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Stable organic radical qubits and their applications in quantum information science 稳定的有机基量子比特及其在量子信息科学中的应用
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-06-21 DOI: 10.1016/j.xinn.2024.100662
Aimei Zhou, Zhecheng Sun, Lei Sun
{"title":"Stable organic radical qubits and their applications in quantum information science","authors":"Aimei Zhou, Zhecheng Sun, Lei Sun","doi":"10.1016/j.xinn.2024.100662","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100662","url":null,"abstract":"The past century has witnessed the flourishing of organic radical chemistry. Stable organic radicals are highly valuable for quantum technologies thanks to their inherent room temperature quantum coherence, atomic-level designability, and fine tunability. In this comprehensive review, we highlight the potential of stable organic radicals as high-temperature qubits and explore their applications in quantum information science, which remain largely underexplored. Firstly, we summarize known spin dynamic properties of stable organic radicals and examine factors that influence their electron spin relaxation and decoherence times. This examination reveals their design principles and optimal operating conditions. We further discuss their integration in solid-state materials and surface structures, and present their state-of-the-art applications in quantum computing, quantum memory, and quantum sensing. Finally, we analyze the primary challenges associated with stable organic radical qubits and provide tentative insights to future research directions.","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"61 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-06-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141548798","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Scientists eager for Chang’e-6 lunar farside samples to bring new discoveries 科学家渴望嫦娥六号月球远侧样品带来新发现
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-06-19 DOI: 10.1016/j.xinn.2024.100660
Wei Yang, Yuyang He, Yuqi Qian, Zongyu Yue
{"title":"Scientists eager for Chang’e-6 lunar farside samples to bring new discoveries","authors":"Wei Yang, Yuyang He, Yuqi Qian, Zongyu Yue","doi":"10.1016/j.xinn.2024.100660","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100660","url":null,"abstract":"","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"58 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-06-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141504340","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Toward a nomenclature consensus for diverse intelligent systems: Call for collaboration 为多样化智能系统达成术语共识：呼吁合作
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-06-17 DOI: 10.1016/j.xinn.2024.100658
Brett J. Kagan, Michael Mahlis, Anjali Bhat, Josh Bongard, Victor M. Cole, Phillip Corlett, Christopher Gyngell, Thomas Hartung, Bianca Jupp, Michael Levin, Tamra Lysaght, Nicholas Opie, Adeel Razi, Lena Smirnova, Ian Tennant, Peter Thestrup Wade, Ge Wang
{"title":"Toward a nomenclature consensus for diverse intelligent systems: Call for collaboration","authors":"Brett J. Kagan, Michael Mahlis, Anjali Bhat, Josh Bongard, Victor M. Cole, Phillip Corlett, Christopher Gyngell, Thomas Hartung, Bianca Jupp, Michael Levin, Tamra Lysaght, Nicholas Opie, Adeel Razi, Lena Smirnova, Ian Tennant, Peter Thestrup Wade, Ge Wang","doi":"10.1016/j.xinn.2024.100658","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100658","url":null,"abstract":"Disagreements about language use are common both between and within fields. Where interests require multidisciplinary collaboration or the field of research has the potential to impact society at large, it becomes critical to minimize these disagreements where possible. The development of diverse intelligent systems, regardless of the substrate (e.g., silicon vs. biology), is a case where both conditions are met. Significant advancements have occurred in the development of technology progressing toward these diverse intelligence systems. Whether progress is silicon based, such as the use of large language models, or through synthetic biology methods, such as the development of organoids, a clear need for a community-based approach to seeking consensus on nomenclature is now vital. Here, we welcome collaboration from the wider scientific community, proposing a pathway forward to achieving this intention, highlighting key terms and fields of relevance, and suggesting potential consensus-making methods to be applied.","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"26 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141504304","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Selectivity switch via tuning surface static electric field in photocatalytic alcohol conversion 在光催化酒精转化过程中通过调节表面静电场实现选择性转换
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-06-17 DOI: 10.1016/j.xinn.2024.100659
Zhiwei Chen, Hongru Zhou, Fanhao Kong, Zhaolin Dou, Min Wang
{"title":"Selectivity switch via tuning surface static electric field in photocatalytic alcohol conversion","authors":"Zhiwei Chen, Hongru Zhou, Fanhao Kong, Zhaolin Dou, Min Wang","doi":"10.1016/j.xinn.2024.100659","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100659","url":null,"abstract":"Photocatalysis has shown powerful capabilities in organic reactions, while controlling the selectivity is a long-standing goal and challenge due to the involvement of various radical intermediates. In this study, we have realized selectivity control in the photocatalytic conversion of alcohols via engineering the surface static electric field of the CdS semiconductor. By leveraging the Au–CdS interaction to adjust lattice strain, which influences the intensity of the surface static electric field, we altered the pathways of alcohol conversion. The increased intensity of the surface static electric field changed the activation pathways of the C–H/O–H bond, leading to the selective formation of targeted C/O-based radical intermediates and altering the selectivity from aldehydes to dimers. A wide range of alcohols, such as aromatic alcohol and thiophenol alcohol, were selectively converted into aldehyde or dimer. This work provides an effective strategy for selectively controlling reaction pathways by generating a surface electric field.","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"15 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141548800","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Forecasting fierce floods with transferable AI in data-scarce regions 在数据稀缺地区利用可转移的人工智能预测凶猛洪水
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-05-29 DOI: 10.1016/j.xinn.2024.100652
Hui-Min Wang, Xiao Peng, Xiaogang He
{"title":"Forecasting fierce floods with transferable AI in data-scarce regions","authors":"Hui-Min Wang, Xiao Peng, Xiaogang He","doi":"10.1016/j.xinn.2024.100652","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100652","url":null,"abstract":"","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"185 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-05-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141517606","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Surface-adaptive interfaces: Bioresorbable ultrasound biomedical devices for noninvasive monitoring and imaging of deep-tissue homeostasis 表面自适应界面：用于无创监测和成像深层组织稳态的生物可吸收超声生物医学装置
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-05-27 DOI: 10.1016/j.xinn.2024.100651
Jiyu Li, Yingying Zhou, Xiazi Huang, Puxiang Lai, Yuan Huang
{"title":"Surface-adaptive interfaces: Bioresorbable ultrasound biomedical devices for noninvasive monitoring and imaging of deep-tissue homeostasis","authors":"Jiyu Li, Yingying Zhou, Xiazi Huang, Puxiang Lai, Yuan Huang","doi":"10.1016/j.xinn.2024.100651","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100651","url":null,"abstract":"","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"127 21-22 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-05-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141254880","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
H2O2-modified NiOx for perovskite photovoltaic modules 用于过氧化物光伏组件的 H2O2 改性氧化镍
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-05-27 DOI: 10.1016/j.xinn.2024.100650
Jianlong Xie, Qiyin Chen, Qin Xue, Igor F. Perepichka, Guohua Xie
{"title":"H2O2-modified NiOx for perovskite photovoltaic modules","authors":"Jianlong Xie, Qiyin Chen, Qin Xue, Igor F. Perepichka, Guohua Xie","doi":"10.1016/j.xinn.2024.100650","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100650","url":null,"abstract":"","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"52 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-05-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141254780","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
FlowerMate 2.0: Identifying plants in China with artificial intelligence FlowerMate 2.0：用人工智能识别中国的植物
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-05-07 DOI: 10.1016/j.xinn.2024.100636
Gan Xie, Jing Xuan, Bing Liu, Yibo Luo, Yufei Wang, Xinhui Zou, Min Li
{"title":"FlowerMate 2.0: Identifying plants in China with artificial intelligence","authors":"Gan Xie, Jing Xuan, Bing Liu, Yibo Luo, Yufei Wang, Xinhui Zou, Min Li","doi":"10.1016/j.xinn.2024.100636","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100636","url":null,"abstract":"","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"42 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-05-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140934136","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Decoding the brain: Unveiling comprehensive cellular atlases through multiomics mega-data 解码大脑：通过多组学巨型数据揭示全面的细胞图谱
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-05-06 DOI: 10.1016/j.xinn.2024.100637
Qianwen Wang, Wenli Tang, Lukui Chen, Lin Deng, Guangchuang Yu
{"title":"Decoding the brain: Unveiling comprehensive cellular atlases through multiomics mega-data","authors":"Qianwen Wang, Wenli Tang, Lukui Chen, Lin Deng, Guangchuang Yu","doi":"10.1016/j.xinn.2024.100637","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100637","url":null,"abstract":"","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"171 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140934138","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
6PPD-quinone affects the photosynthetic carbon fixation in cyanobacteria by extracting photosynthetic electrons 6PPD-quinone 通过提取光合电子影响蓝藻的光合碳固定
IF 32.1 1区 综合性期刊
The Innovation Pub Date : 2024-04-26 DOI: 10.1016/j.xinn.2024.100630
Xiuqi You, Ximin Chen, Yi Jiang, Huan Chen, Juan Liu, Zhen Wu, Weiling Sun, Jinren Ni
{"title":"6PPD-quinone affects the photosynthetic carbon fixation in cyanobacteria by extracting photosynthetic electrons","authors":"Xiuqi You, Ximin Chen, Yi Jiang, Huan Chen, Juan Liu, Zhen Wu, Weiling Sun, Jinren Ni","doi":"10.1016/j.xinn.2024.100630","DOIUrl":"https://doi.org/10.1016/j.xinn.2024.100630","url":null,"abstract":"Photosynthetic carbon fixation by cyanobacteria plays a pivotal role in the global carbon cycle but is threatened by environmental pollutants. To date, the impact of quinones, with electron shuttling properties, on cyanobacterial photosynthesis is unknown. Here, we present the first study investigating the effects of an emerging quinone pollutant, i.e., 6PPD-Q (N-(1,3-dimethylbutyl)-N′-phenyl--phenylenediamine-quinone), on the cyanobacterium sp. over a 400-generation exposure period. sp. exhibited distinct sequential phases, including hormesis, toxicity, and eventual recovery, throughout this exposure. Extensive evidence, including results of thylakoid membrane morphological and photosynthetic responses, carbon fixation rate, and key gene/protein analyses, strongly indicates that 6PPD-Q is a potent disruptor of photosynthesis. 6PPD-Q accepts photosynthetic electrons at the Q site in photosystem II (PSII) and the A site in PSI, leading to a sustained decrease in the carbon fixation of cyanobacteria after an ephemeral increase. This work revealed the specific mechanism by which 6PPD-Q interferes with photosynthetic carbon fixation in cyanobacteria, which is highly important for the global carbon cycle.","PeriodicalId":36121,"journal":{"name":"The Innovation","volume":"61 1","pages":""},"PeriodicalIF":32.1,"publicationDate":"2024-04-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140882784","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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