Accounts of materials research最新文献

{"title":"","authors":"Hengrui Zhang, Alexandru B. Georgescu, Suraj Yerramilli, Christopher Karpovich, Daniel W. Apley, Elsa A. Olivetti, James M. Rondinelli* and Wei Chen*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"6 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":14.0,"publicationDate":"2025-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/accountsmr.5c00011","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144489193","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"","authors":"Yoonhee Kim, Yuna Kwak, Jihyeon Choi and Jwa-Min Nam*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"6 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":14.0,"publicationDate":"2025-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/accountsmr.5c00043","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144489189","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"","authors":"Zhixue Liu, Junyi Chen and Chunju Li*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"6 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":14.0,"publicationDate":"2025-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/accountsmr.5c00071","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144489187","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Multifunctional Spin-Dependent Tunneling: From Tunnel Magnetodielectric to Magneto-Optic and Faraday Effects","authors":"Yang Cao, Nobukiyo Kobayashi, Hanae Kijima-Aoki, Jun Zhang, Hiroshi Masumoto","doi":"10.1021/accountsmr.5c00113","DOIUrl":"https://doi.org/10.1021/accountsmr.5c00113","url":null,"abstract":"Magnetic granular nanocomposites, consisting of magnetic nanogranules dispersed within a host matrix, represent a versatile class of functional materials that enable control over electrical, magnetic, and thermal properties at the nanoscale. Over the past decade, by leveraging electrons as carriers of spin, charge, and heat, these features have enabled the discovery of a family of tunnel related phenomena: tunnel magnetoresistance (TMR), tunnel magneto-Seebeck (TMS), tunnel magnetodielectric (TMD), and most recently tunnel magneto-optical (TMO) effects. Their structural features allow for tuning of granular size, distribution, and intergranular spacing, positioning these materials as promising candidates for miniaturized magnetic field sensors, antennas, microwave devices, and spintronic components.","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"183 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144237478","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Promise and Perspectives of Garnet-Based Anode-Free Solid-State Batteries","authors":"Jiayun Wen, Yiming Dai, Qian Yu, Zhiyuan Ouyang, Wei Luo, Yunhui Huang","doi":"10.1021/accountsmr.4c00129","DOIUrl":"https://doi.org/10.1021/accountsmr.4c00129","url":null,"abstract":"With the rapid advancement of energy storage technologies, lithium-ion batteries (LIBs) based on graphite anodes and liquid organic electrolytes have achieved remarkable progress. Nevertheless, the limited specific capacity of graphite anodes and the safety concerns associated with organic electrolytes hinder further enhancement of LIBs. In pursuit of higher energy density and improved safety, solid-state Li metal batteries (SSLMBs) have drawn significant attention. Furthermore, anode-free solid-state batteries (AFSSBs), as a particularly promising innovation in the field of energy storage, have gained increasing interest in recent years. With increasing research investment and continuous technological optimization, AFSSBs hold great potential for widespread applications including electric vehicles, grid energy storage, and beyond.","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"08 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144237479","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Wet Spinning Enabled Advanced PEDOT:PSS Composite Fibers for Smart Devices","authors":"Haodi Zeng, Chunxia Gao, Yuanyuan Yu, Mengjin Jiang, Tingyin Deng, Jiadeng Zhu","doi":"10.1021/accountsmr.5c00076","DOIUrl":"https://doi.org/10.1021/accountsmr.5c00076","url":null,"abstract":"Poly(3,4-ethylenedioxythiophene): poly(styrenesulfonate) (PEDOT:PSS) is a derivative of polythiophene and an intrinsically conductive polymer (CP). Due to its excellent conductivity, processability, and biocompatibility, it has received widespread attention in the past decade and has become a popular material for wearable electronic devices. Thin films and fibers are the two primary dimensions that PEDOT:PSS has been made into. Compared with two-dimensional (2D) thin films, 1D fibers have natural advantages in integration and structural design, remarkably accelerating practical applications.","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"519 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144237481","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Biomimetic Bone Tissue Engineering Scaffolds Combined with Physical Stimulation to Reconstruct Piezoelectric Network for Functional Regeneration in Critical Bone Defects","authors":"Qihong Li, Chen Li, Xiaomei Bie, Jianzheng Zhang, Yantao Zhao","doi":"10.1021/accountsmr.5c00029","DOIUrl":"https://doi.org/10.1021/accountsmr.5c00029","url":null,"abstract":"In addition to supporting and protecting mobility, bone is essential for regulating systemic homeostasis. Large bone defects have always been a clinical challenge because of their complicated composition and structure, which makes them difficult to repair on their own. Currently, clinical operations employ primarily autologous, allogeneic, and synthetic bone grafting methods, which are still limited by factors such as donor scarcity, complications from infections, and market acceptance. Thus, novel biomimetic artificial bone tissue engineering scaffolds can be created by designing and regulating the composition and structure of materials, drawing inspiration from the intrinsic properties of genuine bone tissue. The combined application of bioactive substances and biomaterials in bone repair has achieved multiple satisfactory clinical outcomes. In this Account, based on the principles of bionic tissue engineering, we constructed various bone repair scaffolds through multidimensional approaches and systematically evaluated their capabilities in vascular regeneration, nerve ingrowth, and osteogenesis. The technological development of scaffolds demonstrated a distinct progressive relationship: The initial stage focused on the bionics of natural bone tissue’s matrix and structure; the advanced stage integrated bioactive components like BMP2 to achieve functional osteoinduction; the deepening stage introduced piezoelectric signals to directly regulate the osteogenic function of scaffolds, while simultaneously controlling angiogenesis and nerve ingrowth to indirectly promote bone repair and regeneration. Ultimately, an innovative bone repair paradigm based on “Piezoelectric Network Theory” was proposed. Extracellular matrix (ECM) engineered scaffolds were reconstructed to provide endogenous effects through surface morphology modulation and bioactive component modification. The synergistic responses between endogenous effect and exogenous physical stimulation achieve rapid repair of a variety of large segmental bone defects in various areas. This advancement will establish new theoretical foundations for functional bone reconstruction and significantly enhance the treatment efficacy for large segmental bone defects.","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"1 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144210993","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"3D Graphene for Energy Technologies: Chemical Strategies and Industrial Challenges","authors":"Bibhuti Kumar Jha, Jong-Chul Yoon, Ji-Hyun Jang","doi":"10.1021/accountsmr.4c00381","DOIUrl":"https://doi.org/10.1021/accountsmr.4c00381","url":null,"abstract":"Graphene, a groundbreaking two-dimensional (2D) material, has attracted significant attention across various fields due to its exceptional properties. However, 2D graphene sheets tend to restack or agglomerate, reducing their performance and active surface area. To overcome these limitations and expand graphene’s potential applications, researchers have developed three-dimensional (3D) graphene structures with diverse architectures, including 3D graphene fibers, foams, aerogels, hydrogels, tubes, and cages. These structures, along with modifications such as functionalization, doping, preintercalation, and compositing, prevent stacking and enhance specific properties for targeted applications.","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"157 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144193003","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"4D Synchrotron X-ray Nanoimaging for Early Age Cement Curing: Where Are We and Where Should We Go?","authors":"Miguel A.G. Aranda","doi":"10.1021/accountsmr.5c00018","DOIUrl":"https://doi.org/10.1021/accountsmr.5c00018","url":null,"abstract":"The production of cement is a key indicator of a region’s level of development. As such, its use is essential for any society aiming to create healthy, comfortable, safe and secure living and working environments. However, these benefits come at a price; Portland cement production accounts for ≈8% of the total anthropogenic CO₂ emissions. If cement fabrication was considered a country, it would rank as the third largest emitter, after China and the United States. Consequently, reducing the CO₂ footprint of the construction industry is a societal need. Numerous low-carbon cement alternatives have been proposed, primarily involving the partial substitution of Portland clinker with materials that possess much lower CO₂ footprints. However, these cements have not been widely adopted because they exhibit reduced mechanical strength at 1 day of hydration, failing to meet current practices for formwork stripping. Therefore, a primary objective is to elucidate the mechanisms of early age cement hydration to accelerate their hydration rates.","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"9 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-05-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144177270","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Toward Ideal Biointerfacing Electronics Using Organic Electrochemical Transistors","authors":"Peiyun Li, Ting Lei","doi":"10.1021/accountsmr.5c00030","DOIUrl":"https://doi.org/10.1021/accountsmr.5c00030","url":null,"abstract":"The biointerface between biological tissues and electronic devices serves as a medium for matter transport, signal transmission, and energy conversion. However, significant disparities in properties, such as mechanical modulus and water content, between tissues and electronics, present a key challenge in bioelectronics, leading to biointerface mismatches that severely impact their performance and long-term stability. Organic electrochemical transistors (OECTs), fabricated with soft, hydrophilic organic semiconductors, offer unique advantages, including low operating voltage, high transconductance, and compatibility with aqueous environments. These attributes position OECTs as promising candidates for ideal biointerfaces. As neural probes, OECTs have demonstrated superior biocompatibility and signal detection capabilities compared to conventional metal electrodes and inorganic semiconductors. Despite these advantages, the applications of OECT as biointerfaces remain constrained by several limitations, including limited performance, poor stability, mismatches among p-type, n-type, and ambipolar semiconductors, relatively high Young’s modulus, and unsatisfactory biointerfacial properties.","PeriodicalId":72040,"journal":{"name":"Accounts of materials research","volume":"6 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-05-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144165743","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}