P. Menegasso, J. Souza, I. Vinograd, Z. Wang, S. Edwards, P. Pagliuso, N. Curro, R. Urbano
{"title":"Hyperfine couplings as a probe of orbital anisotropy in heavy-fermion materials","authors":"P. Menegasso, J. Souza, I. Vinograd, Z. Wang, S. Edwards, P. Pagliuso, N. Curro, R. Urbano","doi":"10.1103/PhysRevB.104.035154","DOIUrl":"https://doi.org/10.1103/PhysRevB.104.035154","url":null,"abstract":"The transferred hyperfine interaction between nuclear and electron spins in an heavy fermion material depends on the hybridization between the $f$-electron orbitals and those surrounding a distant nucleus. In CeMIn$_5$ (M=Rh, Ir, Co), both the hyperfine coupling to the two indium sites as well as the crystalline electric field at the Ce are strongly dependent on the transition metal. We measure a series of CeRh$_{1-x}$Ir$_x$In$_5$ crystals and find that the hyperfine coupling reflects the orbital anisotropy of the ground state Ce 4$f$ wavefunction. These findings provide direct proof that the localized to itinerant transition is dominated by hybridization out of the Ce-In plane in this system.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"3 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"79840821","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Finite-temperature symmetric tensor network for spin-1/2 Heisenberg antiferromagnets on the square lattice","authors":"D. Poilblanc, M. Mambrini, F. Alet","doi":"10.21468/SCIPOSTPHYS.10.1.019","DOIUrl":"https://doi.org/10.21468/SCIPOSTPHYS.10.1.019","url":null,"abstract":"Within the tensor network framework, the (positive) thermal density operator can be approximated by a double layer of infinite Projected Entangled Pair Operator (iPEPO) coupled via ancilla degrees of freedom. To investigate the thermal properties of the spin-1/2 Heisenberg model on the square lattice, we introduce a family of fully spin-$SU(2)$ and lattice-$C_{4v}$ symmetric on-site tensors (of bond dimensions $D=4$ or $D=7$) and a plaquette-based Trotter-Suzuki decomposition of the imaginary-time evolution operator. A variational optimization is performed on the plaquettes, using a full (for $D=4$) or simple (for $D=7$) environment obtained from the single-site Corner Transfer Matrix Renormalization Group fixed point. The method is benchmarked by a comparison to quantum Monte Carlo in the thermodynamic limit. Although the iPEPO spin correlation length starts to deviate from the exact exponential growth for inverse-temperature $beta gtrsim 2$, the behavior of various observables turns out to be quite accurate once plotted w.r.t the inverse correlation length. We also find that a direct $T=0$ variational energy optimization provides results in full agreement with the $betarightarrowinfty$ limit of finite-temperature data, hence validating the imaginary-time evolution procedure. Extension of the method to frustrated models is described and preliminary results are shown.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"1 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"72571196","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
T. Kobayashi, Q. Ding, H. Taniguchi, K. Satoh, A. Kawamoto, Y. Furukawa
{"title":"Charge disproportionation in the spin-liquid candidate \u0000κ−(ET)2Cu2(CN)3\u0000 at 6 K revealed by \u0000Cu63\u0000 NQR measurements","authors":"T. Kobayashi, Q. Ding, H. Taniguchi, K. Satoh, A. Kawamoto, Y. Furukawa","doi":"10.1103/physrevresearch.2.042023","DOIUrl":"https://doi.org/10.1103/physrevresearch.2.042023","url":null,"abstract":"The spin-liquid candidate $kappa$-(ET)$_2$Cu$_2$(CN)$_3$ [ET: bis(ethylenedithio)tetrathiafulvalene] does not exhibit magnetic ordering down to a very low temperature, but shows a mysterious anomaly at 6 K. The origin of the so-called 6 K anomaly is still under debate. We carried out nuclear quadrupole resonance (NQR) measurements on the copper sites of the insulating layers, which are sensitive to the charge dynamics unlike the conventional spin-1/2 nuclear magnetic resonance (NMR). The main finding of this study is that the observation of a sharp peak behavior in the nuclear spin-lattice relaxation rate $T_1^{-1}$ of $^{63}$Cu NQR at 6 K while $T_1^{-1}$ of both $^{13}$C and $^{1}$H NMR show no clear anomaly. This behavior can be understood as a second-order phase transition related to charge disproportionation in the ET layers.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"4 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76342167","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Statistics-tuned entanglement of the boundary modes in coupled Su-Schrieffer-Heeger chains","authors":"Saikat Santra, A. Agarwala, S. Bhattacharjee","doi":"10.1103/PhysRevB.103.195134","DOIUrl":"https://doi.org/10.1103/PhysRevB.103.195134","url":null,"abstract":"We show that mutual statistics between quantum particles can be tuned to generate emergent novel few particle quantum mechanics for the boundary modes of symmetry-protected topological phases of matter. As a concrete setting, we study a system of pseudofermions, defined as quantum particles with tunable algebra, which lie on two distinct Su-Schrieffer-Heeger (SSH) chains. We find that as the mutual statistics of the particles are tuned -- the boundary modes present in the two chains gets non-trivially entangled showing a sudden jump in their mutual entanglement entropy. We further show that, such tuning of statistics engenders a first-order transition between two topologically non-trivial phases which differ in the behavior of inter-chain entanglement. Using a combination of analytical and numerical techniques and effective modeling, we uncover the rich physics that this system hosts. The results are of particular relevance in context of the study of the effective low energy quantum mechanics of topological edge modes in one hand and their recent realization in ultracold atoms on the other. This then provides for controlled manipulation of such low energy modes.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"58 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"80529879","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Formation of spatial patterns by spin-selective excitations of interacting fermions","authors":"T. Köhler, S. Paeckel, C. Meyer, S. Manmana","doi":"10.1103/physrevb.102.235166","DOIUrl":"https://doi.org/10.1103/physrevb.102.235166","url":null,"abstract":"We describe the formation of charge- and spin-density patterns induced by spin-selective photoexcitations of interacting fermionic systems in the presence of a microstructure. As an example, we consider a one-dimensional Hubbard-like system with a periodic magnetic microstructure, which has a uniform charge distribution in its ground state, and in which a long-lived charge-density pattern is induced by the spin-selective photoexcitation. Using tensor-network methods, we study the full quantum dynamics in the presence of electron-electron interactions and identify doublons as main decay channel for the induced charge pattern. Our setup is compared to the OISTR mechanism, in which ultrafast optically induced spin-transfer in Heusler and magnetic compounds is associated to the difference of the local density of states of the different elements in the alloys. We find that applying a spin-selective excitation there induces spatially periodic patterns in local observables. Implications for pump-probe experiments on correlated materials and experiments with ultracold gases on optical lattices are discussed.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"34 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"78875440","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Ab initio\u0000 construction of the energy density functional for electron systems with the functional-renormalization-group-aided density functional theory","authors":"Takeru Yokota, T. Naito","doi":"10.1103/PhysRevResearch.3.L012015","DOIUrl":"https://doi.org/10.1103/PhysRevResearch.3.L012015","url":null,"abstract":"We show an $textit{ab initio}$ construction of the energy density functional (EDF) for electron systems using the functional renormalization group. The correlation energies of the homogeneous electron gas given in our framework reproduce the exact behavior at high density and agree with the Monte-Carlo data in a wide range of densities. Our analytic technique enables us to get the correlation energies efficiently for various densities, which realizes the determination of EDF in the local density approximation (LDA) without any fitting for physically relevant densities. Applied to the Kohn-Sham calculation for the noble-gas atoms, our EDF shows comparable results to those of other conventional ones in LDA.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"92 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"85864732","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Generalized diagonalization scheme for many-particle systems","authors":"S. Sykora, A. Hubsch, K. Becker","doi":"10.1103/PhysRevB.102.165122","DOIUrl":"https://doi.org/10.1103/PhysRevB.102.165122","url":null,"abstract":"Despite the advances in the development of numerical methods analytical approaches still play the key role on the way towards a deeper understanding of many-particle systems. In this regards, diagonalization schemes for Hamiltonians represent an important direction in the field. Among these techniques the method, presented here, might be that approach with the widest range of possible applications: We demonstrate that both stepwise and continuous unitary transformations to diagonalize the many-particle Hamiltonian as well as perturbation theory and also non-perturbative treatments can be understood within the same theoretical framework. The new method is based on the introduction of generalized projection operators and allows to develop a renormalization scheme which is used to evaluate directly the physical quantities of a many-particle system. The applicability of this approach is shown for two important elementary many-particle problems.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"39 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76664079","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
S. Gao, Ling-Fang Lin, A. May, B. Rai, Qiang Zhang, E. Dagotto, A. Christianson, M. Stone
{"title":"Weakly coupled alternating \u0000S=12\u0000 chains in the distorted honeycomb lattice compound \u0000Na2Cu2TeO6","authors":"S. Gao, Ling-Fang Lin, A. May, B. Rai, Qiang Zhang, E. Dagotto, A. Christianson, M. Stone","doi":"10.1103/physrevb.102.220402","DOIUrl":"https://doi.org/10.1103/physrevb.102.220402","url":null,"abstract":"Spin-1/2 chains with alternating antiferromagnetic (AF) and ferromagnetic (FM) couplings exhibit quantum entanglement like the integer-spin Haldane chains and might be similarly utilized for quantum computations. Such alternating AF-FM chains have been proposed to be realized in the distorted honeycomb-lattice compound Na$_2$Cu$_2$TeO$_6$, but to confirm this picture a comprehensive understanding of the exchange interactions including terms outside of the idealized model is required. Here we employ neutron scattering to study the spin dynamics in Na$_2$Cu$_2$TeO$_6$ and accurately determine the coupling strengths through the random phase approximation and density functional theory (DFT) approaches. We find the AF and FM intrachain couplings are the dominant terms in the spin Hamiltonian, while the interchain couplings are AF but perturbative. This hierarchy in the coupling strengths and the alternating signs of the intrachain couplings can be understood through their different exchange paths. Our results establish Na$_2$Cu$_2$TeO$_6$ as a weakly-coupled alternating AF-FM chain compound and reveal the robustness of the gapped ground state in alternating chains under weak interchain couplings.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"60 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"90609751","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Hidefumi Takahashi, K. Aono, Y. Nambu, R. Kiyanagi, T. Nomoto, M. Sakano, K. Ishizaka, R. Arita, S. Ishiwata
{"title":"Competing spin modulations in the magnetically frustrated semimetal EuCuSb","authors":"Hidefumi Takahashi, K. Aono, Y. Nambu, R. Kiyanagi, T. Nomoto, M. Sakano, K. Ishizaka, R. Arita, S. Ishiwata","doi":"10.1103/physrevb.102.174425","DOIUrl":"https://doi.org/10.1103/physrevb.102.174425","url":null,"abstract":"The competing magnetic ground states of the itinerant magnet EuCuSb, which has a hexagonal layered structure, were studied via magnetization, resistivity, and neutron diffraction measurements on single-crystal samples. EuCuSb has a three-dimensional semimetallic band structure as confirmed by band calculation and angle-resolved photoelectron spectroscopy, consistent with the nearly isotropic metallic conductivity in the paramagnetic state. However, below the antiferromagnetic transition temperature of TN1 (8.5 K), the resistivity, especially along the hexagonal axis, increases significantly. This implies the emergence of anisotropic magnetic ordering coupled to the conducting electrons. Neutron diffraction measurements show that the Eu spins, which order ferromagnetically within each layer, are collinearly modulated (up-up-down-down) along the hexagonal axis below TN1, followed by the partial emergence of helical spin modulation below TN2 (6 K). Based on the observation of anomalous magnetoresistance with hysteretic behavior, we discuss the competing nature of the ground state inherent in a frustrated Heisenberg-like spin system with a centrosymmetric structure.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"142 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77766187","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Quantum operator growth bounds for kicked tops and semiclassical spin chains","authors":"Chao Yin, A. Lucas","doi":"10.1103/PhysRevA.103.042414","DOIUrl":"https://doi.org/10.1103/PhysRevA.103.042414","url":null,"abstract":"We present a framework for understanding the dynamics of operator size, and bounding the growth of out-of-time-ordered correlators, in models of large-$S$ spins. Focusing on the dynamics of a single spin, we show the finiteness of the Lyapunov exponent in the large-$S$ limit; our bounds are tighter than the best known Lieb-Robinson-type bounds on these systems. We numerically find our upper bound on Lyapunov exponents is within an order of magnitude of numerically computed values in classical and quantum kicked top models. Generalizing our results to coupled large-$S$ spins on lattices, we show that the butterfly velocity, which characterizes the spatial speed of quantum information scrambling, is finite as $Srightarrowinfty$. We emphasize qualitative differences between operator growth in semiclassical large-spin models, and quantum holographic systems including the Sachdev-Ye-Kitaev model.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"30 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"73720401","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}