07.002

Heng Zhao , Chunyang Zeng , Noritatsu Tsubaki

{"title":"A mini review on recent advances in thermocatalytic hydrogenation of carbon dioxide to value-added chemicals and fuels","authors":"Heng Zhao , Chunyang Zeng , Noritatsu Tsubaki","doi":"10.1016/j.recm.2022.07.002","DOIUrl":"https://doi.org/10.1016/j.recm.2022.07.002","url":null,"abstract":"<div><p>The development of industrialization has led to the increased demands for carbon-based energy resources, meanwhile, excessive carbon dioxide (CO<sub>2</sub>) emission caused by industrialization has aroused enormous environmental concerns. With the proposal of global carbon neutrality, much attention has been paid to the thermocatalytic hydrogenation of CO<sub>2</sub> into value-added chemicals and fuels, which is widely considered as a promising way to alleviate carbon emission and energy shortage. CO<sub>2</sub> hydrogenation to hydrocarbons mainly undergoes a CO<sub>2</sub>-modified Fischer-Tropsch synthesis (CO<sub>2</sub>-FTS) route or a methanol-mediated (MeOH) route. However, each route needs to be further optimized and possesses its own advantages and disadvantages. In the present review, the mechanisms and primary intermediates of these two routes are firstly summarized. Hereafter, the current understandings of the relationship among catalytic performance, physical-chemical properties of catalysts and reaction conditions for each route are overviewed according to different target products, including light olefins, gasoline, jet fuel, diesel and aromatics. Finally, we provide an outlook of dual-pathway catalysts on future direction of CO<sub>2</sub> hydrogenation.</p></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"1 3","pages":"Pages 230-248"},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772443322000277/pdfft?md5=d48c93d60818c61534557e9b139d7546&pid=1-s2.0-S2772443322000277-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"91773614","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 7

Recent developments on carbon-carbon cross-coupling reactions using rare-earth metals-derived coordination polymers as efficient and selective Pd catalytic systems 利用稀土金属衍生配位聚合物作为高效、选择性钯催化体系的碳-碳交叉偶联反应研究进展

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/j.recm.2022.08.002

Valerian Dragutan , Ileana Dragutan , Gang Xiong , Lixin You , Yaguang Sun , Fu Ding

{"title":"Recent developments on carbon-carbon cross-coupling reactions using rare-earth metals-derived coordination polymers as efficient and selective Pd catalytic systems","authors":"Valerian Dragutan , Ileana Dragutan , Gang Xiong , Lixin You , Yaguang Sun , Fu Ding","doi":"10.1016/j.recm.2022.08.002","DOIUrl":"10.1016/j.recm.2022.08.002","url":null,"abstract":"<div><p>Most recent progress on the Suzuki-Miyaura, Heck and Sonogashira cross-coupling reactions, induced by heterobimetallic Pd-Ln coordination polymers as heterogeneous catalysts has been accurately reviewed. Physical-chemical characterization of the Pd-Ln composite materials by adequate physical methods revealed the distinct structure and configuration of the two- and three-dimensional frameworks. The important contribution of the coordination polymers as catalyst supports to finely modulating the catalytic activity and chemoselectivity has been considered. Published results illustrate the high activity and chemoselectivity of Pd-Ln coordination polymers in cross-coupling reactions, excellent catalyst recoverability and recyclability as well as low catalyst loading or metal leaching, under optimized reaction conditions. The particular effect of the solvent, base, aryl halide or related reagents in governing the main steps of the Pd catalytic cycle has been particularly outlined. In addition, the well-established cooperative effect of the lanthanides with palladium, with emphasis on the synergism between different metals in heterobimetallic catalytic systems, has been highlighted.</p></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"1 3","pages":"Pages 325-338"},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772443322000435/pdfft?md5=7f20ae72a3d682373c39474549e9b260&pid=1-s2.0-S2772443322000435-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"73359290","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 2

Swelling-induced morpholine functionalized adamantane-containing poly(aryl ether ketone) membranes for vanadium flow batteries 含钒液流电池用溶胀诱导的morpholine功能化含金刚烷聚芳醚酮膜

Resources Chemicals and Materials Pub Date : 2022-09-01 DOI: 10.1016/j.recm.2022.06.003

Bengui Zhang , Xueting Zhang , Qian Liu , Minghui Zhao , Zhirong Yang , Yanshi Fu , Enlei Zhang , Kangjun Wang , Guosheng Wang , Zhigang Zhang , Shouhai Zhang

{"title":"Swelling-induced morpholine functionalized adamantane-containing poly(aryl ether ketone) membranes for vanadium flow batteries","authors":"Bengui Zhang , Xueting Zhang , Qian Liu , Minghui Zhao , Zhirong Yang , Yanshi Fu , Enlei Zhang , Kangjun Wang , Guosheng Wang , Zhigang Zhang , Shouhai Zhang","doi":"10.1016/j.recm.2022.06.003","DOIUrl":"https://doi.org/10.1016/j.recm.2022.06.003","url":null,"abstract":"<div><p>Swelling-induced morpholine functionalized adamantane-containing poly(aryl ether ketone) (MAPEK) membranes were prepared for vanadium flow batteries. MAPEK membranes were prepared from chloromethylated polymer and morpholine and further swelling-induced with hot phosphoric acid to obtain membranes with enhanced ionic conductivity. The swelling, selectivity, and ionic conductivity of MAPEK membranes were regulated by varying the swelling temperature. Selective swelling-induced microphase separation in MAPEK membranes, forming wider ion transport pathways and resulting in low area resistance. The unique rigid adamantane-containing backbone limited the swelling of membranes. Consequently, MAPEK membranes showed excellent selectivity and conductivity (vanadium ion permeability coefficient of MAPEK membranes was lower than 3.82 × 0<sup>−7</sup> cm<sup>2</sup>min<sup>−1</sup>) (Nafion212 membrane, 42.5 × 0<sup>−7</sup> cm<sup>2</sup>min<sup>−1</sup>), and MAPEK-150 membrane exhibited low area resistance (0.17 Ωcm<sup>2</sup>). The vanadium flow batteries (VFB) with MAPEK-150 membrane exhibited high energy efficiency (91.1% at 80 mAcm<sup>−2</sup>, 81.4% at 200 mAcm<sup>−2</sup>). Furthermore, MAPEK membranes showed good stability in VFB and oxidative electrolytes. The swelling-induced method utilized in this work is a versatile and facile method to enhance the conductivity of ion-exchange membranes.</p></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"1 3","pages":"Pages 268-274"},"PeriodicalIF":0.0,"publicationDate":"2022-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S277244332200023X/pdfft?md5=88df140c413fdf2f2a36bb5144a8f937&pid=1-s2.0-S277244332200023X-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"91773617","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 2