ACS Applied Materials & Interfaces最新文献_第6页

Tailoring Functionalized Dipole Molecules for Enhanced Efficiency and Stability of Perovskite Solar Cells. 定制功能化偶极子分子以提高钙钛矿太阳能电池的效率和稳定性。

IF 8.3 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23 Epub Date: 2025-07-14 DOI: 10.1021/acsami.5c09592

Wenxuan Lv, Kangwei Que, Zikang Chen, Ao Shen, Mengling Gong, Chengxi Sun, Mangmang Gao, Wenchao Huang, Runfeng Chen, Ligang Xu

{"title":"Tailoring Functionalized Dipole Molecules for Enhanced Efficiency and Stability of Perovskite Solar Cells.","authors":"Wenxuan Lv, Kangwei Que, Zikang Chen, Ao Shen, Mengling Gong, Chengxi Sun, Mangmang Gao, Wenchao Huang, Runfeng Chen, Ligang Xu","doi":"10.1021/acsami.5c09592","DOIUrl":"10.1021/acsami.5c09592","url":null,"abstract":"Dipole interlayer molecules have been incorporated into perovskite solar cells (PSCs) to enhance the energy level alignment between the perovskite and charge transport layers, improving charge extraction and device performance. However, the conventional dipole interlayer with a singular functionality is inadequate for high-efficiency PSCs with excellent long-term stability. Here, we design a functionalized dipole interlayer (FDI) between perovskite and electron transport layers that integrates multiple functionalities onto a novel dipole molecule. The FDI not only realizes the field-effect function of the conventional dipole interlayer for tuning energy level matching but also extends the function of the dipole interlayer for diminishing defects, fortifying the perovskite's resistance to moisture, and impeding the migration of I- ions within the perovskite layer across perovskite interface. Consequently, FDI proves to be beneficial to air-processed PSCs under a high relative humidity of 45%, yielding enhanced power conversion efficiencies from 19.44 to 21.13%. Furthermore, unencapsulated devices exhibit excellent humidity stability and thermal stability under the standardized International Summit on Organic Photovoltaic Stability (ISOS) protocols for over 1000 h (ISOS-D-1) and 700 h (ISOS-D-2I), respectively. This work extends new functions for dipole interlayers and offers a convenient and effective approach for enhancing the performance of PSCs prepared in air environments.","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":" ","pages":"42011-42019"},"PeriodicalIF":8.3,"publicationDate":"2025-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144635705","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Advances in Interface Engineering of MoS2-Based Heterostructures as Bifunctional Electrodes for Efficient Water Splitting. 基于二硫化钼异质结构的高效水分解双功能电极界面工程研究进展。

IF 9.5 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23 DOI: 10.1021/acsami.5c08374

Malatesh S Pujar,Anita Padasalagi

引用次数: 0

Sandwich Nanoparticles Mediated by Ytterbium Sublattice for Advanced Photonic Applications. 镱亚晶格介导的夹层纳米粒子在先进光子应用中的研究。

IF 9.5 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23 DOI: 10.1021/acsami.5c11653

Longchi Li,Chunwen Yuan,Yujie Chen,Zewen Su,Kai Yang,Gongxun Bai,Liang Chen

引用次数: 0

A Machine Learning-Enabled SERS Sensor: Multiplex Detection of Lipopolysaccharides from Foodborne Pathogenic Bacteria. 基于机器学习的SERS传感器：多重检测食源性致病菌中的脂多糖。

IF 9.5 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23 DOI: 10.1021/acsami.5c08361

Mahmoud Matar Abed,Cassandra L Wouters,Clarice E Froehlich,Timmy B Nguyen,Rhea Caldwell,Katie L Riley,Punarbasu Roy,Theresa M Reineke,Christy L Haynes

{"title":"A Machine Learning-Enabled SERS Sensor: Multiplex Detection of Lipopolysaccharides from Foodborne Pathogenic Bacteria.","authors":"Mahmoud Matar Abed,Cassandra L Wouters,Clarice E Froehlich,Timmy B Nguyen,Rhea Caldwell,Katie L Riley,Punarbasu Roy,Theresa M Reineke,Christy L Haynes","doi":"10.1021/acsami.5c08361","DOIUrl":"https://doi.org/10.1021/acsami.5c08361","url":null,"abstract":"Foodborne pathogenic bacteria pose a global threat to public health, causing dangerous and expensive outbreaks. While therapeutics are being developed to target antibiotic-resistant and foodborne pathogenic bacteria, approaches to minimize their spread are also crucial. As estimated by the World Health Organization, each year around 600 million cases of foodborne illnesses are reported, with over 420,000 deaths annually. Lipopolysaccharides (LPS) are glycolipids found on the outer membrane of Gram-negative bacteria, serving as biomarkers for pathogenic strains. With a clear need for a sensing platform to quickly and cost-effectively detect and identify microbial pathogens, this work focuses on surface-enhanced Raman scattering (SERS)-based bacterial sensors for the detection of LPS from various pathogenic bacteria. Specifically, linear polymer affinity agents with a broad affinity for LPS immobilized on metal film over nanosphere plasmonic substrates and the integration of machine learning analysis are used to characterize and discriminate between the Raman \"fingerprints\" of LPS from Salmonella typhimurium, Escherichia coli O111:B4, and Escherichia coli O26:B6. Our findings demonstrate the feasibility of a linear polymer-based SERS sensing platform coupled to machine learning analysis with principal component analysis and support vector machines for the sensitive detection and differentiation of LPS from different bacterial species, even in a complex food matrix like apple juice, highlighting its potential for real-world applications in food safety monitoring.","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"696 1","pages":""},"PeriodicalIF":9.5,"publicationDate":"2025-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144693543","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Infrared Detection Achieved by Controlling Thermionic Emission in Organic Transistors. 控制有机晶体管热离子发射实现红外探测。

IF 9.5 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23 DOI: 10.1021/acsami.5c08922

Yanpeng Wang,Shixuan Zhao,Bokun Rong,Yao Fu,Shougang Sun,Jiannan Qi,Yongxu Hu,Yinan Huang,Zhongwu Wang,Shuguang Wang,Xiaosong Chen,Rongmei Si,Liqiang Li,Wenping Hu

{"title":"Infrared Detection Achieved by Controlling Thermionic Emission in Organic Transistors.","authors":"Yanpeng Wang,Shixuan Zhao,Bokun Rong,Yao Fu,Shougang Sun,Jiannan Qi,Yongxu Hu,Yinan Huang,Zhongwu Wang,Shuguang Wang,Xiaosong Chen,Rongmei Si,Liqiang Li,Wenping Hu","doi":"10.1021/acsami.5c08922","DOIUrl":"https://doi.org/10.1021/acsami.5c08922","url":null,"abstract":"Commercial inorganic infrared (IR) photodetectors have important applications in night vision, medical imaging, remote sensing, and other fields, but still face the challenges of operating at low temperatures and high costs. Organic semiconductor (OSC)-based IR detectors can operate at room temperature and have the advantages of flexibility and large-area processing. Consequently, they have important application prospects. However, high-performance OSCs usually have wide bandgaps, which makes it difficult for them to directly absorb IR light for detection. Overcoming the bandgap limitations of OSCs to achieve IR detection is extremely challenging. Herein, the organic field-effect transistors (OFETs) are prepared using poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) electrodes that exhibit photothermal effects under infrared irradiation and can form Schottky contacts with numerous OSCs. The electrodes can effectively absorb IR light and release heat, which increases the temperature of the electrode-OSC contact region and promotes thermionic emission, resulting in a change in the electrical properties of the device to achieve an IR response. Using this strategy, the prepared OFET exhibits a high photosensitivity of 1.42 × 105 and a detectivity of 2.12 × 108 Jones at 808 nm and also exhibits a distinguishable IR response at different light intensities. Moreover, the invisible IR light signal is converted into a visible green light signal via a circuit design. This study provides a universally applicable solution to achieve IR detection using OFETs, which furthers their application potential.","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"53 1","pages":""},"PeriodicalIF":9.5,"publicationDate":"2025-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144693564","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Correction to "Antifouling Dendrimer-Entrapped Copper Sulfide Nanoparticles Enable Photoacoustic Imaging-Guided Targeted Combination Therapy of Tumors and Tumor Metastasis". 更正“防污树枝状包裹的硫化铜纳米颗粒使光声成像引导肿瘤和肿瘤转移的靶向联合治疗”。

IF 8.3 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23 DOI: 10.1021/acsami.5c14132

Zhijun Ouyang, Du Li, Zhijuan Xiong, Cong Song, Yue Gao, Renna Liu, Mingwu Shen, Xiangyang Shi

引用次数: 0

IF 8.3 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23

Rui Zhang, Mingyu Zhu, Yang Liu, Liqiu Hu, Pinghang Chen, Junqin Wang, Bin Tang, Chao Liu and Fuzeng Ren*,

引用次数: 0

IF 8.3 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23

Peipei Xi, Xiangyu Wei, Yuting Huang, Yunan Wang, Nengjie Yang, Yongxin Xu, Hao Zhang, Yujuan Zhu* and Zhifeng Gu*,

引用次数: 0

IF 8.3 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23

Siriporn Kosawatthanakun, Poobodin Mano, Pawan Boonyoung, Nadhita Chanchaona, Kittipong Chainok, Suwadee Jiajaroen, Supaporn Nualyai, Kajornsak Faungnawakij, Supawadee Namuangruk* and Bunyarat Rungtaweevoranit*,

引用次数: 0

IF 8.3 2区材料科学

ACS Applied Materials & Interfaces Pub Date : 2025-07-23

Athina Papadopoulou*, Maria Isabel Pintor-Monroy*, Sreeshma Dayaran, Irina Skvortsova, João Pedro de Sousa Gouveia dos Anjos, Sownder Subramaniam, Wenya Song, Itai Lieberman, Yinghuan Kuang, Johan Hofkens, Maarten B. J. Roeffaers, Sara Bals, Robert Gehlhaar and Jan Genoe,

引用次数: 0