Advanced Sustainable Systems最新文献_第4页

Tailoring MOF-303 Reinforced Biopolymer Hybrid Coatings with Hierarchically Porous Architectures for Precision Nitrogen Delivery in Sustainable Agriculture (Adv. Sustainable Syst. 8/2025) 定制具有分层多孔结构的MOF-303增强生物聚合物杂化涂层，用于可持续农业的精准氮输送（ad . Sustainable system . 8/2025）

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-27 DOI: 10.1002/adsu.70107

Mingchuan Yang, Chunyan Tang, Meiqi Han, Zhaohui Tong, Yuechao Yang, Liwen Gao, Boning Su, DengLun Chen, Junyin Li, Long Zhang, Shugang Zhang

引用次数: 0

Evaluation of Absorbent Solutions for the Integrated CO2 Desorption and Electrolysis 综合CO2解吸和电解吸收溶液的评价

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-25 DOI: 10.1002/adsu.202500846

Fabian Hauf, Ricarda Kollmuß, Stefan Haufe, Elias Klemm

{"title":"Evaluation of Absorbent Solutions for the Integrated CO2 Desorption and Electrolysis","authors":"Fabian Hauf, Ricarda Kollmuß, Stefan Haufe, Elias Klemm","doi":"10.1002/adsu.202500846","DOIUrl":"https://doi.org/10.1002/adsu.202500846","url":null,"abstract":"CO2 electrolysis is an approach that contributes to mitigating global warming. Integrated CO2 electrolysis is a possibility to reduce operating costs by combining desorption and electrolysis. In this approach, it is important to provide sufficient CO2 directly from the absorbent solution to the catalyst, whereby the physically absorbed CO2 appears to play a central role. Therefore, the absorbent solution used for integrated electrolysis must meet a wide range of requirements, as it needs to supply sufficient CO2 while being compatible with the process conditions in the cell. In this study, it is demonstrated that KOH and piperazine (PZ) are suitable absorbent solutions for integrated CO2 electrolysis among the three tested groups of absorbents – namely, inorganic, amines, and physical absorbents. The results reveal that physical absorbents provide the highest amount of accessible CO2 for electrolysis, whereas inorganic absorbents exhibit the highest compatibility with the membranes. KOH and PZ demonstrate the ability to withstand the electrochemical conditions during CO2 electrolysis and the capability to produce C2+ products during integrated CO2 electrolysis. These results highlight the critical importance of absorbent selection and demonstrate the feasibility of using KOH as well as amine-based solutions, such as PZ, for integrated CO2 electrolysis.","PeriodicalId":7294,"journal":{"name":"Advanced Sustainable Systems","volume":"9 10","pages":""},"PeriodicalIF":6.1,"publicationDate":"2025-08-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/adsu.202500846","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145341778","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Molten Salt Preparation of Rice Husk Biocarbon for Lightweight and Efficient Microwave Absorption 稻壳生物碳轻质高效微波吸收熔盐制备研究

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-25 DOI: 10.1002/adsu.202500736

Yuhao Zhang, Bin Li, Chaoen Li, Jie Zhao, Dongjing Liu

引用次数: 0

A Review on Rubber Nanocomposites for Strain Sensing Applications 橡胶纳米复合材料应变传感研究进展

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-23 DOI: 10.1002/adsu.202500893

Drisya Mottammal, Jayesh Cherusseri, Susmi Anna Thomas, Deepthi N. Rajendran, Cheol Joo Moon, Myong Yong Choi

{"title":"A Review on Rubber Nanocomposites for Strain Sensing Applications","authors":"Drisya Mottammal, Jayesh Cherusseri, Susmi Anna Thomas, Deepthi N. Rajendran, Cheol Joo Moon, Myong Yong Choi","doi":"10.1002/adsu.202500893","DOIUrl":"https://doi.org/10.1002/adsu.202500893","url":null,"abstract":"Rubber nanocomposites play a unique role in modern translational research due to its tunable properties and wide-ranging applications. Rubber is a natural material that finds use in diverse fields, including sanitation, health care, households, energy storage, and sensors. The properties of natural rubber can be modified by preparing nanocomposites with secondary fillers such as carbon nanotubes, graphene, and conducting polymers to achieve the desired characteristics. Rubber nanocomposites are sustainable materials that are highly eco-friendly, low-cost, and scalable. A comprehensive review in the area of rubber nanocomposites for strain sensing applications is currently lacking in the literature. This gap motivated us to write a review on rubber nanocomposites for strain sensing applications. Initially, the key properties of rubber nanocomposites are discussed. Subsequently, various synthesis approaches used to prepare rubber nanocomposites are presented. Furthermore, the strain sensing properties of rubber nanocomposites are highlighted, with a detailed discussion on its strain sensing capabilities. This review proclaims the advancement of sustainable rubber nanocomposite-based materials for strain sensing applications, emphasizing their high selectivity, flexibility, and specificity for integration into next-generation on-body wearable electronic devices.","PeriodicalId":7294,"journal":{"name":"Advanced Sustainable Systems","volume":"9 10","pages":""},"PeriodicalIF":6.1,"publicationDate":"2025-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145341899","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Multifunctional Molybdenum Disulfide Nanoarchitectures for Advanced Lithium-Sulfur Batteries: Comprehensive Strategies for Cathode Catalysis, Separator Modification, and Anode Stabilization 先进锂硫电池的多功能二硫化钼纳米结构：阴极催化，分离器改性和阳极稳定的综合策略

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-23 DOI: 10.1002/adsu.202501043

Hongwei Guo, Xiao-Chen Liu, Yu Zhang, Kui Chen, Guangning Wu

{"title":"Multifunctional Molybdenum Disulfide Nanoarchitectures for Advanced Lithium-Sulfur Batteries: Comprehensive Strategies for Cathode Catalysis, Separator Modification, and Anode Stabilization","authors":"Hongwei Guo, Xiao-Chen Liu, Yu Zhang, Kui Chen, Guangning Wu","doi":"10.1002/adsu.202501043","DOIUrl":"https://doi.org/10.1002/adsu.202501043","url":null,"abstract":"Lithium-sulfur (Li-S) batteries have garnered significant attention due to their exceptional theoretical energy density (2600 Wh kg−1), utilization of earth-abundant sulfur resources, and environmental compatibility. However, their practical implementation faces substantial challenges, including shuttle effects, sluggish sulfur redox kinetics, and uncontrolled lithium dendrite formation. Molybdenum disulfide (MoS2) nanosheets are demonstrated to serve as a versatile catalytic platform to concurrently mitigate these fundamental limitations. This comprehensive review aims to systematically summarize recent advances in MoS2-engineered modification strategies across three key domains: 1) sulfur cathode hosts for enhanced electrocatalysis, 2) functional separator/interlayer designs, and 3) lithium anode stabilization approaches. Furthermore, persistent challenges are critically analyzed, and strategic research directions are proposed for optimizing MoS2-engineered systems, aiming to design high-energy-density and long-life Li-S batteries in the future.","PeriodicalId":7294,"journal":{"name":"Advanced Sustainable Systems","volume":"9 10","pages":""},"PeriodicalIF":6.1,"publicationDate":"2025-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145341898","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Fully Plant-Based and Optically Transparent Wood Substrates with Improved Thermal Insulating Properties 完全基于植物和光学透明的木材基材，具有改进的隔热性能

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-21 DOI: 10.1002/adsu.202500564

Liya Antony, Antonella Giuri, Simone Bruno, Sudipto Pal, Sonia Carallo, Iolena Tarantini, Antonio Licciulli, Marco Pugliese, Vincenzo Maiorano, Carola Esposito Corcione, Barbara Cortese, Luisa De Marco, Aurora Rizzo

{"title":"Fully Plant-Based and Optically Transparent Wood Substrates with Improved Thermal Insulating Properties","authors":"Liya Antony, Antonella Giuri, Simone Bruno, Sudipto Pal, Sonia Carallo, Iolena Tarantini, Antonio Licciulli, Marco Pugliese, Vincenzo Maiorano, Carola Esposito Corcione, Barbara Cortese, Luisa De Marco, Aurora Rizzo","doi":"10.1002/adsu.202500564","DOIUrl":"https://doi.org/10.1002/adsu.202500564","url":null,"abstract":"Transparent wood composites are gaining interest for their superior properties over natural wood (PW), including superior transparency, thermal insulation, and stability. These composites are manufactured via infiltration of bio-based polymers into porous bleached wood (BW), offering a sustainable alternative to glass and plastic in applications such as energy-efficient windows and smartphone displays. In this study, the highest level of transparency in transparent wood (TW) substrates is achieved using biobased resins and an environmentally friendly bleaching process. Pristine balsa wood is bleached using non-toxic chemicals and subsequently infiltrated with two bio-based commercial resins, both sustainable and biocompatible. The performance of these bio-based composites is compared to conventional epoxy resin. Resin viscosity is shown to influence the physical, optical, thermal, and mechanical characteristics of the final composite due to its ability to penetrate and interact with the wood's porous structure. Notably, the plant-based soya resin-infiltrated TW achieves exceptional properties, as 91% transparency at 550 nm, alongside remarkable UV stability and hydrophobicity. Additionally, this bio-based composite shows a ≈50% reduction in thermal conductivity compared to standard glass (≈1 W m·K−1), highlighting its potential as a thermally insulative, energy-efficient material for building-integrated applications.","PeriodicalId":7294,"journal":{"name":"Advanced Sustainable Systems","volume":"9 10","pages":""},"PeriodicalIF":6.1,"publicationDate":"2025-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/adsu.202500564","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145341458","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Surface Modification of MoS2 Via Fluorine and Bromine Doping for Efficient Catalysis in Oxygen Evolution and Dye Degradation 氟溴掺杂对二硫化钼表面改性对析氧和染料降解的高效催化作用

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-21 DOI: 10.1002/adsu.202500317

Tania Shahzadi, Sobia Dilpazir, Muhammd Imran, Sawaira Moeen, Anwar Ul-Hamid, Ghafar Ali, Muhammad Ikram, Souraya Goumri-Said, Mohammed Benali Kanoun

{"title":"Surface Modification of MoS2 Via Fluorine and Bromine Doping for Efficient Catalysis in Oxygen Evolution and Dye Degradation","authors":"Tania Shahzadi, Sobia Dilpazir, Muhammd Imran, Sawaira Moeen, Anwar Ul-Hamid, Ghafar Ali, Muhammad Ikram, Souraya Goumri-Said, Mohammed Benali Kanoun","doi":"10.1002/adsu.202500317","DOIUrl":"https://doi.org/10.1002/adsu.202500317","url":null,"abstract":"Tailoring highly efficient and robust bifunctional catalysts for enhanced oxygen evolution reaction (OER) as well as organic dye degradation is intriguing but still a triggering concern. Herein, variable concentrations (1 and 3 wt.%) of fluorine (F) with a fixed amount (3%) of bromine (Br) are effectively synthesized in doped molybdenum disulfide (MoS2) nanosheets by a facile hydrothermal strategy. This research aimed to efficiently degrade Rhodamine B (RhB) dye together with significant OER kinetics. Optical properties, structural morphology, functional group analysis, elemental composition, and crystallinity of synthesized catalysts are investigated by employing cutting-edge techniques. Among all samples, the optimized sample (3% F/Br-MoS2) exhibited maximum RhB reduction efficacy in a basic medium. Linear sweep voltammetry (LSV), cyclic voltammetry (CV), Tafel plot, and electrochemical impedance spectroscopy (EIS) are conducted to evaluate the electrochemical OER performance of synthesized electrocatalysts. The optimized sample exhibited minimal overpotential, Tafel slope, and charge transfer resistance, indicating the highest OER activity. First-principles calculations of OH− adsorption energies on pristine and F/Br-doped MoS2 monolayers suggest that F/Br doping may enhance OER activity. This work paves a pathway to the design of unique, cost-effective, and promising materials for synthetic dye removal and high-performance catalysts for water splitting.","PeriodicalId":7294,"journal":{"name":"Advanced Sustainable Systems","volume":"9 10","pages":""},"PeriodicalIF":6.1,"publicationDate":"2025-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145341457","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Engineering Poly(Lactic Acid)/Cellulose Nanocrystal Composites: A Comparative Review of Preparation Strategies and their Influence on Structure-Property Relationships 工程聚乳酸/纤维素纳米晶复合材料的制备策略及其对结构-性能关系的影响

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-21 DOI: 10.1002/adsu.202500654

Jimin Ryoo, Dongyeop X. Oh, Jeyoung Park

{"title":"Engineering Poly(Lactic Acid)/Cellulose Nanocrystal Composites: A Comparative Review of Preparation Strategies and their Influence on Structure-Property Relationships","authors":"Jimin Ryoo, Dongyeop X. Oh, Jeyoung Park","doi":"10.1002/adsu.202500654","DOIUrl":"https://doi.org/10.1002/adsu.202500654","url":null,"abstract":"The incorporation of cellulose nanocrystals (CNCs) into poly(lactic acid) (PLA) matrices has emerged as a promising approach to enhance the mechanical, thermal, and rheological properties of bioplastics. However, the final properties of PLA/CNC nanocomposites are dependent on the preparation methods employed. This review explores the impact of various synthesis techniques, including chemical grafting, melt processing, and solution-based approaches, on the dispersion, interfacial adhesion, and performance of PLA/CNC composites. While melt processing methods such as extrusion offer scalable production, they often lead to CNC aggregation, limiting reinforcement efficiency. In contrast, solution-based methods provide improved CNC dispersion but introduce challenges related to solvent removal and processing complexity. Recent advancements in reactive extrusion and surface-modified CNCs have demonstrated potential in mitigating these limitations. By comparing the effects of these preparation strategies on crystallinity, mechanical reinforcement, and rheological behavior, this review provides insights into optimizing PLA/CNC nanocomposite formulations for diverse applications, including packaging, biomedical devices, and additive manufacturing.","PeriodicalId":7294,"journal":{"name":"Advanced Sustainable Systems","volume":"9 10","pages":""},"PeriodicalIF":6.1,"publicationDate":"2025-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/adsu.202500654","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145341838","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

n-Bi2MoO6 Nanoflake-Decorated p-CuBi2O4 Microrod Photoanode for Simultaneous Hydrogen Evolution and Rhodamine B Degradation in Alkaline Electrolyte and Natural Seawater n-Bi2MoO6纳米片修饰的p-CuBi2O4微棒光阳极在碱性电解质和自然海水中同时析氢和罗丹明B降解

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-20 DOI: 10.1002/adsu.202500701

Sadanan Boochakiat, Burapat Inceesungvorn, Klaudia Wagner, Jun Chen

{"title":"n-Bi2MoO6 Nanoflake-Decorated p-CuBi2O4 Microrod Photoanode for Simultaneous Hydrogen Evolution and Rhodamine B Degradation in Alkaline Electrolyte and Natural Seawater","authors":"Sadanan Boochakiat, Burapat Inceesungvorn, Klaudia Wagner, Jun Chen","doi":"10.1002/adsu.202500701","DOIUrl":"https://doi.org/10.1002/adsu.202500701","url":null,"abstract":"Herein, n-Bi2MoO6 nanoflake-decorated p-CuBi2O4 microrod photoanode (CB) is successfully fabricated. To the best of the knowledge, this is the first report demonstrating the simultaneous photoelectrocatalysistic (PEC) of RhB degradation and hydrogen evolution using a single photoanode under visible light in both alkaline electrolyte and natural seawater. The enhanced performance of the composite photoanode is attributed to improved charge separation efficiency via the creation of an internal electric field as supported by Mott–Schottky, transient photocurrent, and EIS studies. The proposed PEC mechanism reveals that direct hole oxidation played a decisive role in the degradation of RhB and that the presence of RhB can boost the H2 production. In natural seawater, the PEC degradation of RhB is markedly improved, attributed to the high conductivity of seawater. Although the hydrogen evolution is significantly suppressed in seawater due mainly to the deposition of Mg(OH)2 and Ca(OH)2 at Pt cathode, the findings are the first to show the potential application of p-CuBi2O4/n-Bi2MoO6 photoanode for PEC water purification and simultaneous renewable energy production in natural seawater. This work may pave the way for more sustainable solutions in water and energy management for real-world applications.","PeriodicalId":7294,"journal":{"name":"Advanced Sustainable Systems","volume":"9 10","pages":""},"PeriodicalIF":6.1,"publicationDate":"2025-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145341642","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Solar-Driven Plastic Upcycling Coupled with Valuable Reduction Reactions 太阳能驱动的塑料升级回收加上有价值的还原反应

IF 6.1 3区材料科学

Advanced Sustainable Systems Pub Date : 2025-08-20 DOI: 10.1002/adsu.202500735

Xiang Gao, Longfei Hong, Huiyan Zhang, Sheng Chu

{"title":"Solar-Driven Plastic Upcycling Coupled with Valuable Reduction Reactions","authors":"Xiang Gao, Longfei Hong, Huiyan Zhang, Sheng Chu","doi":"10.1002/adsu.202500735","DOIUrl":"https://doi.org/10.1002/adsu.202500735","url":null,"abstract":"Solar-powered valorization of plastic waste has emerged as a promising strategy to address the dual challenges of environmental pollution and sustainable carbon resource utilization. By harnessing solar energy and enabling spatially separated redox reactions, solar-driven systems facilitate integrated upcycling pathways that couple oxidative upcycling of plastic with value-added reductive transformations, which overcome the thermodynamic constraints of conventional single transformation, enhance the charge carrier utilization, and economic benefits. This review highlights recent advances in solar-driven photocatalytic and photoelectrocatalytic plastic upcycling integrated with valuable reduction reactions, with a focus on charge transfer properties at substrate-catalyst interfaces, and structure-property relationships. The photooxidative conversion of different plastic wastes is first discussed (such as polyethylene terephthalate, polyolefins, polystyrene, polyvinyl chloride, and polylactic acid) into valuable chemical products. Then, the progress of solar-driven plastic waste-assisted H2 evolution, CO2 reduction, and H2O2 synthesis is summarized. Finally, the challenges and the perspectives on solar-driven plastic upcycling coupled with valuable reduction reactions are also put forward. This review aims to offer insight on the design of next-generation solar-driven platforms for a circular and sustainable plastics economy.","PeriodicalId":7294,"journal":{"name":"Advanced Sustainable Systems","volume":"9 10","pages":""},"PeriodicalIF":6.1,"publicationDate":"2025-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145341640","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0