Md. Mahmudur Rahman, Songita Rani Adhikary, M Mohinur Rahman Rabby, Md. Mahafujul Hassan, Salah Knani, Syed Hasibul Akhfer, Md. Khalid Al Zuhanee
{"title":"Production of functionalized clay-CNC based biopolymeric nanocomposite from agro-waste biomass for bulky industrial wastewater treatment via continuous column adsorption study with mathematical modeling: A critical review","authors":"Md. Mahmudur Rahman, Songita Rani Adhikary, M Mohinur Rahman Rabby, Md. Mahafujul Hassan, Salah Knani, Syed Hasibul Akhfer, Md. Khalid Al Zuhanee","doi":"10.1016/j.jclepro.2025.145883","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.145883","url":null,"abstract":"Due to extensive industrialization, fluctuating technologies, and an overgrowing population a colossal amount of hazardous effluent is generated every moment and discharged directly into the environment. This crude wastewater can contaminate the environment and food cycle; causing serious damage not only to the ecosystem but also to public health. Therefore, it is critical to treat this wastewater by improving an ecological and economical technology before discharging/reusing. However, researchers are exasperating to improve an efficient and effective technology for the refinement of the bulky industrial wastewater. Here, some state-of-the-art production techniques of the FC-CNC bionanosorbents have been proposed for the effective purification of bulky effluent via a continuous adsorption system. This technology is superior to other methods due to its lower cost, higher efficiency, innovative and beneficial nature, and high selectivity. Instead, the precursors (cellulose and clay) are more available, nontoxic, ecofriendly, biodegradable, thermally and mechanically stable, and have shown high surface area, porous structure, possessed substantial active binding sites that could have been busting their adsorption performances. Still there are several complications concerning the effective processing/modification of the main precursors, production techniques, mechanism, and mode of application while purifying the crude wastewater. Henceforth, this review paper would be devoted by concentrating the modification process, advance production methods, synergistic mechanism to support the mono and/or multilayer physisorption, chemisorption, diffusion/deep penetration, and mode of application addressing the bulky wastewater treatment. By discovering the gaps and suggesting impending instructions, this study aims to expand the fabrication, categorization, and application of the FC-CNC bionanoadsorbents.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"58 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144192680","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Subsidizing repair: implications for the formal and informal circular economy","authors":"Wim Van Opstal, Lize Borms","doi":"10.1016/j.jclepro.2025.145898","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.145898","url":null,"abstract":"As the linear economy faces increasing pressure due to high material footprints and waste generation, repair emerges as a promising circular strategy to extend product lifespans. Repair can occur formally or informally, such as through self-repair or community repair, but little is currently known about the interaction between formal and informal repair decisions. This paper analyses the effects of a repair subsidy for household appliances on formal and informal repair sectors in Flanders (Belgium). Employing a Computable General Equilibrium (CGE) model and household survey data, we find that a subsidy increases formal repair expenditure and employment while also slightly increasing paid informal repair activities, indicating a complementary relationship. However, repair subsidies may crowd out unpaid informal repair among households primarily motivated by cost-saving. Nonetheless, unpaid informal repair decisions remain mainly influenced by household characteristics, risk preferences, environmental values, and perceived habits. This paper is the first to combine macroeconomic modelling with survey data on formal and informal repair decisions. We recommend policymakers to complement repair subsidies with strategies to formalise undeclared informal repair activities and fostering the development of repair skills, enabling repair as a circular strategy that contributes to a just circular transition.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"13 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144201404","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Luis Garrido Mateos, Fernando Rodríguez-López, José Ignacio Sánchez-Macías
{"title":"The Three-Stage Evolution in the Economic Valuation of Nature: Externalities, Ecosystem Services, and Natural Capital Accountability.","authors":"Luis Garrido Mateos, Fernando Rodríguez-López, José Ignacio Sánchez-Macías","doi":"10.1016/j.jclepro.2025.145899","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.145899","url":null,"abstract":"This review analyzes the evolution of the economic valuation of environmental assets and services as a succession of paradigms, which we identify as (i) valuation of the environment, (ii) valuation of ecosystem services, and (iii) natural capital accountability. In this evolution, the field has moved from an academic, supply-driven approach to an operative, market-oriented one, in which more and more often institutions and businesses are being held accountable for their impacts on natural capital. Aims, techniques, and methods have been adapted to the evolution of needs. The concept of value itself has shifted from ontological to responsible, moving the focus from notional worth to impacts, dependencies, and decision-making.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"9 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144201406","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Life Cycle Assessment of Scaled-up Pyrite-based Solid-state Batteries for Energy Storage Applications","authors":"Md Rashed Hossain, Muyue Han, Lin Li","doi":"10.1016/j.jclepro.2025.145861","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.145861","url":null,"abstract":"The growing demand for sustainable and safer energy storage solutions has driven increased interest in emerging battery technologies. While liquid-based lithium-ion batteries are widely adopted, concerns over safety, environmental impact, and the scarcity of critical raw materials have prompted a shift toward solid-state alternatives. With higher energy density, greater inherent stability, and improved sustainability, solid-state batteries present a compelling alternative. However, quantitative assessments of their environmental impacts across different life cycle phases remain limited. Existing studies focus on transportation applications using lab-scale production data, leaving the life cycle impacts of solid-state batteries for large-scale energy storage underexplored. This study conducts a life cycle assessment to evaluate the environmental performance of pyrite-based solid-state batteries with scaled-up production for energy storage applications, considering cradle-to-gate and cradle-to-use phases. Key environmental impact indicators, including global warming potential, ecotoxicity, smoke and fog, and crustal scarcity indicator, are analyzed across five scenarios incorporating different battery performance metrics. Additionally, a sustainable and lower-impact development path is proposed by linking environmental performance with battery use-phase parameters across various application scales, from general-purpose storage to grid-level systems. Results indicate that under the U.S. energy mix, the global warming potential can be reduced by 35%, while overall environmental impacts across the selected categories can be lowered by 50% through optimized energy sourcing, improved battery chemistry, and strategic usage patterns.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"37 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144192947","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Camillo Bosco , Karen Nessler Seglem , Edvard Sivertsen , Oriana Jovanović , Herman Helness
{"title":"Developing a framework to assess water smartness and sustainability of circular economy solutions in the water sector","authors":"Camillo Bosco , Karen Nessler Seglem , Edvard Sivertsen , Oriana Jovanović , Herman Helness","doi":"10.1016/j.jclepro.2025.145874","DOIUrl":"10.1016/j.jclepro.2025.145874","url":null,"abstract":"<div><div>The transition to a circular economy in the water sector is challenged by the lack of comprehensive tools to assess and compare the performance of innovative solutions across multiple sustainability dimensions. This study aims to develop a structured framework of indicators to support such assessments and guide the sector toward achieving the United Nations Sustainable Development Goals (SDGs). The framework was co-developed with stakeholders and encompasses technical, social, environmental, economic, and governance dimensions. It is organized into four hierarchical layers: dimensions, objectives, criteria, and indicators. Objectives were designed to be broadly applicable, while criteria and indicators were formulated to assess alignment with these objectives and capture the multifaceted nature of “water smartness.” The framework was tested and validated through workshops and structured engagement activities across six demonstration cases. Results from exploratory data analysis confirmed the framework's relevance for decision-making, highlighting its capacity to compare alternatives under diverse scenarios and its alignment with the SDGs. Additionally, the testing process pointed out the differentiated responsibilities of involved stakeholders, offering practical insights for advancing full-scale implementation of circular economy models in the water sector.</div></div>","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"517 ","pages":"Article 145874"},"PeriodicalIF":9.7,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144201409","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Joel Kostensalo , Kirsi Silvennoinen , Marita Kettunen , Vesa Lampi
{"title":"Optimal design of national food waste monitoring for the food service sector","authors":"Joel Kostensalo , Kirsi Silvennoinen , Marita Kettunen , Vesa Lampi","doi":"10.1016/j.jclepro.2025.145889","DOIUrl":"10.1016/j.jclepro.2025.145889","url":null,"abstract":"<div><div>The countries of the European Union have committed to monitoring and lowering food waste (FW) levels, including in the food service sector. In this work, the relative importance of factors such as food service type, outlet size, seasonal and weekday variation, and length of measurement period for monitoring originally edible and total FW is explored. We provide the first sample size estimates needed for national-level monitoring, and take the length of the observation period carefully into account and whether the food service type, outlet size, and regional variation are controlled for, and what size of a change in FW one wants to be able to observe. Two datasets collected as part of the Finnish national monitoring system were used. The first consisted of 192 two-week measurements from outlets of various sizes. The second consisted of three long-term (1.5–2 year) monitoring efforts. The food service type is by far the most important factor, explaining 66 % and 54 % of the variance in edible and total FW, respectively. The next factor is monthly variation (13 % and 10 %), municipal level variation (5 % and 9 %), and weekday-variation (6 % and 5 %), with the outlet size being relatively unimportant (2 % and 8 %). At the smallest, a sample size of n = 68 is needed to observe a change of 30 % in the total national FW levels. With two-week measurements n = 72 is sufficient, highlighting the fact that longer measurement periods are not resource efficient, because between-outlet variation tends to be greater than within-outlet variation. The results can be used to develop national data collection in other countries, to optimize the limited resources available for monitoring, and to improve the comparability of measurements between years.</div></div>","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"517 ","pages":"Article 145889"},"PeriodicalIF":9.7,"publicationDate":"2025-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144189002","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Comprehensive evaluation of Filament Winding process and part design: effects on winding time and Life Cycle impacts","authors":"Iacopo Bianchi, Archimede Forcellese, Chiara Mignanelli, Michela Simoncini, Tommaso Verdini","doi":"10.1016/j.jclepro.2025.145888","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.145888","url":null,"abstract":"Filament Winding (FW) is an automated process that allows the production of axisymmetric components in Fiber Reinforced Polymers (FRPs). As compared to traditional composites production technologies, FW enables the achievement of cost and environmental impacts reduction. In this framework, the present paper aims at developing a comprehensive model for the evaluation of process time, cost and environmental impacts of filament winding of FRP composite, at different process parameters, such as winding angle and speed, part design obtained varying mandrel length and/or mandrel diameter, and material characteristics, such as towpreg bandwidth. To this purpose, process simulations were carried out to assess the effect of process parameters and material variables on process time, material and energy use. A statistical approach was used to predict these outputs for a generic FRP component at different parameters. Furthermore, Life Cycle Assessment and Life Cycle Costing spreadsheets were developed to quantify the environmental and economic sustainability of the FRP structure. The results have proven the excellent capability of the model in predicting winding time, in particular R<sup>2</sup>, adjusted R<sup>2</sup>, Mean Squared Error (MSE) are respectively equal to 99.48%, 99.33%, and 0.133 min<sup>2</sup>. The relation between the process parameters and the winding time was used in spreadsheet to evaluate cost and environmental impacts of FW process of FRP structures from the early design stages, promoting a sustainable approach in the manufacturing of FRP composite sector.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"37 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144189013","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Carolina M. Pereira , Henrique Vieira , Nuno P.F. Gonçalves , Guilherme Ascensão , Rui M. Novais
{"title":"Innovative waste-containing 3D-printed geopolymer structures for enhanced acoustic comfort in built environments","authors":"Carolina M. Pereira , Henrique Vieira , Nuno P.F. Gonçalves , Guilherme Ascensão , Rui M. Novais","doi":"10.1016/j.jclepro.2025.145857","DOIUrl":"10.1016/j.jclepro.2025.145857","url":null,"abstract":"<div><div>The reduction of noise pollution in buildings, a critical global public health concern, demands the development of novel acoustic barriers that meet with the sustainability requirements envisioned for future building materials. Herein, additive manufacturing was explored to develop 3D-printed geopolymer structures combining high porosity, mechanical strength, and remarkable acoustic properties, a pioneering study in this area. The results demonstrate that lattice design can effectively tailor the acoustic performance of these novel materials. A 21-mm thick structure with filaments rotated by 45° between layers exhibited an impressive sound absorption coefficient across the studied frequency range (α reaching 0.90 at 3150 Hz) alongside a compressive strength (6.9 MPa). In contrast, a structure with filaments rotated by 90° showed slightly lower sound absorption performance (α = 0.84) but significantly higher strength (12.6 MPa). These promising findings could pave the way for the broader use of environmentally conscious geopolymers in acoustic applications.</div></div>","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"517 ","pages":"Article 145857"},"PeriodicalIF":9.7,"publicationDate":"2025-05-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144189015","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Sayak Saha Chowdhury , Biswajit Bera , Manoj Peddiraju , Sirshendu De
{"title":"Green synthesis of sulfonated hydroxyapatite incorporated carbonaceous composite (C-aHAp-S) for efficient adsorptive separation of lead in water: an experimental and theoretical approach","authors":"Sayak Saha Chowdhury , Biswajit Bera , Manoj Peddiraju , Sirshendu De","doi":"10.1016/j.jclepro.2025.145839","DOIUrl":"10.1016/j.jclepro.2025.145839","url":null,"abstract":"<div><div>A facile in-situ co-precipitation strategy was devised to produce novel sulfonated aluminium substituted hydroxyapatite nanoparticle (designated as aHAp-S) immobilized macro-scale granular charcoal composite (referred as C-aHAp-S). The green synthesis strategy (water used as reaction medium) involving minimal energy and non-toxic nature of the products enhance the scalability and sustainability of the material. The developed aHAp-S showed higher specific surface area (S<sub><em>BET</em></sub> = 120.36 m<sup>2</sup>/g) and pore volume (<em>v</em><sub><em>p</em></sub> = 0.20 cm<sup>3</sup>/g) relative to the unmodified counterpart, aHAp (S<sub><em>BET</em></sub> = 81.91 m<sup>2</sup>/g, <em>v</em><sub><em>p</em></sub> = 0.14 cm<sup>3</sup>/g). High S<sub><em>BET</em></sub> of C-aHAp-S (310.56 m<sup>2</sup>/g) facilitated enhanced pore diffusion of lead ions to be adsorbed on the active sites inside the carbon matrix. aHAp-S showed enhanced maximum Pb uptake capacity (<em>Q</em><sub><em>L</em></sub>) in aqueous phase (<em>Q</em><sub><em>L</em></sub> = 1282.0 mg/g at 30 °C using Langmuir model) than aHAp (<em>Q</em><sub><em>L</em></sub> = 823.0 mg/g). C-aHAp-S demonstrated <em>Q</em><sub><em>L</em></sub> of 200.0 mg/g. High activation energy (<em>E</em><sub><em>a</em></sub> > 20 kJ/mol) indicated chemisorption of Pb. A fundamental pore diffusion-adsorption model was utilized for analyzing the kinetics of the batch process along with the conventional pseudo-first order and pseudo-second order models. The strong selectivity and credible reusability (5 cycles) was also highlighted. Fixed bed columns with C-aHAp-S packing were used to elucidate an effective continuous mode Pb adsorption performance with breakthrough volume as high as 860 times the fixed bed packing volume. An appropriate diffusion-convection-adsorption based transport model was employed to generate simulated concentration profiles and analyze the breakthrough trends for column studies which were subsequently used to predict the long-term performance.</div></div>","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"517 ","pages":"Article 145839"},"PeriodicalIF":9.7,"publicationDate":"2025-05-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144183956","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Harnessing low-cost adsorbents for removal of heavy metals and metalloids in contaminated water: Progress in the past decade and future perspectives","authors":"Zhiliang Li, Guining Lu, Daolin Du, Dongye Zhao","doi":"10.1016/j.jclepro.2025.145845","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.145845","url":null,"abstract":"Heavy metals and metalloids have been a major environmental concern due to their adverse effects on the environmental and human health. Consequently, more cost-effective technologies have been sought for decades to remove the contaminants from contaminated water. As metals and metalloids are nondegradable, adsorption based on low-cost materials has garnered broad interest for its cost-effectiveness, easy operation, and lower environmental impact, especially in developing countries or underserved communities. This review encapsulates the latest progress and the state of the technology on the type, preparation and applications of low-cost adsorbents ranging from natural minerals, biosorbents, materials, agricultural wastes, and modified natural materials to synthetic composite adsorbents. The focus was placed on the technical feasibility, economic effectiveness, pros and cons, as well as influencing factors for treating a range of heavy metals (e.g., lead, zinc, and copper) and metalloids (e.g., arsenic, selenium, tellurium, and antimony) in water. In addition, the underlying adsorption mechanisms were discussed and the technical practicality and economic viability are analyzed by considering the pros and cons as well as relevant environmental factors. Overall, low-cost adsorbents may offer an effective alternative for remediation of water contaminated with metal(loid)s, especially for underdeveloped communities and for non-potable water treatment. Modified or composite adsorbents composed of multiple low-cost materials have shown great promise. This review also identified some critical research needs and knowledge gaps, including eight action items, which may guide the future material and technology development.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"4 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-05-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144183954","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}