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Features of Polyimide Films with Molecular Imprints of Erythrosine and Indigocarmine 具有赤藓红和靛红分子印迹的聚酰亚胺薄膜的特征
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-05-07 DOI: 10.1134/S1061933X24600088
S. A. Khalzova, A. N. Zyablov, A. Yu. Vybornyi
{"title":"Features of Polyimide Films with Molecular Imprints of Erythrosine and Indigocarmine","authors":"S. A. Khalzova,&nbsp;A. N. Zyablov,&nbsp;A. Yu. Vybornyi","doi":"10.1134/S1061933X24600088","DOIUrl":"10.1134/S1061933X24600088","url":null,"abstract":"<p>Polyimide films with molecular imprints of erythrosine and indigocarmine have been obtained. The structure and morphology of the film surfaces have been studied by scanning probe microscopy and IR spectroscopy. It has been found that the surface roughness of molecularly imprinted polymers (MIPs) increases, while the relief height amounts to 3–4 nm. The removal of template molecules leads to a redistribution of pores over sizes in the polymers with molecular imprints. The adsorption of dyes by MIP films has been carried out under static conditions. The degrees of extraction and the imprinting factors have been calculated for polymers with molecular imprints of the dyes. The high values of these parameters indicate the selectivity of MIPs to the target template molecules.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 2","pages":"297 - 305"},"PeriodicalIF":1.4,"publicationDate":"2024-05-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140885450","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermal Ice Melting Performance of Femtosecond Laser Metal Micro-Nano-Structured Surface 飞秒激光金属微纳结构表面的热融冰性能
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-04-10 DOI: 10.1134/S1061933X23601166
Ziyuan Liu, Qing Ma, Tingsong Zhang, Yujia Dai
{"title":"Thermal Ice Melting Performance of Femtosecond Laser Metal Micro-Nano-Structured Surface","authors":"Ziyuan Liu,&nbsp;Qing Ma,&nbsp;Tingsong Zhang,&nbsp;Yujia Dai","doi":"10.1134/S1061933X23601166","DOIUrl":"10.1134/S1061933X23601166","url":null,"abstract":"<p>Improving thermal ice melting efficiency is very important in the practical application of anti-icing surfaces. This work investigated the thermal ice melting performance of micro-nano-structured surfaces fabricated by femtosecond laser. To the best of our knowledge, we found that the micro-nano-structured surfaces significantly improve the ice melting time for the first time. The shortest melting time was on the porous micro-nano-structured surface, about one third of the original surface. Moreover, it was proven that the accelerated ice melting surface had good durability. The research in this paper showed that the micro-nano-structured surfaces are very suitable for the surface that needs to be heated to melt ice, providing essential guidance for the design of the anti-icing surface.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 2","pages":"315 - 322"},"PeriodicalIF":1.4,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140600949","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Development of a New Biocompatible Colloid System to Improve the Solubility of Celecoxib 开发新型生物相容性胶体系统以提高塞来昔布的溶解度
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-04-10 DOI: 10.1134/S1061933X23601270
Alireza Salabat,  Nesa Ghorbani
{"title":"Development of a New Biocompatible Colloid System to Improve the Solubility of Celecoxib","authors":"Alireza Salabat,&nbsp; Nesa Ghorbani","doi":"10.1134/S1061933X23601270","DOIUrl":"10.1134/S1061933X23601270","url":null,"abstract":"<p>In this research work, a new biocompatible microemulsion containing castor oil has been formulated to increase the solubility of celecoxib, as a well-known anti-inflammatory drug. In this formulation castor oil has also anti-inflammatory properties. The proposed oil-in-water microemulsion composed of Tween 80 as surfactant, isobutanol as co-surfactant, and castor oil as the oil phase. In the first step, the phase diagrams of the proposed colloid systems with surfactant to co-surfactant mass ratios of 4 : 1 and 2 : 1 were prepared at ambient temperature. Then, using the obtained phase diagrams, the appropriate formulations were selected by combining different percentages of water, oil, surfactant and co-surfactant in the microemulsion region. Some of physico-chemical properties, such as electrical conductivity, density, refractive index, surface tension and particle size of the selected microemulsion formulations have been determined at 298 K. After that, the solubility of celecoxib in the selected formulations was determined and compared with other reported microemulsion formulations. Interesting results from this section indicated that the solubility of celecoxib significantly increased compared to pure water and the previous proposed formulations. The results of this study can be used to provide suitable formulations based on the biocompatible microemulsions for celecoxib in pharmaceutical industry.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 2","pages":"323 - 329"},"PeriodicalIF":1.4,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140600950","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Symmetric and Asymmetric Supercapacitor Fabrication Based on Green Synthesized NiO Nanoparticles and Graphene 基于绿色合成氧化镍纳米粒子和石墨烯的对称和不对称超级电容器制造
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-04-10 DOI: 10.1134/S1061933X23600914
A. Zemieche, L. Chetibi, D. Hamana, S. Achour, V. D. Noto
{"title":"Symmetric and Asymmetric Supercapacitor Fabrication Based on Green Synthesized NiO Nanoparticles and Graphene","authors":"A. Zemieche,&nbsp;L. Chetibi,&nbsp;D. Hamana,&nbsp;S. Achour,&nbsp;V. D. Noto","doi":"10.1134/S1061933X23600914","DOIUrl":"10.1134/S1061933X23600914","url":null,"abstract":"<p>Nickel oxide nanoparticles (NiO NPs) are synthesized using olive leaf extract (OLE), which contains a range of polyphenols. These polyphenols serve as both reducing and capping agents, stabilizing the nanoparticles. Aqueous nickel acetate is employed as a precursor. Simultaneously, exfoliated graphene (EG) is obtained via electrochemical exfoliation of graphite in aqueous solutions. These materials were employed as electroactive components in supercapacitor applications. Characterization of NiO and EG involved thermogravimetric analysis (TGA), X-ray diffraction (XRD), Raman spectroscopy (RS), X-ray photoelectron spectroscopy (XPS), and scanning/transmission electron microscopy (SEM/TEM), alongside Brunauer−Emmett−Teller (BET) analysis, confirming the formation of crystalline NiO NPs with a cubic phase and <i>Fm</i>-3<i>m</i> space group. Micrographs revealed nanoscale dimensions for both NiO and EG with a substantial surface area, as verified by BET analysis. Symmetric (NiO/NiO, EG/EG) and asymmetric (NiO/EG) supercapacitors were fabricated using the doctor blade method. Electrode evaluation, employing field-emission scanning electron microscopy FESEM, cyclic voltammetry (CV), and electrochemical impedance spectroscopy (EIS), demonstrated promising morphological and electrochemical characteristics. At low scan rates, both symmetric and asymmetric supercapacitors exhibited a notable gravimetric capacitance (221, 111, and 162 F g<sup>–1</sup> at 1 mV s<sup>–1</sup>). Additionally, they revealed higher power density (173, 137, and 161 W kg<sup>–1</sup> at 10 mV s<sup>–1</sup>), showcasing pseudocapacitive and electric double-layer capacitor (EDLC) behavior for NiO NPs and EG, respectively. This research significantly contributes valuable insights by presenting a sustainable synthesis route for NiO NPs, developing high-performance supercapacitor electrodes, and achieving a comprehensive understanding of the electrochemical behavior of NiO NPs and EG.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 2","pages":"330 - 345"},"PeriodicalIF":1.4,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140600988","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Kinetic Regularities of the Synthesis of Silica Nanoparticles by Heterogeneous Hydrolysis of Tetraethoxysilane Using L-Arginine as a Catalyst 以 L-精氨酸为催化剂异构水解四乙氧基硅烷合成二氧化硅纳米粒子的动力学规律性
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-04-10 DOI: 10.1134/S1061933X23601257
V. M. Masalov, N. S. Sukhinina, D. N. Sovyk, V. G. Ralchenko, G. A. Emel’chenko
{"title":"Kinetic Regularities of the Synthesis of Silica Nanoparticles by Heterogeneous Hydrolysis of Tetraethoxysilane Using L-Arginine as a Catalyst","authors":"V. M. Masalov,&nbsp;N. S. Sukhinina,&nbsp;D. N. Sovyk,&nbsp;V. G. Ralchenko,&nbsp;G. A. Emel’chenko","doi":"10.1134/S1061933X23601257","DOIUrl":"10.1134/S1061933X23601257","url":null,"abstract":"<p>The kinetics of the synthesis of silica nanoparticles (&lt;50 nm) has been studied under the conditions of heterogeneous hydrolysis of tetraethoxysilane (TEOS) using <i>L</i>-arginine as an alkaline catalyst. The rates of silica formation have been determined in a temperature range of 10–95°C at catalyst concentrations of 6–150 mM. It has been shown that the activation energy of the process depends on catalyst concentration and varies in a range of 21.5–13.9 kJ/mol, while decreasing linearly with increasing concentration of <i>L</i>-arginine in the system. The criterion of maintaining the monodispersity has been estimated for SiO<sub>2</sub> particles being grown “onto seeds.” The density of submicron-sized silica particles has been experimentally determined as depending on the annealing temperature. Within a temperature range of 200–1000°C, the particle density varies from 2.04 to 2.20 g/cm<sup>3</sup>.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 2","pages":"248 - 257"},"PeriodicalIF":1.4,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S1061933X23601257.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140600982","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Influence of Homogeneous Nucleation on the Intensity of Evaporation/Condensation Processes 均匀成核对蒸发/凝结过程强度的影响
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-04-10 DOI: 10.1134/S1061933X23601361
V. Yu. Levashov, A. P. Kryukov, I. N. Shishkova
{"title":"Influence of Homogeneous Nucleation on the Intensity of Evaporation/Condensation Processes","authors":"V. Yu. Levashov,&nbsp;A. P. Kryukov,&nbsp;I. N. Shishkova","doi":"10.1134/S1061933X23601361","DOIUrl":"10.1134/S1061933X23601361","url":null,"abstract":"<p>An approach based on the direct numerical solution of the Boltzmann kinetic equation is proposed to take into account the influence of homogeneous nucleation on the mass transfer intensity in the evaporation/condensation (recondensation) problem. On the basis of the comparison between the scales of the formation time of a critical-size droplet and the time of supersaturation propagation, it is shown that it is possible to describe the considered problem in two stages, i.e., without taking into account the influence of droplets at the first stage and with taking into account their influence at the second stage. The calculation results show that, in the case of immobile droplets, there is a strong influence of bulk condensation on the intensity of the evaporation/condensation process.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 2","pages":"232 - 240"},"PeriodicalIF":1.4,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140600948","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Synthesis and Study of Superhigh-Concentrated Organosols of Silver Nanoparticles 超高浓缩银纳米颗粒有机溶剂的合成与研究
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-04-10 DOI: 10.1134/S1061933X23601294
S. A. Vorobyev, M. Yu. Flerko, S. A. Novikova, E. V. Mazurova, Ye. V. Tomashevich, M. N. Likhatski, S. V. Saikova, A. S. Samoilo, N. A. Zolotovsky, M. N. Volochaev
{"title":"Synthesis and Study of Superhigh-Concentrated Organosols of Silver Nanoparticles","authors":"S. A. Vorobyev,&nbsp;M. Yu. Flerko,&nbsp;S. A. Novikova,&nbsp;E. V. Mazurova,&nbsp;Ye. V. Tomashevich,&nbsp;M. N. Likhatski,&nbsp;S. V. Saikova,&nbsp;A. S. Samoilo,&nbsp;N. A. Zolotovsky,&nbsp;M. N. Volochaev","doi":"10.1134/S1061933X23601294","DOIUrl":"10.1134/S1061933X23601294","url":null,"abstract":"<p>Due to their unique properties, organosols of silver nanoparticles are widely used in optical and semiconductor devices, to produce electrically and thermally conductive films, as catalysts, antibacterial materials, etc. This work proposes a simple and highly productive method for the preparation of silver organosols, which have a metal concentration as high as 1800 g/L and contain spherical nanoparticles with low polydispersity and a median size of 9.1 nm. The method consists in the initial preparation of silver nanoparticle hydrosols with a concentration of higher than 30 g/L followed by the transfer of the NPs into an organic phase of <i>o</i>-xylene. A set of physical research methods has been employed to study the regularities of the extraction of silver nanoparticles with <i>o</i>-xylene in the presence of cetyltrimethylammonium bromide (CTAB) and ethanol and to determine the optimal process conditions, under which the extraction degree is as high as 62.5%. It has been found that bromine anions contained in CTAB molecules cause the aggregation of some amount of silver nanoparticles with the formation of silver metal sediment in the aqueous phase. According to X-ray photoelectron spectroscopy data, the sediment contains bromide ions (up to 4 at %) on the particle surface. Organosols synthesized under optimal conditions are stable for more than 7 months and withstand repeated cycles of drying and redispersing. Silver organosols have been used to obtain metal films with an electrical conductivity of about 68 500 S/cm, which increases to 412 000 and 509 500 S/cm (87.8% of the electrical conductivity of bulk silver) after thermal treatment at 150 and 250°C, respectively.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 2","pages":"208 - 217"},"PeriodicalIF":1.4,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S1061933X23601294.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140600983","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Mechanochemical Synthesis of Nanocomposites with Specified Composition in the Presence of a Solvent for Precursors 在前驱体溶剂存在的情况下以机械化学方法合成具有特定成分的纳米复合材料
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-04-10 DOI: 10.1134/S1061933X23601245
F. Kh. Urakaev
{"title":"Mechanochemical Synthesis of Nanocomposites with Specified Composition in the Presence of a Solvent for Precursors","authors":"F. Kh. Urakaev","doi":"10.1134/S1061933X23601245","DOIUrl":"10.1134/S1061933X23601245","url":null,"abstract":"<p>The objective of this work is an attempt to introduce into scientific practice the method of “mechanochemical recrystallization” in solid-phase systems with small additives of a liquid solvent. Dimethyl sulfoxide (DMSO), a universal bipolar aprotic solvent, has been used as the additive. As an example, the mechanical activation of reaction AgNO<sub>3</sub> + NH<sub>4</sub>I + <i>z</i> NH<sub>4</sub>NO<sub>3</sub> (diluent) + <i>y</i>S + <i>x</i>DMSO = AgI + <i>y</i>S* + (<i>z</i>+1)NH<sub>4</sub>NO<sub>3</sub> + <i>x</i>DMSO has been studied, where <i>z</i> ≈ 5, <i>y</i> ≈ 1, and <i>x</i> <span>( ll )</span> 1 are molar fractions. The formation of sulfur (S<b>*</b>) and silver iodide (AgI) nanoparticles has been revealed, and/or S*/AgI nanocomposites with controlled contents of the components have been synthesized. The use of NH<sub>4</sub>NO<sub>3</sub>, which is a non-target product of the mechanosynthesis, as a diluent leads to the stabilization of nanoparticle sizes. The nanoparticles are formed in the medium of DMSO due to the conventional recrystallization (continuous process of dissolution–crystallization of sulfur) or the reactional recrystallization (process of dissolution of AgNO<sub>3</sub> and NH<sub>4</sub>I followed by their interaction with the AgI crystallization) rather than the direct mechanical activation. The former and latter mechanisms are realized when obtaining S* and AgI, respectively. The target products (S*, AgI, and S*/AgI) are purified from water-soluble components (NH<sub>4</sub>NO<sub>3</sub>, DMSO) by washing in an ultrasonic bath. The proposed technical solution of the problem has been realized in planetary ball mills with different milling tools.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 2","pages":"278 - 286"},"PeriodicalIF":1.4,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140601325","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Investigation of the Mechanical and Chemical Stability of Superhydrophobic Coatings Based on Reactive Copolymers of Glycidyl Methacrylate and Fluoroalkyl Methacrylates 基于甲基丙烯酸缩水甘油酯和甲基丙烯酸氟烷基酯反应共聚物的超疏水涂层的机械和化学稳定性研究
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-03-18 DOI: 10.1134/S1061933X23601208
V. V. Klimov, O. V. Kolyaganova, E. V. Bryuzgin, A. V. Navrotskiy, I. A. Novakov
{"title":"Investigation of the Mechanical and Chemical Stability of Superhydrophobic Coatings Based on Reactive Copolymers of Glycidyl Methacrylate and Fluoroalkyl Methacrylates","authors":"V. V. Klimov,&nbsp;O. V. Kolyaganova,&nbsp;E. V. Bryuzgin,&nbsp;A. V. Navrotskiy,&nbsp;I. A. Novakov","doi":"10.1134/S1061933X23601208","DOIUrl":"10.1134/S1061933X23601208","url":null,"abstract":"<p>This work is devoted to studying the stability of polymer coatings formed from reactive copolymers of glycidyl methacrylate and fluoroalkyl methacrylates and applied onto textured aluminum and cotton textile surfaces. The stability is determined with respect to the action of aggressive media and mechanical stress. The resulting coatings provide the achievement of long-term stable heterogeneous wetting with initial contact angles as large as 170°, thus preventing the penetration of corrosive agents into the hierarchical structure. The study has shown the influence of the composition of the reactive copolymers containing 3–7 fluorine atoms in a monomer unit on the stability of the polymer coatings with respect to the prolonged exposure to media with different acidities, as well as to cavitation, and abrasive wear.</p>","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 1","pages":"52 - 63"},"PeriodicalIF":1.4,"publicationDate":"2024-03-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140169644","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Editorial Column 社论专栏
IF 1.4 4区 化学
Colloid Journal Pub Date : 2024-03-18 DOI: 10.1134/S1061933X23601324
L. B. Boinovich, A. M. Emelyanenko, M. A. Kalinina
{"title":"Editorial Column","authors":"L. B. Boinovich,&nbsp;A. M. Emelyanenko,&nbsp;M. A. Kalinina","doi":"10.1134/S1061933X23601324","DOIUrl":"10.1134/S1061933X23601324","url":null,"abstract":"","PeriodicalId":521,"journal":{"name":"Colloid Journal","volume":"86 1","pages":"1 - 3"},"PeriodicalIF":1.4,"publicationDate":"2024-03-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140468292","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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