Cell Reports Physical Science最新文献

Lignin as a bioderived modular surfactant and intercalant for Ti₃C₂T_x MXene stabilization and tunable functions. 木质素作为一种生物来源的模块化表面活性剂和插层剂，用于 Ti3C2Tx MXene 的稳定和可调功能。

IF 7.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-11-20 DOI: 10.1016/j.xcrp.2024.102259

Pan Jiang, Xiaodan Hong, Jin Zhang, Jiali Sheng, Jiahui Kang, Olli Ikkala, Fuxiang Chu, Bo Peng, Yanming Han, Zhong-Peng Lv

{"title":"Lignin as a bioderived modular surfactant and intercalant for Ti3C2Tx MXene stabilization and tunable functions.","authors":"Pan Jiang, Xiaodan Hong, Jin Zhang, Jiali Sheng, Jiahui Kang, Olli Ikkala, Fuxiang Chu, Bo Peng, Yanming Han, Zhong-Peng Lv","doi":"10.1016/j.xcrp.2024.102259","DOIUrl":"10.1016/j.xcrp.2024.102259","url":null,"abstract":"Controlled tailoring of atomically thin MXene interlayer spacings by surfactant/intercalants (e.g., polymers, ligands, small molecules) is important to maximize their potential for application. However, challenges persist in achieving precise spacing tunability in a well-defined stacking, combining long-term stability and dispersibility in various solvents. Here, we discovered that lignin can be used as surfactants/intercalants of Ti3C2Tx MXenes. The resulting MXene@lignin complexes exhibit superior colloidal stability and oxidation resistance in both water and different organic solvents. More important, we reveal a dynamic interaction between MXene and lignin that enables a wide-range fine interlayer distance tuning at a sub-nanometer scale. Such dynamic interaction is sparse in the reported organic surfactants/intercalants containing single types of functional groups. We also demonstrate the tunability of electrical conductivity, infrared emissivity, and electromagnetic interference shielding effectiveness. Our approach offers a starting point to explore the potential of MXene-biomacromolecule composites for electronics and photonics applications.","PeriodicalId":9703,"journal":{"name":"Cell Reports Physical Science","volume":"5 11","pages":"102259"},"PeriodicalIF":7.9,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11582023/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142709368","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Amino acid-dependent phase equilibrium and material properties of tetrapeptide condensates. 四肽缩合物的氨基酸相平衡和材料特性。

IF 7.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-10-16 Epub Date: 2024-09-23 DOI: 10.1016/j.xcrp.2024.102218

Yi Zhang, Ramesh Prasad, Siyuan Su, Daesung Lee, Huan-Xiang Zhou

引用次数: 0

Paper microfluidic sentinel sensors enable rapid and on-site wastewater surveillance in community settings 纸质微流控哨点传感器可在社区环境中快速进行现场废水监测

IF 8.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-09-19 DOI: 10.1016/j.xcrp.2024.102154

Yuwei Pan, Baojun Wang, Jonathan M. Cooper, Zhugen Yang

{"title":"Paper microfluidic sentinel sensors enable rapid and on-site wastewater surveillance in community settings","authors":"Yuwei Pan, Baojun Wang, Jonathan M. Cooper, Zhugen Yang","doi":"10.1016/j.xcrp.2024.102154","DOIUrl":"https://doi.org/10.1016/j.xcrp.2024.102154","url":null,"abstract":"Tracking genomic sequences as microbial biomarkers in wastewater has been used to determine community prevalence of infectious diseases, contributing to public health surveillance programs worldwide. Here, we report upon a low-cost, rapid, and user-friendly paper microfluidic platform for severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2) and influenza detection, using loop-mediated isothermal amplification, with signal read using a mobile phone camera. Sample-to-answer results were collected in less than 1.5 h, providing rapid multiplexed detection of viruses in wastewater, with a detection limit of <20 copies mL−1. The device was subsequently used for on-site testing of SARS-CoV-2 in wastewater samples from four quarantine hotels at London Heathrow Airport, showing comparable results to those obtained using polymerase chain reaction. This sensing platform, which enables rapid and localized testing without requiring samples to be sent to centralized laboratories, provides a potentially important public health tool for pandemic preparedness, with a variety of future wastewater surveillance applications in community settings.","PeriodicalId":9703,"journal":{"name":"Cell Reports Physical Science","volume":"3 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2024-09-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264634","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Catalyzing deep decarbonization with federated battery diagnosis and prognosis for better data management in energy storage systems 利用联合电池诊断和预测催化深度脱碳，改善储能系统的数据管理

IF 8.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-09-19 DOI: 10.1016/j.xcrp.2024.102215

引用次数: 0

Solid-electrolyte fracture models driven by lithium metal plating require electrochemical mechanical couplings 锂金属镀层驱动的固体电解质断裂模型需要电化学机械耦合

IF 8.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-09-18 DOI: 10.1016/j.xcrp.2024.102207

Taeho Jung, Eric A. Carmona, Yueming Song, Paul Albertus

{"title":"Solid-electrolyte fracture models driven by lithium metal plating require electrochemical mechanical couplings","authors":"Taeho Jung, Eric A. Carmona, Yueming Song, Paul Albertus","doi":"10.1016/j.xcrp.2024.102207","DOIUrl":"https://doi.org/10.1016/j.xcrp.2024.102207","url":null,"abstract":"A common failure mode for solid-state lithium-metal batteries is solid-electrolyte fracture during lithium plating, but fracture initiation is complicated to diagnose. Here, an electrochemically and mechanically coupled steady-state lithium-plating model is implemented numerically to study fracture initiation at the lithium/solid-electrolyte interface. The solid electrolyte is treated as a linear elastic solid, while lithium is modeled as a Newtonian fluid. An electrochemical connection between the two phases is made via the stress-modified Butler-Volmer equation at the Gaussian-curved interface, where lithium protrudes into the solid electrolyte. The model simulations demonstrate that the couplings result in significantly different electrochemical and mechanical behaviors from those predicted by the model without the couplings. The J-integrals—an indicator of fracture—of the coupled and uncoupled models are six orders of magnitude apart. The coupled model supports a shear-traction-driven fracture concentrated at the asperity base instead of the commonly attributed pressure-driven fracture at the asperity tip. Finally, our sensitivity analysis reveals that lithium pseudo-viscosity and asperity geometry are important parameters determining fracture initiation.","PeriodicalId":9703,"journal":{"name":"Cell Reports Physical Science","volume":"19 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264642","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Doping regulation of highly conductive PBTTT films 高导电性 PBTTT 薄膜的掺杂调节

IF 8.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-09-18 DOI: 10.1016/j.xcrp.2024.102197

Yanwei Fan, Jie Liu, Ping-An Chen, Dongdong Xia, Jiawei Wang, Yuanyuan Hu, Zitong Liu, Yunqi Liu, Lang Jiang

{"title":"Doping regulation of highly conductive PBTTT films","authors":"Yanwei Fan, Jie Liu, Ping-An Chen, Dongdong Xia, Jiawei Wang, Yuanyuan Hu, Zitong Liu, Yunqi Liu, Lang Jiang","doi":"10.1016/j.xcrp.2024.102197","DOIUrl":"https://doi.org/10.1016/j.xcrp.2024.102197","url":null,"abstract":"Doping is a key strategy for enhancing the charge mobility and thermoelectric properties of polymers. While advancements utilizing the anion exchange technique have notably enhanced doping efficiency, there is a need for further optimization of the doping process. This study introduces a two-step doping approach combining solid-state diffusion with anion exchange, applied to poly[2,5-bis(3-tetradecylthiophen-2-yl)thieno[3,2-b]thiophene] (PBTTTC14) films. Initial 2,3,5,6-tetrafluoro-7,7,8,8-tetracyano-quinodimethane (F4TCNQ) diffusion doping followed by anion exchange with F4TCNQ/ionic liquid achieved higher conductivity than one-step anion exchange doping. Spectral and structural analyses elucidated the enhanced doping mechanism. Additionally, adjusting the molecular weight (MW) of PBTTTC14 from 11,867 to 175,199 improved doping levels and conductivity, reaching 1,103.8 S cm−1. A medium MW (MW = 99,407) optimized thermoelectric performance by balancing conductivity and Seebeck coefficients. These findings provide insights into controlling doping and performance of conductive semiconductor polymers through a two-step doping process and MW engineering.","PeriodicalId":9703,"journal":{"name":"Cell Reports Physical Science","volume":"11 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264641","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Deformation of collagen-based tissues investigated using a systematic review and meta-analysis of synchrotron x-ray scattering studies 利用同步辐射 X 射线散射研究的系统回顾和荟萃分析研究胶原基组织的变形

IF 8.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-09-18 DOI: 10.1016/j.xcrp.2024.102212

Lander Manrique, Mahmoud S. Moussa, Muhammad Talal Khan, Kawkab Tahboub, Robert O. Ritchie, Meisam Asgari, Elizabeth A. Zimmermann

{"title":"Deformation of collagen-based tissues investigated using a systematic review and meta-analysis of synchrotron x-ray scattering studies","authors":"Lander Manrique, Mahmoud S. Moussa, Muhammad Talal Khan, Kawkab Tahboub, Robert O. Ritchie, Meisam Asgari, Elizabeth A. Zimmermann","doi":"10.1016/j.xcrp.2024.102212","DOIUrl":"https://doi.org/10.1016/j.xcrp.2024.102212","url":null,"abstract":"Collagen fibrils are the building blocks of many tissues from fish scales and tendons to bone. Synchrotron small-angle X-ray scattering (SAXS) with in situ mechanical testing is a powerful tool to investigate collagen fibril deformation. There is a need to combine data from SAXS studies to investigate structure-function relationships. A literature search used the concepts of mechanical properties, collagen, and SAXS, with 52 articles meeting the eligibility criteria. Here, we report that mineralized tissues transfer a greater proportion of tissue-scale deformation to the fibril: 67% for cortical bone, 49% for tendon, 10% for ligament, and 3% for skin. Across non-mineralized tissues, tissues with less complexity and greater elastin content transfer less deformation to the fibril. The meta-analysis finds 20%–40% lower fibril strain in human aging and disease compared to controls, which contributes toward fracture risk. This synthesis demonstrates how variations in composition and structure tune material properties in collagen-based tissues.","PeriodicalId":9703,"journal":{"name":"Cell Reports Physical Science","volume":"20 1","pages":""},"PeriodicalIF":8.9,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264638","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Insights into polarization relaxation of electromagnetic wave absorption 对电磁波吸收的偏振弛豫的见解

IF 8.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-09-18 DOI: 10.1016/j.xcrp.2024.102206

Shijie Zhang, Di Lan, Jiajun Zheng, Zhiwei Zhao, Zirui Jia, Guanglei Wu

引用次数: 0

Catalysis for plastic deconstruction and upcycling 用于塑料解构和升级再循环的催化作用

IF 8.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-09-18 DOI: 10.1016/j.xcrp.2024.102209

Ding Ma, Ye Wang, Michele L. Sarazen, Cyrille Boyer, Tomonori Saito, Haohong Duan, Wenyu Huang

引用次数: 0

4.8-V all-solid-state garnet-based lithium-metal batteries with stable interface 界面稳定的 4.8 V 全固态石榴石型锂金属电池

IF 8.9 2区综合性期刊

Cell Reports Physical Science Pub Date : 2024-09-18 DOI: 10.1016/j.xcrp.2024.102213

引用次数: 0