Atmospheric Pollution Research最新文献

筛选
英文 中文
Source apportionment of primary and secondary fine particulate matter in Eskisehir/Türkiye using conventional and dispersion-normalized positive matrix factorization Eskisehir/ t<s:1> rkiye中初级和次级细颗粒物的源解析使用常规和分散归一化的正矩阵分解
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-15 DOI: 10.1016/j.apr.2025.102653
Akif Ari , Pelin Ertürk Ari , Eftade O. Gaga
{"title":"Source apportionment of primary and secondary fine particulate matter in Eskisehir/Türkiye using conventional and dispersion-normalized positive matrix factorization","authors":"Akif Ari ,&nbsp;Pelin Ertürk Ari ,&nbsp;Eftade O. Gaga","doi":"10.1016/j.apr.2025.102653","DOIUrl":"10.1016/j.apr.2025.102653","url":null,"abstract":"<div><div>In this study, the organic and inorganic components of atmospheric fine particulate matter (PM<sub>2.5</sub>) were monitored daily in Eskisehir City/Türkiye, for one year, and the contributions of primary and secondary sources to the PM mass were investigated. A total of 94 components were characterized in PM<sub>2.5</sub> samples, including 5 anions, 46 trace elements, Organic and Elemental Carbon (OC &amp; EC), 16 Polycyclic Aromatic Hydrocarbons (PAHs), 26 n-alkanes, levoglucosan, and 8 carboxylic acids to obtain a more holistic mass closure. In addition, the principal sources of PM<sub>2.5</sub> were apportioned by the Conventional and Dispersion-Normalized Positive Matrix Factorization (C-PMF and DN-PMF) to assess dispersion/dilution characteristics of local meteorological conditions on source contributions of PM. The main sources of PM were classified into 8 factors. A significant seasonal variation was observed in combustion-related PM<sub>2.5</sub> constituents, which increased in the winter, while the contribution of Secondary Organic Carbon (SOC) enhanced during the summer period. In addition, a visual effect of seasonal atmospheric dilution/dispersion conditions on measured pollutant levels was observed as a function of Ventilation Coefficients (VC). The mass percent of SOC in PM<sub>2.5</sub> varied between 2.3 % and 13.0 %, and the annual mean contribution was over 7.5 %.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102653"},"PeriodicalIF":3.9,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144633947","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The input-optimized and supplemented MEGAN improves biogenic volatile organic compounds estimation accuracy in China 投入优化和补充后的MEGAN提高了中国生物源性挥发性有机物估算的准确性
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-14 DOI: 10.1016/j.apr.2025.102650
Bin Cai , Haomiao Cheng , Tianfang Kang , Yu Wang , Wentao Han , Wei Wang
{"title":"The input-optimized and supplemented MEGAN improves biogenic volatile organic compounds estimation accuracy in China","authors":"Bin Cai ,&nbsp;Haomiao Cheng ,&nbsp;Tianfang Kang ,&nbsp;Yu Wang ,&nbsp;Wentao Han ,&nbsp;Wei Wang","doi":"10.1016/j.apr.2025.102650","DOIUrl":"10.1016/j.apr.2025.102650","url":null,"abstract":"<div><div>To reduce the uncertainty in biogenic volatile organic compound (BVOC) emission estimates by MEGAN model, this study introduces targeted optimizations in the input conditions driven by plant functional types (PFTs), emission factors (EFs), and leaf area index (LAI), and supplements the missing BVOC emissions from urban green spaces (U-BVOC emissions). To verify the optimization effect of the input-improved MEGAN, the study conducted a comparative validation of the estimated BVOC emission levels in representative regions of northern and southern China using formaldehyde vertical column densities and accumulation-based estimates through stock volume conversion. The results indicate that the input-improved MEGAN can provide more reasonable BVOC estimates with a more notable improvement in the southern region, and the estimated isoprene emissions show better spatiotemporal correlation with formaldehyde vertical column densities. The optimization of PFT + EF and LAI input conditions both effectively improve the model's estimation accuracy. Although the U-BVOC emissions are significantly lower than the BVOC emissions from non-urban environment, the newly added U-BVOC emission inventory is expected to help improve the performance of existing air quality models in simulating O<sub>3</sub> and particulate matter pollution in urban areas.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102650"},"PeriodicalIF":3.9,"publicationDate":"2025-07-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144703477","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effects of altitude on light gasoline vehicles: fuel consumption and air pollution 海拔对轻型汽油车的影响:燃料消耗和空气污染
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-14 DOI: 10.1016/j.apr.2025.102652
Yanxu Ren, Wenhan Yu, Lijun Hao, Yunshan Ge
{"title":"Effects of altitude on light gasoline vehicles: fuel consumption and air pollution","authors":"Yanxu Ren,&nbsp;Wenhan Yu,&nbsp;Lijun Hao,&nbsp;Yunshan Ge","doi":"10.1016/j.apr.2025.102652","DOIUrl":"10.1016/j.apr.2025.102652","url":null,"abstract":"<div><div>Driven by the global carbon neutrality goal and emission regulations, gasoline vehicles' fuel consumption and emission characteristics in the plateau environment have received extensive attention. In this paper, the running resistance of light gasoline vehicles in a high-altitude environment laboratory is corrected by coasting resistance tests to ensure the accuracy of laboratory tests. Finally, a constant speed fuel consumption test and a New European Driving Cycle emission test were carried out in the high-altitude environment laboratory. The results of fuel consumption characteristics show that at low-to-medium speeds (below 5,000m altitude), fuel efficiency generally improved with increasing altitude. For the high-speed range, air resistance becomes more prominent below 5000m, which reduces overall fuel consumption. However, once the altitude approaches 5000m, all speed ranges show an upward trend in fuel consumption. Fuel consumption at high speeds enters an upward trend earlier (at relatively low altitudes). The results of emission characteristics show that the emission of CO and THC increases significantly with the increase of altitude due to combustion deterioration. The contribution of the cold start-up phase increased significantly (77.1 % CO and 66.3 % THC), which became the core factor of the increase in emissions. Due to the game between the combustion temperature and the efficiency of the three-way catalytic converter (TWC), NOx emission shows a trend of first decreasing and then increasing. Its instantaneous emission characteristics are not stable because of the gradual decline of TWC performance. In general, these results can be used to drive vehicle energy efficiency and emission reduction targets.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102652"},"PeriodicalIF":3.9,"publicationDate":"2025-07-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144695222","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Long-term evolution and synoptic meteorological modulation of PM2.5 and PM10 in Seoul 首尔地区PM2.5和PM10的长期演变及天气气象调制
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-14 DOI: 10.1016/j.apr.2025.102649
Wooseok Jang , Simon Wang , Hyun Cheol Kim , Jee-Hoon Jeong , Changhyun Yoo , Jin-Young Choi , Jin-Ho Yoon
{"title":"Long-term evolution and synoptic meteorological modulation of PM2.5 and PM10 in Seoul","authors":"Wooseok Jang ,&nbsp;Simon Wang ,&nbsp;Hyun Cheol Kim ,&nbsp;Jee-Hoon Jeong ,&nbsp;Changhyun Yoo ,&nbsp;Jin-Young Choi ,&nbsp;Jin-Ho Yoon","doi":"10.1016/j.apr.2025.102649","DOIUrl":"10.1016/j.apr.2025.102649","url":null,"abstract":"<div><div>Addressing particulate matter (PM) pollution in megacities like Seoul is crucial for public health and environmental sustainability, necessitating a comprehensive understanding of its long-term evolution and meteorological drivers. This study investigated the key factors affecting long-term PM concentrations in Seoul, South Korea, from 2000 to 2021, with a focus on the winter (DJF) and spring (MAM) seasons. To address the gap in PM research caused by the shorter observation period of PM<sub>2.5</sub> compared with PM<sub>10</sub>, we used an extended PM<sub>2.5</sub> dataset. This enabled a detailed analysis of PM<sub>2.5</sub> and its relationship with PM<sub>10</sub>, which, despite some differences, generally displayed similar variability. Both PM<sub>2.5</sub> and PM<sub>10</sub> exhibited decreasing trends in winter as well as spring, although the rate of decline slowed in the last decade (2011–2020) compared with the earlier decade (2000–2010). Both seasons exhibited a strengthened interannual correlation between PM<sub>2.5</sub> and PM<sub>10</sub> in the last decade. Daily PM<sub>2.5</sub> and PM<sub>10</sub> levels generally fluctuated in a similar pattern in both seasons, which can be attributed to synoptic-scale meteorological systems, particularly migratory systems from Northwest China, which can remain stationary over Korea for several days, particularly in winter. This pattern continues into spring, albeit with a lower intensity. These findings provide valuable insights into PM<sub>2.5</sub> variability and its correlation with PM<sub>10</sub> over time, which may inform future PM<sub>2.5</sub> mitigation strategies.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102649"},"PeriodicalIF":3.9,"publicationDate":"2025-07-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144703476","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Characteristics and influencing factors of ambient ozone pollution in Hangzhou in the relative humidity range with high ozone levels 杭州高臭氧水平相对湿度区环境臭氧污染特征及影响因素
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-10 DOI: 10.1016/j.apr.2025.102648
Yu Lu , Lingdong Kong , Jiandong Shen , Beibei Liu , Yixuan An , Yuwen Wang , Jie Tan , Lin Wang
{"title":"Characteristics and influencing factors of ambient ozone pollution in Hangzhou in the relative humidity range with high ozone levels","authors":"Yu Lu ,&nbsp;Lingdong Kong ,&nbsp;Jiandong Shen ,&nbsp;Beibei Liu ,&nbsp;Yixuan An ,&nbsp;Yuwen Wang ,&nbsp;Jie Tan ,&nbsp;Lin Wang","doi":"10.1016/j.apr.2025.102648","DOIUrl":"10.1016/j.apr.2025.102648","url":null,"abstract":"<div><div>With the rapid economic growth and urbanization, despite improvements in particulate matter (PM<sub>2.5</sub>) pollution control, ozone (O<sub>3</sub>) pollution has emerged as a pressing environmental issue in China. This study systematically investigates O<sub>3</sub> pollution dynamics in Hangzhou (2021–2023) in the relative humidity (RH) range with high ozone levels using observational data and generalized additive modeling (GAM). Key findings reveal distinct temporal patterns: diurnal O<sub>3</sub> peaks at 14:00 (lagging solar radiation by about 2 h), seasonal maxima in summer (157.58 μg m<sup>−3</sup>) driven by temperature-photochemistry coupling, and non-monotonic annual trends (116.21–123.77 μg m<sup>−3</sup>) despite NO<sub>x</sub> decline, reflecting transitional chemical regimes. Alkenes (36.94 %) and oxygenated VOCs (OVOCs, 36.54 %) dominated O<sub>3</sub> formation potential, with acetaldehyde, ethylene, and 1-butene as top contributors, highlighting the significant contributions of industrial and vehicular emission sources to O<sub>3</sub> formation. GAM analysis identified temperature as the primary driver, exhibiting exponential O<sub>3</sub> enhancement above 30 °C. In particular, NO<sub>2</sub> and peroxyacetyl nitrate showed synergistic effects, suggesting their dual roles as both precursors and indicators of radical cycling efficiency under the RH range. The 40 %–60 % RH range optimizes hydroxyl radical production while minimizes aerosol hydration, establishing it as a critical threshold for photochemical O<sub>3</sub> generation. These findings emphasize the importance of considering specific RH ranges and precursor reactivity in formulating refined O<sub>3</sub> pollution control strategies, providing a new theoretical basis for O<sub>3</sub> pollution control in the Yangtze River Delta region.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102648"},"PeriodicalIF":3.9,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144597291","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Improving PM2.5 simulations using LSTM: a study on spatiotemporal generalization 利用LSTM改进PM2.5模拟:时空概化研究
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-08 DOI: 10.1016/j.apr.2025.102647
Xingtian Chen , Yuhang Zhang , Kai Cao , Dongxing Li , Qizhong Wu
{"title":"Improving PM2.5 simulations using LSTM: a study on spatiotemporal generalization","authors":"Xingtian Chen ,&nbsp;Yuhang Zhang ,&nbsp;Kai Cao ,&nbsp;Dongxing Li ,&nbsp;Qizhong Wu","doi":"10.1016/j.apr.2025.102647","DOIUrl":"10.1016/j.apr.2025.102647","url":null,"abstract":"<div><div>Deep learning models, particularly long short-term memory (LSTM) networks, have shown strong potential for bias correction in air quality simulations. Although LSTM-based models have demonstrated success in improving PM<sub>2.5</sub> simulations during specific periods such as winter months or heavy pollution events, their ability to generalize across varying temporal intervals and geographical locations remains underexplored. This study systematically investigates the spatiotemporal generalization capabilities of LSTM-based (LSTM<sub>Local</sub>, LSTM<sub>Regional</sub>, LSTM<sub>Regional-idx</sub>, LSTM<sub>Regional-sub</sub>) models across 12 monthly intervals and 34 monitoring sites in Beijing. Benchmark comparisons with alternative deep learning models (RNN, GRU, BPNN, CNN) demonstrate the superiority of LSTM-based model in improving predictive performance. Seasonal analysis reveals that the LSTM<sub>Local</sub> and LSTM<sub>Regional-sub</sub> model achieved modest gains during summer half-year (May to October) but achieved significant improvements during winter half-year (November to April), with average RMSE reductions of −5.89 % (November), −17.40 % (December), −6.37 % (January), 0.36 % (February), −5.87 % (March) and −1.57 % (April). Spatially, urban sites show moderate gains, but suburban sites exhibit greater improvement, with average RMSE of −5.14 % (Center), −2.26 % (South-East), −7.05 % (North-East), −8.39 % (South-West) and −12.37 % (North-West). These findings highlight the robust spatiotemporal generalization of LSTM-based models and support their applicability for real-time bias correction, long-term forecasting, and air quality dataset enhancement at fine spatial and temporal resolutions.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102647"},"PeriodicalIF":3.9,"publicationDate":"2025-07-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144686007","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Comparison of MERRA-2 black carbon aerosols and ground observation at a high-altitude mountainous site in southern China 中国南方高海拔山区MERRA-2黑碳气溶胶与地面观测的比较
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-05 DOI: 10.1016/j.apr.2025.102644
Cheng Liu , Lichen Deng , Aijun Yan , Xinjie Liu , Jiening Huang , Xinrui Miao , Yue Qian , Renguo Zhu , Xiaozhen Fang , Wei Guo
{"title":"Comparison of MERRA-2 black carbon aerosols and ground observation at a high-altitude mountainous site in southern China","authors":"Cheng Liu ,&nbsp;Lichen Deng ,&nbsp;Aijun Yan ,&nbsp;Xinjie Liu ,&nbsp;Jiening Huang ,&nbsp;Xinrui Miao ,&nbsp;Yue Qian ,&nbsp;Renguo Zhu ,&nbsp;Xiaozhen Fang ,&nbsp;Wei Guo","doi":"10.1016/j.apr.2025.102644","DOIUrl":"10.1016/j.apr.2025.102644","url":null,"abstract":"<div><div>Black carbon (BC) is an important light-absorbing component of atmospheric aerosols and plays a crucial role in regional/global climate and human health. In contrast to the predominant focus on urban BC aerosols in existing literature, this study comprehensively compared and studied the temporal variations of BC concentration at a high-altitude mountainous site (Mt. Lushan) in southern China based on long-term (2008–2022) ground observations and elevation-corrected MERRA-2 reanalysis. Results indicate that both the observed and MERRA-2 annual mean BC concentrations show a downward trend over the years. However, the observed decline rate (−0.115 μg m<sup>−3</sup> yr<sup>−1</sup>) is considerably larger than that of MERRA-2 (−0.045 μg m<sup>−3</sup> yr<sup>−1</sup>), mainly attributed to MERRA-2's static emission inventory after 2013. Both datasets capture a “V-shaped” monthly variation pattern, but MERRA-2 overestimates winter BC by 68 % and underestimates summer BC by 8 %. Despite notable discrepancies during winter and at night, the diurnal variations of MERRA-2 and observed BC exhibit a consistent unimodal distribution, with its peak occurring between 12:00 and 17:00 local standard time (LST). This pattern contrasts with those observed in urban areas. A comparison reveals that using ground-level MERRA-2 reanalysis against the observation at Mt. Lushan results in larger biases than that using station elevation-matched product. This suggests that station elevation plays a significant role in the temporal variation of BC concentration, and it is preferable to use model-level BC data from MERRA-2 that corresponds to the actual station altitude for comparison at such high-altitude sites. These results could provide a referenced evaluation and promote the understanding on the applicability and accuracy of the MERRA-2 BC variation pattern over high-altitude sites.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102644"},"PeriodicalIF":3.9,"publicationDate":"2025-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144562858","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Investigation on vehicle emission factors in urban tunnels through mobile measurements with an optimized estimation method 基于优化估算方法的城市隧道车辆排放因子移动测量研究
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-05 DOI: 10.1016/j.apr.2025.102646
Chaowen Jiang , Chao Lin , Yu Zhao , Zhiwen Luo , Tianyi Zhao
{"title":"Investigation on vehicle emission factors in urban tunnels through mobile measurements with an optimized estimation method","authors":"Chaowen Jiang ,&nbsp;Chao Lin ,&nbsp;Yu Zhao ,&nbsp;Zhiwen Luo ,&nbsp;Tianyi Zhao","doi":"10.1016/j.apr.2025.102646","DOIUrl":"10.1016/j.apr.2025.102646","url":null,"abstract":"<div><div>Urban traffic pollution, driven by vehicle exhaust emissions, necessitates accurate assessment through Emission Factors (EFs). While tunnel measurements are commonly used, previous studies relied on fixed sampling points near tunnel entrances and exits, making results vulnerable to external influences. This study aims to elucidate the spatial patterns of EFs within tunnels and their influencing factors using multi-season mobile measurements, providing a reference for optimizing the selection of fixed testing points. Through the mobile measurements of Lianhuashan Tunnel in Dalian, real-time particulate matter concentration data were collected during vehicular transit, and variations in EFs at different locations were analyzed. The average EFs in spring, summer, and winter were 3.07 ± 0.84, 0.56 ± 0.12, and 0.90 ± 0.41 (mg/veh/km), respectively. Factors influencing the distribution characteristics of EFs within the tunnel include complex traffic conditions, characteristics specific to the EFs calculation equation employed in mobile measurement, and the influence of natural wind direction at the tunnel exit. Congestion or intermittent movement causes uneven EFs distribution. In cases of short sampling distances, small fluctuations in pollutant concentrations may result in overestimated EFs. Reverse winds at the exit may also inflate EFs due to pollutant accumulation. It is suggested that the optimal locations for fixed measurements lie within the range of 30 %–84 % of the tunnel length from the entrance.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102646"},"PeriodicalIF":3.9,"publicationDate":"2025-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144597289","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Study on the NO2 pollution and its connection with PM2.5 and O3 in Dazhou based on source apportionment 基于源解析的达州市NO2污染及其与PM2.5、O3的关系研究
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-04 DOI: 10.1016/j.apr.2025.102645
Xu Liu , Pulong Chen , Congwu Huang , Tijian Wang , Tao Niu , Mengmeng Li , Rong Li , Hao Wu , Yawei Qu
{"title":"Study on the NO2 pollution and its connection with PM2.5 and O3 in Dazhou based on source apportionment","authors":"Xu Liu ,&nbsp;Pulong Chen ,&nbsp;Congwu Huang ,&nbsp;Tijian Wang ,&nbsp;Tao Niu ,&nbsp;Mengmeng Li ,&nbsp;Rong Li ,&nbsp;Hao Wu ,&nbsp;Yawei Qu","doi":"10.1016/j.apr.2025.102645","DOIUrl":"10.1016/j.apr.2025.102645","url":null,"abstract":"<div><div>Dazhou, as one of the key construction cities in the Sichuan-Chongqing economic belt, has experienced accelerated economic development, accompanied by a dense population, extensive infrastructure construction, and rapid industrial growth. Consequently, air pollution has become increasingly severe, with the mass concentration of NO<sub>2</sub>, a primary pollutant, being a significant constraint on air quality management in the city. This study utilizes the WRF-CMAQ (Weather Research and Forecasting Model-Community Multi-scale Air Quality) model to quantitatively analyze the main sector sources of NO<sub>2</sub> in Dazhou during different seasons in 2022. The findings reveal that industrial sources contribute the most to NO<sub>2</sub> pollution in spring and winter, while transportation sources dominate in autumn. Additionally, the correlation between PM<sub>2.5</sub>, O<sub>3</sub>, and NO<sub>2</sub> concentrations, which exhibit significant seasonal variations, was examined. Notably, in summer, a negative correlation between O<sub>3</sub> and NO<sub>2</sub> concentrations was observed, while a positive correlation between PM<sub>2.5</sub> and NO<sub>2</sub> concentrations was evident in winter. Furthermore, the correlation between NO<sub>2</sub>, O<sub>3</sub> and PM<sub>2.5</sub> concentrations across different sectors was analyzed using ISAM (The Integrated Source Apportionment Method). In spring, the energy sources of NO<sub>2</sub> and the transportation sources of O<sub>3</sub> are significantly negatively correlated, with a correlation coefficient of −0.94. Additionally, the residential sources of NO<sub>2</sub> are significantly positively correlated with the transportation sources of PM<sub>2.5</sub>, with a correlation coefficient of 0.96. In autumn, the energy sources of NO<sub>2</sub> exhibit the most significant correlations with the industrial sources of O<sub>3</sub> and the transportation sources of NO<sub>2</sub> and PM<sub>2.5</sub>. In winter, the correlations among various sectors for O<sub>3</sub> pollution are not significant, with correlation coefficients ranging from 0.02 to 0.63. The highest correlation is observed between the industrial sources of NO<sub>2</sub> and the residential sources of PM<sub>2.5</sub>, reaching 0.98. This study analyzed the main source sectors of NO<sub>2</sub> in Dazhou City and the correlation with the source sectors of O<sub>3</sub> and PM<sub>2.5</sub> by using the CMAQ-ISAM source apportionment method, revealing the importance of seasonal cooperation in air pollution control in Dazhou and emphasizing its significance for long-term pollution management.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102645"},"PeriodicalIF":3.9,"publicationDate":"2025-07-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144572821","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Reanalysis-based retrieval of near-surface ozone concentrations and its implications for ozone pollution events across China 基于再分析的近地表臭氧浓度反演及其对中国臭氧污染事件的影响
IF 3.9 3区 环境科学与生态学
Atmospheric Pollution Research Pub Date : 2025-07-03 DOI: 10.1016/j.apr.2025.102643
Lili Wang , Xingchuan Yang , Haili Zhou , Yang Yang , Jiantao Dong , Shuo Dong , Wenji Zhao , Minghui Tao , Pengfei Ma
{"title":"Reanalysis-based retrieval of near-surface ozone concentrations and its implications for ozone pollution events across China","authors":"Lili Wang ,&nbsp;Xingchuan Yang ,&nbsp;Haili Zhou ,&nbsp;Yang Yang ,&nbsp;Jiantao Dong ,&nbsp;Shuo Dong ,&nbsp;Wenji Zhao ,&nbsp;Minghui Tao ,&nbsp;Pengfei Ma","doi":"10.1016/j.apr.2025.102643","DOIUrl":"10.1016/j.apr.2025.102643","url":null,"abstract":"<div><div>Ozone (O<sub>3</sub>) pollution has become a serious environmental issue in China, posing a significant threat to human health. However, existing satellite-based surface ozone concentration retrieval products are often restricted by data gaps and low spatial resolution, which limit their accuracy and applicability. Therefore, this study integrated reanalysis data from the National Centers for Environmental Prediction (NCEP) and ground-based observations, employing the XGBoost machine learning algorithm to estimate near-surface ozone concentrations across China at a high spatial resolution of 1 km. The model performed excellently in sample-based 10-fold cross-validation, achieving an R<sup>2</sup> of 0.91 and an RMSE of 13 μg/m<sup>3</sup>. Case studies of ozone pollution in two typical industrial cities (Tianjin and Dongguan) revealed the spatial heterogeneity of ozone pollution, supporting fine-scale regional monitoring. With the advantages of high spatial resolution and full coverage, our dataset successfully captured a prolonged ozone exposure event in eastern China from 12 June to July 15, 2023. This dataset holds great potential for applications in ozone exposure assessment and environmental impact studies.</div></div>","PeriodicalId":8604,"journal":{"name":"Atmospheric Pollution Research","volume":"16 11","pages":"Article 102643"},"PeriodicalIF":3.9,"publicationDate":"2025-07-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144564025","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
0
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
相关产品
×
本文献相关产品
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信