Resources Chemicals and Materials最新文献

Corrigendum regarding updated Declaration of Competing Interest statements in previously published articles 关于先前发表的文章中更新的竞争利益声明的勘误表

Resources Chemicals and Materials Pub Date : 2025-09-01 DOI: 10.1016/j.recm.2025.100144

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Outside Back Cover 外封底

Resources Chemicals and Materials Pub Date : 2025-09-01 DOI: 10.1016/S2772-4433(25)00052-2

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Development of wastewater treatment methods for palm oil mill effluent (POME): A comprehensive review 棕榈油厂废水处理方法的发展综述

Resources Chemicals and Materials Pub Date : 2025-08-07 DOI: 10.1016/j.recm.2025.100130

Andriy Anta Kacaribu , Yuliani Aisyah , Febriani , Darwin

{"title":"Development of wastewater treatment methods for palm oil mill effluent (POME): A comprehensive review","authors":"Andriy Anta Kacaribu , Yuliani Aisyah , Febriani , Darwin","doi":"10.1016/j.recm.2025.100130","DOIUrl":"10.1016/j.recm.2025.100130","url":null,"abstract":"<div><div>As the world’s largest palm oil producer, Indonesia significantly benefits from its palm oil industry but also faces serious environmental challenges from palm oil mill effluent (POME)—a high-strength wastewater containing substantial organic matter, nutrients, suspended solids, and various chemical compounds. Sustainable and effective wastewater treatment strategies are urgently needed to address this issue. This review presents a comprehensive analysis of existing POME treatment technologies, including anaerobic digestion (AD), advanced oxidation processes (AOPs), membrane filtration, adsorption, phytoremediation, and microalgae-based systems. Each method is examined in terms of treatment efficiency, operational feasibility, and potential for implementation under Indonesian conditions. While advanced processes, such as AOPs and membrane filtration, achieve high pollutant removal, they are often limited by operational costs. In contrast, biological approaches, such as AD and phytoremediation, offer both environmental benefits and economic value through the recovery of biogas, biofertilizers, and biomass. This review highlights the potential for integrating wastewater purification with resource recovery and valorization, supporting a shift toward more circular and sustainable management of POME. The insights provided are intended to guide future research, inform policy decisions, and facilitate the industrial adoption of optimized treatment systems.</div></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"4 4","pages":"Article 100130"},"PeriodicalIF":0.0,"publicationDate":"2025-08-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144885595","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Magnesium leaching from dunite slurry and CO2 mineralization to form hydrated MgCO3 with different morphologies 镁浸出与CO2矿化形成不同形态的水合MgCO3

Resources Chemicals and Materials Pub Date : 2025-08-05 DOI: 10.1016/j.recm.2025.100125

Jacob Rubel , Joren De Brabander , Dharmjeet Madhav , Yukun Ji , Veerle Vandeginste

{"title":"Magnesium leaching from dunite slurry and CO2 mineralization to form hydrated MgCO3 with different morphologies","authors":"Jacob Rubel , Joren De Brabander , Dharmjeet Madhav , Yukun Ji , Veerle Vandeginste","doi":"10.1016/j.recm.2025.100125","DOIUrl":"10.1016/j.recm.2025.100125","url":null,"abstract":"<div><div>This study investigates the leaching and purification processes for dunite slurry, a common mining waste material, and the carbonation processes for the mineralization of CO<sub>2</sub> with <figure><img></figure> . Results indicate that HCl is a promising leaching agent, and pH and temperature are major factors in controlling the efficiency of the leaching process, with leaching efficiencies of 82% achieved after 4 h using 2 M HCl solution at 75 °C. The removal of other ions like <figure><img></figure> , <figure><img></figure> , and <figure><img></figure> through the purification of the leachate using ammonium hydroxide was also proven to be effective, completely removing iron and aluminum from the leachate from starting concentrations of 3.10 and 0.40 g/L, respectively. The carbonation of magnesium at room temperature was investigated with both purified leachate and pure MgCl<sub>2</sub> aqueous solution. Nesquehonite crystals began to form after 1.5 h with a conversion of <figure><img></figure> to nesquehonite of approximately 5%. The produced crystals possess a needle-like shape, which could be modified using the biopolymers pectin and xanthan. Pectin had a limited influence on the length of the crystals, reducing the needle length with increasing pectin concentration. Xanthan, on the other hand, shortened and widened the needle-like structure into a column shape as more xanthan was added. This study demonstrates the potential for this process to utilize mining wastes and sequester CO<sub>2</sub>, producing useful mineral products in the process.</div></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"4 4","pages":"Article 100125"},"PeriodicalIF":0.0,"publicationDate":"2025-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144841374","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Natural rubber composites incorporating alkali lignin: Property characterization and functional evaluation 含碱木质素的天然橡胶复合材料：性能表征和功能评价

Resources Chemicals and Materials Pub Date : 2025-07-17 DOI: 10.1016/j.recm.2025.100126

Skulrat Pichaiyut , Bunyarit Panyapinyopol , Parinvadee Chukaew , Yuwanda Thongpanich , Fuangfa Utrarachkij , Sanchai Kuboon , Wasawat Kraithong , Pongtanawat Khemthong , Kriangsak Riewklang , Kamonwat Nakason , Wanwitoo Wanmolee

{"title":"Natural rubber composites incorporating alkali lignin: Property characterization and functional evaluation","authors":"Skulrat Pichaiyut , Bunyarit Panyapinyopol , Parinvadee Chukaew , Yuwanda Thongpanich , Fuangfa Utrarachkij , Sanchai Kuboon , Wasawat Kraithong , Pongtanawat Khemthong , Kriangsak Riewklang , Kamonwat Nakason , Wanwitoo Wanmolee","doi":"10.1016/j.recm.2025.100126","DOIUrl":"10.1016/j.recm.2025.100126","url":null,"abstract":"<div><div>Conventional natural rubber (NR) fillers pose several environmental concerns. This study presents the sustainable development of NR composites incorporating sugarcane leaf (SCL)-derived alkali lignin and commercial alkali lignin as functional fillers. The primary objective was to evaluate the mechanical properties, aging resistance, thermal stability, and antimicrobial activity of the NR composites. Various NR composites were prepared by different filler types, including KOH-extracted SCL lignin, commercial alkali lignin, and butylated hydroxytoluene (BHT). The results show that NR composites containing KOH-extracted SCL lignin exhibited superior mechanical properties (crosslink density 126 mol/m<sup>3</sup>), improved aging resistance (aging coefficient 80.08 %), and enhanced thermal stability (the thermal degradation with 50 % weight loss (T<sub>50</sub>) and the highest degradation rate occurs (T<sub>d</sub>) of 394 and 383 °C, respectively) compared to all other samples. NR composites with commercial lignin demonstrated the highest reduction in <em>Staphylococcus aureus</em> populations (56.25 %). The NR composites with KOH-extracted SCL lignin displayed limited antimicrobial efficacy (37.78 %), suggesting that its primary contribution lies in mechanical and thermal reinforcement rather than microbial inhibition. These findings highlight the potential of eco-friendly lignin from SCL biomass as a sustainable bio-based filler for NR composites.</div></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"4 4","pages":"Article 100126"},"PeriodicalIF":0.0,"publicationDate":"2025-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144711732","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Catalytic decomposition of methane over Fe2O3-Al2O3 catalysts with high iron contents and at high CH4 space velocities 高铁含量、高CH4空速的Fe2O3-Al2O3催化剂催化甲烷分解

Resources Chemicals and Materials Pub Date : 2025-07-16 DOI: 10.1016/j.recm.2025.100123

Shuang Li , Junyi Liao , Zhanguo Zhang , Guangwen Xu

{"title":"Catalytic decomposition of methane over Fe2O3-Al2O3 catalysts with high iron contents and at high CH4 space velocities","authors":"Shuang Li , Junyi Liao , Zhanguo Zhang , Guangwen Xu","doi":"10.1016/j.recm.2025.100123","DOIUrl":"10.1016/j.recm.2025.100123","url":null,"abstract":"<div><div>Catalysts Fe<sub>2</sub>O<sub>3</sub>-Al<sub>2</sub>O<sub>3</sub> with high Fe<sub>2</sub>O<sub>3</sub> contents (50–90wt%) were prepared by co-precipitation method and tested for methane decomposition and production of high-purity carbon nanofibers (CNFs). Catalytic tests were conducted in a fixed-bed reactor at atmospheric pressure, different temperatures and high CH<sub>4</sub> space velocities. The catalytic tests performed at 700 °C showed that Fe<sub>2</sub>O<sub>3</sub>-Al<sub>2</sub>O<sub>3</sub> catalysts containing 60–80wt% Fe<sub>2</sub>O<sub>3</sub> enable a maximal CH<sub>4</sub> conversion of around 56 % and production of CNFs with a purity above 95 %. Further, the catalytic results recorded over 80 % Fe<sub>2</sub>O<sub>3</sub>-Al<sub>2</sub>O<sub>3</sub> catalyst at varied temperatures and space velocities revealed the following: (1) increasing temperature leads to an increased maximum CH<sub>4</sub> conversion but a reduced CNFs productivity per unit weight of catalyst, and (2) CNFs productivity can be maximized at each temperature by lowering CH<sub>4</sub> space velocity to an appropriate rate through reducing CH<sub>4</sub> feed rate or increasing the amount of catalyst fed in the reactor. Moreover, typical SEM, Raman and TEM characterization results confirmed that the CNFs obtained are of a relatively narrow diameter distribution of 20–40 nm and graphitic nanostructure in appearance. Furthermore, electroconductivity measurement of typical CNFs products confirmed their good electrical conductivity, suggesting their potential direct use for formulation of anti-static CNFs reinforced plastic composites.</div></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"4 4","pages":"Article 100123"},"PeriodicalIF":0.0,"publicationDate":"2025-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144748702","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Facilitated hydrogenation of furfural into furfuryl alcohol over catalyst CuSiAlOx made with infrared-heating calcination 红外加热煅烧催化剂CuSiAlOx催化糠醛加氢生成糠醇

Resources Chemicals and Materials Pub Date : 2025-06-14 DOI: 10.1016/j.recm.2025.100122

Mengjuan Zhang , Xiaoyu Wu , Chao Wang , Jiarui He , Guoguo Liu , Peng Zheng , Zhennan Han , Jinggang Zhao , Kangjun Wang

{"title":"Facilitated hydrogenation of furfural into furfuryl alcohol over catalyst CuSiAlOx made with infrared-heating calcination","authors":"Mengjuan Zhang , Xiaoyu Wu , Chao Wang , Jiarui He , Guoguo Liu , Peng Zheng , Zhennan Han , Jinggang Zhao , Kangjun Wang","doi":"10.1016/j.recm.2025.100122","DOIUrl":"10.1016/j.recm.2025.100122","url":null,"abstract":"<div><div>A CuSiAlO<sub>x</sub> catalyst was prepared through infrared-heating calcination and employed to catalyze vapor furfural (FFR) hydrogenation in a fixed-bed reactor. Its catalytic performance was systematically evaluated and compared to that of a catalyst derived from the same precursor but calcined using an electric oven. The hydrogenation tests were performed at temperatures varying in 140 ∼ 180 °C, H<sub>2</sub>/FFR (mol/mol) ratios in 4:1 ∼ 8:1, and liquid hourly space velocity (LHSVs) in 0.6 ∼ 1.0 h<sup>-1</sup>. The catalyst CuSiAlO<sub>x</sub>-IH (prepared by infrared-heating calcination) demonstrated higher FFR conversion than CuSiAlO<sub>x</sub>-EH (prepared by electric-oven heating) did. Under the conditions of a H<sub>2</sub>/FFR ratio of 6:1, a temperature of 140 °C, and an LHSV of 0.6 h<sup>-1</sup>, the CuSiAlO<sub>x</sub>-IH catalyst achieved a 99.70 % FFR conversion and 95.72 % selectivity to furfur alcohol (FOL) in a continuous test for 18 h. This time duration with good stability was twice longer than that enabled by CuSiAlO<sub>x</sub>-EH. Characterization of the fresh, reduced, and spent catalysts revealed that the catalyst CuSiAlO<sub>x</sub>-IH, compared to CuSiAlO<sub>x</sub>-EH, possessed more Cu defects, a higher BET surface area, a smaller average size, and the narrower size distribution of active-species particles. These structural advantages thus rendered the CuSiAlO<sub>x</sub>-IH catalyst superior in its catalysis of the FFR hydrogenation reactions.</div></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"4 3","pages":"Article 100122"},"PeriodicalIF":0.0,"publicationDate":"2025-06-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144331304","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Advanced cellulose-based materials for flexible energy storage systems 用于柔性储能系统的先进纤维素基材料

Resources Chemicals and Materials Pub Date : 2025-06-07 DOI: 10.1016/j.recm.2025.100120

Zehong Chen , Hongzhi Zheng , Jiwang Yi , Tanglong Liu , Haihong Lai , Shuai Zhang , Wei Huang , Yunlong Yin , Xiaofang Huang , Yifan Tong , Dianen Liang , Runsen Li , Linxin Zhong , Chaoqun Zhang , Huili Zhang

{"title":"Advanced cellulose-based materials for flexible energy storage systems","authors":"Zehong Chen , Hongzhi Zheng , Jiwang Yi , Tanglong Liu , Haihong Lai , Shuai Zhang , Wei Huang , Yunlong Yin , Xiaofang Huang , Yifan Tong , Dianen Liang , Runsen Li , Linxin Zhong , Chaoqun Zhang , Huili Zhang","doi":"10.1016/j.recm.2025.100120","DOIUrl":"10.1016/j.recm.2025.100120","url":null,"abstract":"<div><div>The rapid development of portable electronics, wearable technologies, and healthcare monitoring systems necessitates the innovation of flexible energy storage systems. Considering environmental pollution and the depletion of fossil resources, the utilization of renewable resources to engineer advanced flexible materials has become especially crucial. Cellulose, the most abundant natural polymer, has emerged as a promising precursor for advanced functional materials due to its unique structure and properties. Typically, the easy processability, tunable chemical structure, self-assembly behavior, mechanical strength, and reinforcing capability enable its utilization as binder, substrate, hybrid electrode, separator, and electrolyte reservoir for flexible energy storage devices. This review comprehensively summarizes the design, fabrication, and mechanical and electrochemical performances of cellulose-based materials. The structure and unique properties of cellulose are first briefly introduced. Then, the construction of cellulose-based materials in the forms of 1D fibers/filaments, 2D films/membranes, 3D hydrogels and aerogels is discussed, and the merits of cellulose in these materials are emphasized. After that, the various advanced applications in supercapacitors, lithium-ion batteries, lithium-sulfur batteries, sodium-ion batteries, metal-air batteries, and Zn-ion batteries are presented in detail. Finally, an outlook of the potential challenges and future perspectives in advanced cellulose-based materials for flexible energy storage systems is discussed.</div></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"4 3","pages":"Article 100120"},"PeriodicalIF":0.0,"publicationDate":"2025-06-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144253582","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Assembly of two-dimensional nanosheets of copper sulfide on nickel foam for high-efficiency energy storage applications: Exploring the effect of pH 在泡沫镍上组装二维硫化铜纳米片用于高效储能：探讨pH值的影响

Resources Chemicals and Materials Pub Date : 2025-06-02 DOI: 10.1016/j.recm.2025.100119

Akashdeep Dey, Mahendra S. Gaikwad, S. Noyel Victoria

{"title":"Assembly of two-dimensional nanosheets of copper sulfide on nickel foam for high-efficiency energy storage applications: Exploring the effect of pH","authors":"Akashdeep Dey, Mahendra S. Gaikwad, S. Noyel Victoria","doi":"10.1016/j.recm.2025.100119","DOIUrl":"10.1016/j.recm.2025.100119","url":null,"abstract":"<div><div>Two-dimensional (2D) CuS/Cu<sub>9</sub>S<sub>5</sub> nanostructures are quite popular owing to their intriguing electrochemical properties. In-situ hydrothermal deposition of 2D CuS/Cu<sub>9</sub>S<sub>5</sub> nanostructures on nickel foam at different pH was studied. The X-ray diffraction analysis confirmed two different stoichiometric forms, namely CuS and Cu<sub>9</sub>S<sub>5</sub>, in different proportions with a change in the synthesis pH. Morphological and compositional analysis exhibited a strong impact of pH on the CuS/Cu<sub>9</sub>S<sub>5</sub> deposits. The samples prepared at pH 6.5 presented less agglomerated and densely distributed 2D nanosheets. Transmission electron microscopic studies under high resolution for the deposits synthesized at pH 6.5 showed hexagonal CuS and rhombohedral Cu<sub>9</sub>S<sub>5</sub> particles of 32 nm average particle size. The electrochemical characterization of the samples for energy storage devices by cyclic voltammetry (CV) study revealed the specific capacitance from 1781 Fg<sup>−1</sup> to 1589 Fg<sup>−1</sup> at 10 mVs<sup>−1</sup>. The findings of CV and galvanostatic charge/discharge (GCD) analysis matched well. Rate capability studies showed the values between 72.9% and 50.24% at 7.5 Ag<sup>−1</sup> for various samples. The sample prepared at pH 6.5 exhibited 73.07% of its starting capacitance at 10 Ag<sup>−1</sup> after 2500 charging and discharging sequences. Electrochemical impedance spectroscopy runs (EIS) showed the existence of two constant phase elements (CPE) in series and the relaxation time constants from 0.01 to 0.5 seconds, which are preferred for energy storing purposes. Symmetric supercapacitor device prepared from sample deposited at pH 6.5 displayed 29.16 Wh energy per kg of material and a power density of 900 W kg<sup>−1</sup>, highlighting its suitability for high-efficiency energy storage applications.</div></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"4 3","pages":"Article 100119"},"PeriodicalIF":0.0,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144231661","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Essential strategies for efficient low–tar biomass gasification: in-bed intensification and interactive two–stage reactions 有效的低焦油生物质气化的基本策略：床内强化和相互作用的两阶段反应

Resources Chemicals and Materials Pub Date : 2025-06-01 DOI: 10.1016/j.recm.2024.11.002

Chao Wang , Xinyu Wang , Zhennan Han , Mengjuan Zhang , Lianfeng Zhu , Xin Jia , Ping An , Dingrong Bai , Fang Wang , Guoqing Guan , Guangwen Xu

{"title":"Essential strategies for efficient low–tar biomass gasification: in-bed intensification and interactive two–stage reactions","authors":"Chao Wang , Xinyu Wang , Zhennan Han , Mengjuan Zhang , Lianfeng Zhu , Xin Jia , Ping An , Dingrong Bai , Fang Wang , Guoqing Guan , Guangwen Xu","doi":"10.1016/j.recm.2024.11.002","DOIUrl":"10.1016/j.recm.2024.11.002","url":null,"abstract":"<div><div>Gasification is a highly effective technology for converting biomass into fuel gas or syngas. While various gasifiers have been commercialized for fuel gas production, mitigating tar formation in gasifiers remains challenging. This review is devoted to summarizing the general strategies adopted in various gasifiers to reduce tar formation for high-efficiency clean gasification. For single-bed and staged-gasification processes, their low-tar strategies are typically different. In the single-bed processes, the low-tar strategies involve in-bed intensification achieved by controlling flow directions of gas and particles inside the gasifier. During the gasification, these two components often have different temperatures to facilitate thermochemical interactions between them. Meanwhile, the two-stage gasifiers are generally designed to decouple pyrolysis, gasification and tar cracking reactions for maximizing the benefits (such as yield and efficiency) realized from the interactions among these reactions. In addition to minimizing tar formation, the approach of reaction decoupling can also raise the calorific value of product gas, even without use of oxygen, and/or improve the adaptability of gasification technology to the feedstocks with various moisture contents and particle sizes. The reanalysis based on those essential low-tar strategies is expected to gain alternative insights into the reaction principles implicated in most advanced biomass gasification technologies.</div></div>","PeriodicalId":101081,"journal":{"name":"Resources Chemicals and Materials","volume":"4 2","pages":"Article 100087"},"PeriodicalIF":0.0,"publicationDate":"2025-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144713517","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0