Advanced Powder Materials最新文献

筛选
英文 中文
Al2O3 nanoparticles as surface modifier enables deposition of high quality perovskite films for ultra-flexible photovoltaics Al2O3纳米颗粒作为表面改性剂,可以沉积高质量的钙钛矿薄膜,用于超柔性光伏电池
Advanced Powder Materials Pub Date : 2023-06-17 DOI: 10.1016/j.apmate.2023.100142
Zhiyong Wang , Qingshun Dong , Ying Yan , Zikeng Fang , Guojun Mi , Mingzhu Pei , Shuhong Wang , Linghui Zhang , Jing Liu , Min Chen , Hongru Ma , Ruiting Wang , Jie Zhang , Chun Cheng , Yantao Shi
{"title":"Al2O3 nanoparticles as surface modifier enables deposition of high quality perovskite films for ultra-flexible photovoltaics","authors":"Zhiyong Wang ,&nbsp;Qingshun Dong ,&nbsp;Ying Yan ,&nbsp;Zikeng Fang ,&nbsp;Guojun Mi ,&nbsp;Mingzhu Pei ,&nbsp;Shuhong Wang ,&nbsp;Linghui Zhang ,&nbsp;Jing Liu ,&nbsp;Min Chen ,&nbsp;Hongru Ma ,&nbsp;Ruiting Wang ,&nbsp;Jie Zhang ,&nbsp;Chun Cheng ,&nbsp;Yantao Shi","doi":"10.1016/j.apmate.2023.100142","DOIUrl":"10.1016/j.apmate.2023.100142","url":null,"abstract":"<div><p>Advanced photovoltaics, such as ultra-flexible perovskite solar cells (UF-PSCs), which are known for their lightweight design and high power-to-mass ratio, have been a long-standing goal that we, as humans, have continuously pursued. Unlike normal PSCs fabricated on rigid substrates, producing high-efficiency UF-PSCs remains a challenge due to the difficulty in achieving full coverage and minimizing defects of metal halide perovskite (MHP) films. In this study, we utilized Al<sub>2</sub>O<sub>3</sub> nanoparticles (NPs) as an inorganic surface modifier to enhance the wettability and reduce the roughness of poly-bis(4-phenyl) (2,4,6-trimethylphenyl) amine simultaneously. This approach proves essentials in fabricating UF-PSCs, enabling the deposition of uniform and dense MHP films with full coverage and fewer defects. We systematically investigated the effect of Al<sub>2</sub>O<sub>3</sub> NPs on film formation, combining simulation with experiments. Our strategy not only significantly increases the power conversion efficiency (PCE) from 11.96% to 16.33%, but also promotes reproducibility by effectively addressing the short circuit issue commonly encountered in UF-PSCs. Additionally, our UF-PSCs demonstrates good mechanical stability, maintaining 98.6% and 79.0% of their initial PCEs after 10,000 bending cycles with radii of 1.0 and 0.5 ​mm, respectively.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"3 1","pages":"Article 100142"},"PeriodicalIF":0.0,"publicationDate":"2023-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772834X23000349/pdfft?md5=5105a9f7649ddccf65ba4477aa2ddcc6&pid=1-s2.0-S2772834X23000349-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"72738101","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Functional inorganic additives in composite solid-state electrolytes for flexible lithium metal batteries 柔性锂金属电池用复合固态电解质中的功能性无机添加剂
Advanced Powder Materials Pub Date : 2023-06-13 DOI: 10.1016/j.apmate.2023.100141
Honglan Huang , Chao Liu , Ziya Liu , Yunyan Wu, Yifan Liu, Jinbo Fan, Gen Zhang, Pan Xiong, Junwu Zhu
{"title":"Functional inorganic additives in composite solid-state electrolytes for flexible lithium metal batteries","authors":"Honglan Huang ,&nbsp;Chao Liu ,&nbsp;Ziya Liu ,&nbsp;Yunyan Wu,&nbsp;Yifan Liu,&nbsp;Jinbo Fan,&nbsp;Gen Zhang,&nbsp;Pan Xiong,&nbsp;Junwu Zhu","doi":"10.1016/j.apmate.2023.100141","DOIUrl":"10.1016/j.apmate.2023.100141","url":null,"abstract":"<div><p>Flexible lithium metal batteries with high capacity and power density have been regarded as the core power resources of wearable electronics. However, the main challenge lies in the limited electrochemical performance of solid-state polymer electrolytes, which hinders further practical applications. Incorporating functional inorganic additives is an effective approach to improve the performance, including increasing ionic conductivity, achieving dendrite inhibiting capability, and improving safety and stability. Herein, this review summarizes the latest developments of functional inorganic additives in composite solid-state electrolytes for flexible metal batteries with special emphasis on their mechanisms, strategies, and cutting-edge applications, in particular, the relationship between them is discussed in detail. Finally, the perspective on future research directions and the key challenges on this topic are outlooked.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"3 1","pages":"Article 100141"},"PeriodicalIF":0.0,"publicationDate":"2023-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772834X23000337/pdfft?md5=a4a4906316b59b7ea169b1725e083595&pid=1-s2.0-S2772834X23000337-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"75683410","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Chemically bonded BiVO4/Bi19Cl3S27 heterojunction with fast hole extraction dynamics for continuous CO2 photoreduction 化学键合BiVO4/Bi19Cl3S27异质结与快速空穴萃取动力学的连续CO2光还原
Advanced Powder Materials Pub Date : 2023-06-05 DOI: 10.1016/j.apmate.2023.100140
Baojing Huang , Xinxin Fu , Kai Wang , Liang Wang , Hualei Zhang , Zhongyi Liu , Bin Liu , Jun Li
{"title":"Chemically bonded BiVO4/Bi19Cl3S27 heterojunction with fast hole extraction dynamics for continuous CO2 photoreduction","authors":"Baojing Huang ,&nbsp;Xinxin Fu ,&nbsp;Kai Wang ,&nbsp;Liang Wang ,&nbsp;Hualei Zhang ,&nbsp;Zhongyi Liu ,&nbsp;Bin Liu ,&nbsp;Jun Li","doi":"10.1016/j.apmate.2023.100140","DOIUrl":"10.1016/j.apmate.2023.100140","url":null,"abstract":"<div><p>Surface charge localization and inferior charge transfer efficiency seriously restrict the supply of reactive hydrogen and the reaction dynamics of CO<sub>2</sub> photoreduction performance of photocatalysts. Herein, chemically bonded BiVO<sub>4</sub>/Bi<sub>19</sub>Cl<sub>3</sub>S<sub>27</sub> (BVO/BCS) S-scheme heterojunction with a strong internal electric field is designed. Experimental and density function theory calculation results confirm that the elaborated heterojunction accelerates the vectorial migration of photogenerated charges from BiVO<sub>4</sub> to Bi<sub>19</sub>Cl<sub>3</sub>S<sub>27</sub> via the interfacial chemical bonding interactions (i.e., Bi-O and Bi-S bonds) between Bi atoms of BVO and S atoms of BCS or Bi atoms of BCS and O atoms of BVO under light irradiation, breaking the interfacial barrier and surface charge localization of Bi<sub>19</sub>Cl<sub>3</sub>S<sub>27</sub>, and further decreasing the energy of reactive hydrogen generation, CO<sub>2</sub> absorption and activation. The separation efficiency of photogenerated carriers is much more efficient than that counterpart individual in BVO/BCS S-scheme heterojunction system. As a result, BVO/BCS heterojunction exhibits a significantly improved continuous photocatalytic performance for CO<sub>2</sub> reduction and the 24 ​h CO yield reaches 678.27 ​μmol·g<sup>−1</sup>. This work provides an atomic-level insight into charge transfer kinetics and CO<sub>2</sub> reduction mechanism in S-scheme heterojunction.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"3 1","pages":"Article 100140"},"PeriodicalIF":0.0,"publicationDate":"2023-06-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772834X23000325/pdfft?md5=2fef6f28965db0538dbed05d7f27317d&pid=1-s2.0-S2772834X23000325-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"73223877","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 8
Selective laser melting of GH3536 superalloy: Microstructure, mechanical properties, and hydrocyclone manufacturing GH3536高温合金激光粉末床熔合:组织、力学性能及旋流器制造
Advanced Powder Materials Pub Date : 2023-05-28 DOI: 10.1016/j.apmate.2023.100134
Chengzhe Yu , Nan Chen , Ruidi Li , Tiechui Yuan , Shisen Huang , Xin Ma , Yi Zhang , Min Huang , Liang Lv , Ruoyu Liu , Yuanyuan Jiang , Xingyan Liu , Duan Lai
{"title":"Selective laser melting of GH3536 superalloy: Microstructure, mechanical properties, and hydrocyclone manufacturing","authors":"Chengzhe Yu ,&nbsp;Nan Chen ,&nbsp;Ruidi Li ,&nbsp;Tiechui Yuan ,&nbsp;Shisen Huang ,&nbsp;Xin Ma ,&nbsp;Yi Zhang ,&nbsp;Min Huang ,&nbsp;Liang Lv ,&nbsp;Ruoyu Liu ,&nbsp;Yuanyuan Jiang ,&nbsp;Xingyan Liu ,&nbsp;Duan Lai","doi":"10.1016/j.apmate.2023.100134","DOIUrl":"10.1016/j.apmate.2023.100134","url":null,"abstract":"<div><p>The effect of scanning strategy on the microstructure and properties of GH3536 Ni-based superalloy prepared by Laser Powder Bed Fusion was investigated, for the purpose of building high quality hydrocyclone part. The results show that the strength of Z67° (a zone with 67° hatch angle strategy) specimen is the highest among the four scanning strategies (0°, 67°, 90°and Z67°), with yield strength and tensile strength of 681 ​MPa and 837 ​MPa, respectively. Selective orientation of crystals occurs during the forming process because the longitudinal section of the specimen exhibits a high texture strength in (001). As the stretching proceeds, the plastic deformation mechanism of the specimen gradually changes from slip to twin-dominated, a substantial amount of twinning is observed in the region where the deformation of the specimen reaches 80%. The additive manufacturing simulation suite: Ansys Additive is used to simulate the stress and deformation of the part during the process, and the displacement results are consistent with the experimental phenomena. According to the simulation results, the structure design is optimized and the surface quality of the part is improved. The results show that the support of the part is more reasonable when the overhang angle is 45°.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"3 1","pages":"Article 100134"},"PeriodicalIF":0.0,"publicationDate":"2023-05-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772834X2300026X/pdfft?md5=846fb78d5849193bd4f56aaf0c87d4c6&pid=1-s2.0-S2772834X2300026X-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"81472888","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Insights into atomically dispersed reactive centers on g-C3N4 photocatalysts for water splitting g-C3N4光催化剂上原子分散反应中心的研究进展
Advanced Powder Materials Pub Date : 2023-04-01 DOI: 10.1016/j.apmate.2022.100094
Wenzhe Shang , Wei Liu , Xiangbin Cai , Jinwen Hu , Jingya Guo , Cuncun Xin , Yuehui Li , Naitian Zhang , Ning Wang , Ce Hao , Yantao Shi
{"title":"Insights into atomically dispersed reactive centers on g-C3N4 photocatalysts for water splitting","authors":"Wenzhe Shang ,&nbsp;Wei Liu ,&nbsp;Xiangbin Cai ,&nbsp;Jinwen Hu ,&nbsp;Jingya Guo ,&nbsp;Cuncun Xin ,&nbsp;Yuehui Li ,&nbsp;Naitian Zhang ,&nbsp;Ning Wang ,&nbsp;Ce Hao ,&nbsp;Yantao Shi","doi":"10.1016/j.apmate.2022.100094","DOIUrl":"https://doi.org/10.1016/j.apmate.2022.100094","url":null,"abstract":"<div><p>Co-catalysts decorations provide unique opportunity in promoting the photocatalytic water splitting performance of graphite carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) system, while mechanistic understanding of this complex catalytic network remains elusive. Here, taking the single-atom-based photocatalysts (M<sub>1</sub>-g-C<sub>3</sub>N<sub>4</sub>) as an unprecedented simplified model system, we theoretically tracked the photocatalytic kinetics for a comprehensive understanding of the photocatalytic process and afforded the descriptor <em>α</em><sub>S1-T1/</sub><em>α</em><sub>T1-S0</sub> (ratio of the extent of S<sub>1</sub>-T<sub>1</sub> and T<sub>1</sub>-S<sub>0</sub> state mixing) and Δ<em>G</em><sub>H∗</sub> (hydrogen adsorpti on free energy) for rational screening of photocatalysts. The targeted Fe<sub>1</sub>-g-C<sub>3</sub>N<sub>4</sub> yields an excellent H<sub>2</sub> evolution rate (ca. 3.2 ⋅mmol·g<sub>cat</sub><sup>−1</sup>·h<sup>−1</sup> under full arc), two order of magnitude improvement relative to pristine g-C<sub>3</sub>N<sub>4</sub> counterpart and also outperforms other representative 3d-transition-metal-based photocatalysts. This work presents a comprehensive understanding of the essential role of isolated atomic sites in the photocatalytic course and sheds light on the design of photocatalysts from both photophysical and photochemical aspects.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"2 2","pages":"Article 100094"},"PeriodicalIF":0.0,"publicationDate":"2023-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49734771","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 17
MXenes in tribology: Current status and perspectives 摩擦学中的MXenes:现状与展望
Advanced Powder Materials Pub Date : 2023-04-01 DOI: 10.1016/j.apmate.2022.100092
Xiaonan Miao , Zhangpeng Li , Shuwen Liu , Jinqing Wang , Shengrong Yang
{"title":"MXenes in tribology: Current status and perspectives","authors":"Xiaonan Miao ,&nbsp;Zhangpeng Li ,&nbsp;Shuwen Liu ,&nbsp;Jinqing Wang ,&nbsp;Shengrong Yang","doi":"10.1016/j.apmate.2022.100092","DOIUrl":"https://doi.org/10.1016/j.apmate.2022.100092","url":null,"abstract":"<div><p>MXenes are an emerging class of new two-dimensional materials, which have been widely used in energy storage, catalysis, sensing, biology, and other fields due to their unique structure and properties. The distinct structure, low shear resistance, and easy-to-modify ability endow MXenes with particularly superior lubrication potentials. This review highlights the research status and applications of MXenes lubrication categorized into solid lubricants, lubricant additives, and reinforcement phase parts, summaries the influencing factors and lubrication mechanisms of MXenes lubrication, points out some unexplored research fields and unsettled questions, and then puts forwards possible solutions and prospects for the future research. The lubrication advances and potentials of MXenes are fully verified. Predictably, the emerging MXenes lubricants will exhibit remarkable application prospects in advanced manufacturing such as machining industries, automotive industries, micro/nano-electromechanical systems, and spacecraft components.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"2 2","pages":"Article 100092"},"PeriodicalIF":0.0,"publicationDate":"2023-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49716200","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 20
Elemental segregation inhibits hydrogen embrittlement in aluminium alloys 元素偏析抑制铝合金中的氢脆
Advanced Powder Materials Pub Date : 2023-04-01 DOI: 10.1016/j.apmate.2022.100099
Jun Hui , Biao Wang , Jiapeng Chen , Xiaoyong Zhang
{"title":"Elemental segregation inhibits hydrogen embrittlement in aluminium alloys","authors":"Jun Hui ,&nbsp;Biao Wang ,&nbsp;Jiapeng Chen ,&nbsp;Xiaoyong Zhang","doi":"10.1016/j.apmate.2022.100099","DOIUrl":"https://doi.org/10.1016/j.apmate.2022.100099","url":null,"abstract":"<div><p>In this study, we performed first-principles calculations to determine the effects of four metallic solutes (Y, Zr, Mg, and Zn) on the hydrogen embrittlement (HE) of aluminum alloys with the Σ5(210) grain boundary (GB). The segregation energy, associated segregation concentration, and binding energy of these solutes were examined to identify their states. Moreover, the ability of the aforementioned solutes to inhibit or promote HE in the aforementioned alloys through GB energy, free surface energy, and adhesion was investigated. The Griffith and Rice–Wang–Scheiber models were used to determine the effect of nonequilibrium concentration on adhesion. Tensile tests were performed using the uniaxial strain loading method to determine the ultimate tensile strength and GB elongation of the considered alloys. The mechanism of HE inhibition by the four solutes was investigated by examining the charge density, Bader charge, and crystal orbital Hamiltonian population of the alloys. Finally, the calculation results of this study were validated through experiments.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"2 2","pages":"Article 100099"},"PeriodicalIF":0.0,"publicationDate":"2023-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49716137","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Assembling of low-dimensional aggregates with interlaminar electromagnetic synergy network for high-efficient microwave absorption 利用层间电磁协同网络组装低维聚集体实现高效微波吸收
Advanced Powder Materials Pub Date : 2023-04-01 DOI: 10.1016/j.apmate.2022.100100
Fei Pan , Xiaofen Wu , Dan Batalu , Wei Lu , Hongtao Guan
{"title":"Assembling of low-dimensional aggregates with interlaminar electromagnetic synergy network for high-efficient microwave absorption","authors":"Fei Pan ,&nbsp;Xiaofen Wu ,&nbsp;Dan Batalu ,&nbsp;Wei Lu ,&nbsp;Hongtao Guan","doi":"10.1016/j.apmate.2022.100100","DOIUrl":"https://doi.org/10.1016/j.apmate.2022.100100","url":null,"abstract":"<div><p>Considering the risk of a sudden degeneration caused by the oxidation of MXenes in dielectric and microwave absorption properties, to enhance the oxidation resistance of multilayer MXenes can make them more applicable as microwave absorbers than those with few-layer. However, there remains disadvantage in optimizing the poor impedance matching and inherent aggregation of multilayer MXenes via rational assembling. In the present study, a facile self-assembly process is conducted to obtain 2D MXenes/1D MnO<sub>2</sub>/0D NiCo<sub>2</sub>S<sub>4</sub> assembled low-dimensional aggregate with hierarchical structure and interlaminar electromagnetic synergy network. In addition to bridging adjacent MXenes lamellas for the enhancement of internal electron transport, high-density MnO<sub>2</sub> can also combine with NiCo<sub>2</sub>S<sub>4</sub> to form an electromagnetic synergy network between lamellas, thus improving microwave attenuation. Though the modulation of components and assembled structures, it is achievable to effectively adjust and optimize the performance in impedance matching and microwave absorption. Given the thickness of 2.17 ​mm, the optimal reflection loss of −59.23 ​dB, and the effective absorption bandwidth of 5.8 ​GHz are achieved. Moreover, the RCS simulations is performed to demonstrate its excellent performance. Thus, the present work contributes a facile method to the development of multi-layer MXenes based-MAs via interlaminar electromagnetic network design.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"2 2","pages":"Article 100100"},"PeriodicalIF":0.0,"publicationDate":"2023-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49716136","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 16
Construction of zinc metal-Tin sulfide polarized interface for stable Zn metal batteries 稳定锌金属电池中锌金属-硫化锡极化界面的构建
Advanced Powder Materials Pub Date : 2023-04-01 DOI: 10.1016/j.apmate.2022.100093
Yingzhu Hu , Chunyan Fu , Simin Chai , Qiong He , Yijiang Wang , Mingyang Feng , Yifang Zhang , Anqiang Pan
{"title":"Construction of zinc metal-Tin sulfide polarized interface for stable Zn metal batteries","authors":"Yingzhu Hu ,&nbsp;Chunyan Fu ,&nbsp;Simin Chai ,&nbsp;Qiong He ,&nbsp;Yijiang Wang ,&nbsp;Mingyang Feng ,&nbsp;Yifang Zhang ,&nbsp;Anqiang Pan","doi":"10.1016/j.apmate.2022.100093","DOIUrl":"https://doi.org/10.1016/j.apmate.2022.100093","url":null,"abstract":"<div><p>Aqueous Zn metal batteries have become competitive electrochemical energy storage systems owing to their material abundance, low cost, high capacity, and nontoxicity. Nevertheless, the notorious Zn dendrites and poor anode reversibility caused by the insulating by-products and “dead Zn” are still formidable challenges for their practical application. Herein, an SnS-based layer coated on the Zn anode is reported to tackle these problems. The semiconducting SnS with a higher work function can drive the electrons from the Zn anode, which constructs a polarized interface between the SnS layer and Zn. The semiconducting importance of the coating layer is verified through theoretical simulations, which can migrate the polarization layer from the electrode surface to a well-protected spot beneath the coating layer. This polarization interface is effective in homogenizing the Zn<sup>2+</sup> flux and repelling the anions from electrochemical corrosion. Compared with the bare Zn, the SnS-coated Zn anode exhibits a notable 14.7-fold enhancement in plating/stripping lifetime (over 3000 ​h), high reversibility (with CE of 99.74%), and superior stability in full cells when paired with vanadium- and manganese-based cathodes.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"2 2","pages":"Article 100093"},"PeriodicalIF":0.0,"publicationDate":"2023-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49715964","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 15
Laser powder bed fusion of a novel high strength quasicrystalline Al–Fe–Cr reinforced Al matrix composite 激光粉末床熔接一种新型高强度准晶Al - fe - cr增强Al基复合材料
Advanced Powder Materials Pub Date : 2023-04-01 DOI: 10.1016/j.apmate.2022.100108
Nan Kang , Yuan Zhang , Mohamed El Mansori , Xin Lin
{"title":"Laser powder bed fusion of a novel high strength quasicrystalline Al–Fe–Cr reinforced Al matrix composite","authors":"Nan Kang ,&nbsp;Yuan Zhang ,&nbsp;Mohamed El Mansori ,&nbsp;Xin Lin","doi":"10.1016/j.apmate.2022.100108","DOIUrl":"https://doi.org/10.1016/j.apmate.2022.100108","url":null,"abstract":"<div><p>Quasicrystal (QC)-reinforced metal matrix composites fabricated by rapid solidification present promising new opportunities to develop high-strength alloys with multiple functions. In this research, specially designed Al–Fe–Cr samples possessing an Al–Fe–Cr quasicrystal-reinforced Al matrix structure were manufactured using a laser powder bed fusion (LPBF) process. Based on the optimized process parameters of laser scanning speed and hatch distance, an almost dense (99.8%) free-crack sample was obtained with the multiscaled heterogenous structure induced by the nonuniform rapid solidification in a single molten pool. The results show that nanosized Al–Fe–Cr quasicrystalline particles of different sizes are heterogeneously distributed in the α-Al columnar grain structure. In detail, the coarse flower-like and spherical QC particles can be observed at the molten pool boundary, and the fine spherical Al–Fe–Cr QC is located inside the laser fusion zone. The orientation relationship between the Al matrix and the icosahedral Al–Fe–Cr QC is as follows: Al [ ​− ​112 ] ∥ i5 with a semicoherency feature. The novel designed LPBF-processed Al–Fe–Cr alloy exhibits high mechanical strength due to the ultrafine multireinforced microstructure-induced Orowan strengthening effect. For instance, the ultimate tensile strength, yield strength and elongation of the sample processed with LPBF are 530.80 ​± ​3.19 ​MPa, 395.06 ​± ​6.44 ​MPa, and 4.16% ​± ​0.38%, respectively. The fractographic analysis shows that the fracture mechanism presents a combination of ductile‒brittle fracture.</p></div>","PeriodicalId":7283,"journal":{"name":"Advanced Powder Materials","volume":"2 2","pages":"Article 100108"},"PeriodicalIF":0.0,"publicationDate":"2023-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49716273","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
0
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
相关产品
×
本文献相关产品
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信